Polyurethanes Modified by Ionic Liquids and Their Applications

Article Polymer Science

Enhancement of flame retardancy of solid polymer electrolyte based on phosphorus-containing ionic liquid polyurethane membrane for safe lithium batteries

Jia Chen et al.

Summary: Phosphorus-containing flame retardant ionic liquid polyurethane (FR-ILPU) membrane is an effective approach to overcome the defects of polyurethane solid electrolytes and improve the cycling performance and safety of lithium batteries.

POLYMER (2023)

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Article Chemistry, Multidisciplinary

3D Printed Solid Polymer Electrolytes with Bicontinuous Nanoscopic Domains for Ionic Liquid Conduction and Energy Storage

Daniele Melodia et al.

Summary: Tunable solid polymer electrolytes (SPEs) with enhanced mechanical properties and conductivities were prepared via digital light processing 3D printing. The polymerization-induced microphase separation (PIMS) technique allowed for the fabrication of nanostructured ion-conducting materials, with a rigid crosslinked scaffold providing high shear modulus and soft domains containing an ionic liquid contributing to high ionic conductivity. These 3D-printed SPEs are promising for use in all solid energy storage devices, including supercapacitors.

SMALL (2023)

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Article Instruments & Instrumentation

Effect of branched structure on microphase separation and electric field induced bending actuation behaviors of poly(urethane-urea) elastomers

Haibing Zeng et al.

Summary: In this study, branch-structured poly(urethane-urea) elastomers (PUUs) were fabricated to improve bending actuation performance and understand the relationship between structure and electromechanical properties. The results showed that the mechanical loss and bending actuation stress of PUUs were significantly improved by incorporating a small amount of branch structure into the PUU chains. The bending deformation and bending actuation stress of the branch-structured PUUs were 76.3 and 79 times higher than those of the PUUs without branch structure, respectively.

SMART MATERIALS AND STRUCTURES (2023)

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Article Chemistry, Physical

Fabrication of Carboxylic Acid and Imidazolium Ionic Liquid Functionalized Porous Cellulosic Materials for the Efficient Conversion of Carbon Dioxide into Cyclic Carbonates

Yunlong Yang et al.

Summary: Cellulosic poly(ionic liquid)s ([Cellmim][Br]) were successfully synthesized via the transesterification reaction of cellulose with 1-(2-methoxyacetyl)-3-methyl imidazole bromide IL ([Mmim][Br]). The resulting POF-[Cellmim][Br] materials functioned as efficient catalysts for cycloaddition reactions of epoxides and carbon dioxide. The work provided insights into the cooperative effects of porous properties and nucleophilic anions on the reaction.

ACS APPLIED ENERGY MATERIALS (2023)

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Article Materials Science, Composites

Transparent and flexible electromagnetic interference shielding film based on Ag nanowires/ionic liquids/thermoplastic polyurethane ternary composites

Chengbao Wang et al.

Summary: In this study, a simple yet effective method was proposed to fabricate flexible, transparent, and high electromagnetic interference (EMI) shielding films using Ag nanowires (AgNWs)/ionic liquids (ILs)/thermoplastic polyurethane (TPU) ternary composites. The prepared AgNWs/ILs/TPU film exhibited a transmittance of 67% and an EMI shielding effectiveness of about 26.8 dB at 10 GHz, attributed to the low-density but highly interconnected AgNW network and synergistic effect of AgNWs and ILs on composite conductivity. Additionally, the film showed excellent durability and stability in EMI shielding properties even after 1000 bending cycles or exposure to acidic or alkali solutions. These exceptional performances make the prepared film highly promising for flexible and transparent EMI shielding applications.

COMPOSITES COMMUNICATIONS (2023)

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Article Chemistry, Multidisciplinary

Functional Ionic Liquid Polymer Stabilizer for High-Performance Perovskite Photovoltaics

Yunxiu Shen et al.

