☆ 4.7 Review

Electrocatalytic seawater splitting for hydrogen production: Recent progress and future prospects

JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY (2023)

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Stable p-block metals electronic perturbation in PtM@CNT (M=Ga, In, Pb and Bi) for acidic seawater hydrogen production at commercial current densities

Nanzhu Nie et al.

Summary: We present a novel strategy using SMSI and Pt-p-block alloys to achieve stable acidic seawater hydrogen production at commercial current densities. The optimized Pt61Ga39@CNT exhibits high stability and catalytic activity in acidic seawater.

APPLIED CATALYSIS B-ENVIRONMENTAL (2023)

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Article Chemistry, Physical

Bifunctional zeolitic imidazolate framework-67 coupling with CoNiSe electrocatalyst for efficient hydrazine-assisted water splitting

Wentao Liu et al.

Summary: By employing hydrazine oxidation reaction (HzOR) instead of oxygen evolution reaction (OER), energy-saving hydrogen generation can be realized. Here, a combined experimental and theoretical investigation of zeolitic imidazolate framework-67 coupling with CoNiSe-3 (ZIF67@CoNiSe-3) as an efficient electrocatalyst towards both hydrogen evolution reaction (HER) and HzOR is introduced. The as-prepared ZIF67@CoNiSe-3 with nanoflower structure and highly porous ultrathin nanosheet arrays endow advanced electrocatalytic properties for HER and HzOR.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2023)

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Article Chemistry, Physical

Au nanocluster coupling with Gd-Co2B nanoflakes embedded in reduced TiO2 nanosheets: Seawater electrolysis at low cell voltage with high selectivity and corrosion resistance

Tanveer ul Haq et al.

Summary: A novel seawater electrolysis electrode design has been proposed, which demonstrates outstanding performance in overall seawater splitting with high selectivity for oxygen and hydrogen, strong corrosion resistance, and practical viability.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Chemistry, Multidisciplinary

Design strategies of phosphorus-containing catalysts for photocatalytic, photoelectrochemical and electrocatalytic water splitting

Lei Chen et al.

Summary: The review focuses on the recent progress of P-containing catalysts in water splitting and their design strategies to enhance catalytic activity. It delves into the theory-structure-property relationship and discusses research directions and challenges in the field.

GREEN CHEMISTRY (2022)

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Article Chemistry, Physical

Cost effective and facile low temperature hydrothermal fabrication of Cu2S thin films for hydrogen evolution reaction in seawater splitting

T. Marimuthu et al.

Summary: Electrolysis of seawater for hydrogen production is an attractive approach for renewable energy technologies. In this study, Cu2S electrocatalyst was fabricated on Ni foam using a low temperature hydrothermal growth method. The Cu2S catalyst grown for 1 hour exhibited low overpotentials and superior electrocatalytic behavior for hydrogen evolution reaction in both deionized water and seawater. The results suggest that the cost-effective and low temperature fabrication of Cu2S electrocatalyst holds great potential for large-scale seawater splitting.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2022)

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Article Energy & Fuels

Nickel-Based Electrocatalysts for Water Electrolysis

Zuraya Angeles-Olvera et al.

Summary: Currently, there is a need to develop alternative methods for hydrogen production due to the emission of pollutants from the current reforming process. Water electrolysis, which does not produce carbon-based pollutants, is an ideal option for large-scale hydrogen production. However, the current electrocatalysts required for water electrolysis are expensive noble metals, making them inaccessible for industrial applications. Nickel-based electrocatalysts, which are economically accessible, have been extensively researched for hydrogen and oxygen evolution. The review of recent progress in this field provides valuable insights for the development of efficient nickel-based electrocatalysts.

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Water Resources Liability Measurement and the Driving Factors of Water Resources Liability Intensity

Dan-dan Zhang et al.

Summary: This study examines water resources liability (WRL) and water resources liability intensity (WLI). It finds that the total amount of WRL in China has decreased, indicating improved water use efficiency. There are spatial differences in WLI, with higher WLI in the western region and lower WLI in the eastern region. The urbanization rate and degree of economic openness significantly drive the reduction of WLI.

