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Article
Chemistry, Physical
Yurong Zhou et al.
Advanced Energy Materials
(2023)
Review
Chemistry, Physical
Muhammad Sufyan Javed et al.
Summary: Zn-ion hybrid supercapacitors (ZHSCs) combine Zn-ion batteries with supercapacitors to meet the energy and power needs of portable devices and electric automobiles. This review provides an in-depth investigation and summarization of the charge storage mechanisms, advantages/disadvantages, recent development of cathode materials, and new design of device fabrications for ZHSCs, highlighting the importance of developing new cathode materials.
ADVANCED ENERGY MATERIALS
(2023)
Article
Nanoscience & Nanotechnology
Jianbin Ruan et al.
Summary: This work proposes a design concept of 3D artificial array interface engineering to achieve stable Zn metal anode in aqueous Zn-ion batteries. Through multi-scale characterization techniques, the mechanism of MXene array interface on modulating the growth kinetics and deposition behavior of Zn atoms is revealed. The engineered electrode exhibits comprehensive enhancements in corrosion resistance, rate capability, and cyclic stability, offering potential for high-performance rechargeable batteries.
NANO-MICRO LETTERS
(2023)
Article
Chemistry, Physical
Xiangcheng Xu et al.
Summary: Zinc-ion hybrid supercapacitors (ZHCs) based on multivalent ion storage principle are considered promising for large-scale energy storage. To meet demands for portable and miniaturized devices, a compact three-dimensional porous graphene cathode was designed to balance porous structure and high density, achieving high volumetric energy density with no sacrifice of power density. The ZHC with this cathode demonstrated excellent volumetric performance, long cycle stability, and extremely high volumetric energy density.
Article
Chemistry, Physical
Yue Zhao et al.
Summary: By synthesizing N/P co-doped graphene (NPG) through a one-step hydrothermal method, this study highlights the efficient synthesis and excellent performance of NPG cathode materials, promoting the rapid development and great application of high-performance Zn-ion hybrid capacitors.
JOURNAL OF POWER SOURCES
(2022)
Review
Chemistry, Physical
Sadayappan Nagamuthu et al.
Summary: Metal ion capacitors (MICs) combine the advantages of supercapacitors and rechargeable batteries, offering high energy density and long cycle life. Research on non-lithium based MICs has made significant progress in recent years.
JOURNAL OF MATERIALS CHEMISTRY A
(2022)
Article
Chemistry, Physical
Ke Wang et al.
Summary: This study demonstrates the use of renewable polymers as a surface coating layer to protect zinc anodes in zinc-iodine batteries, effectively suppressing triiodide ion shuttling and zinc dendrite formation. The results show that the introduction of renewable polymers significantly improves the stability and cycle life of the batteries.
JOURNAL OF MATERIALS CHEMISTRY A
(2022)
Article
Chemistry, Physical
Jiaming Wang et al.
Summary: By optimizing porous bamboo carbons, a flexible and high-performance Zn-ion hybrid supercapacitor was successfully constructed, showing superior specific capacitance and high energy density, as well as remarkable cycling stability and the ability to withstand various deformations.
APPLIED SURFACE SCIENCE
(2022)
Article
Chemistry, Physical
Shaojie Kuang et al.
Summary: A biomass hydrogel electrolyte with double cross-linked structure was successfully synthesized, which exhibited excellent mechanical strength and high ionic conductivity. The resulting flexible supercapacitors based on this electrolyte achieved high specific capacitance and excellent energy density, and maintained their performance even when folded at different angles. Zinc ion capacitors constructed using this electrolyte also showed high capacity retention after a large number of cycles.
JOURNAL OF ALLOYS AND COMPOUNDS
(2022)
Article
Chemistry, Physical
Yujia Long et al.
Summary: The corrosion mechanism of the zinc anode in aqueous Zn-ion hybrid supercapacitors (ZHSCs) was studied and a method for modifying the zinc anode with an in-situ grown zeolitic imidazolate framework-8 (ZIF-8) layer was reported. The ZIF-8 layer with hydrophobicity can inhibit zinc corrosion, promote zinc deposition, and improve the cycling stability and capacity retention of ZHSCs.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2022)
Article
Chemistry, Physical
Zhanpeng Huang et al.
