☆ 4.7 Review

Recent advances in cellulosic materials for aqueous zinc-ion batteries: An overview

CARBOHYDRATE POLYMERS (2023)

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A strategy for generating value-added aromatic monomers and lignocellulosic nanofibrils simultaneously from lignocellulosic biomass via polyoxometalate-mediated oxidative fractionation

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Summary: This study presents an efficient strategy for separating lignocellulosic biomass into valuable products, including phenolic products derived from lignin and LCNFs derived from cellulose. The lignin can be completely removed and disassembled into phenolic products, while most of the cellulose remains as fibrous water-insoluble solid. In addition, a mild disk grinding strategy is proposed to fibrillate cellulose-rich WIS into LCNFs, which can be tailored to different diameters.

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Active-site and interface engineering of cathode materials for aqueous Zn-gas batteries

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Summary: Aqueous rechargeable Zn-gas batteries are considered promising energy storage and conversion devices due to their safety and environmental friendliness. However, their energy efficiency and power density are limited by slow cathode reactions. This review introduces battery configurations and fundamental reactions, summarizes recent advances in active site engineering and cathode material regulation strategies, and provides personal perspectives on the future development of Zn-gas batteries.

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Review Chemistry, Physical

Active-site and interface engineering of cathode materials for aqueous Zn-gas batteries

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Summary: This review introduces aqueous rechargeable Zn-gas batteries and the challenges they face, discusses recent advances in enhancing the intrinsic catalytic activities of cathode catalysts and optimizing the performance of Zn-gas batteries, and presents personal perspectives for future development.

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Ion Sieve: Tailoring Zn2+ Desolvation Kinetics and Flux toward Dendrite-Free Metallic Zinc Anodes

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Summary: This study presents an ion sieve coating that effectively inhibits dendrite growth on metallic zinc anodes, improving the rechargeability of aqueous zinc metal batteries. Experimental and theoretical analyses demonstrate that the coating facilitates the desolvation of zinc clusters, weakens hydrogen evolution reaction, and homogenizes ion flux, resulting in dendrite-free zinc deposition. The symmetric cell with the ion sieve coating shows a lifespan of up to 3000 hours, highlighting the enhanced performance of zinc metal batteries.

ACS NANO (2022)

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Article Chemistry, Physical

Manipulating Ion Concentration to Boost Two-Electron Mn4+/Mn2+ Redox Kinetics through a Colloid Electrolyte for High-Capacity Zinc Batteries

Xuesong Xie et al.

Summary: By using an ion concentration/dilution strategy, the capacity and efficiency of Zn/MnO2 batteries can be improved, leading to enhanced performance in terms of capacity release, cycle life, and elevated-temperature endurance.

ADVANCED ENERGY MATERIALS (2022)

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Article Chemistry, Physical

Cotton-derived cellulose film as a dendrite-inhibiting separator to stabilize the zinc metal anode of aqueous zinc ion batteries

Weijun Zhou et al.

Summary: This study utilizes a cotton-derived cellulose film as a separator for AZIBs, which effectively inhibits zinc dendritic growth and harmful side reactions due to its excellent mechanical properties and ionic conductivity. Batteries with this separator show stability and high capacity, as well as improved rate capability and cyclability.

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Article Engineering, Environmental

Manipulating Zn-ion flux by two-dimensional porous g-C3N4 nanosheets for dendrite-free zinc metal anode

Yi Yang et al.

Summary: Zinc metal anode is a promising choice in aqueous zinc ion batteries, but zinc dendrite growth compromises its practicability. In this study, a modified separator was developed by coating g-C3N4 nanosheets onto commercial cellulose fiber separator. The g-C3N4 coated separator enables dendrite-free zinc deposition and improves the reversibility of zinc metal anodes.

