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Article
Chemistry, Multidisciplinary
Yulu Yang et al.
Summary: Lithium metal batteries (LMBs) with high-voltage nickel-rich cathode and Li metal anode have the potential for high capacity and power density, but electrolytes that can withstand oxidation on the cathode at high cut-off voltage are urgently needed. This study presents an armor-like inorganic-rich cathode electrolyte interphase (CEI) strategy using pentafluorophenylboronic acid (PFPBA) as an additive to explore oxidation-resistant electrolytes for sustaining 4.8 V Li||LiNi0.6Co0.2Mn0.2O2 (NCM622) batteries. The CEI, which consists of armored lithium borate and abundant LiF, improves the mechanical stability and Li+ conductivity, leading to excellent cycling performance and capacity retention even at 4.8 V cut-off voltage.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2023)
Article
Engineering, Environmental
Shyam Chand Pal et al.
Summary: The emerging problem in the chemical industry is the efficient and cost-effective selective capture and separation of gases from mixtures. Cu-PSB, as a Prussian blue analogue, shows great potential as an energy-efficient gas separation material, exhibiting excellent separation performance for C2H2/C2H4, biogas, and flue gas mixtures.
CHEMICAL ENGINEERING JOURNAL
(2023)
Review
Chemistry, Applied
Prakas Samanta et al.
Summary: This article provides a comprehensive review on the development of cost-effective and environmentally friendly energy storage devices, focusing on the application of environmentally viable water-in-salt electrolytes in high-performance energy storage devices. The water-in-salt electrolyte exhibits a wide electrochemical stability window, high safety, non-flammability, and superior electrochemical performance compared to conventional salt-in-water electrolytes. The article systematically reviews the strategic application of water-in-salt electrolytes in rechargeable metal-ion batteries and supercapacitors with potentially improved electrochemical performance, and discusses the unique advantages, future prospects, and challenges of water-in-salt electrolytes.
JOURNAL OF ENERGY CHEMISTRY
(2023)
Review
Engineering, Environmental
Yu Zhang et al.
Summary: Environmental pollution is a global issue that has attracted widespread attention. Metal-organic frameworks (MOFs) have shown promise in the removal of environmental contaminants, but their efficiency needs improvement. Researchers have been modifying MOFs to introduce new functionalities for better pollutant removal. This review highlights the progress in functional modification of MOFs for air and water pollutant treatment, discussing their classification, modification approaches, applications, stability, and future trends.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Engineering, Environmental
Anna A. Lysova et al.
Summary: This study thoroughly investigated the adsorption and separation of light saturated hydrocarbons (methane, ethane, and propane) on a series of metal-organic frameworks. The impact of the size and nature of the glycol moiety on the adsorption parameters was revealed. The studied metal-organic frameworks showed exceptional performance in the practical separation of natural gas or other relevant mixtures of light alkanes.
CHEMICAL ENGINEERING JOURNAL
(2023)
Review
Engineering, Environmental
Mohan Gopalakrishnan et al.
Summary: Rechargeable aqueous zinc-ion batteries (AZIBs) have gained much interest due to their high energy density, safety, and low cost. However, issues such as anode side reactions, passivation, corrosion, hydrogen evolution, and Zn dendrite growth continue to hinder their widespread application. This review presents metal-organic frameworks (MOFs) as potential solutions to these problems by enhancing the performance of Zn anode materials, electrolytes, and electrolyte additives through their porous structure and active sites. The review also proposes directions for the rational design of MOF-based Zn anodes and understanding the mechanisms affecting Zn2+ solvation in high-performance AZIBs, aiming to extend the cycling lifetime and promote the commercialization of AZIBs.
CHEMICAL ENGINEERING JOURNAL
(2023)
Review
Engineering, Environmental
Borui Jie et al.
Summary: This review explores the application of luminescent metal organic frameworks (LMOFs) in detecting pollutants. The relationship between detection mechanism and signal emission is analyzed based on the structural characteristics of LMOFs, and various strategies for constructing and synthesizing LMOFs are proposed. Additionally, recent research progress in using LMOFs as fluorescent sensors to distinguish different types of pollutants is systematically summarized.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Chemistry, Multidisciplinary
Rupam Sahoo et al.
Summary: The effective design of new efficient crystalline solid-state proton conductors (SSPCs) is necessary for clean energy applications. In this study, a coordination polymer (CP), IITKGP-101, is presented as a highly scalable and robust SSPC that exhibits superprotonic conductivity. The CP utilizes coordinated water molecules as the sole intrinsic proton sources, allowing for efficient proton migration and high conductivity values.
MATERIALS CHEMISTRY FRONTIERS
(2023)
Article
Chemistry, Physical
Ha Huu Do et al.