Summary: Interfacial engineering using a metal-organic framework cation reservoir as a zincophile interphase offers a solution to manipulate zinc-ion flux, suppress side reactions, and improve the performance of zinc metal anodes.
JOURNAL OF POWER SOURCES
(2022)
Article
Chemistry, Physical
Jiwei Chen et al.
Summary: This study reports a stiff and tough poly(vinyl alcohol) hydrogel electrolyte for flexible supercapacitor. A solvent-exchange strategy was used to introduce kosmotropic ions and promote self-assembly of PVA chains into a homogeneous network. The resulting hydrogel electrolytes exhibited remarkable stiffness and toughness, and a flexible supercapacitor assembled with these electrolytes showed high areal specific capacitance and resistance to mechanical stimuli.
JOURNAL OF POWER SOURCES
(2022)
Article
Chemistry, Physical
Hongyang Wang et al.
Summary: In this study, a robust flexible aqueous zinc-ion hybrid supercapacitor (ZHSC) was fabricated using an anti-freezing and anti-drying organohydrogel electrolyte. The electrolyte showed good conductivity and stable flexibility, and the ZHSC exhibited resistance to mechanical damage. It achieved high energy and power densities, broad temperature adaptability, and retained capacitance after storage and cycling tests.
JOURNAL OF POWER SOURCES
(2022)
Article
Chemistry, Multidisciplinary
Xiaoqing Zhu et al.
Summary: In this study, a freeze-tolerant hydrogel electrolyte with high ionic conductivity and superior mechanical properties was developed for portable zinc-ion hybrid supercapacitors. The hydrogel exhibited excellent durability and stable electrochemical performance at low temperatures.
Article
Chemistry, Physical
Li Wen et al.
Summary: Rechargeable zinc-based aqueous systems are attractive for energy storage technology due to their safety, low cost, and ecological friendliness. This study verifies the feasibility of using TiSe2 as an intercalated anode for aqueous zinc ion batteries and zinc ion hybrid supercapacitors. TiSe2 exhibits excellent electrical charge transport characteristics and demonstrates good performance in terms of capacity, working potential window, and recyclability.
Article
Electrochemistry
Qiuhong Chen et al.
Summary: In this study, a high-performance solid hydrogel with adequate flexibility and strong low-temperature tolerance was developed for flexible supercapacitors. By using this hydrogel as the electrolyte in a flexible zinc-ion hybrid supercapacitor, wide voltage window and excellent cycling stability were achieved. The device demonstrated high specific energy and the ability to operate at ultralow temperatures, showcasing its great potential for advanced flexible electronic devices.
Article
Chemistry, Physical
Jinwoo Park et al.
Summary: Considering the need for environmental friendliness and cost effectiveness, increasing the energy density of aqueous supercapacitors is highly desired. Recently, concentrated aqueous electrolytes known as water-in-salt electrolytes (WiSEs) have gained attention due to their broad electrochemical stability window. In addition, the development of redox-active electrolytes provides an opportunity to improve capacitance. A supercapacitor containing a dual redox-active WiSE is demonstrated, which significantly increases the energy density and delivers a constant power output.
ACS ENERGY LETTERS
(2022)
Article
Chemistry, Physical
Zhixiao Xu et al.
Summary: In this study, aqueous zinc ion capacitors (ZICs) were developed to work under extreme conditions, such as ultrafast rates, sub-million cycles, high loadings, and wide temperatures. The incorporation of activated carbon (AC), aqueous binder, and concentrated electrolyte enabled the ZICs to achieve unprecedented performance, including large capacitance, high rate capability, long cycle life, high loadings, and wide temperature operation. The AC electrode revealed a proton/Zn2+ ion co-interaction mechanism. This work opens up possibilities for practical supercapacitors beyond normal conditions.
