期刊
CHEMICAL COMMUNICATIONS
卷 51, 期 58, 页码 11654-11657出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cc02913a
关键词
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资金
- Major State Basic Research Development Program of China (973 Program) [2012CB822102]
- National High Technology Research and Development Program of China [2012AA021504]
- National Natural Science Foundation of China [21172135, 21372145]
- Development Fund for Collaborative Innovation Center of Glycoscience of Shandong University
- NIH [R01HD065122]
The diversity-oriented chemoenzymatic synthesis of alpha-dystroglycan (alpha-DG) core M1 O-mannose glycans has been achieved via a three-step sequential one-pot multienzyme (OPME) glycosylation of a chemically prepared disaccharyl serine intermediate. The high flexibility and efficiency of this chemoenzymatic strategy was demonstrated for the synthesis of three more complex core M1 O-mannose glycans for the first time along with three previously reported core M1 structures.
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