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A high strength, anti-corrosion and sustainable separator for aqueous zinc-based battery by natural bamboo cellulose

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Summary: The use of bamboo cellulose membrane as a separator for zinc-based batteries has been found to greatly improve battery performance. The membrane's natural nano-scale pores and high tensile strength effectively block zinc dendrite penetration and facilitate uniform deposition. Additionally, the membrane exhibits excellent corrosion resistance.

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Facile and green synthesis of nanocellulose with the assistance of ultraviolet light irradiation for high-performance quasi-solid-state zinc-ion batteries

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An Ion-Sieving Janus Separator toward Planar Electrodeposition for Deeply Rechargeable Zn-Metal Anodes

Xiaotan Zhang et al.

Summary: A Janus separator was constructed using spin-coating technique, which can continuously regulate the growth of zinc and achieve a locked crystallographic orientation of zinc(002) texture to intercept dendrites. The separator also has the capability to repel SO42- and anchor H+ while allowing effective transport of Zn2+. This work demonstrates the importance of continuous regulation for achieving crystallographic homogeneity of the Zn anode in metal batteries.

ADVANCED MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Synergic Effect of Dendrite-Free and Zinc Gating in Lignin-Containing Cellulose Nanofibers-MXene Layer Enabling Long-Cycle-Life Zinc Metal Batteries

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Summary: This study reports a bifunctional layer to stabilize the interface of zinc anode, which improves the performance of the battery through zinc gating and diffusion limited dendrite suppression. In Zn//Cu asymmetric cells, the LM layer achieves high coulombic efficiency and low overpotential. In Zn//MnO2 full cells, the LM layer enables high-capacity retention, surpassing the cells without a protective layer.

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Achieving ultra-long lifespan Zn metal anodes by manipulating desolvation effect and Zn deposition orientation in a multiple cross-linked hydrogel electrolyte

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Summary: A novel polyacrylamide-poly (ethylene glycol) diacrylate-carboxymethyl cellulose (PMC) hydrogel electrolyte is designed to overcome the obstacles of high desolvation energy barrier and inhomogeneous Zn2+ flux in aqueous zinc-ion batteries (ZIBs). The PMC hydrogel electrolyte reduces the desolvation energy barrier and guides the preferential orientation of Zn deposition, leading to improved performance and an ultra-long cycle life of 5000 hours with a high coulombic efficiency of 99.5%.

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A piece of common cellulose paper but with outstanding functions for advanced aqueous zinc-ion batteries

Zefang Yang et al.

Summary: The direct implantation of commercially available cellulose paper in aqueous zinc-ion batteries improves their overall performance by reducing by-product accumulation and preventing the shuttle of vanadium ions, leading to an outstanding long cycle life and high performance.

MATERIALS TODAY ENERGY (2022)

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Sorbitol-modified cellulose hydrogel electrolyte derived from wheat straws towards high-performance environmentally adaptive flexible zinc-ion batteries

Yuhui Quan et al.

Summary: In this study, a food-grade sorbitol-modified cellulose hydrogel electrolyte with concentrated ZnCl2 was developed, which exhibited excellent mechanical properties, strong adhesion, high transparency, good moldability, rich porosity, ultralow freezing point, and large ionic conductivity. The modified hydrogel electrolyte enabled high zinc stripping/plating reversibility even under extreme temperatures, resulting in superior electrochemical performances in the assembled flexible Zn-PANI battery.

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PBC@cellulose-filter paper separator design with efficient ion transport properties toward stabilized zinc-ion battery

Linbo Li et al.

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Environmentally adaptable hydrogel electrolyte with the triple interpenetrating network in the flexible zinc-ion battery with ultralong stability

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Summary: With the increasing demand for stable flexible batteries in wearable electronic devices, the limitations of traditional aqueous electrolytes in cold conditions have hindered the practical application of aqueous zinc ion batteries. In this study, a hydrogel electrolyte with a triple interpenetrating network was developed, which exhibited stable mechanical compression deformation and broadened the operating temperature range. The hydrogel electrolyte enabled highly reversible Zn2+ insertion/extraction and accelerated ion transfer, leading to high capacity and cycling stability of the zinc ion batteries.

