期刊
CHEMICAL COMMUNICATIONS
卷 51, 期 89, 页码 16107-16110出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cc05508c
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资金
- MEXT, Japan
Described herein is a highly enantioselective synthesis of fused piperidine and pyrrolidine derivatives with all-carbon stereogenic centers. The enantioselective reductive amination from Cs-symmetric 1,3-dione derivatives proceeded in a highly stereoselective manner by taking advantage of the desymmetrization approach to afford fused heterocycles with contiguous stereogenic centers in good to excellent enantioselectivities (up to 98% ee).
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