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Article
Biochemistry & Molecular Biology
Enmin Zong et al.
Summary: This study presents a novel magnetically recyclable bio-adsorbent for removing Congo red dye from water. The adsorbent exhibits easy separation and excellent anti-interference capability, with a removal efficiency of 92% after five consecutive cycles. This work provides a sustainable strategy for the development of efficient, separable, and recyclable bio-derived adsorbents for organic dye removal.
INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES
(2023)
Article
Nanoscience & Nanotechnology
Wenwen Jia et al.
Summary: Excessive use of pesticides poses serious environmental risks and harm to human health. This study developed gel capsules based on metal-organic frameworks (MOFs) for pesticide detection and removal. The capsules showed sensitive detection of pesticide residues and could be used for water decontamination and food safety control.
ACS APPLIED MATERIALS & INTERFACES
(2023)
Article
Nanoscience & Nanotechnology
Kunyao Cao et al.
Summary: An ultralight Ni-MOF-rGO aerogel with broad bandwidth and strong absorption, as well as lightweight and thin matching thickness, was fabricated through hydrothermal treatment, freeze-drying, and annealing. The composite achieved outstanding microwave absorption performance with a thickness of 1.9 mm and 2 wt% filling content, showing strong absorption (-51.19 dB) and broad effective absorption bandwidth (6.32 GHz). The unique multiple layered structure of GO and the hollow core-shell structure of Ni@C microsphere contribute to the extraordinary microwave absorption performance.
ACS APPLIED MATERIALS & INTERFACES
(2023)
Article
Chemistry, Multidisciplinary
Ilia Kochetygov et al.
Summary: In this work, a new strategy for ligand design is proposed, using piperazine and dihydrophenazine units as substitutes for benzene rings, via simple nucleophilic aromatic substitution reactions without using transition metal catalysts. 21 carboxylate-based ligands with varying sizes, shapes, and denticity and 15 linear di- and tetra-nitriles were successfully synthesized. Moreover, 16 structurally diverse MOFs with surface areas up to 3100 m(2) g(-1) were synthesized using these ligands as building blocks.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2023)
Article
Agricultural Engineering
Lijun Li et al.
Summary: A Cu2+-doped lignin-based adsorbent (Cu-AL) was prepared for massive and selective adsorption of cationic dyes Azure B (AB) and Saffron T (ST) through amination and Cu2+ doping of industrial alkali lignin. The adsorption capacities of AB and ST on Cu-AL reached up to 1168 and 1420 mg g-1, respectively, due to electrostatic attraction, pi-pi interaction, H-bonding, and Cu2+ coordination. Cu-AL showed high removal efficiency for dyes even after 4 reuses (>80%), and could efficiently remove and separate AB and ST from dye mixtures in real time.
BIORESOURCE TECHNOLOGY
(2023)
Article
Chemistry, Applied
Zhiqiang Wang et al.
Summary: By integrating renewable chitin, lignin, and plant oil, fully biobased sustainable elastomers with excellent mechanical strength and UV-blocking property were developed. The incorporation of a dynamic cross-linked network further improved the macroscopic behavior of these chitin graft elastomers. This strategy is versatile and can inspire the further development of fully biobased sustainable materials.
CARBOHYDRATE POLYMERS
(2023)
Article
Engineering, Environmental
Vinayak Hegde et al.
Summary: In recent years, porous metal-organic frameworks (MOFs) and biopolymer-based materials have been widely used as adsorbents for wastewater purification. However, they have some drawbacks such as stability concerns, recovery difficulty, and high synthetic cost. To overcome these limitations, a novel porous composite of keratin biopolymer and cerium MOF (Ce-UiO-66 MOF) was designed for the treatment of dye-contaminated wastewater. The designed composite showed excellent removal efficiency and adsorption capacity, as well as promising performance in the presence of interfering ions, real-time sample analysis, and recyclability.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Biochemistry & Molecular Biology
Boyu Du et al.
Summary: The application of lignin activation by demethylation has attracted intensive attention recently for its potential to improve reactivity and enrich multiple functions. Nevertheless, the low reactivity and complexity of the lignin structure pose a challenge. This study explored an effective demethylation method utilizing microwave assistance to enhance the hydroxyl (-OH) content and preserve the lignin structure. The demethylated lignin showed promising performance in the removal of heavy metal ions and wound healing applications, demonstrating its high value potential.
INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES
(2023)
Article
Biochemistry & Molecular Biology
Zhenyu Jing et al.
Summary: Zirconium alginate/graphene oxide (ZA/GO) hydrogel spheres were prepared and used as the substrate for the in-situ growth of UiO-67 crystal. The ZA/GO/UiO-67 aerogel spheres showed a high adsorption capacity of 1105.23 mg/g for methylene blue, following the pseudo-first-order kinetic model and single-layer adsorption. This study highlights the potential of ZA/GO/UiO-67 aerogel spheres for efficient adsorption and reuse.
INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES
(2023)
Article
Biochemistry & Molecular Biology
Chao Wang et al.
Summary: In this study, bio-based hydrogels (LN-NH-SA hydrogel) were prepared from aminated lignin and sodium alginate. The physical and chemical properties of the hydrogel were characterized using various techniques. The LN-NH-SA@3 hydrogel showed high adsorption efficiency for methylene blue and maintained good adsorption efficiency after multiple cycles. Overall, the environmentally friendly and cost-effective LN-NH-SA@3 hydrogel shows promise for dye adsorption.
INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES
(2023)
Article
Nanoscience & Nanotechnology
Norah Alsadun et al.
Summary: The ongoing global industrialization and population growth pose a challenge to the global environment and water and food needs. Therefore, an improved irrigation management system and refined chemical sensors for soil-moisture monitoring are of great importance. However, the challenge lies in designing and constructing stable materials with the necessary sensitivity, selectivity, and high performance.
ACS APPLIED MATERIALS & INTERFACES
(2023)
Article
Nanoscience & Nanotechnology
Xiang Liu et al.
Summary: A novel metal-organic framework adsorbent (UiO-FHD) is developed, which efficiently and selectively captures lead ions by introducing multiple ligands. The maximum adsorption capacity of lead ions is 433.15 mg/g at pH 5. The adsorption process follows pseudo-second-order kinetic and Langmuir isotherm models, and appropriate temperature reduction facilitates the removal of Pb(II). Performance tests show that UiO-FHD maintains a high removal rate of 90.35% for Pb(II) after four consecutive adsorption-desorption cycles.
ACS APPLIED MATERIALS & INTERFACES
(2023)
Article
Agricultural Engineering
Hanjun Zhou et al.
Summary: In this study, honeycomb lignin-based biochar (HLB) was prepared by hydrothermal activation using industrial lignin as raw material for the removal of norfloxacin from water. Batch adsorption tests showed that HLB has a strong and selective ability to remove norfloxacin at various pH levels with a high adsorption capacity. The highly aromatized structure of HLB and the abundant oxygen-containing functional groups contribute to the effective removal of norfloxacin.
BIORESOURCE TECHNOLOGY
(2023)
Article
Chemistry, Applied
Zhi Chen et al.
Summary: In this study, a polyethyleneimine-modified chitosan/Ce-UIO-66 composite hydrogel (PEI-CS/Ce-UIO-66) was successfully prepared using the ex-situ blend method. The synthesized composite hydrogel was characterized and its adsorption performance for methyl orange (MO) was evaluated. The results showed that PEI-CS/Ce-UIO-66 exhibited excellent adsorption properties for MO through electrostatic interaction, pi-pi stacking, and hydrogen bonding. These findings suggest that the PEI-CS/Ce-UIO-66 composite hydrogel has potential for the adsorption of anionic dyes.
CARBOHYDRATE POLYMERS
(2023)
Article
Chemistry, Applied
Shadpour Mallakpour et al.
Summary: A novel effective bio adsorbent, Zn-Al LDH@NH2-MIL-125(Ti) hybrid, was produced and used to remove congo red and methylene blue dyes from water matrices. The hybrid showed good adsorption capacity and efforts were made to improve reusability and prevent secondary contamination.
CARBOHYDRATE POLYMERS
(2023)
Article
Environmental Sciences
Mengying Xu et al.
Summary: Effective strategies are critical to improve charge separation in semiconductor particles for enhancing the photodegradation of organic pollutants. In this study, Bi2MoO6 (BMOMOF) nanoparticles and quantum dots were synthesized from a bismuth-based metal-organic framework (Bi-MOF) precursor. The combination of surface defects, NPs and QDs in BMOMOF improved charge separation and facilitated redox reactions. The BMOMOF photocatalyst was more efficient in degrading widely-used antibiotics and carcinogenic pollutants compared to BMO derived from uncoordinated Bi. Loading BMOMOF on biopolymer bacterial cellulose significantly enhanced photocatalytic performance and facilitated material recovery after water treatment processes.
Article
Environmental Sciences
Yue Gao et al.
Summary: A robust EDTA-UiO-66-NH2/CFC material was prepared for simultaneous removal of heavy metals, dyes, and chemical warfare agents. The material showed high adsorption and catalytic performance, and could be reused multiple times without loss of efficiency. This study provides a simple and versatile synthetic strategy for developing high-performance environmental materials for multiple pollutants remediation.
ENVIRONMENTAL POLLUTION
(2023)
Article
Agricultural Engineering
Yongchang Sun et al.
