☆ 4.7 Review

Unlocking the potential of metal-organic frameworks-based mixed matrix membranes for hydrogen separation and purification

JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY (2023)

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Article Energy & Fuels

In-situ interfacial crosslinking of NH2-MIL-53 and polyimide in MOF-incorporated mixed matrix membranes for efficient H2 purification

Yan Jia et al.

Summary: The key to avoiding degradation of gas separation performance in mixed matrix membranes (MMMs) is to enhance the interfacial compatibility between fillers and the polymer matrix. This study introduces a method of preparing MMMs by crosslinking metal organic frameworks (MOF) and polyamic acid (PAA) to improve interfacial force and compatibility, leading to enhanced H2/CO2 separation. The resulting MMMs loaded with 30 wt% MOF exhibit high H2 permeability (384.1 Barrer) and H2/CO2 selectivity (16.7), surpassing the 2008 Robeson upper bound. These membranes also show improved mechanical properties and long-term stability. This work highlights the potential of in-situ cross-linking strategies to enhance membrane performance for gas separation applications.

FUEL (2023)

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Review Energy & Fuels

Mixed matrix membranes for H2/CO2 gas separation- a critical review

Fayez Nasir Al-Rowaili et al.

Summary: Membrane technology plays a significant role in the separation processes of modern industries, especially in gas separation. Mixed matrix membranes (MMMs) have been widely studied and applied to improve the gas separation performance. This paper reviews the choice of advanced materials, recent research developments, and applications of MMMs in gas separation, with a focus on H2/CO2.

FUEL (2023)

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Article Engineering, Chemical

In-situ etching MOF nanoparticles for constructing enhanced interface in hybrid membranes for gas separation

Huiyuan Jiao et al.

Summary: Metal-organic frameworks (MOFs) based hybrid membranes with nearly defect-free interfaces were constructed through a distinctive interfacial design strategy via in-situ etching ZIF-8 nanoparticles. The hybrid membranes exhibited enhanced permeability and selectivity, surpassing the upper bound of 2008 and approaching the upper bound of 2015 for several gas pairs. The CO2 plasticization resistance also achieved significant improvement. This work provides an effective and robust strategy to enhance the interfacial compatibility of hybrid membranes.

JOURNAL OF MEMBRANE SCIENCE (2023)

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Article Chemistry, Multidisciplinary

Challenges in Developing MOF-Based Membranes for Gas Separation

Dun-Yen Kang et al.

Summary: This article discusses the challenges for the future development of MOF-based membranes based on past research, including the overstudy of certain MOF compounds, the lack of correlation between gas adsorption and diffusion in MOFs, and the importance of characterizing gas distribution in MOFs. For MOF-based mixed matrix membranes, engineering the MOF-polymer interface is crucial and defect engineering is proposed as an efficient approach for enhancing the interfacial morphology and achieving desired gas separation performance.

LANGMUIR (2023)

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Review Energy & Fuels

Issues and challenges in hydrogen separation technologies

Muhammad Amin et al.

Summary: Depleting energy resources, global warming, and environmental problems call for the substitution of conventional fuels with more efficient and sustainable resources. Hydrogen (H2) has emerged as the ultimate choice due to its low carbon emissions, cleanliness, and efficiency. However, the production, separation, and storage of H2 pose challenges that need to be addressed. This paper provides a comprehensive review of the issues and challenges in the separation of H2 using various technologies, with a focus on membrane technology as the most promising method.

ENERGY REPORTS (2023)

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Article Engineering, Chemical

Performance optimization of imidazole containing copolyimide/functionalized ZIF-8 mixed matrix membrane for gas separations

Xiya Yuan et al.

Summary: The combination of functionalized metal organic frameworks with a polymer with structural similarity is a feasible route to enhance binary phase adhesion of hybrid membranes. The incorporation of amine-modified ZIF-8 with a permeable imidazole-containing copolyimide produces compatible mixed matrix membranes (MMMs) with optimized gas separation performance. The hydrogen bonding created between amine groups and the polymer matrix significantly improves interfacial adhesion and leads to increased membrane permeability, thermal stability, and gas selectivity, especially under sub-ambient temperatures for CO2/CH4 and H-2/CH4 separations.

