期刊
JOURNAL OF HAZARDOUS MATERIALS
卷 460, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.jhazmat.2023.132405
关键词
Septic system; Micropollutant; Endocrine disrupting chemical; Pharmaceuticals and personal care products; Risk assessment; Wastewater
This study is the first comprehensive effort to assess the occurrence of emerging contaminants in the Chesapeake Bay. The results revealed varying concentrations of antibiotics, hormones, UV filters, and sucralose at different locations, some of which were associated with wastewater and septic systems.
Previous studies have reported select contaminants of emerging concern (CECs) in limited areas of the Chesapeake Bay (USA), but no comprehensive efforts have been conducted. In this work, 43 antibiotics, 9 hormones, 11 UV filters, and sucralose, were measured in matched water, sediment, and oyster samples from 58 sites. The highest sucralose concentration was 3051 ng L-1 in a subwatershed with 4.43 million liters of wastewater effluent per day (MLD) and 4385 septic systems. Although antibiotic occurrence was generally low in subwatersheds located in less populated areas, 102 ng L-1 ciprofloxacin was detected downstream of 0.58 MLD wastewater effluent and 10 animal feeding operations. Hormones were not regularly detected in water (2%) or oysters (37%), but the high detection frequencies in sediment (74%) were associated with septic systems. UV filters were ubiquitously detected in oysters, and octisalate exhibited the highest concentration (423 ng g-1). Oyster-phase oxybenzone and aqueous-phase sucralose concentrations were significantly correlated to wastewater effluent and septic systems, respectively. Toxicity outcomes were predicted for homosalate and octisalate throughout the Bay, and antimicrobial resistance concerns were noted for the Chester River. The geospatial and co-occurrence relationships constitute crucial advances to understanding CEC occurrence in the Chesapeake Bay and elsewhere.
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