☆ 4.6 Review

Applications of Carbon-Based Materials in Activated Peroxymonosulfate for the Degradation of Organic Pollutants: A Review

CHEMICAL RECORD (2023)

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Article Chemistry, Multidisciplinary

Low Concentration of Peroxymonosulfate Triggers Dissolved Oxygen Conversion over Single Atomic Fe-N3O1 Sites for Water Decontamination

Zhiyu Zhao et al.

Summary: This study reveals the triggering role of low-concentration peroxymonosulfate (PMS) in dissolved oxygen (DO) conversion over a single-atom Fe catalyst, inspiring the development of resource-saving, cost-effective, and environmentally-friendly catalytic oxidation systems.

SMALL (2023)

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Article Engineering, Chemical

Singlet oxygen-dominated non-radical oxidation in biochar/peroxymonosulfate system for efficient degradation of tetracycline hydrochloride: Surface site and catalytic mechanism

Rui Zhang et al.

Summary: In this study, Camellia oleifera shell-derived biochar (COSB) was prepared by one-step pyrolysis. The catalytic efficiency of COSB was found to be tunable by the pyrolysis temperature, with COSB-1000 prepared at 1000 degrees C showing the optimal activity in peroxymonosulfate (PMS) activation. The COSB-1000/PMS system exhibited good anti-interference ability and wide pH applicability, and the degradation of tetracycline hydrochloride (TC) was mainly dominated by the non-radical oxidation process, with the generated O-1(2) playing a vital role.

JOURNAL OF THE TAIWAN INSTITUTE OF CHEMICAL ENGINEERS (2023)

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Article Engineering, Chemical

Nonradical pathway dominated activation of peroxymonosulfate by ZnFe2O4/C composites to eliminate tetracycline hydrochloride: Insight into the cycle of Zn/Fe and electron transfer

Yawen Yu et al.

Summary: Magnetic ZnFe2O4 nanoparticles embedded into carbon substrate exhibit efficient catalytic activity in peroxymonosulfate (PMS) activation, thanks to the anchoring effect and improved electron transfer. The composites show wide pH adaptation range and good stability. This work provides a simple strategy for the preparation of magnetic ZnFe2O4/C heterogeneous catalyst, and promotes the application of spinel nano-materials in environmental remediation.

SEPARATION AND PURIFICATION TECHNOLOGY (2023)

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Article Engineering, Environmental

Co@C core-shell nanostructures anchored on carbon cloth for activation of peroxymonosulfate to degrade tetracycline

Quanzhi Zhang et al.

Summary: Co@C/CC immobilized catalyst shows enhanced catalytic activity and lower Co ion leaching in persulfate activation for organic pollutant degradation. The Co@C/CC/PMS system efficiently degrades tetracycline with high durability, interference resistance, and wide pH adaptability. Non-free radical pathway (1O2) dominates the degradation process. Density functional theory calculations indicate C-C as the primary attack site in tetracycline and provide possible degradation pathways. Importantly, the Co@C/CC catalyst enables fast and simple collection and regeneration.

JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING (2023)

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Article Engineering, Environmental

Degradation of antibiotic pollutants by persulfate activated with various carbon materials

Yuan Gao et al.

Summary: Antibiotic residues are widespread in water sources, posing ecological risks, with AOPs showing great potential for their removal; Carbon materials can activate persulfate effectively, but there is a lack of comprehensive studies on their behavior; This study provides insight into the degradation of antibiotics by carbon-activated persulfate system and discusses the synergistic effects with other strategies.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Engineering, Environmental

Reduced graphene oxide-supported hollow Co3O4@N-doped porous carbon as peroxymonosulfate activator for sulfamethoxazole degradation

Yanling Chen et al.

Summary: A novel Co3O4@NPC/rGO composite material was successfully synthesized and showed high catalytic activity for the removal of sulfamethoxazole. The study differentiated and calculated the contribution ratio of different reactive oxidative species in the system for the first time, and proposed a possible degradation mechanism. This work expands the environmental application of metal-organic frameworks-derived hollow nanomaterials and provides a promising heterogeneous catalyst for the elimination of refractory contaminants.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Engineering, Environmental

Decomposition of perfluorooctanic acid by carbon aerogel with persulfate

Yu Chi Lee et al.

Summary: The addition of Carbon aerogel (CA) in the thermally-activated persulfate (PS) system significantly improves the decomposition and defluorination of Persistent perfluorooctanoic acid (PFOA). This enhancement reduces activation energies and increases reaction rates, leading to potential energy savings and shorter process times.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Environmental Sciences

Can biochar and hydrochar be used as sustainable catalyst for persulfate activation

Mohamed Faisal Gasim et al.

