期刊
JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY
卷 -, 期 -, 页码 -出版社
SPRINGER
DOI: 10.1007/s10967-023-09096-9
关键词
TIMS; Nuclear debris; Cesium; Nuclear forensics
Cs-135/Cs-137 measurements were conducted on debris samples from the Trinity nuclear test, revealing variations in condensation times and Cs-135/Cs-137 ratios. The measurements also showed heterogeneities in Cs-135/Cs-137 ratios within different trinitite lithologies in a single sample.
Cs-135/Cs-137 measurements were performed on a set of debris samples from the first nuclear test, Trinity. Debris from several locations around ground zero of the event were purified and analyzed for Cs-135/Cs-137 by thermal ionization mass spectrometry (TIMS). The Cs-isotopic measurements presented here are the first high precision TIMS Cs-135/Cs-137 measurements of trinitite from variable locations and cooling histories relative to ground zero. Our measurements show a large fractionation from the predicted fission yields, all with a relative enrichment in Cs-137. Cs-135/Cs-137 ratios indicate that condensation times varied between different debris forms, however they are not consistent with an unfractionated decay to Cs from independent fission products. Variations in Cs-135/Cs-137 ratios are observed with relative distance from ground zero as well as Cs-135/Cs-137 heterogeneities between different trinitite lithologies within a single sample.
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