Summary: The stability-related issues of perovskite precursor inks, films, device structures, and interdependence have not been explored sufficiently. In this study, a ionic-liquid polymer (poly[Se-MI][BF4]) was designed to stabilize the entire device fabrication process. The functional moieties of carbonyl (C=O), selenium (Se+), and tetrafluoroborate (BF4-) ions in the polymer effectively stabilized the lead polyhalide colloids and perovskite precursor inks. The poly[Se-MI][BF4] also suppressed the dissociation and migration of iodine (I-) in perovskite films with the help of anchored selenium ions and passivated defects by BF4-. High efficiencies of 25.10% and 20.85% were achieved by a 0.062-cm(2) device and 15.39-cm(2) module, respectively, with over 90% retention of initial efficiency after 2200 hours of operation.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2023)

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Article Chemistry, Physical

Flexible multisensory sensor based on hierarchically porous ionic liquids/ thermoplastic polyurethane composites

Meiling Peng et al.

Summary: In this study, a lightweight and flexible multisensory sensor based on hierarchically porous ILs/TPU composite was developed. The sensor demonstrated excellent sensing performance, including strain and temperature sensing capabilities, ultra-low detection limit, ultra-wide sensing range, fast response/recovery time, and outstanding durability. This work provides an effective and simple strategy for fabricating high-performance multisensory sensors.

APPLIED SURFACE SCIENCE (2023)

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Article Polymer Science

Design of healable, porous polyurethane with large ionic liquids loading amounts towards ultra-durable pressure sensor

Mingguang Zhang et al.

Summary: A novel porous capacitance pressure sensor with ultra-durability was successfully prepared by impregnating highly conductive ionic liquids into a polyurethane matrix. The sensor exhibited excellent self-healing ability, ultra-absorption ability, good sensitivity, and outstanding antifatigue ability. It also maintained stable electronic signals even after 100 days of storage at room temperature, demonstrating its ultra-durability.

EUROPEAN POLYMER JOURNAL (2023)

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Article Chemistry, Multidisciplinary

High-performance and multifunctional organic field-effect transistors

Yujie Zhao et al.

Summary: Organic field-effect transistors (OFETs) are field-effect transistors that utilize organic semiconductors as channel materials. They are expected to be used in emerging technologies such as wearable electronics, sensors, flexible displays, internet-of-things, and neuromorphic computing due to the advantages of organic materials like solution processability and flexibility. Improving the electrical performance and developing multifunctional OFETs are two major aspects of OFETs research, and progress in one aspect will promote the other, bringing more confidence for future OFETs development. This review summarizes the recent progress in high-performance OFETs and multifunctional OFETs.

CHINESE CHEMICAL LETTERS (2023)

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Article Engineering, Environmental

Scalable anti-infection polyurethane catheters with long-acting and autoclavable properties

Zongpeng Xiu et al.

Summary: In this study, antibacterial catheter materials were prepared by modifying polyurethane with an efficient imidazole ionic liquid-typed cationic antibacterial agent, Mim-BU. The modified materials showed efficient and long-term antibacterial properties against various bacteria, while maintaining good mechanical properties and biocompatibility. The facile synthetic route of the antibacterial agent allowed for large-scale production of the catheters. Animal experiments confirmed the in vivo anti-infection performance of the antibacterial catheters. This study provides a feasible strategy for the development and application of long-term antibacterial catheters.

CHEMICAL ENGINEERING JOURNAL (2023)

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Article Nanoscience & Nanotechnology

Flexible and Transparent Pressure/Temperature Sensors Based on Ionogels with Bioinspired Interlocked Microstructures

Youqun Xu et al.

Summary: This study presents a flexible and transparent skin-like sensor inspired by the interlocked structure of natural skin. It exhibits outstanding pressure and temperature sensing properties, along with antibacterial and strain sensing capabilities. This novel design strategy may inspire future research in the field of e-skin sensors.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Chemistry, Multidisciplinary

A Self-Healing and Ionic Liquid Affiliative Polyurethane toward a Piezo 2 Protein Inspired Ionic Skin

Chao Chen et al.

Summary: A self-healing ionic polyurethane (i-PU) with compatibility and strong interaction is successfully synthesized by using an ionic chain extender containing an ammonium cationic group, allowing for complete self-healing at room temperature. The material demonstrates excellent compatibility and strong interaction through electrostatic interaction and chain diffusion, as proven by low contact angle and DFT calculation.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Article Materials Science, Biomaterials

Highly stretchable, self-healable, and self-adhesive ionogels with efficient antibacterial performances for a highly sensitive wearable strain sensor

Haibo Wang et al.