Summary: There has been a surge of interest in using biomass-derived char as an activator for persulfate to remove anthropogenic pollutants. While char has shown potential as a persulfate activator, its sustainability over prolonged application is unclear. This review assesses the knowledge gap related to the sustainability of char as a persulfate activator and provides potential research directions.

CHEMOSPHERE (2022)

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Review Environmental Sciences

Novel insights into the adsorption of organic contaminants by biochar: A review

Zirui Luo et al.

Summary: Biochar plays a crucial role in wastewater and polluted soil decontamination as an adsorbent for organic contaminants. However, further research is needed on aspects such as dynamic adsorption, potential environmental risks, interactions between biochar and soil microbes to facilitate its practical application. This research will contribute to a better understanding of organic contaminants' adsorption removal by biochar.

CHEMOSPHERE (2022)

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Article Engineering, Environmental

N, S co-doped magnetic mesoporous carbon nanosheets for activating peroxymonosulfate to rapidly degrade tetracycline: Synergistic effect and mechanism

Dongdong He et al.

Summary: A novel N, S co-doped magnetic mesoporous carbon nanosheets were prepared in this study, demonstrating high degradation efficiency for tetracycline within 10 minutes due to non-radical pathway, with pyridinic N as the main active site.

JOURNAL OF HAZARDOUS MATERIALS (2022)

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Article Engineering, Chemical

Degradation of tetracycline hydrochloride through efficient peroxymonosulfate activation by B, N co-doped porous carbon materials derived from metal-organic frameworks: Nonradical pathway mechanism

Jinling Xie et al.

Summary: The study demonstrates that B-NC catalysts show excellent efficiency in the removal of tetracycline hydrochloride, with nitrogen doping changing the degradation pathway and boron doping providing more active sites. Singlet oxygen (O-1(2)) is found to be the major active species in the reaction, while electron transfer is identified as another significant oxidation pathway.

SEPARATION AND PURIFICATION TECHNOLOGY (2022)

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Article Engineering, Environmental

Rational design of CoxMn3-xO4 embedded carbon composites from MOF-74 structure for boosted peroxymonosulfate activation: A dual pathway mechanism

Linjie Wang et al.

Summary: In this study, Spinel structured CoxMn3-xO4 nanoparticles embedded carbon composites (CoxMn3-xO4-C) were designed and prepared using Co/Mn bimetallic metal organic frameworks (MOFs) as the template. Among them, Co1.5Mn1.5O4-C showed the highest degradation efficiency and could completely degrade BPA within 3 minutes. Furthermore, Co1.5Mn1.5O4-C exhibited limited leaching of Co2+ in the Co1.5Mn1.5O4-C/PMS system. The research revealed that hydroxyl radical and singlet oxygen were the main active species in the reaction system, contributing to a dual pathway mechanism for BPA degradation. Additionally, Co1.5Mn1.5O4-C showed promising recyclability in different water matrices.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Engineering, Environmental

High efficient activation of peroxymonosulfate by Co9S8 anchored in N, S, O co-doped carbon composite for degradation of sulfamethoxazole: Effect of sulfur precursor and sulfur doping content

Shizong Wang et al.

Summary: Cobalt sulfides as persulfate activator have been studied for their catalytic activity in persulfate-based advanced oxidation process. This study successfully prepared Co9S8 anchored in N, S, O heteroatoms co-doped carbon composite, which showed high catalytic activity in activating peroxymonosulfate for sulfamethoxazole degradation. The study also investigated the effect of various factors on the degradation process and identified the active sites and intermediate products involved.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Engineering, Environmental

Transition metal single-atom embedded on N-doped carbon as a catalyst for peroxymonosulfate activation: A DFT study

Jiahui Hu et al.

Summary: This study used density functional theory calculations to investigate the electronic structures and activation mechanisms of peroxymonosulfate (PMS) on transition metal single-atom catalysts. The results showed that electron transfer mediated by surface activated PMS plays a dominant role in all MeN@C/PMS systems, leading to the generation of various reactive oxygen species (ROS). Different adsorption configurations and subsequent PMS activation result in the formation of different types of ROS.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Chemistry, Inorganic & Nuclear

Synthesis of Carbon Nanoparticles with Cobalt-Rich Shell via Pyrolysis of Zn-ZIF@Co/Zn-ZIF: Relevance of Co(III) Precursors

Jiachen Ge et al.

Summary: This study reports the rapid one-pot synthesis of a unique core-shell-structured ZIF using Co(III) and Zn(II) precursors and discusses the growth mechanism of the synthesized ZIF particles and the differences between synthesized ZIF and conventional Co(II)-ZIF-67.

INORGANIC CHEMISTRY (2022)

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Review Engineering, Environmental

Multi-heteroatom-doped carbocatalyst as peroxymonosulfate and peroxydisulfate activator for water purification: A critical review

Zheng-Yi Choong et al.