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Cellulose-Acetate Coating by Integrating Ester Group with Zinc Salt for Dendrite-Free Zn Metal Anodes

Xu Liu et al.

Summary: The study demonstrates the effectiveness of ion-affiliative cellulose acetate (CA) coating with Zn(CF3SO3)(2) on Zn anode in suppressing zinc dendrite formation and growth in aqueous electrolytes. The symmetric CAZ@Zn//CAZ@Zn battery shows significantly improved reversible plating/stripping performance compared to bare Zn, while the full cell with optimized Zn anode and NH4V4O10 cathode achieves substantially stable performance, outperforming bare Zn.

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Wood-based electrodes enabling stable, anti-freezing, and flexible aqueous zinc-ion batteries

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Summary: A wood-based quasi-solid-state aqueous zinc ion battery has been developed to address the issues of low reversibility and tolerance to low-temperature environments. The wood-based electrode exhibits good conductivity and affinity to the electrolyte, and effectively stabilizes the zinc deposition behavior. The assembled wood-based battery delivers superior performance even at low temperatures and under bending.

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Stable Thermochromic Hydrogel for a Flexible and Wearable Zinc- Ion Yarn Battery with High-Temperature Warning Function

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Summary: This study developed a hydrogel-based zinc-ion yarn battery with excellent thermochromic features and electrochemical performance. It has great potential for high-temperature warning and effectively avoiding low-temperature scalding, providing a new approach and application for developing reliable, durable, and wearable smart batteries.

ACS APPLIED ENERGY MATERIALS (2022)

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Esterification of cellulose using carboxylic acid-based deep eutectic solvents to produce high-yield cellulose nanofibers

Suling Liu et al.

Summary: This study utilized carboxylic acid-based deep eutectic solvents for pretreating cellulose, resulting in the production of cellulose nanofibers with widths less than 100 nm through simultaneous esterification modifications. Esterification modifications prevented over-hydrolysis and dissolution of cellulose while maintaining the cellulose I crystal structure. The esterified cellulose nanofibers showed improved dispersibility and interfacial compatibility with polylactic acid, leading to mechanical enhancement of CNF/PLA composites.

CARBOHYDRATE POLYMERS (2021)

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Article Electrochemistry

Modifying hydrogel electrolyte to induce zinc deposition for dendrite-free zinc metal anode

Yachun Mao et al.

Summary: In recent years, research on flexible aqueous Zn-ion batteries has been promoted, but dendrite growth on the anode and poor mechanical properties of the flexible polymer electrolyte remain challenges. A CMC/PAM hydrogel electrolyte with a double-network structure has been constructed to address these issues, showing promising potential in improving the performance of flexible ZIBs.

ELECTROCHIMICA ACTA (2021)

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Crossroads in the renaissance of rechargeable aqueous zinc batteries

Junhua Song et al.

Summary: Aqueous zinc batteries are dominating the primary battery market with alkaline chemistries and are now being developed as rechargeable devices for grid-scale energy storage applications. Significant progress has been made in improving cyclability in alkaline, neutral, and mild acidic systems, with a focus on static closed cell designs in this review. Challenges and advancements in developing highly rechargeable alkaline and mild acidic batteries are examined, while flow batteries and open systems like zinc-air batteries are excluded due to space constraints.

MATERIALS TODAY (2021)

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Electrolyte Concentration Regulation Boosting Zinc Storage Stability of High-Capacity K0.486V2O5 Cathode for Bendable Quasi-Solid-State Zinc Ion Batteries

Linpo Li et al.

Summary: By regulating the concentration of ZnCl2 electrolyte, the cycle life of Vanadates in AZIBs can be greatly improved without the need to approach the water-in-salt threshold. Additionally, a novel CMC-ZnCl2 gel electrolyte with high ionic conductivity was designed for the first time, enabling the assembly of a quasi-solid-state AZIB with excellent stability and energy density.