Summary: A multi-functional ionogel has been developed using Ag-Lignin nanoparticles, polyurethane, and ionic liquids, with excellent mechanical properties, self-healing ability, and favorable antibacterial and UV absorption properties. The sensor based on this ionogel shows good and stable sensing performance, indicating broad application prospects in human movement and personalized physiological health monitoring.

JOURNAL OF MATERIALS CHEMISTRY B (2022)

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Review Polymer Science

Textile-Based Flexible Pressure Sensors: A Review

Jia-wen Zhang et al.

Summary: Textile-based flexible pressure sensors offer promising potential for integration into modern garments and applications in electronic skin, healthcare, and human motion capture. Challenges and prospects in the development of these sensors are also discussed.

POLYMER REVIEWS (2022)

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Review Instruments & Instrumentation

Applications of characterization methods in polyurethane materials: analysis of microphase-separated structures

Qinqin Zhang et al.

Summary: Polyurethanes (PUs) are widely used for their versatile properties of elasticity and hardness, usually with microphase-separated structures. Characterization methods such as FTIR, AFM, DSC, and SAXS are used to study these structures and their relationship with PU properties, laying a theoretical foundation for improving PU application performance.

APPLIED SPECTROSCOPY REVIEWS (2022)

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Article Polymer Science

An antifatigue and self-healable ionic polyurethane/ionic liquid composite as the channel layer for a low energy cost synaptic transistor

Shuai Han et al.

Summary: In this study, a novel ion-conductive transistor with a flexible channel layer made of a synthesized ionic polyurethane and blended with an ionic liquid was successfully constructed. The material exhibited high transparency, stability, antifatigue, and stretchability. The transistor showed good self-healing property and antifatigue performance, making it a promising candidate for flexible electronics.

EUROPEAN POLYMER JOURNAL (2022)

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Review Materials Science, Characterization & Testing

A review of microphase separation of polyurethane: Characterization and applications

Bing-Xu Cheng et al.

Summary: This study summarizes the characterization methods and applications of microphase separation in polyurethane, filling the gap in related research.

POLYMER TESTING (2022)

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Review Nanoscience & Nanotechnology

Biological Effects, Applications and Design Strategies of Medical Polyurethanes Modified by Nanomaterials

Jianrong Wang et al.

Summary: This review summarizes the current applications of nano-modified medical PUs and analyzes the underlying mechanisms for efficiency optimization. It provides insights for the design of novel and appropriate PUs for clinical requirements.

INTERNATIONAL JOURNAL OF NANOMEDICINE (2022)

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Article Nanoscience & Nanotechnology

Liquid-Free Ion-Conducting Elastomer with Environmental Stability for Soft Sensing and Thermoelectric Generating

Rong Zhou et al.

Summary: In this study, a free-liquid ionic conducting elastomer (LFICE) was successfully fabricated, which exhibited superior tensile strength, stretchability, and ionic conductivity. The LFICE also showed sensitive strain and temperature response as well as durable environmental stability. In terms of applications, LFICE demonstrated potential in sensor and thermoelectric generator (TEG), enabling precise detection and energy harvesting.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Chemistry, Multidisciplinary

Integrated Bending Actuation and the Self-Sensing Capability of Poly(Vinyl Chloride) Gels with Ionic Liquids

Zhiwei Liu et al.

Summary: In this study, the integration of bending actuation and capacitance pressure self-sensing is achieved in polyvinyl chloride (PVC) gels by adding a plasticizer and imidazolium type ionic liquids (ILs). The results show that the bending actuation performance and sensing behavior are influenced by the migrability of movable ions from ILs.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Review Chemistry, Applied

Research progress on dielectric properties of PU and its application on capacitive sensors and OTFTs

Sixu Liu et al.

Summary: This paper reviews the research status of polyurethane (PU) as a dielectric layer in electronic devices. It briefly introduces the common preparation methods of the PU dielectric layer, discusses its advantages and existing modification methods. The application of PU as a dielectric layer in capacitive sensors and organic thin film transistors (OTFTs) is highlighted, and the problems faced by the PU dielectric layer and its prospects for future application are summarized.

REACTIVE & FUNCTIONAL POLYMERS (2022)

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Review Materials Science, Characterization & Testing

Ionic liquids as antistatic additives for polymer composites-A review

Szymon Kosinski et al.