WATER RESOURCES MANAGEMENT (2022)

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Article Chemistry, Physical

High Selectivity Electrocatalysts for Oxygen Evolution Reaction and Anti-Chlorine Corrosion Strategies in Seawater Splitting

Shanshan Jiang et al.

Summary: Seawater is an abundant and clean hydrogen resource, and direct electrolysis using renewable energy is a promising technology for hydrogen production. However, challenges such as chlorine corrosion and low oxygen selectivity need to be addressed. Researchers are focusing on developing efficient and corrosion-resistant electrocatalysts for seawater splitting.

CATALYSTS (2022)

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Article Energy & Fuels

Highly active bifunctional electrocatalyst: Nanoporous (Ni,Co)0.85Se anchored on rGO for water and hydrazine oxidation

Zhongbao Feng et al.

Summary: The bifunctional (Ni,Co)(0.85)Se/rGO catalyst fabricated via electrodeposition shows superior electrocatalytic activity and stability towards hydrazine electrooxidation and oxygen evolution reaction. Its advantages include high electrochemical surface area, high electrical conductivity, and rapid release of bubbles from electrode surface. This study presents a versatile, cost-effective, and industrial strategy for producing highly active catalysts.

INTERNATIONAL JOURNAL OF ENERGY RESEARCH (2022)

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Article Chemistry, Physical

Synthesis of bristlegrass-like Co-doped Ni2P composites on Ni foam for overall seawater splitting

Xiangfei Sun et al.

Summary: Seawater, as the most abundant resource on earth, requires the development of efficient electrocatalysts for seawater splitting. This study presents the synthesis of a unique morphological Co-Ni2P composite with excellent electrocatalytic activity and stability.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2022)

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Review Chemistry, Physical

Recent advances in electrocatalysts for seawater splitting in hydrogen evolution reaction

Jiao Li et al.

Summary: This review examines the mechanisms, challenges, and recent progress in electrocatalytic seawater splitting for H-2 production, and provides suggestions for future work.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2022)

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Article Nanoscience & Nanotechnology

Cobalt Molybdenum Nitride-Based Nanosheets for Seawater Splitting

Xiang Wang et al.

Summary: This article reports a simple approach for preparing nitride composite materials using a metal-organic framework sacrificial template, and demonstrates the excellent catalytic performance and corrosion resistance of these composite materials in seawater splitting. By supporting cobalt molybdenum nitride catalyst on nitrogen-doped carbon nanosheets, high current density can be achieved at low overpotentials, providing potential for cost-effective implementation of water electrolysis technology.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Review Environmental Sciences

Assessing the Role of Water Resources Protection Practice for Sustainable Water Resources Management: A Review

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Summary: This review paper focuses on groundwater and surface water protection in South Africa and proposes a novel policy monitoring framework to improve sustainable water resource utilization in the country.

WATER (2022)

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Review Nanoscience & Nanotechnology

Strategies of Anode Design for Seawater Electrolysis: Recent Development and Future Perspective

Tanveer ul Haq et al.

Summary: This review discusses the additional challenges of seawater electrolysis compared to freshwater splitting and summarizes the current effective strategies. It provides insights for the rational design of high-performance anodes and proposes a perspective on the fabrication of high-performance anodes for direct seawater electrolysis.

SMALL SCIENCE (2022)

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Review Chemistry, Applied

Recent advances in spinel-type electrocatalysts for bifunctional oxygen reduction and oxygen evolution reactions

Xiao-Meng Liu et al.

Summary: The demand for efficient and environmentally-benign electrocatalysts is rapidly increasing, with a focus on high-performance bifunctional oxygen electrocatalysts. Spinel-type catalysts, with their versatility and advantages, have garnered attention in the field. This review provides insights into the design of spinel-type bifunctional oxygen electrocatalysts, emphasizing the relationship between structure and property.

JOURNAL OF ENERGY CHEMISTRY (2021)

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Review Chemistry, Multidisciplinary

Design Strategies of Transition-Metal Phosphate and Phosphonate Electrocatalysts for Energy-Related Reactions

Hui Zhao et al.

