期刊
CHEMICAL COMMUNICATIONS
卷 51, 期 96, 页码 17104-17107出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cc07455j
关键词
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资金
- Ministry of Science & Technology of Taiwan [MOST-104-2628-M-001-005-MY4]
- Academia Sinica Career Development Award [104-CDA-M08]
para-CH activation of pyridine with allylbenzene is described by Ni/Al cooperative catalysis in combination with a bulkier NHC ligand and a Lewis acid, leading to linear hydroheteroarylation products. Interestingly, the branch selectivity can be achieved by using the combination of a less sterically hindered amino-NHC ligand and AlMe3 through tandem reaction of facile alkene isomerization followed by a slow CH bond activation process.
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