JOURNAL OF MEMBRANE SCIENCE (2022)

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Article Engineering, Chemical

Insights into the progress of polymeric nano-composite membranes for hydrogen separation and purification in the direction of sustainable energy resources

Nishel Saini et al.

Summary: This paper analyzes key rules regarding material engineering and separation mechanisms for improved hydrogen separation membranes, focusing on using different polymer membrane materials to design matrices with better characteristics. Research suggests that polymer nanocomposite membranes have the potential to compete with conventional methods.

SEPARATION AND PURIFICATION TECHNOLOGY (2022)

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Article Engineering, Chemical

Polyimide/ZIFs mixed matrix membranes with tunable interfacial interaction for efficient gas separation

Yan Liu et al.

Summary: Adjusting the functionality of fillers and polyimides enables precise control of membrane interfacial bonding behavior, resulting in a high-performance mixed matrix membrane with tunable separation performance.

JOURNAL OF MEMBRANE SCIENCE (2022)

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Article Materials Science, Multidisciplinary

Capturing CO2 by a Fixed-Site-Carrier Polyvinylamine-/Matrimid-Facilitated Transport Membrane

Wrya Aframehr et al.

Summary: Facilitated transport membranes based on polyimide and polyvinyl amine are fabricated and their gas separation performance is studied by incorporating silica nanoparticles. The results show that the addition of polyvinyl amine and silica can greatly enhance the permeance and selectivity of CO2.

ACS APPLIED POLYMER MATERIALS (2022)

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Article Chemistry, Applied

Activated carbon in mixed-matrix membranes

Jeremy Lewis et al.

Summary: This review critically analyzes the state-of-the-art on using activated carbon (AC) as a filler in mixed matrix membranes (MMMs), covering aspects such as AC fabrication, MMM fabrication, properties, and performance. It also discusses various applications and predictive models specifically utilized for AC-MMMs.

SEPARATION AND PURIFICATION REVIEWS (2021)

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Article Nanoscience & Nanotechnology

Constructing Strong Interfacial Interactions under Mild Conditions in MOF-Incorporated Mixed Matrix Membranes for Gas Separation

Zhenggong Wang et al.

Summary: A study introduced an efficient and less destructive method to cross-link MOFs/PI mixed matrix membranes, significantly improving membrane stability and mechanical strength under relatively mild conditions without destroying membrane structure. The resulting cross-linked membranes showed significantly enhanced CO2 antiplasticization pressure and gas permeability, while also improving gas separation performance.

ACS APPLIED MATERIALS & INTERFACES (2021)

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A review - The development of hollow fibre membranes for gas separation processes

Guoqiang Li et al.

Summary: This article reviews the importance, process and performance of gas separation using hollow fibre membranes. Improvements in gas separation performance of thin film composite hollow fibre membranes can be achieved by modifying coating solutions and adding layers.

INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL (2021)

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Article Chemistry, Physical

Surface and interface engineering in CO2-philic based UiO-66-NH2-PEI mixed matrix membranes via covalently bridging PVP for effective hydrogen purification

S. Ashtiani et al.

Summary: The defect-free mixed-matrix membrane based on PEI matrix with uniformly dispersed UiO-66-NH2 filler shows enhanced CO2/H-2 separation performance with improved polymer-filler interface interactions. The CO2 permeability reached 394 Barrer and the separation factor of 12, surpassing the 2008 Robeson reverse upper bound limit, due to the combination of diffusion-solution mechanism and preferential adsorption of CO2 via reversible reactions with amino groups in the membrane structure.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2021)

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Review Energy & Fuels

Hydrogen Production Technologies: From Fossil Fuels toward Renewable Sources. A Mini Review

Pedro J. Megia et al.

Summary: This study reviews and compares different technologies for hydrogen production using renewable and non-renewable resources. The results show that biomass gasification and steam reforming technologies have promising features in terms of hydrogen yield, energy efficiency, and operational costs.