Summary: A novel Fe-modified lignin-based biochar (Fe-LB) was successfully fabricated for methylene blue (MB) removal, demonstrating high specific surface area and micropore volume compared to traditional LB. Fe-LB exhibited quick adsorption of MB with a maximum adsorption capacity of 2.7-fold higher than LB, achieving 100% removal efficiency in 15 minutes. Furthermore, Fe-LB showed selective adsorption preference for MB in a wide pH range and high salt environments, making it a promising candidate for dye wastewater treatment.
BIORESOURCE TECHNOLOGY
(2022)
Article
Engineering, Environmental
Sheng-Nan Zhuo et al.
Summary: The biomass pretreatment liquor (PL) produced from rice straw pretreatment can be used as a new flocculant to effectively remove anionic dyes from wastewater. This research is significant for future water environment remediation and material development.
JOURNAL OF HAZARDOUS MATERIALS
(2022)
Article
Nanoscience & Nanotechnology
Chuan Zhou et al.
Summary: A series of defected granular UiO-66-NH2 metal-organic gels were synthesized for the removal of sulfur mustard simulant 2-CEES, showing high degradation rate and adsorption capacity.
ACS APPLIED MATERIALS & INTERFACES
(2022)
Article
Agricultural Engineering
Marut Jain et al.
Summary: Activated biochar derived from cow-dung shows excellent adsorption capacity for phenol in wastewater, with an adsorption efficiency of approximately 98.8%.
BIORESOURCE TECHNOLOGY
(2022)
Article
Environmental Sciences
Ji Won Heo et al.
Summary: Research on low-cost bio-adsorbents for the removal of harmful substances from effluents has gained significant attention. This study prepared three types of amino-silane-modified lignins and investigated their adsorption behavior towards cationic and anionic dyes. The results showed that the amino-silane reagents resulted in different molecular self-assembly structures on the lignin surface. The ASLs exhibited excellent adsorption capacities and selectivity based on the pH conditions.
Article
Chemistry, Multidisciplinary
Qian Wang et al.
Summary: In this study, polyoxometalate-based molybdenum trioxide composites were successfully prepared and exhibited excellent adsorption capacity for anionic dyes through strong electrostatic interactions. Among the composites, Al-13-3.34%@MoO3 showed the most remarkable adsorption capacity and maintained stable performance after five consecutive adsorption/desorption cycles.
CHINESE CHEMICAL LETTERS
(2022)
Article
Engineering, Chemical
Xueting Liu et al.
Summary: In this study, metal-organic frameworks (MOFs) catalysts with NH2-UiO-66-xHAc structure were synthesized using acetic acid (HAc) as a modulator, and applied to the cycloaddition reaction. The results showed that the modulation by HAc influenced the morphologies and structures of the MOFs, and optimizing the amount of HAc could enhance the catalytic activity of NH2-UiO-66-xHAc.
CHINESE JOURNAL OF CHEMICAL ENGINEERING
(2022)
Article
Engineering, Environmental
Hao Wang et al.
Summary: UiO-66-AMP, a novel zirconium-based adsorption material modified from UiO-66-NH2 with 5-adenosine, showed efficient removal of Pb(II) and Cr(VI) from wastewater. Experimental results confirmed its high adsorption capacity for both metal ions, attributed to surface complexation and electrostatic interactions. The adsorption process followed pseudo-second-order and Langmuir models, indicating a single-layer chemical process.
JOURNAL OF HAZARDOUS MATERIALS
(2022)
Article
Engineering, Environmental
Li-Lan Zhang et al.
JOURNAL OF HAZARDOUS MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Qiao Zhao et al.
Summary: By integrating metal-organic frameworks (MOFs) based biobarcodes with CRISPR/Cas12a assay, the study achieved sensitive detection of microRNAs, presenting a universal strategy for miRNA detection with high sensitivity.
Article
Chemistry, Analytical
Jiali Liu et al.
Summary: In this study, a fluorescence switching nanoprobe based on amine-functionalized UiO-66-NH2 was developed for highly sensitive and selective detection of U(VI) in water. The functionalization with amine groups greatly enhanced the fluorescence emission and selective sensitivity of UiO-66-NH2 towards U(VI). The sensing mechanism was attributed to the static quenching interaction between U(VI) and the rich functionalized amine groups. The findings provide an efficient fluorescence probe for sensitive U(VI) detection and offer a new strategy of tailored plasma functionalization for enhanced fluorescence emission, sensitivity, and selectivity of MOF sensor platforms.
ANALYTICAL CHEMISTRY
(2022)
Article
Energy & Fuels
Wei Ruan et al.