Summary: This review provides an overview on the development of multi-heteroatom-doped carbocatalyst for persulfate activation, evaluating the potential interactions and summarizing the performance for pollutant removal. The preparation strategies, characterization techniques, and prospects for further research are also discussed.

JOURNAL OF HAZARDOUS MATERIALS (2022)

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Article Engineering, Chemical

Outstanding catalytic performance of metal-free peroxymonosulfate activator: Important role of chrysotile

Qian Peng et al.

Summary: In this study, a metal-free peroxymonosulfate catalyst based on chrysotile and graphite carbon nitride (g-C3N4) was synthesized for the first time, which significantly improved the activation efficiency of peroxymonosulfate and showed superior catalytic performance for rhodamine B degradation. Moreover, the catalyst exhibited good cycle performance and universal applicability, providing a new idea for the comprehensive utilization of asbestos tailings and environmental remediation.

SEPARATION AND PURIFICATION TECHNOLOGY (2022)

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Article Engineering, Environmental

Activation of peroxymonosulfate by MnFe2O4@BC composite for bisphenol A Degradation: The coexisting of free-radical and non-radical pathways

Siyu Xu et al.

Summary: In this study, a novel metallic oxide catalyst MnFe2O4@biochar composite was synthesized and used to activate peroxymonosulfate (PMS) for efficient degradation of bisphenol A. The composite showed homogeneously distributed metal oxide particles, strong magnetism, and wide adaptability, effectively removing organic pollutants.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Engineering, Environmental

The enhanced catalytic degradation of sulfamethoxazole over Fe@nitrogen-doped carbon-supported nanocomposite: Insight into the mechanism

Jinkai He et al.

Summary: An environmentally friendly Fe@nitrogen-doped carbon nanocomposite catalyst (Fe@N-CNs) was prepared using carboxymethyl chitosan hydrogel as a template. The catalyst showed excellent catalytic activity for the degradation of sulfamethoxazole (SMX) and exhibited stable performance over a wide pH range and under high-salinity conditions. Singlet oxygen was identified as the dominant reactive species in the catalytic oxidation process. The Fe@N-CNs/PMS system also proved to be effective against antibiotic resistant bacteria and antibiotics resistance genes.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Chemistry, Physical

Cobalt/calcium bimetallic oxides based on bio-waste eggshells for the efficient degradation of norfloxacin by peroxymonosulfate activation

Xinyi Zhang et al.

Summary: Cobalt-calcium bimetallic oxide (ECCO) synthesized from eggshells and cobalt nitrate was found to efficiently activate peroxymonosulfate (PMS) and remove norfloxacin (NOR). ECCO exhibited high degradation efficiency and good reusability due to enhanced electron transfer capability, diversified reactive oxygen species (ROS) production, and active sites on Co and oxygen vacancies.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2022)

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Article Chemistry, Physical

MOF Derived Co-Fe nitrogen doped graphite carbon@crosslinked magnetic chitosan Micro-nanoreactor for environmental applications: Synergy enhancement effect of adsorption-PMS activation

Aiwen Wang et al.

Summary: This study successfully addresses the limitations of adsorption technology in fully mineralizing pollutants and the potential health risks from metal ion leakage. A micro-nanoreactor structure is designed with glutaraldehyde crosslinked chitosan as the backbone and encapsulated MOF-derived Co-Fe nitrogen-doped graphitic carbon as the activated PMS reaction center (Co-Fe/NC@GCS). High concentration sulfamethoxazole can be efficiently enriched through electrostatic attraction and hydrogen bonding, and a small amount of PMS can be rapidly activated.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Engineering, Environmental

Co/N co-doped carbonaceous polyhedron as efficient peroxymonosulfate activator for degradation of organic pollutants: Role of cobalt

Huiwang Dai et al.

Summary: The study synthesized a Co/N co-doped polyhedron carbonaceous catalyst (Co@N-C-2) with abundant mesoporous, high graphitization degree, and cobalt content via the pyrolysis of core-shell MOFs composite (ZIF-8@ZIF-67). The two cobalt species in Co@N-C-2 were found to play different roles in PMS activation, with Co-N-x serving as active sites for the O-1(2) evolution pathway and Co NPs enhancing electron transfer pathway. The catalyst showed superior catalytic performance in removing organic pollutants and high resistance to inorganic anions and natural organic matter.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

Sulfur-containing iron nanocomposites confined in S/N co-doped carbon for catalytic peroxymonosulfate oxidation of organic pollutants: Low iron leaching, degradation mechanism and intermediates

Yangke Long et al.

Summary: By confining iron nano-composites and heteroatoms (S/N) within a porous carbon host, the Fe-S@SNC catalyst exhibits enhanced catalytic performance for various pollutants and effectively resolves the issue of metal leaching-induced secondary pollution. This work provides new insights into the design and activation mechanism of iron-based PMS activators.

