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Review
Chemistry, Multidisciplinary
Pham Thi Phan et al.
Summary: Metal-organic frameworks (MOFs) are versatile porous materials whose selectivity, diffusion kinetics, and catalytic activity are influenced by their design and synthetic procedure. Microwave-assisted synthesis has gained significant attention in the past decade due to its short reaction time, fast rate of nucleation, and modified properties of MOFs. This review provides an overview of the development, properties, and applications of microwave-assisted synthesis of MOFs in various fields.
Article
Chemistry, Multidisciplinary
Guanglai Mo et al.
Summary: Recently, there has been a growing interest in artificial and semi-artificial photosynthesis to address the crisis of energy from fossil fuels and reduce excessive CO2 emissions. Metal-organic frameworks (MOFs) have emerged as ideal platforms for constructing artificial photosynthesis systems due to their unique properties and tunable functionalities. This review discusses the characteristics, superiorities, and challenges of MOF-based photocatalysts, and provides a detailed summary of several common design strategies for MOF-based artificial systems. Additionally, the review highlights the applications, mechanisms, and future research directions of MOF-based photocatalysts.
CHINESE JOURNAL OF CHEMISTRY
(2023)
Article
Chemistry, Physical
Arezoo Abdollahi et al.
Summary: In this paper, a nickel-iron (Ni-Fe) electrocatalyst was electrodeposited on a graphite substrate using cyclic voltammetry method. The optimized factors such as applied potential range, scan rate, and number of cycles were determined. The synthesized Ni-Fe coating on graphite rod exhibited promising hydrogen evolution reaction (HER) activity and excellent performance for the oxygen evolution reaction (OER).
JOURNAL OF ALLOYS AND COMPOUNDS
(2023)
Article
Chemistry, Physical
Dongyu Han et al.
Summary: In this study, prism-like materials of MIL-88 were synthesized by a hydrothermal method, and Co-Ni layered double hydroxides (CoNi-LDHs) nanosheets were directly wrapped on the surface of MIL-88 to form core-shell MIL-88@CoNi-LDHs composites. Due to the distinct structure and synergistic effect between the MIL-88 core and CoNi-LDHs shell, MIL-88@CoNi-LDHs showed outstanding OER activity with a small Tafel slope (45.55 mV dec(-1)), low overpotential (314 mV) at 10 mA cm (2), and superior durability. This study provides a prospective pathway to exploit highly efficient low-cost electrocatalysts for OER.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2023)
Article
Huijie Wei et al.
International Journal of Environmental Research and Public Health
(2023)
Review
Chemistry, Multidisciplinary
Kayode Adesina Adegoke et al.
Summary: Metal-organic frameworks (MOFs)-derived nanomaterials are viable electrocatalysts for converting CO2 to value-added products. This study discusses recent advancements in MOF-derivative nanomaterials for CO2 reduction reaction (CO2RR) and their synthetic techniques, active sites, and selectivity. Confinement engineering and structure-activity relationships of MOF-derived electrocatalysts are also discussed. The study evaluates the efficiency of CO2RR electrocatalysts and identifies obstacles and future research directions for commercial applications.
JOURNAL OF CO2 UTILIZATION
(2023)
Review
Biochemical Research Methods
Alessio Zuliani et al.
Summary: The use of metal-organic frameworks (MOFs) in analytical and bioanalytical applications is a growing research area due to their unique properties. MOFs have high porosity and well-defined channels, and can be easily modified for sensing applications. The interaction of analytes with MOFs results in changes to their structure and physicochemical properties, allowing for measurable signals and efficient analyte adsorption. The potential of MOF-based sensors in various applications is discussed, along with future challenges and opportunities for their translation from academia to industry.
ANALYTICAL AND BIOANALYTICAL CHEMISTRY
(2023)
Article
Chemistry, Physical
Jun Zhang et al.
