4.6 Article

Epoxy modulated multifold enhancement of magnetoelectric response in distributed disc structured composite

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MATERIALS LETTERS
卷 342, 期 -, 页码 -

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ELSEVIER
DOI: 10.1016/j.matlet.2023.134327

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Composites; Magnetic materials; Piezoelectric materials; Magnetoelectricity; Distributed disc structures

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The authors previously introduced a novel magnetoelectric (ME) composite configuration called distributed disc structured (DDS) configuration, which can operate at high temperatures without epoxy. However, a topological study revealed that the absence of epoxy in the DDS composites resulted in material discontinuity and voids at the magnetostrictive/piezoelectric interface, negatively impacting the ME response. In this study, epoxy was used to fill the voids in the DDS composites, resulting in a remarkable improvement in the quasi-static and resonant ME measurements compared to epoxy-free counterparts.
The authors had previously reported a novel magnetoelectric (ME) composite configuration termed as distributed disc structured (DDS) configuration, which was proposed as epoxy-free ME composite to enable them to operate at elevated temperatures. However, a topological study on the epoxy-free DDS composites reveal that the absence of epoxy led to material discontinuity and generation of voids at the magnetostrictive/piezoelectric interface, thereby adversely affecting the output ME response. In this study, the voids at the magnetostrictive/piezoelectric interface in the DDS composites have been filled using epoxy material and quasi-static and resonant ME mea-surements show a remarkable improvement over their epoxy-free counterparts. The maximum ME coefficient of 2.33 V/cm Oe (enhancement of 430 %) and a peak value of 163 V/cm Oe is observed for four-disc structured configuration under quasi-static and resonant operating conditions, respectively. Thus, for the first time, the advantage of the DDS configuration has been combined with the use of epoxy leads to achieve a remarkable enhancement in ME response of Ni/PZT composites.

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