ENERGY STORAGE MATERIALS
(2022)
Article
Chemistry, Physical
Yihan Wu et al.
Summary: This paper presents a novel aqueous zinc-ion hybrid supercapacitor (ZHSC) with a robust and stretchable eutectogel electrolyte. The gel electrolyte is prepared through a one-step gelation process without additional initiators and crosslinkers. The ZHSC exhibits high ionic conductivity, extended voltage window, high energy density, admirable cycling stability, temperature stability, and bendability, making it a promising candidate for flexible wearable electronic devices.
ACS APPLIED ENERGY MATERIALS
(2022)
Article
Nanoscience & Nanotechnology
Meihua Zhu et al.
Summary: This study presents a bio-inspired silk fibroin (SF) coating to stabilize Zn anode via constructing an interface reversible electric field. The SF coating with amphoteric charges can manipulate the transfer kinetics of Zn2+ and reduce anodic polarization. Experimental and theoretical analyses demonstrate that the SF coating facilitates the desolvation of [Zn(H2O)6]2+ and provides nucleation sites for uniform deposition.
NANO-MICRO LETTERS
(2022)
Article
Chemistry, Multidisciplinary
Xiaofeng He et al.
Summary: The study introduces a concept of constructing an anion concentration gradient-assisted solid-electrolyte interphase for metal anodes, which enhances ionic conductivity and suppresses dendritic growth and side reactions. This new approach enables stable plating/stripping of zinc metal and shows improved cycling stability in various types of batteries and supercapacitors.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2022)
Article
Chemistry, Physical
Qinping Jian et al.
Summary: The study formulates a new low-concentration electrolyte to improve the reversibility and stability of zinc anodes in aqueous zinc batteries. By adding DMSO into the electrolyte, a fluorinated interphase is formed on the zinc surface, suppressing dendrite formation and side reactions. This newly formulated electrolyte enables highly reversible zinc plating/stripping and significantly improves the cycle life of zinc batteries.
ENERGY STORAGE MATERIALS
(2022)
Article
Energy & Fuels
Ahmed S. Etman et al.
Summary: This report investigates the use of MXenes as positive electrode materials and surface coating materials in zinc-ion hybrid supercapacitors. The study finds that coating the surface of the zinc anode with a layer of Ti3C2Tz MXene can inhibit side reactions and passivation, allowing for the use of low-cost zinc salt. Moreover, the performance of MXene materials varies in different electrolytes.
JOURNAL OF ENERGY STORAGE
(2022)
Article
Chemistry, Multidisciplinary
Zijing Xia et al.
Summary: Membranes integrating two-dimensional materials have unique ion transport properties and can be used for separation applications in both aqueous and nonaqueous systems. By tuning interlayer spacing and enhancing membrane stability, ion diffusivity can be controlled.
Article
Chemistry, Physical
Haiyan Wang et al.
Summary: Hierarchically porous carbon nanosheets functionalized with oxygen groups and nitrogen dopants derived from biomass are synthesized and used as cathode materials for Zn-ion hybrid supercapacitors. The resulting Zn-ion hybrid supercapacitor exhibits high capacity and energy density, surpassing most state-of-the-art reported ZHSCs. The hierarchical porous structure and nitrogen doping with oxygen functional groups modification are found to enhance both physical and chemical adsorption of Zn2+.
APPLIED SURFACE SCIENCE
(2022)
Article
Engineering, Environmental
Yuan Wang et al.
Summary: This study proposes novel aqueous Zn-ion hybrid supercapacitors with dual redox-active ions enhanced electrolytes, resulting in a significantly higher specific capacity compared to traditional Zn-ion hybrid supercapacitors.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Chemistry, Physical
He Yang et al.
Summary: This study develops a gel polymer electrolyte based on a ternary deep eutectic solvent with a low eutectic point, which shows excellent flexibility and satisfactory mechanical properties. The optimized electrolyte exhibits high ionic conductivity at low temperature and significantly improves the energy density and cycling stability of a ZIHS. The assembled flexible device demonstrates outstanding wide-temperature adaptability and tolerance to harsh conditions.