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Article Chemistry, Multidisciplinary

Delayed Linker Addition (DLA) Synthesis for Hybrid SOD ZIFs with Unsubstituted Imidazolate Linkers for Propylene/Propane and n-Butane/i-Butane Separations

Febrian Hillman et al.

Summary: The delayed linker addition (DLA) synthesis strategy allows for efficient incorporation of Im linkers into ZIF-8 framework, improving gas separation performance. The Im/ZIF-8 synthesized via DLA demonstrates outstanding performance in gas separation.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Review Chemistry, Physical

Advances in hydrogen selective membranes based on palladium ternary alloys

M. Laura Bosko et al.

Summary: This review provides an in-depth analysis of Pd-based ternary alloy membranes for hydrogen separation, focusing on PdAgAu, PdCuAg, and PdCuAu systems. These alloys show improved hydrogen permeability and chemical resistance, with correlations between permeation properties and lattice parameters. Surface segregation behavior is also analyzed in these ternary alloys, even after exposure to CO, CO2, and H2S, indicating the need for further research on developing membranes with improved long-term stability.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2021)

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Article Engineering, Chemical

Mixed matrix membranes with highly dispersed MOF nanoparticles for improved gas separation

Yapeng Shi et al.

Summary: Metal organic frameworks (MOFs) are ideal fillers for preparing mixed matrix membranes (MMMs) due to their molecular sieving property. Highly dispersed ZIF-8 nanoparticles with diameter of around 50 nm were prepared by coating isophthalic dihydrazide (IPD) molecular layer onto their surfaces. The modification of IPD greatly enhances the interfacial affinity between ZIF-8 and 6FDA-Durene polyimide (PI) in MMMs, resulting in improved gas permeation performance.

SEPARATION AND PURIFICATION TECHNOLOGY (2021)

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Review Chemistry, Multidisciplinary

Metal-Organic Framework UiO-68 and Its Derivatives with Sufficiently Good Properties and Performance Show Promising Prospects in Potential Industrial Applications

Xin Ye et al.

Summary: UiO-68 is a Zr-based metal-organic framework with high surface area, exceptional thermal stability, and remaining crystalline at high pressure, making it promising for industrial applications. By adjusting the organic linkers, UiO-68 with desired functionalities can be obtained. UiO-68 and its derivatives have various applications such as catalysts, sorbents, drug delivery, fluorescent probes, and sensors.

CRYSTAL GROWTH & DESIGN (2021)

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Review Chemistry, Multidisciplinary

Zeolitic imidazolate framework membranes for gas separations: Current state-of-the-art, challenges, and opportunities

Mohamad Rezi Abdul Hamid et al.

Summary: This paper presents the latest advances in ZIF membrane processing, focusing on their microstructural features and separation performance, while also providing prospects for future research directions.

JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY (2021)

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Article Engineering, Chemical

Carbon molecular sieve membranes for hydrogen purification from a steam methane reforming process

Linfeng Lei et al.

Summary: Asymmetric carbon molecular sieve (CMS) membranes prepared from cellulose hollow fiber precursors show excellent separation performance and high stability for H2/CO2 separation. A two-stage carbon membrane system is found to be technologically and economically feasible for producing high-purity H2. It is suggested that higher operating temperatures are needed to achieve higher purity hydrogen.

JOURNAL OF MEMBRANE SCIENCE (2021)

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Article Multidisciplinary Sciences

Pre-combustion gas separation by ZIF-8-polybenzimidazole mixed matrix membranes in the form of hollow fibres-long-term experimental study

Adelaida Perea-Cachero et al.

Summary: This study investigates the continuous measurement of H-2/CO2 separation properties of PBI hollow fibers prepared as mixed matrix membranes with MOF ZIF-8 filler. The effects of membrane healing and operation conditions were examined over approximately 51 days, showing H-2 permeance in the 22-17 GPU range with corresponding selectivity values in the 22-32 range.

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Article Chemistry, Physical

Metal organic frameworks for hydrogen purification

Donglai Mao et al.

