期刊
CHEMICAL ENGINEERING JOURNAL
卷 475, 期 -, 页码 -出版社
ELSEVIER SCIENCE SA
DOI: 10.1016/j.cej.2023.146422
关键词
Acid pretreatment; Fermentable sugars; Biomass conversion; Dark fermentation
This study proposes a rapid and effective pretreatment method using molten oxalic acid dihydrate (OAD) to enhance enzymatic saccharification for biohydrogen production. The pretreatment achieves high cellulose retention, hemicellulose removal, and delignification within a short time, resulting in high enzymolysis conversion rate and fermentative hydrogen yield.
Biohydrogen production from lignocellulose presents an enduring challenge due to the tough, rigid, and complex structure that endows the lignocellulose with high resistance to biodegradation. In the present work, a rapid and effective pretreatment method employing molten oxalic acid dihydrate (OAD) was proposed to enhance enzymatic saccharification for biohydrogen production through efficient coextraction of wheat straw. The molten OAD pretreatment at 110 degrees C achieves a 95 % cellulose retention, 95 % hemicellulose removal, and 81.3 % delignification within 5 min. Furthermore, an 85 % enzymolysis conversion rate and 114.04 mL/g total solids (TS) fermentative hydrogen yield can be obtained. The OAD pretreatment enhanced the feasibility of biomass refining and paves the way for a novel, fast and high-efficiency pretreatment method for advancing the productivity stage toward biohydrogen production from lignocellulosic biomass.
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