JOURNAL OF POWER SOURCES
(2022)
Article
Chemistry, Multidisciplinary
Yuanjun Zhang et al.
Summary: In this study, a stable honeycomb-like ZnO passivation protective layer was developed on the Zn surface to inhibit the growth of Zn dendrites, resulting in improved cycling stability and lifespan of the battery.
Article
Energy & Fuels
He Yang et al.
Summary: Zinc ion hybrid supercapacitor (ZIHS) shows great potential in portable electronics and electric vehicles, but the issue of zinc dendrites hinders its practical application. A new supramolecular gel polymer electrolyte (SGPE) is constructed to suppress the growth of zinc dendrites and provide good mechanical performance and high ionic conductivity. The ZIHS assembled with SGPE, activated carbon materials, and zinc metal demonstrates a wide voltage window and impressive cycling life.
JOURNAL OF ENERGY STORAGE
(2022)
Article
Chemistry, Multidisciplinary
Shiqiang Wei et al.
Summary: This study demonstrates the enhancement of stability for zinc metal anodes by constructing self-assembled monolayers (SAMs) on their surfaces. By selectively grafting thiol molecules onto unstable zinc crystal facets, a covalent interface can be engineered to enable uniform zinc deposition and prevent dendrite growth and side reactions. The modified anodes exhibit improved electrochemical performance and cycling stability.
Article
Engineering, Environmental
Bo Zhou et al.
Summary: This study addresses the poor plating/stripping behaviors in zinc metal batteries by constructing vermiculite with fast ion-transport channels on the surface of the zinc metal anodes. The ion channels facilitate zinc ion transport and reduce the presence of water molecules. Experimental results demonstrate dendrite-free plating/stripping behavior and long cycling life of the zinc metal anodes.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Chemistry, Physical
Haiyan Wang et al.
Summary: This study synthesized biomass-derived hierarchical porous carbon nanosheets functionalized with oxygen groups and nitrogen dopants as the cathode for Zn-ion hybrid supercapacitors. The cathode demonstrated high capacity and maintained performance even at high current densities, leading to an ultra-high energy density in the ZHSC. The synergistic effect of nitrogen doping and oxygen functional groups modification in hierarchical porous carbon was shown to enhance Zn-ion storage.
APPLIED SURFACE SCIENCE
(2022)
Article
Chemistry, Multidisciplinary
Cheng Wang et al.
Summary: By developing ZnCl2-based electrolytes, researchers have successfully improved the energy density and cycling life of zinc ion hybrid capacitors. Through the mechanism of desolvation facilitated by chloride ions and the use of a water-in-salt hydrogel electrolyte, they were able to achieve this goal.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2021)
Article
Chemistry, Multidisciplinary
Zhaodong Huang et al.
Summary: Research has shown that involving anions in the reaction process can improve the capacitance and anti-self-discharge ability of ion hybrid capacitors, leading to a stable energy storage mechanism.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2021)
Article
Chemistry, Multidisciplinary
Qingjin Fu et al.
Summary: The flexible zinc-ion hybrid capacitors exhibit excellent low-temperature adaptability and high thermal conductivity, along with a long cycling lifespan, outperforming similar products.
Article
Polymer Science
Guoqiang Li et al.
Summary: In this study, the performance of PAA-based GPEs was improved by incorporating SPEEK chains, resulting in enhanced ionic conductivity and mechanical properties. The supercapacitor developed using the SPEEK-enhanced GPE showed higher specific capacitance and energy density compared to the one using plain PAA GPE.
POLYMER INTERNATIONAL
(2021)
Article
Nanoscience & Nanotechnology
Linpo Li et al.
Summary: By regulating the concentration of ZnCl2 electrolyte, the cycle life of Vanadates in AZIBs can be greatly improved without the need to approach the water-in-salt threshold. Additionally, a novel CMC-ZnCl2 gel electrolyte with high ionic conductivity was designed for the first time, enabling the assembly of a quasi-solid-state AZIB with excellent stability and energy density.
