期刊
CHEMICAL COMMUNICATIONS
卷 51, 期 26, 页码 5706-5709出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cc00591d
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资金
- Deutsche Forschungsgemeinschaft
Reaction of various alkenes with commercially available N-fluorobenzenesulfonimide (NFSI) and TEMPONa provides the corresponding aminooxygenation products inmoderate to good yields. Single electron transfer from readily generated TEMPONa to NFSI allows for clean generation of the corresponding bissulfonylamidyl radical along with TEMPO. N-radical addition to an alkene and subsequent TEMPO trapping provides the corresponding aminooxygenation product.
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