NANO-MICRO LETTERS (2021)

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Article Chemistry, Multidisciplinary

Realizing an All-Round Hydrogel Electrolyte toward Environmentally Adaptive Dendrite-Free Aqueous Zn-MnO2 Batteries

Minfeng Chen et al.

Summary: A all-round hydrogel electrolyte was developed using cotton, tetraethyl orthosilicate, and glycerol, exhibiting high ionic conductivity and excellent mechanical properties.

ADVANCED MATERIALS (2021)

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Article Engineering, Environmental

Highly stable H2V3O8/Mxene cathode for Zn-ion batteries with superior rate performance and long lifespan

Chaozheng Liu et al.

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CHEMICAL ENGINEERING JOURNAL (2021)

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Article Chemistry, Physical

Ultra-stable and highly reversible aqueous zinc metal anodes with high preferred orientation deposition achieved by a polyanionic hydrogel electrolyte

Jianlong Cong et al.

Summary: The newly designed PAMPSZn hydrogel electrolyte shows effectiveness in alleviating side reactions and preventing Zn dendrites formation in AZMBs, allowing for stable Zn plating/stripping and high preferred orientation deposition during cycles. Compared to traditional electrolytes, it exhibits higher coulombic efficiency and cycle stability in both Zn/Cu and Zn/V2O5 cells.

ENERGY STORAGE MATERIALS (2021)

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Article Chemistry, Physical

Modulating Zn deposition via ceramic-cellulose separator with interfacial polarization effect for durable zinc anode

Jin Cao et al.

Summary: A cellulose nanofibers-ZrO2 composite separator (ZC) has been developed to stabilize the zinc anode in aqueous zinc-ion batteries, enabling excellent ionic conductivity and high Zn2+ transfer number. The ZrO2 particles with high dielectric constant offer a directional electric field to regulate uniform zinc deposition, accelerate Zn2+ ions diffusion kinetics, and repel anions, resulting in dendrite-free plating/stripping behavior, high Coulombic efficiency and exceptional cyclability for the zinc anode.

NANO ENERGY (2021)

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Article Nanoscience & Nanotechnology

In Situ Construction of a Multifunctional Quasi-Gel Layer for Long-Life Aqueous Zinc Metal Anodes

Jingyi Ding et al.

Summary: A hydrophilic layer composed of a covalent organic polymer (COP) and carboxylmethyl cellulose (CMC) is designed to improve the performance of aqueous zinc-ion batteries, enhancing Zn2+ transport kinetics, guiding uniform nucleation, and suppressing Zn corrosion and H-2 evolution.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Physical

Integrated design of aqueous zinc-ion batteries based on dendrite-free zinc microspheres/carbon nanotubes/nanocellulose composite film anode

Anran Wang et al.

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JOURNAL OF COLLOID AND INTERFACE SCIENCE (2021)

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Solution-processed perylene diimide-ethylene diamine cathodes for aqueous zinc ion batteries

Biao Jiang et al.

Summary: In this study, high-yield and high-performance organic electroactive compound PDI-EDA/CB composites were prepared via a solution-based method for application as cathodes in ZIBs. The composites showed high specific capacity, stability at high current density, and good cycling stability, outperforming many recently reported ZIB cathodes. The excellent electrochemical performance of PDI-EDA/CB was attributed to its zinc ion storage mechanism and solution-based fabrication method.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2021)

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Jin Cao et al.

Summary: A functional separator composed of cellulose nanofibers and graphene oxide is developed for dendrite-free and stable zinc ion batteries. This separator promotes uniform zinc deposition and significantly enhances the performance of zinc anodes in various types of batteries.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Physical

Impact of Binder Functional Groups on Controlling Chemical Reactions to Improve Stability of Rechargeable Zinc-Ion Batteries

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ACS APPLIED ENERGY MATERIALS (2021)

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