CHEMICAL ENGINEERING JOURNAL (2021)

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Review Engineering, Environmental

A review of the innovations in metal- and carbon-based catalysts explored for heterogeneous peroxymonosulfate (PMS) activation, with focus on radical vs . non-radical degradation pathways of organic contaminants

Mona Kohantorabi et al.

Summary: This review summarizes the rapid development of heterogeneous catalysts for peroxymonosulfate (PMS) activation in sulfate radical-based AOPs, covering various catalysts and discussing their roles in the activation mechanism.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Chemistry, Physical

Optimization of active sites by sulfurization of the core-shell ZIF 67@ZIF 8 for rapid oxygen reduction kinetics in acidic media

Jung Su Lee et al.

Summary: The Co-decorated nitrogen and sulfur co-doped carbon nanostructures (Co-NSC) exhibit high catalytic activity for oxygen reduction reactions, aiming to replace expensive commercial Pt catalysts. The sulfur co-doping dramatically enhances intrinsic catalytic activity, with variation in sulfurization degree influencing overall catalytic performance. Co-NSC 200 with high sulfur doping shows improved onset potential and current density, making it a promising PGM-free catalyst option.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2021)

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Article Chemistry, Physical

Activation of peroxymonosulfate by iron-biochar composites: Comparison of nanoscale Fe with single-atom Fe

Zhuoqian Li et al.

Summary: A convenient and efficient method for fabricating isolated Fe single-atom catalysts (ISA-Fe/MC) on Myriophyllum aquaticum-based biochar was reported for peroxymonosulfate-based organics degradation. Compared to Fe nanoparticles anchored on biochar, ISA-Fe/MC demonstrated better catalytic performance for phenol degradation, attributed to its unique structure and atomically dispersed Fe species facilitating electron transfer for activation.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2021)

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Article Engineering, Environmental

In-situ self-assembly construction of hollow tubular g-C3N4 isotype heterojunction for enhanced visible-light photocatalysis: Experiments and theories

Qinghua Liang et al.

Summary: S doping in a highly reactive hollow tubular g-C3N4 isotype heterojunction (SCN-CN) enhances visible light absorption and directs the transfer of electrons and holes. The tubular structure of SCN-CN facilitates electron transfer in the longitudinal direction, reducing charge carrier recombination. Experimental and theoretical studies were conducted to analyze the optical properties, electronic structure, and electron transfer of SCN-CN.

JOURNAL OF HAZARDOUS MATERIALS (2021)

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Article Engineering, Environmental

Singlet oxygen-dominated activation of peroxymonosulfate by passion fruit shell derived biochar for catalytic degradation of tetracycline through a non-radical oxidation pathway

Yi Hu et al.

Summary: The study demonstrates that the pyrolysis temperature can influence the efficiency of passion fruit shell derived biochar (PFSC) for activating peroxymonosulfate (PMS) to degrade tetracycline hydrochloride (TC), with the PFSC-900/PMS system showing high catalytic performance mainly due to the non-free radical reaction pathway. This research not only showcases biochar as an efficient catalyst for PMS activation, but also provides a value-added reuse pathway for passion fruit shells.

JOURNAL OF HAZARDOUS MATERIALS (2021)

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Article Engineering, Environmental

Enhancing peroxymonosulfate activation by Co-Fe layered double hydroxide catalysts via compositing with biochar

Quanyun Ye et al.

Summary: Efficient and low-cost catalysts for peroxymonosulfate (PMS) activation are essential for pollution prevention and environmental remediation. In this study, biochar (BC) was composited with CoFe layered double hydroxide (CoFe-LDH) to achieve enhanced PMS activation. The synergistic effect between BC and CoFe-LDH resulted in improved catalytic activity and stability, leading to higher production of reactive oxygen species (ROS) in the BC-LDH/PMS system. The degradation efficiency of dimethyl phthalate (DMP) was significantly higher in the BC-LDH/PMS system compared to the CoFe-LDH/PMS system, reaching 100% within 60 minutes.

CHEMICAL ENGINEERING JOURNAL (2021)

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Review Engineering, Environmental

Activation of persulfates by carbonaceous materials: A review

Wuqi Huang et al.

Summary: This paper analyzed the mechanisms of persulfates activation by carbonaceous materials and their composites, explored the synergistic effect for activation improvement in the composites or in the hybrid activation systems. It summarized the influence of environmental conditions on the activation processes, discussed deactivation and regeneration of carbonaceous materials, and reviewed the application of these materials in activating persulfates for remediation of contaminated groundwater and treatment of wastewater, as well as proposed the challenges for such applications.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

The mechanism changes during bisphenol A degradation in three iron functionalized biochar/peroxymonosulfate systems: The crucial roles of iron contents and graphitized carbon layers

Kai Li et al.