Summary: In response to the demand for clean and renewable energy technologies, researchers have developed economically feasible and stable non-precious electrocatalysts for the oxygen evolution reaction (OER). A highly efficient Ni-NCN/CoFe-LDH composite catalyst was produced by embedding Ni nanoparticles into nanoporous carbon nanorods and electrodepositing them on CoFe-layered double hydroxide (LDH) nanosheets. The composite exhibited excellent catalytic activity with low overpotential, small Tafel slope, and good durability, attributed to the synergistic effect of multiple composites, enhanced electron transport, and uniformly dispersed Ni nanoparticles. The Ni-NCN/CoFe-LDH catalyst showed higher OER performance compared to Niundoped carbon nanorod/LDH, indicating the significant contribution of Ni dopant and LDH to overall OER performance.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2023)
Article
Chemistry, Inorganic & Nuclear
A. A. Bhoite et al.
Summary: To meet energy demands, supercapacitors with high capacity, long life, excellent density and fast charge/discharge rates have been extensively researched. This study synthesized binder-free Ni-MOF thin films using a solvothermal method and studied their structural, morphological, and electrochemical characteristics. The Ni-MOF electrode exhibited a crystalline phase and nanosheet-like structure, showing a specific capacitance of 850.42 F/g, energy density of 18.66 Wh/kg, and power density of 1671 W/kg. These results demonstrate the potential of Ni-MOF for supercapacitor applications and future high-performance materials development.
JOURNAL OF SOLID STATE CHEMISTRY
(2023)
Article
Chemistry, Physical
Jelena D. Gojgic et al.
Summary: The hydrogen evolution reaction (HER) was studied in Ni foams with different pore sizes and in Ni-Sn/Ni foam electrodes. Ni-Sn alloys were electrodeposited from a pyrophosphate-glycine bath using the controlled potential coulometry (CPC) technique. Cross-section analysis revealed that rough Ni-Sn alloy covered the complete inner and outer surface of the foam. Compared to bare Ni foams, Ni-Sn samples showed a lower overpotential at j =-200 mA cm-2 and a change in Tafel slopes from -120 mV dec-1 to -50 mV dec-1. The lowest overpotential achieved at -100 mA cm-2 was as low as -77 mV. These cathodes could be promising 3D materials for industrial water electrolysis.
APPLIED CATALYSIS A-GENERAL
(2023)
Article
Chemistry, Physical
Mani Ram Kandel et al.
Summary: A noble-metal-free electrocatalyst with a unique heterostructure architecture, consisting of hybrid Ni2P-MnP nanosheet coupled with Co2P nanoflowers (Ni2P-MnP@Co2P), has been successfully developed for highly competent hydrogen evolution reaction (HER) and oxygen evolution reaction (OER). The tri-phased Ni2P-MnP@Co2P nanocrystal exhibits greatly active and robust electrocatalytic efficacy with low HER (60 mV) and OER (255 mV) potential achieving current densities of (10 and 30) mA cm-2, respectively. The exceptional electrochemical performance is attributed to the distinctive architectural feature, high surface area with optimum porosity, bountiful Ni2P-MnP and Co2P heterointerface interaction, and synergism among Ni2P, MnP, and Co2P multi-active sites.
APPLIED CATALYSIS B-ENVIRONMENTAL
(2023)
Article
Chemistry, Physical
Alagan Muthurasu et al.
Summary: A defect-rich porous framework composed of metal-organic compound networks is developed to create high-performance electrocatalysts with improved electrochemical activity, conductivity, and mass transport properties. The resulting hollow carbon nanostructures with in situ-grown N-doped graphitic carbon matrix and embedded selenium-doped CoS2 hollow spheres exhibit efficient and long-lasting chemical energy conversion functions. Additionally, a zinc-air battery with excellent discharge-charge performance and mechanical stability is successfully constructed using this technique.
APPLIED CATALYSIS B-ENVIRONMENTAL
(2023)
Review
Chemistry, Analytical
I. K. H. Shaikhutdinov et al.
Summary: This article provides a critical review of experimental studies on the efficiency of separating different groups of chemical compounds using metal-organic framework polymers (MOFs) or composite materials with MOFs as a stationary phase in high-performance liquid chromatography. MOFs have demonstrated numerous advantages in high-performance liquid chromatography, showing potential to successfully compete with conventional phases, especially in the determination of low-molecular-weight compounds and optical isomers. Promising options for utilizing this class of materials include the development of monolithic separation columns and hybrid adsorbents that can overcome the limitations of pure MOF-based adsorbents.
JOURNAL OF ANALYTICAL CHEMISTRY
(2023)
Review
Chemistry, Inorganic & Nuclear
Shadpour Mallakpour et al.
Summary: Metal-organic frameworks (MOFs) have gained attention for their adjustable pore sizes, large surface area, and various functionalities, making them suitable for applications in energy storage, CO2 adsorption, catalysis, drug storage, and release.
COORDINATION CHEMISTRY REVIEWS
(2022)
Article
Chemistry, Multidisciplinary
Wei Gong et al.
