期刊
CHEMICAL COMMUNICATIONS
卷 51, 期 35, 页码 7536-7539出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cc01555c
关键词
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资金
- Ministry of Innovation, Science, Research and Technology of North Rhine-Westphalia
- Europaischer Fonds fur Regionale Entwicklung
- European Research Council under the European Union [268309]
A catalytic two-step reaction sequence was developed to access a range of complex heterocyclic frameworks based on biorelevant indole/oxindole scaffolds. The reaction sequence includes catalytic Pictet-Spengler cyclization followed by Au(I) catalyzed intramolecular hydroamination of acetylenes. A related cascade poly-cyclization of a designed beta-carboline embodying a 1,5-enyne group yields the analogues of the alkaloid harmicine.
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