Summary: Three magnetic biochar nanocomposites were prepared with different catalytic performances for bisphenol A degradation, where C800-3 showed the best performance. The dominant role of electron transfer pathway was gradually replaced by the SO4 center dot- pathway with the increase of iron amount and the destruction of graphitized carbon layers.

JOURNAL OF HAZARDOUS MATERIALS (2021)

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Review Environmental Sciences

Preparation of biochar and biochar composites and their application in a Fenton-like process for wastewater decontamination: A review

Xuqin Pan et al.

Summary: Biochar is a carbon-rich material obtained from solid waste pyrolysis, featuring low cost, large specific surface area, and strong adsorption capacity. Biochar composites, produced by loading nano particles onto biochar, have been widely applied in wastewater treatment to enhance the performance of advanced oxidation processes. However, due to the variety of biochar feedstocks and preparation methods, comparing the properties of different biochars can be challenging.

SCIENCE OF THE TOTAL ENVIRONMENT (2021)

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Article Engineering, Chemical

Direct transformation of bulk cobalt foam into cobalt nanoparticles encapsulated in nitrogen-doped carbon nanotubes for peroxymonosulfate activation toward rhodamine B degradation

Jiaxing Cheng et al.

Summary: A simple and straightforward approach was developed to prepare encapsulated Co nanoparticles on nitrogen-doped carbon nanotubes, showing efficient degradation of organic dye RhB. Quenching tests and characterization analysis revealed the degradation mechanisms and possible catalytic active sites of the Co/NCNT material.

SEPARATION AND PURIFICATION TECHNOLOGY (2021)

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Article Engineering, Chemical

Activation of peroxymonosulfate by sewage sludge biochar-based catalyst for efficient removal of bisphenol A: Performance and mechanism

Xiaohui Fan et al.

Summary: This study demonstrates the efficient degradation of bisphenol A (BPA) in water by the combination of sludge-derived biochar (SBC) and peroxymonosulfate (PMS), showing improved removal efficiency and verifying the involvement of active species in a non-radical process.

SEPARATION AND PURIFICATION TECHNOLOGY (2021)

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Article Engineering, Environmental

Non-covalent doping of carbon nitride with biochar: Boosted peroxymonosulfate activation performance and unexpected singlet oxygen evolution mechanism

Huazhe Wang et al.

Summary: By utilizing graphitic biochar as a dopant, electronic properties of polymeric carbon nitride were manipulated effectively while maintaining its robust geometric structure, resulting in improved efficiency in activating peroxymonosulfate. The study decoded a new pathway for singlet oxygen production, expanding the understanding of PMS decomposition mechanisms.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

Thiourea-assisted one-step fabrication of a novel nitrogen and sulfur co-doped biochar from nanocellulose as metal-free catalyst for efficient activation of peroxymonosulfate

Yan Xu et al.

Summary: The N, S co-doped biochar with multistage pore structure was successfully synthesized and found to effectively activate PMS for SMX degradation, showing higher removal efficiency compared to systems activated by common metal oxides. The mechanism of the N, S-BC/PMS process was deduced through experiments, revealing the essential role of surface-bound free radicals and 1O2 in SMX degradation.

JOURNAL OF HAZARDOUS MATERIALS (2021)

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Article Engineering, Environmental

Carbon aerogel from forestry biomass as a peroxymonosulfate activator for organic contaminants degradation

Mingshuo Zhu et al.

Summary: The study synthesized biomass carbon aerogel (CA) derived from poplar powder, which exhibited excellent degradation performance for different types of organic contaminants. The possible mechanism for PMS activation was discussed, indicating that singlet oxygen (1O2) dominated the non-radical pathway for pollutant removal. The study also confirmed that the ketonic/carbonyl groups on the surface of CA could serve as a possible active site to facilitate the generation of 1O2.

JOURNAL OF HAZARDOUS MATERIALS (2021)

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Article Engineering, Environmental

Facile ball milling preparation of sulfur-doped carbon as peroxymonosulfate activator for efficient removal of organic pollutants

Min Huang et al.

Summary: Novel sulfur-doped activated carbon particles were prepared through a simple method and utilized as activators of PMS to efficiently degrade various organic pollutants, with the degradation efficiency being dependent on the S doping content. The study showed that the presence of C-S-C bonds significantly influenced the degradation rate of pollutants like DEP, suggesting their importance in PMS activation.

JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING (2021)

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Article Chemistry, Physical

Oxygen vacant Co3O4in situ embedded on carbon spheres: cooperatively tuning electron transfer for boosted peroxymonosulfate activation

Jian Hu et al.