Summary: This paper reviews the research progress of metal-organic frameworks (MOFs) as catalysts for hydrogen production through water splitting. Different types of electrocatalysts and photocatalysts based on MOFs are discussed. The findings of MOF-based catalysts for hydrogen generation are summarized, and the pros and cons of these materials as catalysts for water splitting are discussed. Current challenges and potential developments of MOFs as catalysts are also provided.
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
(2022)
Editorial Material
Chemistry, Physical
Madhab C. Das et al.
Review
Engineering, Environmental
Li Yan et al.
Summary: The problem of bacterial resistance to antibiotics is becoming increasingly serious, and the development of new antibiotics is much slower than the development of antibiotic resistance in pathogenic bacteria. To overcome antibiotic resistance, new therapeutic strategies need to be sought, and new materials such as metal organic frameworks may be potential candidates.
CHEMICAL ENGINEERING JOURNAL
(2022)
Review
Multidisciplinary Sciences
Avishek Karmakar et al.
Summary: Metal-organic frameworks (MOFs) are a promising material class for sensing and capture of toxic pollutants for environmental remediation. Recent studies have shown that MOFs can selectively detect, capture and remove various toxic pollutants from air and water bodies. Their unique structure, porous nature, and easy tunability make them effective in tackling energy and environmental challenges.
NATIONAL SCIENCE REVIEW
(2022)
Article
Chemistry, Multidisciplinary
Huaping Wang et al.
Summary: By employing an additive strategy, the decomposition of PF6- and the formation of a stable NaF-rich solid electrolyte interphase (SEI) were achieved, resulting in the inhibition of dendrite growth on high-capacity sodium (Na) anodes. The use of electrolytes containing 4-acetylpyridine (4-APD) enabled excellent cycling performance and stability.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2022)
Article
Engineering, Multidisciplinary
Rupam Sahoo et al.
Summary: A highly capacitive two-dimensional nickel-metal organic framework was developed and combined with graphene oxide to create an effective supercapacitor device with high energy and power densities, and excellent cycle life retention.
COMPOSITES PART B-ENGINEERING
(2022)
Article
Chemistry, Physical
Rupam Sahoo et al.
Summary: This article introduces the research progress of metal-organic frameworks and coordination polymers as solid-state proton conductors, and discusses key examples of proton conduction driven by coordinated water molecules. These materials have promising applications due to their structural superiority and wide range of proton conductivity.
ACS ENERGY LETTERS
(2022)
Article
Chemistry, Physical
George Shimizu et al.
Summary: This study demonstrates a rational assembly of a permselective gas diffusion electrode for direct CO2 conversion, achieving high faradaic efficiency by using a metal-organic framework mixed matrix membrane that enables selective permeation of CO2 to a silver electrocatalyst. By preventing loss of current towards parasitic reactions and maintaining constant CO selectivity over time, this approach offers potential for direct utilization of low-concentration CO2 without the need for purified feedstocks.
ACS ENERGY LETTERS
(2022)
Article
Chemistry, Physical
Prakas Samanta et al.
Summary: In this study, an asymmetric-bipolar Zn-ion battery (ZiB) was proposed, in which the cathode and anode work at different pHs to improve energy density. Efficiency of Zn2+ accepting the host was enhanced through modification of the MoS2 layer. Investigation on charge storage mechanisms was conducted.
ACS APPLIED ENERGY MATERIALS
(2022)
Review
Chemistry, Multidisciplinary
Rupam Sahoo et al.
Summary: Efforts have been made to separate CO2 from flue gas and biogas using nonthermal-based separations, such as adsorption-based or membrane-separation technology employing metal-organic frameworks (MOFs). This review summarizes the strategies, performance parameters, and molecular-level mechanisms of such separations, and offers critical insights and future recommendations for further development of MOF materials as flue and biogas separators.
ADVANCED FUNCTIONAL MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Baghendra Singh et al.
Summary: This study demonstrates the control over the structure of precatalysts to tune the properties of active catalysts and their water oxidation activity, where PC-2 can be easily transformed into an active catalyst within 15 CV cycles while PC-1 requires 600 CV cycles. The presence of high valent Co3+ and Fe3+ in AC-2 helps in improving water oxidation activity.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2022)
Review
Chemistry, Multidisciplinary
Jing Zhu et al.