Summary: Transition-metal phosphates and phosphonates have shown great potential for designing efficient electrocatalysts due to their flexible coordination and diverse orientations, but challenges such as low intrinsic catalytic efficiency and electronic conductivity still need to be addressed.

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Article Nanoscience & Nanotechnology

Early Transition-Metal-Based Binary Oxide/Nitride for Efficient Electrocatalytic Hydrogen Evolution from Saline Water in Different pH Environments

Ahmed Badreldin et al.

Summary: The study focuses on using abundant seawater for hydrogen production through electrocatalytic water splitting, but highlights challenges related to seawater's effects on stability and activity of hydrogen evolution reaction (HER) electrocatalysts. The synthesized binary metallic core-sheath nitride@oxynitride electrocatalysts show promising advancements in HER performance in saline water, especially under near-neutral pH conditions. Doping early transition metals in nickel oxynitrides aids in accelerating the rate-determining H2O dissociation step and suppressing chloride deactivation, leading to stable performance even at high current densities in a neutral saline electrolyte.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Efficient Hydrogen Evolution of Oxidized Ni-N3 Defective Sites for Alkaline Freshwater and Seawater Electrolysis

Wenjie Zang et al.

Summary: In the study, atomically dispersed Ni with triple nitrogen coordination (Ni-N-3) was shown to achieve efficient hydrogen evolution reaction (HER) performance in alkaline media. These catalysts exhibited overpotentials as low as 102 and 139 mV at 10 mA cm(-2) in alkaline freshwater and seawater electrolytes, respectively, outperforming previously reported results.

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Article Chemistry, Physical

Rational design of core-shell-structured CoPx@FeOOH for efficient seawater electrolysis

Libo Wu et al.

Summary: The core-shell-structured CoPx@FeOOH catalyst designed for seawater electrolysis for hydrogen generation demonstrates excellent catalytic activity, high conductivity, large surface area, improved turnover frequency, optimal absorption energy to OER intermediates, enhanced chemical stability, and corrosion resistance. The CoPx||CoPx@FeOOH pair also shows great promise for fuel-gas production from seawater, with high Faradaic efficiency and low overpotentials required for certain current densities.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Chemistry, Physical

Sulfur-incorporated nickel-iron layered double hydroxides for effective oxygen evolution reaction in seawater

Sun Young Jung et al.

Summary: The research demonstrates that sulfur-incorporated nickel-iron layered double hydroxide can serve as an effective catalyst for seawater oxidation, showing high catalytic activity and corrosion resistance.

APPLIED SURFACE SCIENCE (2021)

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Article Chemistry, Applied

S and Co co-doped Cu3P nanowires self-supported on Cu foam as an efficient hydrogen evolution electrocatalyst in artificial seawater

Ni Wang et al.

Summary: The S&Co-Cu3P nanowires exhibit excellent hydrogen evolution activity in neutral conditions, with a unique structure, rich active sites, and improved conductivity and stability with a binder-free electrode. The use of seawater as an alternative neutral electrolyte is highly feasible, providing a sustainable and cost-effective option for green hydrogen production.

JOURNAL OF POROUS MATERIALS (2021)

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Article Chemistry, Physical

Modulating Interfacial Charge Density of NiP2-FeP2 via Coupling with Metallic Cu for Accelerating Alkaline Hydrogen Evolution

Ashwani Kumar et al.

Summary: This study successfully developed a NiP2-FeP2/Cu-NW/Cu-f catalyst with superior alkaline HER activity, surpassing the state-of-the-art Pt catalyst. The research also demonstrated that designing catalysts with rich interfaces can enhance the HER reaction.

ACS ENERGY LETTERS (2021)

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Article Chemistry, Physical

Synergism on Electronic Structures and Active Edges of Metallic Vanadium Disulfide Nanosheets via Co Doping for Efficient Hydrogen Evolution Reaction in Seawater

Mengxuan Zhao et al.

Summary: The study introduces Co-doped metallic VS2 nanosheets as superior catalysts for hydrogen evolution from seawater, with abundant active sites and desirable catalytic performance. In simulated seawater, the Co-doped VS2 nanosheets with 10% V substituted by Co exhibit excellent catalytic performance and long-term stability.