Summary: The study synthesized carbon spheres embedded with in situ grown oxygen-vacancy-rich cobalt oxide nanoparticles, which cooperatively accelerated the electron transfer process and boosted the generation of reactive radicals for superior BPA degradation rate.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Engineering, Environmental

Malachite green degradation by persulfate activation with CuFe2O4@biochar composite: Efficiency, stability and mechanism

Quanlong Huang et al.

Summary: The CuFe2O4@biochar composite showed high catalytic efficiency and stability in degrading dye wastewater, making it a promising catalyst for treating contaminated wastewater.

JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING (2021)

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Article Engineering, Environmental

Synthesis of nZVI-Ni@BC composite as a stable catalyst to activate persulfate: Trichloroethylene degradation and insight mechanism

Ali Shan et al.

Summary: The study shows that the nZVI-Ni@BC composite material performs well in activating PS to degrade chlorinated contaminants in water, achieving over 99% TCE degradation. The experimental results also indicate that in acidic environments, both SO4·- and OH· radicals play a dominant role in TCE degradation, while high levels of carbonates, bicarbonates, and NOM inhibit the oxidation reaction of TCE.

JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING (2021)

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Article Engineering, Environmental

Removal of tetracycline via the synergistic effect of biochar adsorption and enhanced activation of persulfate

Junhao Chen et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Iron-mediated activation of persulfate and peroxymonosulfate in both homogeneous and heterogeneous ways: A review

Sa Xiao et al.

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Muhammad Ahmad et al.

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Degradation of norfloxacin by CoFe alloy nanoparticles encapsulated in nitrogen doped graphitic carbon (CoFe@N-GC) activated peroxymonosulfate

Dahu Ding et al.

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Oxidative degradation of tetracycline using persulfate activated by N and Cu codoped biochar

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3D mesoporous α-Co(OH)2 nanosheets electrodeposited on nickel foam: A new generation of macroscopic cobalt-based hybrid for peroxymonosulfate activation

Ruixia Yuan et al.

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Zoha Heidarinejad et al.

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Adsorptive interaction of peroxymonosulfate with graphene and catalytic assessment via non-radical pathway for the removal of aqueous pharmaceuticals

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Nitrogen-doping positively whilst sulfur-doping negatively affect the catalytic activity of biochar for the degradation of organic contaminant

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Elbaite catalyze peroxymonosulfate for advanced oxidation of organic pollutants: Hydroxyl groups induced generation of reactive oxygen species

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Activation of peroxymonosulfate by cobalt-impregnated biochar for atrazine degradation: The pivotal roles of persistent free radicals and ecotoxicity assessment

Banghai Liu et al.

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Enhanced surface activation process of persulfate by modified bagasse biochar for degradation of phenol in water and soil: Active sites and electron transfer mechanism

Hao Zhang et al.

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Transforming goat manure into surface-loaded cobalt/biochar as PMS activator for highly efficient ciprofloxacin degradation

Junmei Luo et al.

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B-doped graphitic porous biochar with enhanced surface affinity and electron transfer for efficient peroxydisulfate activation

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Van Luan Pham et al.

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Defective, oxygen-functionalized multi-walled carbon nanotubes as an efficient peroxymonosulfate activator for degradation of organic pollutants

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Red mud modified sludge biochar for the activation of peroxymonosulfate: Singlet oxygen dominated mechanism and toxicity prediction

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Iron nanoparticles encapsulated within nitrogen and sulfur co-doped magnetic porous carbon as an efficient peroxymonosulfate activator to degrade 1-naphthol

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SCIENCE OF THE TOTAL ENVIRONMENT (2020)

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Carbon nanofibers supported Co/Ag bimetallic nanoparticles for heterogeneous activation of peroxymonosulfate and efficient oxidation of amoxicillin

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JOURNAL OF HAZARDOUS MATERIALS (2020)

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Selective oxidation of H1-antihistamines by unactivated peroxymonosulfate (PMS): Influence of inorganic anions and organic compounds

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WATER RESEARCH (2020)

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Enhanced thermal activation of peroxymonosulfate by activated carbon for efficient removal of perfluorooctanoic acid

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Electrochemical mineralization of antibiotic ceftazidime with SnO2-Al2O3/CNT anode: Enhanced performance by peroxydisulfate/Fenton activation and degradation pathway

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Zero-valent iron/activated carbon microelectrolysis to activate peroxydisulfate for efficient degradation of chlortetracycline in aqueous solution

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Comparative removal of emerging contaminants from aqueous solution by adsorption on an activated carbon

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NiO-NiFe2O4-rGO Magnetic Nanomaterials for Activated Peroxymonosulfate Degradation of Rhodamine B

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Metal-organic framework-derived hollow Co3O4/carbon as efficient catalyst for peroxymonosulfate activation