Summary: In this work, a highly porous and robust metal-organic framework (MOF) called NU-200 was successfully designed and synthesized. Computational simulations showed that the hierarchical bowl-shaped nanopockets in NU-200 played a crucial role in enhancing the affinity for xenon. The unique pocket confinement effect was validated using a similarly sized probe, sulfur dioxide.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2022)
Article
Engineering, Chemical
Xiuying Zhu et al.
Summary: The study developed a highly efficient wood evaporator using Cu-CAT layer on a wooden substrate for seawater desalination and wastewater purification. Additionally, the optimized wood evaporator can generate electricity through the solar vaporization process.
SEPARATION AND PURIFICATION TECHNOLOGY
(2022)
Review
Chemistry, Multidisciplinary
Bing He et al.
Summary: Metal-organic frameworks (MOFs) have shown great potential in electrochemical energy storage and conversion (EESC) due to their unique properties. Freestanding electrodes provide a promising platform for MOF-based materials, enabling superior electrochemical performance. This review provides a comprehensive overview of the structural features, fabrication techniques, and recent advances of freestanding MOF electrodes, as well as discussing the challenges and future perspectives for their scale-up production and commercial applications.
Article
Engineering, Multidisciplinary
Mani Ram Kandel et al.
COMPOSITES PART B-ENGINEERING
(2022)
Review
Biochemistry & Molecular Biology
Bianca Maranescu et al.
Summary: Metal organic frameworks (MOFs) have shown great potential as new drug delivery systems (DDSs) in the last decade. They possess unique properties such as architecture, surface, composition, and chemistry, making them highly attractive. Compared to other systems, MOFs have higher biocompatibility and versatile loading capabilities. This review presents recent research, findings, and challenges of using MOFs as DDSs, with a specific focus on stimuli- and multistimuli-responsive MOFs.
INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES
(2022)
Review
Electrochemistry
Hao Ren et al.
Summary: This review summarizes and emphasizes the mechanisms of different electrochemical synthesis methods for metal-organic frameworks (MOFs). It comprehensively illustrates the applications of MOFs in environmental analysis and evaluates the advantages and disadvantages of electrochemical synthesis methods. Suggestions for optimization and future opportunities are also proposed.
Article
Chemistry, Physical
Seong-Min Ji et al.
Summary: A unique metal-organic framework aided vanadium pentoxide nanorods (MOF-V2O5 NRs-500) has been developed as an OER electrocatalyst under alkaline solutions, demonstrating high catalytic activity, extraordinary durability, and superior electrochemical performance.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2022)
Article
Chemistry, Physical
Yi Peng et al.
Summary: Metal-organic framework (MOF) composites are considered important energy storage materials due to their high porousness, multifunction, various structures, and controllable chemical compositions, but they still face challenges and difficulties in batteries and supercapacitors.
ADVANCES IN COLLOID AND INTERFACE SCIENCE
(2022)
Article
Chemistry, Multidisciplinary
Rui Zheng et al.
Summary: This study demonstrates a novel self-limiting and self-repairing thin-film growth mechanism, which achieves high-quality MOF thin films with preferred in-plane orientations at the bottom. This is very helpful for optimizing the LBL-LPE method, understanding the growth cycle-dependent properties of MOF thin films, and inspiring investigations of biomimetic self-repairing materials.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2022)
Review
Chemistry, Inorganic & Nuclear
M. Sivagami et al.
Summary: Dyes are widely used synthetic organic compounds in various industries, but the effluents released into water bodies cause pollution worldwide. Current methods for reducing toxic compounds in industrial effluents, such as physical, chemical, and biological approaches, are expensive and complex. However, the use of green-synthesized metal/metal oxide nanoparticles from plant extracts provides a cheap, non-toxic, and eco-friendly approach for the photocatalytic degradation of dye effluents.
INORGANIC CHEMISTRY COMMUNICATIONS
(2022)
Review
Chemistry, Physical
Xianxian Xu et al.
Summary: The widespread use of non-renewable energy has led to serious environmental problems. Hydrogen, as a carbon-free fuel, is considered the most promising energy carrier for the future. However, the current production of hydrogen is dominated by fossil-based techniques, which have low conversion efficiency and greenhouse gas emissions. Therefore, finding green and sustainable production routes for hydrogen with low energy consumption and cost is crucial. Bio-hydrogen production technologies have environmental advantages and broad prospects, with each technique having its own advantages, challenges, and applicability.