Summary: This review article presents the current research on the use of ionic liquids as an antistatic modifier in polymer composites. Static electrification can be dangerous, leading to fire or explosion, but ionic liquids offer a solution to this problem.

POLYMER TESTING (2022)

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Article Chemistry, Multidisciplinary

Highly Conductive and Underwater Stable Ionic Skin for All-Day Epidermal Biopotential Monitoring

Tinglei Chen et al.

Summary: This study designs a highly conductive and optically camouflaged ionic skin for epidermal biopotential monitoring under aquatic circumstances. By capturing ions through fluorine-rich segments, the ionic skin exhibits remarkable ionic conductivity, high optical transmittance, and improved mechanical strength. The epidermal electrode based on this ionic skin accurately measures a variety of electrophysiological signals in both atmospheric and aquatic environments, demonstrating robust and excellent signal quality.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Review Construction & Building Technology

Polyurethane as a modifier for road asphalt: A literature review

Gang Huang et al.

Summary: This paper reviews the research progress of polyurethane as an asphalt modifier for roads, including its advantages, preparation processes, and road performance. It also discusses the research directions and development trends of polyurethane in this field.

CONSTRUCTION AND BUILDING MATERIALS (2022)

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Article Polymer Science

Synergistic and counteractive effects of Bi-component plasticizers on structure and electric field-induced bending actuation behaviors of poly (vinyl chloride) (PVC) gels

Beibei Li et al.

Summary: This study investigates the effect of bi-component plasticizers on the structure, mechanical properties, dielectric properties, and electric field induced dynamic bending actuation behaviors of plasticized PVC gels. The results show that the interactions between plasticizers and PVC chains in PVC gels greatly influence the bending displacement, and the synergistic and counteractive effects between bi-component plasticizers also play an important role in the bending actuation of PVC gels.

POLYMER (2022)

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Article Materials Science, Composites

Highly stretchable, self-healable and self-adhesive polyzwitterion ionogels enabled with binary noncovalent interactions

Hui Song et al.

Summary: This study develops a special material, polyzwitterion ionogels, with large stretchability, fatigue resistance, self-healability, and self-adhesion. The material can be used as an ionic conductor in wearable strain sensors, showing excellent sensing performance.

COMPOSITES COMMUNICATIONS (2022)

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Article Electrochemistry

A high-safety electrolyte based on functionalized ionic liquid and polyurethane for lithium batteries

Li Fang et al.

Summary: A heat-resistant and non-flammable electrolyte was developed by introducing a functionalized ionic liquid into a porous polyurethane matrix. The electrolyte showed high compatibility and good electrochemical performance, maintaining high capacity retention at different temperatures.

ELECTROCHIMICA ACTA (2022)

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Article Thermodynamics

Flame retardant effect of 1-aminoethyl-3-methylimidazolium hexafluorophosphate in thermoplastic polyurethane elastomer

Chuanmei Jiao et al.

Summary: This study found that 1-aminoethyl-3-methylimidazolium hexafluorophosphate ([APMIm]PF6) as a flame retardant additive can significantly improve the flame retardancy of thermoplastic polyurethane elastomer (TPU), reducing heat release rate, smoke density, and promoting the formation of a protective carbon layer.

JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY (2021)

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Review Chemistry, Multidisciplinary

Carbon dioxide capture using liquid absorption methods: a review

Friday O. Ochedi et al.

Summary: Anthropogenic emissions of greenhouse gases lead to global warming, ocean acidification, polar ice melting, sea level rise, droughts, and hurricanes, threatening human health and the global economy. To combat this, cost-effective technologies for CO(2) capture are necessary. Current research focuses on developing more economical, effective, green, and sustainable technologies for CO(2) capture. Various methods based on solutions, solvents, and processes have been explored to enhance CO(2) absorption performance, with a particular interest in incorporating membrane and microencapsulation technologies to improve absorption selectivity.

ENVIRONMENTAL CHEMISTRY LETTERS (2021)

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Article Nanoscience & Nanotechnology

Breathable Strain/Temperature Sensor Based on Fibrous Networks of Ionogels Capable of Monitoring Human Motion, Respiration, and Proximity

Jianwen Chen et al.