CHEMCATCHEM (2021)

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Article Chemistry, Physical

Selective anodes for seawater splitting via functionalization of manganese oxides by a plasma-assisted process

Lorenzo Bigiani et al.

Summary: Through a specific material combination, selective triggering of oxygen generation and reduction of chlorine production in seawater has been achieved. The combination of MnO2 and Co3O4 performs the best in alkaline seawater splitting, showing significant results.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Chemistry, Multidisciplinary

Facing Seawater Splitting Challenges by Regeneration with Ni-Mo-Fe Bifunctional Electrocatalyst for Hydrogen and Oxygen Evolution

Carles Ros et al.

Summary: Efficient and earth-abundant electrodes are fabricated in this study to address the challenges of using real seawater for hydrogen production. The Ni-Mo-Fe trimetallic electrocatalyst shows promising electrochemical performance in both seawater and alkaline conditions, with high productivities and low voltages for water splitting. The proposed electrode regeneration method effectively dissolves undesired CaCO3 deposition, making seawater splitting economically feasible with high energy efficiency.

CHEMSUSCHEM (2021)

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Review Engineering, Chemical

An overview and recent advances in electrocatalysts for direct seawater splitting

Hao-Yu Wang et al.

Summary: Compared to pure water, seawater is considered an unlimited resource for direct electrolysis. However, challenges such as chlorine-related competing reactions and various impurities hinder its practical application. The development of efficient electrocatalysts is crucial for addressing these challenges and advancing the technology of direct seawater splitting.

FRONTIERS OF CHEMICAL SCIENCE AND ENGINEERING (2021)

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Article Green & Sustainable Science & Technology

Tapping hydrogen fuel from the ocean: A review on photocatalytic, photoelectrochemical and electrolytic splitting of seawater

Fons Dingenen et al.

Summary: Direct splitting of earth-abundant seawater for hydrogen production faces challenges in selectivity and stability. While direct seawater electrolysis is a well-established technology, light-driven processes like photocatalytic and photoelectrochemical seawater splitting show promise in utilizing renewable solar power. Advances in solar-to-hydrogen efficiencies have been made, reaching around 2% over the past decade.

RENEWABLE & SUSTAINABLE ENERGY REVIEWS (2021)

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Article Chemistry, Applied

High-precision regulation synthesis of Fe-doped Co2P nanorod bundles as efficient electrocatalysts for hydrogen evolution in all-pH range and seawater

Yan Lin et al.

Summary: The study prepared Fe-Co2P bundle of nanorods as a catalyst for the hydrogen evolution reaction in seawater electrolysis, with Fe doping improving the overall reaction performance across the pH range. The Fe-Co2P BNRs exhibited higher catalytic activity compared to 20% Pt/C in seawater at high potentials.

JOURNAL OF ENERGY CHEMISTRY (2021)

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Article Energy & Fuels

A Synergistic Combination of P-doped Zn0.5Cd0.5S and CoP for Dual-Stage Electron Trapping and Its Application in Seawater Splitting

Yi-Hao Chew et al.

Summary: A photocatalytic system combining P-doped Zn0.5Cd0.5S (pZCS) and noble-metal-free CoP was developed to significantly enhance the photocatalytic hydrogen evolution reaction (HER) in seawater, with the synergistic relation between pZCS and CoP playing a crucial role. The system achieved remarkable HER activity in seawater due to the midgap states generated by P dopant, which effectively hindered charge carrier recombination and facilitated rapid assembly of photogenerated electrons in CoP, ultimately enabling a spectacular photocatalytic HER in seawater.

SOLAR RRL (2021)

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Article Chemistry, Physical

Preferential Adsorption of Hydroxide Ions onto Partially Crystalline NiFe-Layered Double Hydroxides Leads to Efficient and Selective OER in Alkaline Seawater

Qingqing Tu et al.

Summary: A NiFe-LDH catalyst with partially crystalline characteristics was synthesized, showing high catalytic activity and stability during seawater electrolysis. The presence of more boundaries in the partially crystalline NiFe-LDH contributes to its higher catalytic efficiency and stability in alkalized seawater.