Summary: Due to the excessive consumption of nonrenewable resources, the exploration of effective and durable materials for sustainable energy conversion and storage is highly sought after. Metal-organic frameworks (MOFs) are a new class of hybrid materials that have gained traction in energy-related fields. Vanadium-MOFs (V-MOFs) possess unique structural characteristics and satisfactory electrochemical properties. Furthermore, V-MOFs-derived materials also exhibit superior electrical conductivity and stability when used as electrocatalysts and electrode materials. This review summarizes the research progress and potential applications of V-MOFs and their derivatives in electrochemical energy conversion and storage. Future possibilities and challenges in terms of design and synthesis are also discussed.
Article
Chemistry, Multidisciplinary
Anh N. Hong et al.
Summary: Pore space partition (PSP) concept is a synthetic design concept that can be used for next-step synthetic planning and execution. PSP provides a tool to design new materials platforms by focusing on chemistry and topology. The growing importance of small-molecule gas storage and separation has led to the development of small-pore materials using the uniquely suited PSP strategy. The partitioned-acs (pacs) platform is the best embodiment of the PSP concept and has resulted in a large family of chemically robust materials with controllable pore metrics and suitable functionalities.
Article
Chemistry, Multidisciplinary
Fahui Xiang et al.
Summary: Stimuli-responsive proton-conducting metal-organic frameworks (MOFs) have attracted attention due to their potential applications. This Perspective highlights the current progress in the rational design and fabrication of switchable proton-conducting MOFs, discussing the dynamic structural changes of proton transfer pathways and the role of trigger molecules. Challenges and new research opportunities for further development are also discussed.
Review
Chemistry, Multidisciplinary
Soheila Sanati et al.
Summary: This review focuses on the use of MOF-derived bimetallic materials in supercapacitors, highlighting their advantages including tunable electrochemical activity, high charge capacity, and improved electrical conductivity. The challenges and perspectives in this research area are also discussed.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2021)
Review
Chemistry, Inorganic & Nuclear
Ehsan Binaeian et al.
Summary: This article discusses the removal of ammonia, hydrogen sulfide, sulfur dioxide, and volatile organic compounds, introducing the design and synthesis achievements of metal-organic frameworks (MOFs) as adsorbents.
COORDINATION CHEMISTRY REVIEWS
(2021)
Article
Materials Science, Multidisciplinary
Cong Li et al.
Summary: Improving discharge-charge reversibility by enhancing structural stability through in situ growth of MOF-derived V2O3 on carbon cloth has demonstrated high capacity retention and cycling stability. The stable cathode structure and oxygen vacancy defects play a crucial role in achieving high discharge specific capacity.
Review
Chemistry, Physical
Shyam Chand Pal et al.
Summary: Solid-state proton-conducting materials, such as hydrogen-bonded organic frameworks (HOFs), are essential in various electrochemical devices like fuel cells. HOFs with well-defined H-bonded networks exhibit high stability with permanent microporosity, making them versatile platforms for solid-state proton conductors showing high conductivity potential. The development of HOFs as proton conductors, along with the considerations of early reports on proton-conducting systems and alternative terminologies, is discussed in depth in this review, with a focus on the design principles and critical features for realizing efficient conduction properties.
ACS ENERGY LETTERS
(2021)
Article
Engineering, Environmental
Yu-Chang Wang et al.
Summary: This article focuses on the research of metal-organic frameworks (MOFs) and their composites as photocatalysts, highlighting their structural strategies, photoelectron trajectories, and structure-function relationship. The potential of these photocatalysts in pollutants degradation, water splitting for H-2 generation, and CO2 reduction is emphasized for future high-efficiency catalyst design.
CHEMICAL ENGINEERING JOURNAL
(2021)
Article
Chemistry, Multidisciplinary
Santanu Chand et al.
Summary: The study developed a metal organic framework-based fluorescent sensor for effective detection of Al(III) with a low detection limit of 17.5 ppb, even in the presence of other metal ions. The research also demonstrated a method of real-time naked eye observation using MOF filter paper tests.
CHEMISTRY-A EUROPEAN JOURNAL
(2021)
Review
Chemistry, Inorganic & Nuclear
Chunfei Wang et al.
Summary: Coordination-based molecular nanomaterials with well-defined chemical structures, high synthetic reproducibility, and diverse functionalities bridge the gap between small molecules and conventional nanomaterials. They have shown great potential in biomedically relevant applications such as biosensing, bioimaging, and therapy.
COORDINATION CHEMISTRY REVIEWS
(2021)
Review
Chemistry, Physical
Rupam Sahoo et al.
Summary: COFs are a promising class of solid-state proton-conducting materials with high structural tunability and excellent properties, making them versatile platforms for electrochemical devices. This review discusses the strategies, structure-function relationships, challenges, and future prospects of COFs as proton conductors in detail.
