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Article
Chemistry, Multidisciplinary
Run Wang et al.
Summary: This study successfully developed the first monolithic tandem multicolor perovskite LED and white LED, solving issues such as solvent incompatibility, ion exchange, and energy transfer between different emission centers by utilizing an optimal intermediate connection layer. The multicolor LED achieved the best external quantum efficiency of 1.8% and the highest luminance of 4844 cd m(-2). The monolithic white LED reached a color gamut of 130%, offering a feasible strategy for developing wide-color gamut perovskite displays.
ADVANCED FUNCTIONAL MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Wei Zhou et al.
Summary: This study has successfully achieved spectrally stable emission of blue PeLEDs by using bifunctional passivators of Lewis-base benzoic acid anions and alkali metal cations. By passivating the under-coordinated lead atoms and suppressing halide ion migration, the performance of the devices has been improved significantly, achieving high external quantum efficiency.
ADVANCED FUNCTIONAL MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Zhenyang Liu et al.
Summary: This study demonstrates the synthesis of 2D Cs2AgInxBi1-xCl6 alloyed double perovskite nanoplatelets with controlled morphology and composition. The obtained NPLs show unique optical properties and good stability, making them suitable for solution-processing in low-cost device manufacturing. Solution-processed light-emitting diodes using Cs2AgIn0.9Bi0.1Cl6 alloyed double perovskite NPLs as the emitting component exhibit good performance.
ADVANCED MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Tianxin Bai et al.
Summary: Double perovskites (DPs) are promising candidates for white light-emitting diodes (WLEDs) due to their intrinsic broadband emission. In this study, a series of highly luminescent one-dimensional DP-inspired materials were synthesized using a fluorinated organic cation, and efficient warm-white photoluminescence was achieved. By doping a small amount of antimony ion, lead-free metal-halide WLEDs with superior performance were fabricated.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2023)
Article
Chemistry, Physical
Peifen Zhu et al.
Summary: This study presents a simple recrystallization process to prepare halide double perovskites (DP) Cs2Ag1-xKxIn0.875Bi0.125Cl6 (x≤0.60) under ligand-free conditions, and improves their optical properties by tuning the composition. With the optimal alloying content, these halide DPs exhibit high-quality white light emission suitable for white LED. This research provides insight into achieving environmentally friendly and high-efficiency white light emission using abundant elements and a low-cost synthesis method.
JOURNAL OF ALLOYS AND COMPOUNDS
(2023)
Article
Chemistry, Multidisciplinary
Jin-Long Li et al.
Summary: Lead-free organic antimony(III) halides with zero-dimensional structure demonstrate promising potential in optoelectronic applications due to their exceptional optical properties. The electrically driven organic light-emitting diodes (OLEDs) based on these materials show significant improvement in luminance, current efficiency, and external quantum efficiency compared to non-doped devices, attributed to enhanced surface morphology and balanced carrier transport in the light-emitting layers.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2022)
Article
Chemistry, Multidisciplinary
Yuqing Zhang et al.
Summary: A novel lead-free double perovskite quantum dots were successfully fabricated for white light-emitting diodes with excellent optoelectronic performance and stability. The device exhibits good luminous properties and stability, making it suitable for future lighting applications.
Article
Chemistry, Multidisciplinary
Xingwen Cheng et al.
Summary: This study reports a unique strategy to achieve efficient self-trapped exciton (STE) emission in alloyed lead-free Cs-2(Ag/Na)InCl6 double perovskites through Cu+ doping. A small amount of Cu+ doping enhances the STE emission in the crystals, and the underlying mechanism is investigated by temperature-dependent photoluminescence and femtosecond transient absorption spectroscopy.
Article
Chemistry, Multidisciplinary
Yong Ha Hwang et al.
Summary: Researchers have successfully developed a fiber WOLED with comparable performance to conventional planar WOLEDs, which can be implemented on fibers. This achievement is significant for the realization of complete textile display technologies.
Review
Optics
Abdur Rehman Anwar et al.
Summary: The demand for high-performance displays is increasing due to their wide applications. Micro-LED display shows potential to replace traditional displays, but faces challenges in mass transfer and manufacturing cost. Another option is using color conversion medium for full-color display.
LASER & PHOTONICS REVIEWS
(2022)
Review
Chemistry, Physical
Run Wang et al.
Summary: Full electroluminescence white-light-emitting diodes (WLEDs) are a focus of research in the development of white light sources due to their potential and advantages in energy saving. Achieving white emission involves balancing the excitation of different color emissive centers, which is challenging due to the different bandgaps of the emitters. Regulating the energy distribution among the emissive centers is crucial for achieving white emission and improving the performance and color quality of WLEDs. Various energy regulation strategies have been proposed, promoting the development of full EL-WLEDs.
