期刊
MICROPOROUS AND MESOPOROUS MATERIALS
卷 224, 期 -, 页码 107-115出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.micromeso.2015.11.034
关键词
Palygorskite; Fluorescence dye; Sol-gel processing; Hybrid fluorescent pigment; Environmental stability
类别
资金
- Xuyi Center of Attapulgite Applied Technology Research Development & Industrialization of the Chinese Academy of Sciences [CASXY2013-02]
- Key Technology R&D Program of Jiangsu [BE2014102]
A new hybrid fluorescent pigment was prepared combining the adsorption of a fluorescent yellow X-10GFF (FY-10G, a coumarin derivative fluorescent dye) on palygorskite (PAL) with the silica encapsulation by the hydrolysis of tetraethoxysilane (TEOS) using acetic acid as catalyst. The photo-stability under UV irradiation and the resistance toward acid, alkali and ethanol of the SiO2@FY-10G/PAL hybrid fluorescent pigments were systematically discussed. The results show that the introduction of PAL not only significantly influences the absorption and fluorescence spectra of the FY-10G, but also enhances the thermal stability of FY-10G due to the supramolecular host/guest interactions. The encapsulation of the silica coating can effectively improve thermal- and photo-stability of FY-10G. Moreover, the fluorescent intensity and the resistance of the hybrid fluorescent pigments to acid and organic solvent enhance with the increase of TEOS concentration. (C) 2015 Elsevier Inc. All rights reserved.
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