4.7 Article

Optimisation of recycling process parameters of carbon fibre in epoxy matrix composites

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COMPOSITE STRUCTURES
卷 315, 期 -, 页码 -

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ELSEVIER SCI LTD
DOI: 10.1016/j.compstruct.2023.116995

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Carbon fibres; Centre composite design; Pyrolysis; Genetic algorithm; Fibre recycling

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This article conducted high-temperature pyrolysis recycling experiments on carbon fiber filaments to improve the mechanical properties of recycled carbon fibers. The influence of residual resin content and fiber oxidation on tensile properties was revealed, and process parameters were optimized for high temperature pyrolysis recycling of resin-matrix carbon fiber composites. The results showed that temperature had the greatest influence, a small amount of resin residue helped improve tensile strength, and pyrolysis time had a parabolic relationship with tensile strength.
In order to improve the mechanical properties of recycled carbon fibres, this article adopted the centre composite design method to conduct high-temperature pyrolysis recycling experiments on carbon fibre filaments. The experimental results revealed the influence of the residual resin content in the recycled carbon fibre bundles and the degree of fibre oxidation on the tensile properties. On the basis, the process parameters were further opti-mised for the high temperature pyrolysis recycling process of resin-matrix carbon fibre composites through multi-island genetic algorithm. The results suggest that (1) in the process of pyrolysis and oxidation, the tem-perature has the greatest influence on the properties of the fibres, and a small amount of resin residue helps improving the tensile strength of the recycled carbon fibres; (2) when the temperature is at a constant value in the range of 400-520 celcius, the pyrolysis time has a parabolic relationship with the tensile strength of recycled carbon fibres; (3) the tensile strength of the recycled carbon fibres reaches 80 % with 5.6 % resin residue remained in the recycled carbon fibre bundle after continuous pyrolysis at 428 degrees C for 4.0 h, and such a strength meets the mechanical performance requirements of recycled carbon fibre.

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