ADVANCED ENERGY MATERIALS
(2021)
Article
Multidisciplinary Sciences
T. Paul et al.
Summary: In this paper, DRT functions are numerically calculated for different systems with impedance data, and the quality of impedance data is checked using Kramers-Kronig relations. The DRTs are calculated using Tikhonov regularization method and the physical significance of peaks are discussed through peak fitting program.
SCIENTIFIC REPORTS
(2021)
Article
Chemistry, Physical
Prakas Samanta et al.
Summary: Rechargeable aqueous Zn-ion batteries have drawn attention for their low cost and environmental friendliness. The performance of these batteries can be enhanced by involving both cationic and anionic redox conversion mechanisms simultaneously.
ACS APPLIED ENERGY MATERIALS
(2021)
Review
Chemistry, Inorganic & Nuclear
Rupam Sahoo et al.
Summary: Gas separation processes have a significant impact on various sectors globally. The removal of C-2 hydrocarbons from natural gas is a crucial step, with MOFs offering promise for such separations. Challenges and future prospects in this area are discussed in detail for further development.
COORDINATION CHEMISTRY REVIEWS
(2021)
Review
Chemistry, Multidisciplinary
Zhigang Hu et al.
Summary: Metal-organic frameworks (MOFs) are formed by the coordination connection of organic linkers to metal clusters, with tunable ligands providing robust molecular porosity. Hafnium (Hf) and tetravalent cerium [Ce(iv)] MOFs have shown promise for practical applications, with a focus on their chemistry, topologies, synthetic strategies, and diverse applications. Future research will explore the development of Hf/Ce-MOFs, including fundamental design, defect engineering, and computational approaches for tailor-made applications.
CHEMICAL SOCIETY REVIEWS
(2021)
Article
Chemistry, Multidisciplinary
Hou-Gan Zhou et al.
Summary: In this study, a pair of isostructural 2D copper(i) organic frameworks with different interlayer stacking structures were successfully prepared by combining the chemistry of MOFs and COFs. The variation in interlayer stacking significantly influences their functionality, including porosity, chemical stability, and catalytic activities. Additionally, a structure transformation between the two frameworks was achieved by a simple addition of trifluoroacetic acid, resulting in in situ acceleration of adoption rate, which is uncommon in 2D MOFs and COFs.
Review
Chemistry, Multidisciplinary
Rui-Biao Lin et al.
Review
Chemistry, Multidisciplinary
Qi Zhang et al.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2020)
Review
Chemistry, Multidisciplinary
Jie Yang et al.
Review
Chemistry, Physical
Tianjie Qiu et al.
ACS ENERGY LETTERS
(2020)
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Hao Luo et al.
Review
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Dae-Woon Lim et al.
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Meena Ghosh et al.
ACS SUSTAINABLE CHEMISTRY & ENGINEERING
(2020)
Review
Chemistry, Multidisciplinary
Xiaoxiao Jia et al.
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Rupam Sahoo et al.
CHEMISTRY-A EUROPEAN JOURNAL
(2020)
Article
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Shenzhen Deng et al.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2020)
Article
Engineering, Environmental
Yongling An et al.
CHEMICAL ENGINEERING JOURNAL
(2020)
Article
Chemistry, Physical
Qiancheng Zhu et al.
JOURNAL OF MATERIALS CHEMISTRY A
(2020)
Review
Chemistry, Multidisciplinary
Ning Zhang et al.
CHEMICAL SOCIETY REVIEWS
(2020)
Review
Chemistry, Physical
Chun-Chao Hou et al.
ADVANCED ENERGY MATERIALS
(2019)
Article
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Youcai Ding et al.
APPLIED SURFACE SCIENCE
(2019)
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Bing He et al.
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Xing Zhou et al.
JOURNAL OF POWER SOURCES
(2019)
Article
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Zhuo Wang et al.
Review
Chemistry, Physical
Aishuak Konarov et al.
ACS ENERGY LETTERS
(2018)
Article
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Haigang Qin et al.
JOURNAL OF MATERIALS CHEMISTRY A
(2018)
Article
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Yaping Hou et al.
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Steven Chu et al.
Review
Engineering, Environmental
Youssef Belmabkhout et al.
CHEMICAL ENGINEERING JOURNAL
(2016)
Review
Chemistry, Inorganic & Nuclear
Lu Wang et al.
COORDINATION CHEMISTRY REVIEWS
(2016)
Review
Chemistry, Multidisciplinary
Elisa Barea et al.
CHEMICAL SOCIETY REVIEWS
(2014)
Review
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Jie-Peng Zhang et al.
Article
Chemistry, Applied
Alexandra Lieb et al.
MICROPOROUS AND MESOPOROUS MATERIALS
(2012)
Article
Chemistry, Multidisciplinary
Michel Latroche et al.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2006)