Summary: In this study, fibrous mats with IL/TPU ionogels were fabricated using electrospinning technique to develop a high-performance multimodal sensor for strain and temperature sensing. The sensor exhibited wide strain working range, fast response and recovery, low detection limit, high sensitivity, and good breathability. These excellent sensing capabilities make the sensor ideal for monitoring human motions, respiration, and proximity in wearable electronics.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Review Chemistry, Multidisciplinary

Polymer-Based Solid Electrolytes: Material Selection, Design, and Application

Guan Xi et al.

Summary: Polymer-based solid electrolytes (PSEs) have attracted significant interest for high safety and energy density, with the potential to replace liquid electrolytes; PSEs have notable applications in all-solid-state lithium ion batteries, lithium-sulfur batteries, and other areas.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Engineering, Environmental

Self-healing, anti-freezing and highly stretchable polyurethane ionogel as ionic skin for wireless strain sensing

Junhuai Xu et al.

Summary: Ionogel devices based on ILs are important in artificial sensors, wearable devices, and soft robots due to their ability to convert stimuli into electrical signals. The PU ionogel, combining ILs and PU network, shows excellent stretchability, self-healing ability, and high conductivity. It also exhibits high sensitivity to different strains and pressures, and maintains sensing capability even after being stored in extreme conditions.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

Flexible, transparent, and antibacterial ionogels toward highly sensitive strain and temperature sensors

Niu Jiang et al.

Summary: The study introduces a flexible and transparent skin-like sensor, with a wide strain range and fast response time, capable of accurately detecting temperature and exhibiting excellent antibacterial activity.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

Scalable inter-diffused zwitterionic polyurethanes for durable antibacterial coatings

Zixu Huang et al.

Summary: A novel zwitterionic polyurethane (ZPU) was designed to eliminate bacterial attachment on polyurethane (PU) coatings, achieving long-lasting surface hydrophilicity and improved toughness through inter-diffusion with acrylic polyurethane (APU). The enriched ZPU on the coating surface demonstrated superior antibacterial efficacy even after mechanical abrasion, making it feasible for large-scale application on commercial vinyl tarpaulin. The inter-diffused PU coating showed low batch-to-batch deviation and no delamination, indicating its potential for scalable production from laboratory to practical use.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Materials Science, Biomaterials

Thermo-mechanical, antimicrobial and biocompatible properties of PVC blends based on imidazolium ionic liquids

Daniela Zampino et al.

Summary: The study developed antimicrobial PVC blends loaded with different concentrations of two ILs, finding that the addition of low concentrations of ILs had little impact on the thermal and mechanical properties of the blends, while imparting antimicrobial activity and hydrophilicity to the blends.

MATERIALS SCIENCE & ENGINEERING C-MATERIALS FOR BIOLOGICAL APPLICATIONS (2021)

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Article Polymer Science

Effect of multi-armed chain extender on microphase morphology, stress-strain behavior and electromechanical properties of polyurethane elastomers

Yongri Liang et al.

Summary: In this study, the microphase separated morphology of thermoplastic polyurethane elastomers was controlled by adjusting the content of four-armed polycaprolactone chain extenders, leading to a J-shaped stress-strain curve with low modulus and high electromechanical properties. The presence of long-chain branched structure significantly affected the hydrogen bonding and crystallization within the material, influencing its mechanical and actuation properties. The results highlighted the importance of the polymer network structure in exhibiting the desired stress-strain behavior, providing insights for the development of high-performance dielectric polyurethane elastomers.

POLYMER (2021)

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Review Engineering, Chemical

Processes and Properties of Ionic Liquid-Modified Nanofiller/Polymer Nanocomposites-A Succinct Review

Ahmad Adlie Shamsuri et al.

Summary: Ionic liquids can be synthesized using various reactions and have been increasingly used in modifying nanofillers for the fabrication of polymer nanocomposites with improved properties. Four types of imidazolium-based ionic liquids are reviewed as modifiers, along with three types of ionic liquid-modified nanofiller/polymer nanocomposites. The effect of imidazolium-based ionic liquids on the properties of polymer nanocomposites is discussed in this review.

PROCESSES (2021)

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Article Polymer Science

Ionic liquids enhanced performance of PVC gels actuator

Imdad Ali et al.

Summary: This study prepared highly deformable and fast responsive PVC/ILs gel films using ILs, and characterized their properties using various techniques. Loading IL fluorides in PVC gel significantly improved its performance, making it a potential candidate for the fabrication of high-performance artificial muscles and tunable soft actuators.