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Biochar-induced Fe(III) reduction for persulfate activation in sulfamethoxazole degradation: Insight into the electron transfer, radical oxidation and degradation pathways

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Optimization and mechanism of Acid Orange 7 removal by powdered activated carbon coupled with persulfate by response surface method

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The simultaneous adsorption of nitrate and phosphate by an organic-modified aluminum-manganese bimetal oxide: Adsorption properties and mechanisms

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Redistribution of π and σ electrons in boron-doped graphene from DFT investigation

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Cobalt-impregnated biochar produced from CO2-mediated pyrolysis of Co/lignin as an enhanced catalyst for activating peroxymonosulfate to degrade acetaminophen

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Activation mechanism of peroxymonosulfate by biochar for catalytic degradation of 1,4-dioxane: Important role of biochar defect structures

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Carbon-based magnetic nanocomposite as catalyst for persulfate activation: a critical review

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From rice straw to magnetically recoverable nitrogen doped biochar: Efficient activation of peroxymonosulfate for the degradation of metolachlor

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Activation of peroxymonosulfate by sludge-derived biochar for the degradation of triclosan in water and wastewater

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Solvent-free synthesis of a 2D biochar stabilized nanoscale zerovalent iron composite for the oxidative degradation of organic pollutants

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Cu@Co-MOFs as a novel catalyst of peroxymonosulfate for the efficient removal of methylene blue

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Insights into heterogeneous catalysis of peroxymonosulfate activation by boron-doped ordered mesoporous carbon

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Enhanced degradation of antibiotic sulfamethoxazole by electrochemical activation of PDS using carbon anodes

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Enhanced degradation of Bisphenol A (BPA) by peroxymonosulfate with Co3O4-Bi2O3 catalyst activation: Effects of pH, inorganic anions, and water matrix

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Heterogeneous activation of peroxymonosulfate over monodispersed Co3O4/activated carbon for efficient degradation of gaseous toluene

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Oxidation of bromophenols by carbon nanotube activated peroxymonosulfate (PMS) and formation of brominated products: Comparison to peroxydisulfate (PDS)

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Activation of persulfate (PS) and peroxymonosulfate (PMS) and application for the degradation of emerging contaminants

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Controlled synthesis of dandelion-like NiCo2O4 microspheres and their catalytic performance for peroxymonosulfate activation in humic acid degradation

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Co-Mn layered double hydroxide as an effective heterogeneous catalyst for degradation of organic dyes by activation of peroxymonosulfate

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Identifying the Nonradical Mechanism in the Peroxymonosulfate Activation Process: Singlet Oxygenation Versus Mediated Electron Transfer

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Catalytic Removal of Aqueous Contaminants on N-Doped Graphitic Biochars: Inherent Roles of Adsorption and Nonradical Mechanisms

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Oxidation of Rhodamine B by persulfate activated with porous carbon aerogel through a non-radical mechanism

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Activated Biochar as an Effective Sorbent for Organic and Inorganic Contaminants in Water

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Sludge biochar-based catalysts for improved pollutant degradation by activating peroxymonosulfate

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Biochar modification significantly promotes the activity of Co3O4 towards heterogeneous activation of peroxymonosulfate

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Exploring the Role of Persulfate in the Activation Process: Radical Precursor Versus Electron Acceptor

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Mechanistic Insight into the Reactivity of Chlorine-Derived Radicals in the Aqueous-Phase UV Chlorine Advanced Oxidation Process: Quantum Mechanical Calculations

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Peroxymonosulfate enhanced photoelectrocatalytic degradation of phenol activated by Co3O4 loaded carbon fiber cathode

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Degradation of sulfamethoxazole by UV, UV/H2O2 and UV/persulfate (PDS): Formation of oxidation products and effect of bicarbonate

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Sulfate radical degradation of acetaminophen by novel iron-copper bimetallic oxidation catalyzed by persulfate: Mechanism and degradation pathways

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Simultaneous enhancement of adsorption and peroxymonosulfate activation of Nitrogen-doped reduced graphene oxide for bisphenol A removal

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Heterogeneous activation of peroxymonosulfate by Fe-Co layered doubled hydroxide for efficient catalytic degradation of Rhoadmine B

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Facile synthesis of nitrogen-doped graphene via low-temperature pyrolysis: The effects of precursors and annealing ambience on metal-free catalytic oxidation

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Review Engineering, Environmental

Application of peroxymonosulfate and its activation methods for degradation of environmental organic pollutants: Review

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Occurrence of radical and nonradical pathways from carbocatalysts for aqueous and nonaqueous catalytic oxidation

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Generation of sulfate radical through heterogeneous catalysis for organic contaminants removal: Current development, challenges and prospects

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Unveiling the active sites of graphene-catalyzed peroxymonosulfate activation

