4.8 Article

The Challenge of Water Competition in Physical Adsorption of CO2 by Porous Solids for Carbon Capture Applications - A Short Perspective

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ADVANCED MATERIALS
卷 -, 期 -, 页码 -

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WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.202301730

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carbon capture; CO2 separations; metal-organic frameworks (MOF); modelling; solid sorbents

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This perspective article provides insights into the design of sorbent materials for carbon capture based on nearly a decade of collaboration across science, engineering, and industry partners. The holistic view of the carbon capture problem is emphasized, highlighting the crucial role of water in evaluating the potential of a physical adsorbent for CO2 capture. It calls for interdisciplinary research and is written for a general audience.
With ever-increasing efforts to design sorbent materials to capture carbon dioxide from flue gas and air, this perspective article is provided based on nearly a decade of collaboration across science, engineering, and industry partners. A key point learned is that a holistic view of the carbon capture problem is critical. While researchers can be inclined to value their own fields and associated metrics, often, key parameters are those that enable synergy between materials and processes. While the role of water in the chemisorption of CO2 is well-studied, in this perspective, it is hoped to highlight the often-overlooked but critical role of water in assessing the potential of a physical adsorbent for CO2 capture. This is a challenge that requires interdisciplinarity. As such, this document is written for a general audience rather than experts in any specific discipline.

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