JOURNAL OF APPLIED POLYMER SCIENCE (2021)

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Review Materials Science, Multidisciplinary

Recent Advances of Flexible Strain Sensors Based on Conductive Fillers and Thermoplastic Polyurethane Matrixes

Tianjiao Chen et al.

Summary: TPU plays a crucial role in flexible strain sensors due to its elastomer-like behavior and ease of combination with conductive materials. By combining different conductive materials, sensors with better stretchability and sensitivity can be designed. The wide applications and multifunctionality of TPU highlight its significance in the design and development of intelligent devices.

ACS APPLIED POLYMER MATERIALS (2021)

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Article Polymer Science

Facilitated phase transformation of PVDF in its composite with an ionic liquid

Huan Zhou et al.

Summary: This study demonstrates that the use of imidazole ionic liquid in composites greatly improves the phase transition ability of PVDF, leading to enhanced phase transition efficiency. During the phase transition, the transformed lamellar morphology depends on the crystallization temperature, while the phase transition efficiency is mainly influenced by the annealing temperature.

POLYMER (2021)

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Article Engineering, Multidisciplinary

Self-healable and recyclable polyurethane-polyaniline hydrogel toward flexible strain sensor

Yuanlai Fang et al.

Summary: The PU-DA-1/1-PANI hydrogel, as a strain sensor, displayed high stretchability, soft modulus, and robust tensile strength. The strain sensors with optimized composition showed ideal conductivity to monitor physical motions precisely, and possess self-healing mechanical performance and conductivity.

COMPOSITES PART B-ENGINEERING (2021)

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Article Materials Science, Composites

Thermoplastic polyurethane/CNT nanocomposites with low electromagnetic resistance property

Chia-Fang Lee et al.

Summary: By adding multi-wall carbon nanotubes to thermoplastic polyurethane, nanocomposites with higher mechanical properties and lower resistance coefficients were obtained. The addition of MWCNTs increased the tensile strength and hardness of the composites, showing potential applications in the electronics industry.

JOURNAL OF COMPOSITE MATERIALS (2021)

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Review Chemistry, Physical

Clays as Inhibitors of Polyurethane Foams' Flammability

Aleksander Hejna

Summary: In the reduction of polyurethane foams' flammability, the incorporation of clays can effectively decrease their combustibility by inducing a labyrinth effect inside the foam, delaying decomposition onset, reducing smoke generation, and inhibiting heat, gas, and mass transfer. Additionally, clays can be easily modified with different organic compounds or used in combination with conventional flame retardants, often resulting in a synergistic effect that significantly reduces the foams' flammability.

MATERIALS (2021)

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Review Chemistry, Multidisciplinary

Flexible Temperature Sensors

Ruping Liu et al.

Summary: Flexible temperature sensors play a crucial role in temperature monitoring, with different types developed based on various principles. Various flexible temperature sensors have been studied and optimized for high integration and multifunctionality. This review delves into the structure, materials, fabrication, and performance of flexible temperature sensors, along with discussing typical applications.

FRONTIERS IN CHEMISTRY (2021)

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Article Materials Science, Multidisciplinary

Active-Matrix-Based Flexible Optical Image Sensor

Yan Xuan et al.

Summary: This study proposes a novel mechanically flexible sensor system that can be utilized for optical imaging and tested for mechanical flexibility, demonstrating successful light distribution mapping under both flat and curved conditions. The flexible sensor system shows promise in advancing light distribution mapping with high resolution and low power consumption.

ADVANCED MATERIALS TECHNOLOGIES (2021)

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Article Chemistry, Multidisciplinary

Hydrogen bond reinforced, transparent polycaprolactone-based degradable polyurethane

Qianyun Zhong et al.

Summary: Transparent and degradable polyurethane elastomers with high strength and toughness are in demand for various applications. This study introduced a facile and efficient strategy by employing imidazolidinyl urea (IU) as a multiple hydrogen-bonding motif to fabricate elastomers with superior breaking strength and toughness. The elastomers showed potential application in post-operative anti-adhesion, with breaking strength reaching up to 49.9 MPa after pre-stretching to 600% strain.