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Decolorization of azo dye by peroxymonosulfate activated by carbon nanotube: Radical versus non-radical mechanism

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Degradation of refractory dibutyl phthalate by peroxymonosulfate activated with novel catalysts cobalt metal-organic frameworks: Mechanism, performance, and stability

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Activation of peroxymonosulfate by graphitic carbon nitride loaded on activated carbon for organic pollutants degradation

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Irradiation treatment of pharmaceutical and personal care products (PPCPs) in water and wastewater: An overview

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Promoting effect of ammonia modification on activated carbon catalyzed peroxymonosulfate oxidation

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Graphene-Based Metal-Free Catalysts for Catalytic Reactions in the Liquid Phase

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Selective decolorization of cationic dyes by peroxymonosulfate: non-radical mechanism and effect of chloride

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Electrochemical catalysis at low dimensional carbons: Graphene, carbon nanotubes and beyond - A review

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Nanocarbons in different structural dimensions (0-3D) for phenol adsorption and metal-free catalytic oxidation

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Carbon nanomaterials synthesized by arc discharge hot plasma

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Effect of activated carbon surface chemistry on the activity of ZVI/AC catalysts for Fenton-like oxidation of phenol

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Effects of nitrogen-, boron-, and phosphorus-doping or codoping on metal-free graphene catalysis

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Heat-activated persulfate oxidation of atrazine: Implications for remediation of groundwater contaminated by herbicides

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Activation of persulfates by carbon nanotubes: Oxidation of organic compounds by nonradical mechanism

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Activation of Peroxymonosulfate by Benzoquinone: A Novel Nonradical Oxidation Process

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Heterogeneous photo-Fenton degradation of acid red B over Fe2O3 supported on activated carbon fiber

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JOURNAL OF HAZARDOUS MATERIALS (2015)

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Ultrasound enhanced heterogeneous activation of peroxymonosulfate by a bimetallic Fe-Co/SBA-15 catalyst for the degradation of Orange II in water

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Activated carbon fiber as heterogeneous catalyst of peroxymonosulfate activation for efficient degradation of Acid Orange 7 in aqueous solution

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Degradation and detoxification of diazinon by sono-Fenton and sono-Fenton-like processes

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Sulfur and Nitrogen Co-Doped Graphene for Metal-Free Catalytic Oxidation Reactions

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Dissolved effluent organic matter: Characteristics and potential implications in wastewater treatment and reuse applications

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N-Doping-Induced Nonradical Reaction on Single-Walled Carbon Nanotubes for Catalytic Phenol Oxidation

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The mechanism of bound hydroxyl radical formation and degradation pathway of Acid Orange II in Fenton-like Co2+-HCO3- system

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Peroxymonosulfate activation by phosphate anion for organics degradation in water

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Degradation of direct yellow 9 by electro-Fenton: Process study and optimization and, monitoring of treated water toxicity using catalase

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Degradation of Toluene by a Selective Ferrous Ion Activated Persulfate Oxidation Process

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Superoxide radical driving the activation of persulfate by magnetite nanoparticles: Implications for the degradation of PCBs

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Current understanding of the growth of carbon nanotubes in catalytic chemical vapour deposition

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Comparison of sulfate and hydroxyl radical based advanced oxidation of phenol

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Influence of pH on the Formation of Sulfate and Hydroxyl Radicals in the UV/Peroxymonosulfate System

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Large-Area Synthesis of High-Quality and Uniform Graphene Films on Copper Foils

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Effects of activation schemes on porous, surface and thermal properties of activated carbons prepared from cotton stalks

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Preparation and characterization of activated carbon from date stones by physical activation with steam

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Adsorption characteristics of selected pharmaceuticals and an endocrine disrupting compound - Naproxen, carbamazepine and nonylphenol - on activated carbon

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Single sheet functionalized graphene by oxidation and thermal expansion of graphite

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Recent advances in laser synthesis of single-walled carbon nanotubes

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JOURNAL OF NANOSCIENCE AND NANOTECHNOLOGY (2006)

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Letter Chemistry, Physical

Heterogeneous activation of oxone using Co3O4

GP Anipsitakis et al.

JOURNAL OF PHYSICAL CHEMISTRY B (2005)

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Article Chemistry, Applied

Production and characterization of activated carbons from olive-seed waste residue

GG Stavropoulos et al.

MICROPOROUS AND MESOPOROUS MATERIALS (2005)

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Review Materials Science, Composites

Advances in the science and technology of carbon nanotubes and their composites: a review

ET Thostenson et al.

COMPOSITES SCIENCE AND TECHNOLOGY (2001)

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Article Agricultural Engineering

Bioadsorption of pentachlorophenol (PCP) from aqueous solution by activated sludge biomass

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BIORESOURCE TECHNOLOGY (2000)

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