Summary: High purity hydrogen is crucial for the lifetime of proton exchange membrane fuel cells, but current industrial processes for producing hydrogen are costly and inefficient. Adsorption and membrane technologies, particularly using MOFs, are promising for hydrogen purification. This review summarizes the performance of MOFs in hydrogen purification and discusses the challenges in commercial application.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2021)

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Review Chemistry, Multidisciplinary

Hydrogen separation and purification with MOF-based materials

Dae-Woon Lim et al.

Summary: Hydrogen has emerged as a promising future energy source due to its high energy density and eco-friendly features. However, challenges exist in its production, utilization, and storage, particularly in achieving high purity and separating valuable hydrogen isotopes like deuterium and tritium. Porous crystalline metal-organic frameworks show potential for addressing these challenges with their designable porosity and functionality.

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High-performance gas separation using mixed-matrix composite membranes containing graphene nanoplatelets

Farhang Pazani et al.

Summary: Embedding graphene nanoplatelets into the Pebax selective layer at different concentrations can significantly improve the CO2 permeability and selectivity of MMCMs. The higher aspect ratio of GNPs contributes to more interactions with Pebax and CO2 gas, leading to enhanced gas separation properties.

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Gabriel Bernardo et al.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2020)

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PBI mixed matrix hollow fiber membrane: Influence of ZIF-8 filler over H2/CO2 separation performance at high temperature and pressure

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Zeolite imidazolate framework (ZIF)-based mixed matrix membranes for CO2 separation: A review

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Troger's base mixed matrix membranes for gas separation incorporating NH2-MIL-53(Al) nanocrystals

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High performance composite hollow fiber membranes for CO2/H2 and CO2/N2 separation

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INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2014)

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Physical aging and carbon dioxide plasticization of thin polyimide films in mixed gas permeation

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JOURNAL OF MEMBRANE SCIENCE (2014)

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CO2-selective membranes for hydrogen production and CO2 capture - Part I: Membrane development

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JOURNAL OF MEMBRANE SCIENCE (2014)

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Bicontinuous Zeolitic Imidazolate Framework ZIF-8@GO Membrane with Enhanced Hydrogen Selectivity

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Review Green & Sustainable Science & Technology

Renewable energy resources: Current status, future prospects and their enabling technology

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RENEWABLE & SUSTAINABLE ENERGY REVIEWS (2014)

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Review Polymer Science

State-of-the-art membrane based CO2 separation using mixed matrix membranes (MMMs): An overview on current status and future directions

Mashallah Rezakazemi et al.

PROGRESS IN POLYMER SCIENCE (2014)

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Article Chemistry, Multidisciplinary

A highly permeable mixed matrix membrane containing CAU-1-NH2 for H2 and CO2 separation

Lujie Cao et al.

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Article Engineering, Chemical

Surface Cross-Linking of ZIF-8/Polyimide Mixed Matrix Membranes (MMMs) for Gas Separation

Sumudu N. Wijenayake et al.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2013)

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Review Chemistry, Multidisciplinary

Polymeric mixed matrix membranes containing zeolites as a filler for gas separation applications: A review

Dariush Bastani et al.

JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY (2013)

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Article Chemistry, Applied

Metal organic framework based mixed matrix membranes: An increasingly important field of research with a large application potential

Beatriz Zornoza et al.

MICROPOROUS AND MESOPOROUS MATERIALS (2013)

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Review Multidisciplinary Sciences

The Chemistry and Applications of Metal-Organic Frameworks

Hiroyasu Furukawa et al.

SCIENCE (2013)

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Article Chemistry, Physical

Challenges and opportunities for mixed-matrix membranes for gas separation

Guangxi Dong et al.

JOURNAL OF MATERIALS CHEMISTRY A (2013)

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Challenging fabrication of hollow ceramic fiber supported Cu3(BTC)2 membrane for hydrogen separation

Shuyuan Zhou et al.

JOURNAL OF MATERIALS CHEMISTRY (2012)

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Article Engineering, Chemical

Functionalized metal organic framework-polyimide mixed matrix membranes for CO2/CH4 separation

Omid Ghaffari Nik et al.

JOURNAL OF MEMBRANE SCIENCE (2012)

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Article Engineering, Chemical

High performance ZIF-8/6FDA-DAM mixed matrix membrane for propylene/propane separations

Chen Zhang et al.