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
(2022)
Review
Chemistry, Multidisciplinary
Ying Li et al.
Summary: Metal-organic frameworks (MOFs) have excellent properties and great potential applications in various fields, but they face limitations in scale-up synthesis and shaping, hindering large-scale commercial applications. This paper outlines the advantages and drawbacks of existing synthetic routes and shaping methods, and proposes perspectives on large-scale synthesis and shaping of MOFs, aiming to provide insights and boost commercial applications of MOFs.
CHEMICAL COMMUNICATIONS
(2022)
Review
Chemistry, Inorganic & Nuclear
Bandhana Devi et al.
Summary: Sustainable energy technology is increasingly demanded due to the depletion and risks associated with fossil fuels. Metal-organic frameworks (MOFs) show great potential in trifunctional electrocatalysis application, thanks to their high surface area, porosity, and other unique physicochemical properties. However, the use of MOFs in this field is still in its early stage and requires further exploration.
DALTON TRANSACTIONS
(2022)
Review
Chemistry, Inorganic & Nuclear
Yue Li et al.
Summary: This article reviews the development and applications of flexible metal-organic frameworks (MOFs) in gas storage and separation. It points out that flexible MOFs have controllable structural changes and breathing phenomena, which give them unique advantages in performance tuning.
DALTON TRANSACTIONS
(2022)
Article
Chemistry, Physical
Huixian Jia et al.
Summary: This study developed a simple strategy to construct Ni/NCNs, which exhibited remarkable performance as a glucose sensor. The sensor showed ultra-low detection limit, wide linear detection ranges, fast response times, and good stability.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2021)
Article
Chemistry, Analytical
Yijing Ai et al.
JOURNAL OF ELECTROANALYTICAL CHEMISTRY
(2020)
Proceedings Paper
Physics, Condensed Matter
Nirmal et al.
DAE SOLID STATE PHYSICS SYMPOSIUM 2019
(2020)
Article
Polymer Science
Sedigheh Jabarian et al.
JOURNAL OF INORGANIC AND ORGANOMETALLIC POLYMERS AND MATERIALS
(2019)
Article
Chemistry, Physical
Xi Ke et al.
ENERGY STORAGE MATERIALS
(2019)
Review
Chemistry, Multidisciplinary
Damien Voiry et al.
NATURE REVIEWS CHEMISTRY
(2018)
Article
Nanoscience & Nanotechnology
Zhenhua Li et al.
ACS APPLIED MATERIALS & INTERFACES
(2018)
Article
Chemistry, Multidisciplinary
Saber Alizadeh et al.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2017)
Article
Nanoscience & Nanotechnology
Jia Lu et al.
ACS APPLIED MATERIALS & INTERFACES
(2016)
Article
Polymer Science
Azadeh Azadbakht et al.
JOURNAL OF INORGANIC AND ORGANOMETALLIC POLYMERS AND MATERIALS
(2016)
Article
Chemistry, Physical
Xiaoping Dai et al.
JOURNAL OF PHYSICAL CHEMISTRY C
(2016)
Article
Chemistry, Physical
Nicolo Campagnol et al.
JOURNAL OF MATERIALS CHEMISTRY A
(2016)
Article
Chemistry, Physical
Fangwang Ming et al.
JOURNAL OF MATERIALS CHEMISTRY A
(2016)
Article
Thermodynamics
Jahan-Bakhsh Raoof et al.
Article
Chemistry, Multidisciplinary
Jun-Sheng Qin et al.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2015)
Article
Multidisciplinary Sciences
Idan Hod et al.
NATURE COMMUNICATIONS
(2015)
Review
Electrochemistry
Hanan Al-Kutubi et al.
Article
Chemistry, Multidisciplinary
Andrew J. Clough et al.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2015)
Article
Chemistry, Physical
Gui Fu Yang et al.
JOURNAL OF MATERIALS CHEMISTRY A
(2014)
Review
Chemistry, Multidisciplinary
Yu-Ri Lee et al.
KOREAN JOURNAL OF CHEMICAL ENGINEERING
(2013)
Article
Chemistry, Physical
Nicolo Campagnol et al.
JOURNAL OF MATERIALS CHEMISTRY A
(2013)
Article
Chemistry, Multidisciplinary
Alberto Martinez Joaristi et al.
CRYSTAL GROWTH & DESIGN
(2012)
Review
Chemistry, Physical
Zeid A. ALOthman