NANO-MICRO LETTERS
(2021)
Article
Chemistry, Multidisciplinary
Xuan Qiu et al.
Summary: In this study, a Zn-based hybrid supercapacitor has been developed with high energy density and high Zn-utilization. By utilizing a metal organic framework derived porous carbon cathode and a specific electrolyte, high rate performance at high mass loading was achieved.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2021)
Article
Chemistry, Multidisciplinary
Ye Zhang et al.
Summary: The microstructure of separators plays a crucial role in determining the behavior of zinc electrodeposition. Porous separators direct zinc to deposit into their pores, leaving dead zinc upon stripping, while nonporous separators prevent zinc penetration. It is essential to preserve the attachment of the separator to the zinc-deposited substrate for accurate observation and conclusions.
Article
Multidisciplinary Sciences
Mutian Hua et al.
Summary: A strategy combining freeze-casting and salting-out treatments produces poly(vinyl alcohol) hydrogels with a multi-length-scale hierarchical architecture, including micrometre-scale honeycomb-like pore walls and interconnected nanofibril meshes. These hydrogels have properties that compare favorably to other tough hydrogels and even natural tendons.
Article
Electrochemistry
Li Zhang et al.
Summary: This study demonstrates the use of a novel electrolyte to construct C-ZIHCs with high energy density, ensuring stability and long cycle life during charging/discharging processes.
Article
Materials Science, Multidisciplinary
Fuyun Li et al.
Summary: Low-temperature-tolerant and durable Zn-ion hybrid supercapacitors (ZHSCs) were fabricated by modulating a co-solvent water/ethylene glycol electrolyte. The electrolyte with ZnSO4/water/ethylene glycol (65%) composition showed high ionic conductivity at low temperatures and effectively prevented dendrite formation in the Zn anode. These ZHSCs demonstrated long-term cyclability and operation at sub-zero temperatures as low as -40 degrees C, making them potentially valuable in next-generation electrochemical energy storage devices.
SCIENCE CHINA-MATERIALS
(2021)
Article
Nanoscience & Nanotechnology
Jianghe Liu et al.
Summary: The gel electrolyte based on the PVA/Zn/ethylene glycol system shows high ionic conductivity and excellent antifreezing performance. The antifreezing Zn-ion hybrid supercapacitor fabricated with this gel electrolyte exhibits outstanding electrochemical properties and cyclic stability, even under low temperatures, demonstrating its potential for flexible energy storage devices in subzero-temperature environments.
ACS APPLIED MATERIALS & INTERFACES
(2021)
Article
Chemistry, Multidisciplinary
Yinglun Sun et al.
Summary: This study introduces a new approach using Zn(ClO4)(2) salty ice as the electrolyte, achieving superior performance of a zinc ion hybrid capacitor even at low temperatures. This discovery provides a new insight for constructing low-temperature EES devices using salty ices as electrolytes.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Chemistry, Physical
Guoshen Yang et al.
Summary: Zinc-ion hybrid supercapacitor (ZHSC) combines the high power density of supercapacitors with the high energy density of batteries, utilizing the environmental and cost benefits of zinc-ion technology. Developing an electrolyte with thermal stability and anti-freezing property is crucial for achieving high energy density ZHSC working in a wide temperature range.
Article
Energy & Fuels
Xinren Zhang et al.
Summary: The use of graphene as surface layer on zinc foil in Zinc ion hybrid supercapacitors (ZIHS) successfully inhibits dendrite formation and significantly improves cyclic stability, leading to an ultra-long cycle life compared to traditional zinc foil anodes. The abundance of active sites on graphene facilitates uniform zinc deposition, contributing to the enhanced performance of the electrode.
JOURNAL OF ENERGY STORAGE
(2021)
Article
Nanoscience & Nanotechnology
Yang Li et al.