JOURNAL OF MEMBRANE SCIENCE (2012)

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Article Chemistry, Physical

Unexpected Molecular Sieving Properties of Zeolitic Imidazolate Framework-8

Chen Zhang et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2012)

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Article Chemistry, Multidisciplinary

Functionalized flexible MOFs as fillers in mixed matrix membranes for highly selective separation of CO2 from CH4 at elevated pressures

Beatriz Zornoza et al.

CHEMICAL COMMUNICATIONS (2011)

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Article Engineering, Chemical

MOF-74 building unit has a direct impact on toxic gas adsorption

T. Grant Glover et al.

CHEMICAL ENGINEERING SCIENCE (2011)

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Article Chemistry, Physical

Oriented Zeolitic Imidazolate Framework-8 Membrane with Sharp H2/C3H8 Molecular Sieve Separation

Helge Bux et al.

CHEMISTRY OF MATERIALS (2011)

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Article Engineering, Chemical

Synthesis, characterization and gas transport properties of MOF-5 membranes

Zhenxia Zhao et al.

JOURNAL OF MEMBRANE SCIENCE (2011)

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Review Chemistry, Multidisciplinary

Synthesis, Structure, and Carbon Dioxide Capture Properties of Zeolitic Imidazolate Frameworks

Anh Phan et al.

ACCOUNTS OF CHEMICAL RESEARCH (2010)

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HKUST-1 membranes on porous supports using secondary growth

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JOURNAL OF MATERIALS CHEMISTRY (2010)

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Influence of temperature on the upper bound: Theoretical considerations and comparison with experimental results

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JOURNAL OF MEMBRANE SCIENCE (2010)

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A three-component mixed-matrix membrane with enhanced CO2 separation properties based on zeolites and ionic liquid materials

Yeny C. Hudiono et al.

JOURNAL OF MEMBRANE SCIENCE (2010)

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Article Chemistry, Multidisciplinary

Steam-Stable Zeolitic Imidazolate Framework ZIF-90 Membrane with Hydrogen Selectivity through Covalent Functionalization

Aisheng Huang et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2010)

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Review Polymer Science

Highly permeable polymers for gas separation membranes

Peter M. Budd et al.

POLYMER CHEMISTRY (2010)

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Review Engineering, Chemical

Performance studies of mixed matrix membranes for gas separation: A review

M. A. Aroon et al.

SEPARATION AND PURIFICATION TECHNOLOGY (2010)

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Review Engineering, Chemical

Membrane Gas Separation: A Review/State of the Art

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INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2009)

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Polymeric membranes for the hydrogen economy: Contemporary approaches and prospects for the future

Lu Shao et al.

JOURNAL OF MEMBRANE SCIENCE (2009)

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Mixed-matrix membranes containing MOF-5 for gas separations

Edson V. Perez et al.

JOURNAL OF MEMBRANE SCIENCE (2009)

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Article Chemistry, Applied

Synthesis of continuous MOF-5 membranes on porous α-alumina substrates

Yunyang Liu et al.

MICROPOROUS AND MESOPOROUS MATERIALS (2009)

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Article Engineering, Chemical

The upper bound revisited

Lloyd M. Robeson

JOURNAL OF MEMBRANE SCIENCE (2008)

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Impact of preparation and handling on the hydrogen storage properties of Zn4O(1,4-benzenedicarboxylate)3 (MOF-5)

Steven S. Kaye et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2007)

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Review Polymer Science

Mixed matrix membranes (MMMs) comprising organic polymers with dispersed inorganic fillers for gas separation

Tai-Shung Chung et al.

PROGRESS IN POLYMER SCIENCE (2007)

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Exceptional chemical and thermal stability of zeolitic imidazolate frameworks

Kyo Sung Park et al.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2006)

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Review Polymer Science

Advanced functional polymer membranes

M Ulbricht

POLYMER (2006)

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Article Chemistry, Multidisciplinary

Very large breathing effect in the first nanoporous chromium(III)-based solids:: MIL-53 or CrIII(OH)•{O2C-C6H4-CO2}•{HO2C-C6H4-CO2H}x•H2Oy

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