MATERIALS CHEMISTRY FRONTIERS (2021)

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Article Chemistry, Multidisciplinary

A novel catalytic two-step process for the preparation of rigid polyurethane foams: synthesis, mechanism and computational studies

Loredana Maiuolo et al.

Summary: The study developed an innovative, eco-sustainable, and cost-effective method for producing high-quality rigid polyurethane foam. By using a single initial addition of a cheap catalyst, the method proved effective for both the pre-polymer formation and polyurethane chain elongation, while also allowing the salt to be regenerated for a new catalytic cycle during the formation of the final polyurethane.

REACTION CHEMISTRY & ENGINEERING (2021)

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Article Materials Science, Multidisciplinary

Gel-Polymer Electrolytes Based on Poly(lonic Liquid)/lonic Liquid Networks

Sudeshna Sen et al.

Summary: The use of electrically charged, polymerized ionic liquids (polylLs) for developing gel-polymer electrolytes shows promising potential, with polyIL/IL GPEs demonstrating superior electrochemical and thermal stability and up to six times greater conductivity compared to materials based on neutral hosts. The distribution of ionic liquids within the polymers influences the properties of the gel electrolytes, and 3D printing of polyIL/IL gels has been successfully demonstrated in this study as a proof-of-concept.

ACS APPLIED POLYMER MATERIALS (2021)

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Article Chemistry, Physical

A highly stretchable strain sensor with both an ultralow detection limit and an ultrawide sensing range

Hua Li et al.

Summary: A stretchable strain sensor with ultra-low detection limit and ultra-wide sensing range was designed by combining the electrospinning and ultrasonication anchoring technique. The sensor exhibits many outstanding merits, such as fast response time and excellent durability during stretching. Additionally, it shows sensitivity to temperature and humidity, indicating potential applications in temperature and humidity sensors.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Multidisciplinary

Recent Progress in Solid Electrolytes for Energy Storage Devices

Tingting Ye et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Engineering, Chemical

Self-Healable and Remoldable Transparent Polyurethane Film with High Dielectric Constant from the Synergistic Effect between Lithium Salt and Ionic Liquid

Danyi Li et al.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2020)

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Article Chemistry, Multidisciplinary

Electrical and Thermal and Self-Healing Properties of Graphene-Thermopolyurethane Flexible Conductive Films

Ke Wang et al.

NANOMATERIALS (2020)

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Article Nanoscience & Nanotechnology

High-k, Ultrastretchable Self-Enclosed Ionic Liquid-Elastomer Composites for Soft Robotics and Flexible Electronics

Ankit et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Nanoscience & Nanotechnology

Transparent Stretchable Dual-Network Ionogel with Temperature Tolerance for High-Performance Flexible Strain Sensors

Ji Lan et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Nanoscience & Nanotechnology

Temperature Sensor with a Water-Dissolvable Ionic Gel for Ionic Skin

Shunsuke Yamada et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Chemistry, Multidisciplinary

Mechanically Robust, Elastic, and Healable Ionogels for Highly Sensitive Ultra-Durable Ionic Skins

Tianqi Li et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Oligoamine ionic liquids supported on mesoporous microspheres for CO2 separation with good sorption kinetics and low cost

Ming Zhou et al.

JOURNAL OF CO2 UTILIZATION (2020)

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Article Chemistry, Multidisciplinary

Synthesis of Active Graphene with Para-Ester on Cotton Fabrics for Antistatic Properties

Mengting Su et al.

NANOMATERIALS (2020)

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Article Engineering, Chemical

High performance polyamide nanofiltration membranes enabled by surface modification of imidazolium ionic liquid

Binyu He et al.

JOURNAL OF MEMBRANE SCIENCE (2020)

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Review Chemistry, Multidisciplinary

Ion Dissociation in Ionic Liquids and Ionic Liquid Solutions

Oscar Nordness et al.

CHEMICAL REVIEWS (2020)

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Article Polymer Science

Effect of diacylhydrazine as chain extender on microphase separation and performance of energetic polyurethane elastomer

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Summary: Flexible mechanical sensors fabricated primarily by printing technologies have shown unique applications in fields such as robotics, human-machine interfaces, and biomedicine. However, this field is still in its exploratory stage with unclear performance standards and long-term objectives.

NANOSCALE

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Polyurethanes Modified by Ionic Liquids and Their Applications

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