Summary: Aqueous Zn-ion hybrid supercapacitors with fibrous carbon cathodes exhibit high gravimetric capacity, superior rate capability, exceptional cycling stability, high energy density, high power density, and good anti-self-discharge performance. Mechanism investigation reveals the roles of various reactions in energy storage of ZHSs.
NANO-MICRO LETTERS
(2021)
Article
Chemistry, Physical
Yahui Li et al.
Summary: This paper presents a novel amorphous Ti3C2Tx/BiCuS2.5 electrode material with an enlarged working voltage window for high specific energy supercapacitors. The material exhibited improved capacity and energy density in aqueous symmetrical supercapacitors and zinc-ion capacitors, attributing to a baton relay mechanism and a combination of intercalation and redox battery-type capacity. This work opens a new direction for the construction of high specific energy supercapacitors.
Article
Chemistry, Multidisciplinary
Shuang Wu et al.
Summary: Zinc anodes with a 3D stacked lamellar matrix (SLM) structure show enhanced thermodynamic stability and rapid zinc ions transport kinetics, reducing dendrite growth and achieving exceptional performance under practical conditions.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Chun-Chao Hou et al.
Summary: Carbon micro/nanocages fabricated using a solid-state gas-steamed metal-organic-framework approach exhibit large openings on walls for enhanced kinetics of mass transport. The carbon cathodes show high operation voltage and ultralong cycling lifespan, resulting in high energy density and superb power density.
ADVANCED MATERIALS
(2021)
Article
Chemistry, Physical
Haonan Cui et al.
Summary: This study successfully synthesized nitrogen-doped MXene and designed a dual crosslinked hybrid polymeric hydrogel/electrolyte, which further improved the performance of Zn-ion hybrid supercapacitors, showing higher ionic conductivity and excellent capacity, stability, and energy density.
JOURNAL OF MATERIALS CHEMISTRY A
(2021)
Article
Chemistry, Multidisciplinary
Dandan Wu et al.
Summary: By developing a hydrogel electrolyte with ionically and covalently double crosslinked network and utilizing nitrogen and sulphur co-doped carbon nanosheets as the cathode material, the challenges of corrosion and dendrite growth in aqueous zinc ion hybrid supercapacitors have been effectively addressed, resulting in superior electrochemical performance and cycling stability.
Article
Chemistry, Physical
Zhongmou Pan et al.
APPLIED SURFACE SCIENCE
(2020)
Article
Chemistry, Multidisciplinary
Yuhang Ye et al.
ADVANCED FUNCTIONAL MATERIALS
(2020)
Article
Nanoscience & Nanotechnology
Qiang Wang et al.
ADVANCED ELECTRONIC MATERIALS
(2020)
Article
Chemistry, Physical
Zhiwei Li et al.
ENERGY STORAGE MATERIALS
(2020)
Article
Nanoscience & Nanotechnology
Young-Geun Lee et al.
ACS APPLIED MATERIALS & INTERFACES
(2020)
Article
Chemistry, Physical
Zhiwei Li et al.
ENERGY STORAGE MATERIALS
(2020)
Article
Chemistry, Physical
Geon-Hyoun An
APPLIED SURFACE SCIENCE
(2020)
Article
Chemistry, Physical
Lvye Yang et al.
JOURNAL OF MATERIALS CHEMISTRY A
(2020)
Review
Engineering, Manufacturing
Nouha Ghorbel et al.
COMPOSITES PART A-APPLIED SCIENCE AND MANUFACTURING
(2019)
Article
Nanoscience & Nanotechnology
Siliang Wang et al.
NANO-MICRO LETTERS
(2019)
Article
Nanoscience & Nanotechnology
Qiang Wang et al.
ADVANCED ELECTRONIC MATERIALS
(2019)
Article
Chemistry, Physical
Minfeng Chen et al.
JOURNAL OF MATERIALS CHEMISTRY A
(2019)
Article
Chemistry, Physical
Qi Li et al.
JOURNAL OF POWER SOURCES
(2017)
Review
Chemistry, Multidisciplinary
Hongwei Zhang et al.