ACS APPLIED ENERGY MATERIALS (2021)

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Review Energy & Fuels

Mini Review on Electrocatalyst Design for Seawater Splitting: Recent Progress and Perspectives

Shan-Chao Ke et al.

Summary: This review summarizes recent advances in the rational design of electrocatalysts for seawater splitting, including constructing hierarchical structures, decorating corrosion resistance layers, and introducing charge redistribution within the system, to address the challenges of seawater complexity. Additionally, a perspective on the development of large-scale seawater electrolysis for hydrogen production is proposed.

ENERGY & FUELS (2021)

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Review Chemistry, Analytical

Electrochemical (bio)sensors based on carbon cloth and carbon paper: An overview

Alvaro Torrinha et al.

Summary: Carbon cloth and carbon paper possess unique characteristics suitable for designing efficient and disposable electrochemical sensors, enabling rapid detection of biomolecules and hazardous compounds. Their easy integration and portability make them promising for point-of-care diagnostics and in-situ measurements.

TRAC-TRENDS IN ANALYTICAL CHEMISTRY (2021)

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Article Chemistry, Physical

Adapting Early Transition Metal and Nonmetallic Dopants on CoFe Oxyhydroxides for Enhanced Alkaline and Neutral pH Saline Water Oxidation

Ahmed Badreldin et al.

Summary: This study synthesized two oxyhydroxide electrocatalysts using a simple method, enhancing their activity and stability in saline electrolysis, potentially leading to the commercialization of seawater electrolysis.

ACS APPLIED ENERGY MATERIALS (2021)

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Article Chemistry, Physical

Stabilizing oxygen intermediates on redox-flexible active sites in multimetallic Ni-Fe-Al-Co layered double hydroxide anodes for excellent alkaline and seawater electrolysis

Enkhbayar Enkhtuvshin et al.

Summary: Multimetallic Ni-Fe-Al-Co LDHs, such as NFAC-MELDHs, are considered as one of the best catalysts for alkaline and seawater oxidation due to synergistic effects among four different redox-flexible metals; NFAC-MELDHs prepared via metal-organic framework and hydrothermal reaction exhibit relatively low overpotentials, demonstrating good activity and stability in electrocatalysis for the OER; The study suggests that designing LDHs using multimetals is a highly promising strategy, with activity and stability improving in the sequence of unary, binary, ternary, and quaternary LDHs.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Inorganic & Nuclear

Sulfur doped FeOx nanosheet arrays supported on nickel foam for efficient alkaline seawater splitting

Weiju Hao et al.

Summary: In this study, sulfur-doped iron oxide nanosheet arrays supported on nickel foam were prepared by a one-pot solvothermal reaction, demonstrating excellent bifunctional catalytic performance in alkaline simulated seawater. The developed electrode showed low overpotentials and high Faraday efficiency, providing a promising strategy for efficient hydrogen production from seawater.

DALTON TRANSACTIONS (2021)

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Review Chemistry, Multidisciplinary

Lattice oxygen redox chemistry in solid-state electrocatalysts for water oxidation

Ning Zhang et al.

Summary: The lattice oxygen-mediated mechanism (LOM) derived from lattice oxygen redox chemistry is playing a significant role in solid-state OER electrocatalysts, providing insights into intrinsic activity and surface reconstruction issues, guiding the exploration of efficient electrocatalysts. Strategies for triggering lattice oxygen redox chemistry to promote intrinsic OER activity, along with theoretical calculations and experimental measurements, are crucial in this research area.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Review Chemistry, Multidisciplinary

Recent progress in water-splitting electrocatalysis mediated by 2D noble metal materials

Lin Tian et al.

Summary: Two-dimensional nanostructures have enabled noble-metal-based nanomaterials to be promising electrocatalysts towards overall water splitting, with inherent structural advantages and beneficial electronic and strain effects. The review highlights the recent progress in advanced electrocatalysts based on 2D noble-metal-based nanomaterials and discusses water-splitting mechanisms, engineering strategies, challenges, and structural merits of 2D nanostructures. Additionally, representative water-splitting electrocatalysts are discussed to showcase the superiorities of 2D noble-metal-based nanomaterials for electrochemical water splitting, while also addressing underlying challenges and future opportunities.