Summary: A novel composite adsorbent, Uio-66-NH2/AHMP, was successfully synthesized and applied for the removal of Hg2+ from aqueous solution. The Uio-66-NH2/AHMP demonstrated excellent adsorption selectivity and regeneration performance, making it a promising material for Hg2+ removal.
Article
Engineering, Environmental
Kamyar Mirzaei et al.
Summary: A series of ZIF-8/OND hybrid nanostructures with different percentages of oxidized nanodiamond (OND) were prepared and investigated for their adsorptive removal performance towards methylene blue (MB). The results showed that the addition of OND significantly enhanced the adsorption capacity and rate of ZIF-8 towards MB. The adsorption of MB onto ZND 5 was found to be an endothermic, spontaneous, and entropy-governed process.
JOURNAL OF WATER PROCESS ENGINEERING
(2022)
Article
Biochemistry & Molecular Biology
Yan Zhou et al.
Summary: A highly efficient adsorbent, amino-functionalization alkali lignin (AAL), was synthesized for mercury ion removal. AAL exhibited excellent adsorption capacity for Hg2+ at neutral pH and demonstrated high performance in removing Hg2+ from aqueous solutions.
INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES
(2022)
Article
Engineering, Environmental
Rania M. Eltabey et al.
Summary: In this study, poly(maleic acid)-grafted cross-linked chitosan/montmorillonite composite nanospheres (PMAL-CTS/MMT) were synthesized for efficient adsorption of organic dyes. The high adsorption capacity of PMAL-CTS/MMT towards both anionic and cationic dyes can be attributed to the presence of abundant functional groups. The surface charges of PMAL-CTS/MMT can be modulated by adjusting the solution pH, resulting in enhanced affinity towards different types of dyes. The proposed adsorption mechanism involves electrostatic interaction, pi - pi interactions, and hydrogen bonding. Additionally, PMAL-CTS/MMT was successfully utilized for the separation of dyes from real-life aquatic environments.
JOURNAL OF HAZARDOUS MATERIALS
(2022)
Article
Environmental Sciences
Fahim Ullah et al.
Summary: The massive generation of medical waste leads to various environmental, social, and ecological problems. This study focuses on the use of pyrolysis and activation to obtain activated biochar from medical waste and investigates its adsorption mechanism and properties for dyes. The results show that activated biochar has excellent potential for adsorbing both cationic and anionic dyes, making it an economical and efficient adsorbent.
ENVIRONMENTAL POLLUTION
(2022)
Article
Chemistry, Analytical
Muhammad Altaf Nazir et al.
Summary: The research focuses on developing systematic materials to remove hazardous dyes from water. The ZIF-8@ZnAl-LDH composite material shows excellent adsorption capacity for malachite green and methyl orange, indicating its potential for water purification.
MICROCHEMICAL JOURNAL
(2021)
Article
Biochemistry & Molecular Biology
Wenkun Zhang et al.
Summary: The Chitosan crosslinked with MOF-199@aminated graphene oxide aerogel was prepared as an adsorbent for formaldehyde and methyl orange. Characterization and stability tests showed that the aerogel had good adsorption capacity and stability. Adsorption of pollutants followed Freundlich isotherm model and pseudo-second-order model for kinetic behavior.
INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES
(2021)
Article
Chemistry, Multidisciplinary
Kun Dai et al.
Summary: A novel adsorbent lignin-calcium with mesoporous and coarse surface was prepared via a simple method, showing excellent adsorption capability for methylene blue following the Langmuir model, applicable across a wide pH range and regenerable with high efficiency.
Article
Engineering, Environmental
Ehsan Binaeian et al.
Summary: This study developed a new type of Zr-based MOF with higher surface area/vacant, characterized by enhanced ammonia and hydrogen adsorption capacities. The modified MOFs showed stable adsorption performance after multiple cycles and regenerations under different temperature and pressure conditions.
JOURNAL OF HAZARDOUS MATERIALS
(2021)
Article
Engineering, Environmental
Jun Li et al.
Summary: Experimental and calculation methods were used to investigate the adsorption performances of g-C3N4 surface for organic dye pollutants. A molecular-orientation and force-dominance mechanism adsorption model was proposed based on the combined experimental and calculation results. The study revealed the dominating interactions for MB+ and MO- adsorption, providing fundamental basis for the removal of organic dye pollutants by g-C3N4.
JOURNAL OF HAZARDOUS MATERIALS
(2021)
Article
Biochemistry & Molecular Biology
AbdulKarim-Talaq Mohammad et al.
INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES
(2019)
Article
Chemistry, Physical
Jan Gerit Brandenburg et al.
JOURNAL OF CHEMICAL PHYSICS
(2018)
Article
Chemistry, Physical
Jian-Han Huang et al.
COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS
(2008)