NANOSCALE (2021)

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Review Chemistry, Multidisciplinary

Layered double hydroxide-based electrocatalysts for the oxygen evolution reaction: identification and tailoring of active sites, and superaerophobic nanoarray electrode assembly

Daojin Zhou et al.

Summary: Understanding the structure and active sites of LDHs is crucial for designing and regulating high-performance electrocatalysts. Recent advancements and strategies for enhancing OER activity in LDHs, such as doping, intercalation, and defect-making, are discussed in this review. The concept of superaerophobicity and certain operating standards for OER measurements are also highlighted to improve the performance of LDHs in large scale water splitting applications.

CHEMICAL SOCIETY REVIEWS (2021)

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Article Materials Science, Multidisciplinary

Self-assembly of functionalized Echinops-like Rh porous nanostructure electrocatalysts for highly efficient seawater splitting

Xue Jiang et al.

Summary: This study successfully synthesized novel polyethyleneimine (PEI) functionalized Echinops-like Rh porous nanostructures with high efficiency in both hydrogen and oxygen evolution reactions under neutral conditions. The structures exhibited excellent stability and enhanced activity compared to commercial catalysts, showing potential for improving the efficiency of seawater splitting.

JOURNAL OF MATERIALS CHEMISTRY C (2021)

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Article Chemistry, Multidisciplinary

Carbon nanopore and anchoring site-assisted general construction of encapsulated metal (Rh, Ru, Ir) nanoclusters for highly efficient hydrogen evolution in pH-universal electrolytes and natural seawater

Rong Ding et al.

Summary: Utilizing nitrogen-doped hollow carbon spheres as supporting matrices, well-distributed and ligand-free metal nanoclusters (NCs) were successfully synthesized for efficient hydrogen evolution in various electrolytes. Among them, Rh/NHCSs exhibited superior electrocatalytic activity, stability, and long-term durability in the whole pH range, outperforming commercial Pt/C and most previously reported catalysts. This work proposes a simple and effective method to fabricate highly dispersed MNCs with high performance for pH-universal water/seawater splitting.

GREEN CHEMISTRY (2021)

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Article Chemistry, Physical

NixFeyN@C microsheet arrays on Ni foam as an efficient and durable electrocatalyst for electrolytic splitting of alkaline seawater

Boran Wang et al.

Summary: The study investigates the use of self-supported nickel-iron nitride microsheet arrays coated with carbon as an electrocatalyst for splitting alkaline seawater. The results show that the catalyst exhibits superior durability and efficient electrolysis performance, making it a promising candidate for hydrogen production from seawater electrolysis.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Physical

High-performance anion exchange membrane alkaline seawater electrolysis

Yoo Sei Park et al.

Summary: A Ni-doped FeOOH anode was developed for high-efficiency anion exchange membrane alkaline seawater electrolysis, showing good catalytic activity in half-cell tests and higher performance in 1.0 M KOH + seawater. The anion exchange membrane electrolyzer catalyzed by Ni-doped FeOOH exhibited a high current density and energy conversion efficiency in seawater conditions.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Review Chemistry, Multidisciplinary

Advances in hydrogen production from electrocatalytic seawater splitting

Cheng Wang et al.

Summary: Seawater is a promising electrolyte for industrial hydrogen production and refining of edible salt. Efficient and stable electrocatalysts are essential for water electrolysis, leading to significant achievements in recent years.

NANOSCALE (2021)

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Article Chemistry, Multidisciplinary

A general MOF-intermediated synthesis of hollow CoFe-based trimetallic phosphides composed of ultrathin nanosheets for boosting water oxidation electrocatalysis

Cheng Wang et al.

Summary: Hollow CoFeM trimetallic phosphides prepared through MOF-mediated synthesis exhibit superior electrocatalytic performance for the oxygen evolution reaction (OER). Bi and P doping optimizes the electronic structure of Co and Fe, reducing the adsorption energy of oxygen intermediates. The hollow microsphere structure provides rich surface active sites to enhance the OER electrocatalysis.

NANOSCALE (2021)

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Article Chemistry, Physical

Bifunctional Pt-Co3O4 electrocatalysts for simultaneous generation of hydrogen and formate via energy-saving alkaline seawater/methanol co-electrolysis

Kun Xiang et al.

Summary: The study demonstrates an organic-oxidation-assisted strategy to suppress the undesired oxygen evolution reaction and chlorine evolution reaction during seawater electrocatalytic splitting, leading to simultaneous hydrogen and formate generation with low energy consumption. The integrated two-electrode electrolyzer using Pt-Co3O4/CP bifunctional electrocatalysts shows high efficiency and durability in producing hydrogen and formate simultaneously.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Multidisciplinary

Construction of self-supporting, hierarchically structured caterpillar-like NiCo2S4 arrays as an efficient trifunctional electrocatalyst for water and urea electrolysis

Wenjiao Song et al.

Summary: In this study, self-supporting caterpillar-like spinel NiCo2S4 arrays are developed for the oxygen evolution reaction (OER), hydrogen evolution reaction (HER), and urea oxidation reaction (UOR). The bimetallic synergistic effect, unique hierarchical nanostructure, and self-supporting nature contribute to the high activities of the NiCo2S4/CC electrode. Electrolysis experiments demonstrate its excellent performance in both water electrolysis and urea electrolysis for hydrogen production.

NANOSCALE (2021)

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Review Chemistry, Physical

Seawater electrocatalysis: activity and selectivity

Sakila Khatun et al.

Summary: Seawater is considered a major hydrogen reservoir, but the presence of multielements and interference in electrochemistry, particularly chlorine chemistry, make electrocatalytic water splitting challenging. To achieve sustainable seawater electrolysis, focus should not only on electrocatalyst activity but also on selective oxygen evolution reaction to suppress corrosive chlorine chemistry.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Review Chemistry, Physical

Seawater electrocatalysis: activity and selectivity

Sakila Khatun et al.

Summary: Seawater is considered a major hydrogen reservoir, but the presence of multiple elements and interference in electrochemistry, especially chlorine chemistry, make seawater electrolysis challenging. To make seawater electrolysis sustainable, efficient oxygen evolution reaction and suppression of corrosive chlorine chemistry by electrocatalysts are highly desirable.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Physical

Heterogeneous lamellar-edged Fe-Ni(OH)2/Ni3S2 nanoarray for efficient and stable seawater oxidation

Baihua Cui et al.

Summary: The study presents a heterostructure of Ni3S2 nanoarray with Fe-Ni(OH)(2) edges for efficient catalysis in seawater electrolysis, demonstrating high Faraday efficiency for oxygen evolution reaction and good stability. The introduction of Fe activator and heterostructure design offer massive active and selective sites, providing insights for the rational design of high-performance Fe-based electrodes for industrial seawater electrolysis.

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Active and stable graphene supporting trimetallic alloy-based electrocatalyst for hydrogen evolution by seawater splitting

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Electrocatalytic Selective Oxygen Evolution of Carbon-Coated Na2Co1-xFexP2O7 Nanoparticles for Alkaline Seawater Electrolysis

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ACS CATALYSIS (2020)

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Electronic modulation of cobalt phosphide nanosheet arrays via copper doping for highly efficient neutral-pH overall water splitting

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Oxygen-Defect-Rich Cobalt Ferrite Nanoparticles for Practical Water Electrolysis with High Activity and Durability

Bharati Debnath et al.

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Metal-organic frameworks derived carbon-incorporated cobalt/dicobalt phosphide microspheres as Mott-Schottky electrocatalyst for efficient and stable hydrogen evolution reaction in wide-pH environment

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JOURNAL OF COLLOID AND INTERFACE SCIENCE (2020)

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Hydrogen Generation from Seawater Electrolysis over a Sandwich-like NiCoNINixPINiCoN Microsheet Array Catalyst

Luo Yu et al.

ACS ENERGY LETTERS (2020)

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Article Energy & Fuels

Efficient hydrogen production from solar energy and fossil fuel via water- electrolysis and methane-steam-reforming hybridization

Jiyuan Sui et al.

APPLIED ENERGY (2020)

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