ACS ENERGY LETTERS
(2022)
Article
Chemistry, Multidisciplinary
Ji Jiang et al.
Summary: Efficient red PeLEDs with high EQE and maximum brightness have been achieved by finely controlling the phase distribution of quasi-2D perovskite and passivation of defects in perovskite films.
ADVANCED MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Gangyi Zhang et al.
Summary: An all-inorganic bismuth halide perovskite Cs2AgBiCl6 single crystal is reported to achieve efficient broadband NIR emission by introducing Na ions. The NIR emission originates from self-trapped excitons (STE) emission, which can be enhanced by weakening the strong coupling between electrons and phonons.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2022)
Article
Optics
Rui Sun et al.
Summary: This study presents a promising method for fabricating white perovskite LEDs using lanthanide (Ln(3+)) ions doped CsPbCl3 perovskite nanocrystals. By tuning the perovskite bandgap and surface-capping with a multi-functional ligand, efficient and stable white light emission is achieved. This work provides an optimal solution for the development of low-cost and simple white perovskite LEDs.
LIGHT-SCIENCE & APPLICATIONS
(2022)
Article
Chemistry, Multidisciplinary
Zhuangzhuang Ma et al.
Summary: Perovskite light-emitting diodes (LEDs) are promising light sources for future lighting and display technologies. However, achieving yellow electroluminescence, environmental stability, and lead toxicity are challenges. By incorporating a hole-transporting polymer into the CsCu2I3 emitter, the electroluminescent performance of the LEDs is improved, resulting in significantly enhanced device performances. The external quantum efficiency of the yellow LEDs is increased by 8.5 times, and the half-lifetime reaches 14.6 hours, making them the most stable yellow LEDs based on perovskite systems reported so far.
Editorial Material
Nanoscience & Nanotechnology
Jiawei Chen et al.
Summary: Thanks to the advancements in WLEDs and their design principles, modular crystalline hybrids are providing energy-efficient alternatives for lighting.
NATURE REVIEWS MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Zheming Liu et al.
Summary: This study demonstrates how to enhance the photoluminescence quantum yield (PLQY) of yellow-emissive Bi-doped Cs2Ag1-xNaxInCl6 double perovskite nanocrystals (NCs). By preventing the formation of Ag0 particles and partially replacing Na+ with K+ ions, the PLQY of the NCs can be increased. This work further reveals the parameters influencing carrier trapping/relaxation and provides a strategy to improve the PL efficiency of double perovskite NCs.
Article
Optics
Jiawei Chen et al.
Summary: Halide perovskite LEDs are a new type of white light-emitting diode that utilizes efficient and low-cost lighting technologies, featuring a single broadband emissive layer without the need for phosphors. These LEDs operate with high peak luminance and external quantum efficiency, with potential for further improvements in the future through advancements in fabrication technology and mechanistic understanding.
Article
Chemistry, Physical
Jidong Lin et al.
Summary: This research introduces a method using perovskite quantum dots to produce nanocomposites in glass with superior optical performance and stability, which can be used to improve the color gamut and rendition of LCD. By physically diluting to eliminate the inner filter effect and effectively isolating them from the external environment, the quantum yield and stability of the quantum dots have been significantly enhanced. The backlit LCD designed using this technology showed a color gamut reaching 152% of commercial LCD and 103% of NTSC, showcasing great potential in the optoelectronic industry.
ACS ENERGY LETTERS
(2021)
Article
Chemistry, Physical
Ziming Chen et al.
Summary: The main challenges in the metal-halide-perovskite light-emitting diode (PeLED) field are low light extraction efficiency (LEE) and difficulty in achieving white emission. A high-performance white PeLED with enhanced LEE was successfully constructed by coupling a blue PeLED with a red perovskite nanocrystal (PeNC) down-converter through a multilayer semitransparent electrode. This approach not only improved LEE by over 50%, but also achieved a high external quantum efficiency and luminance, representing state-of-the-art results in the field.
Article
Optics
Peipei Dang et al.
Summary: The development of a highly efficient red-emitting phosphor, CEGO, with high color purity and excellent thermal stability shows great potential as a red component for pc-WLEDs, providing a new perspective for developing new phosphor materials.
LIGHT-SCIENCE & APPLICATIONS
(2021)
Article
Chemistry, Physical
Shai Levy et al.
Summary: Lead-free double perovskites are being studied as alternatives to lead halide perovskites in optoelectronic applications, with a focus on the role of metallic silver nanoparticles in crystal growth. The nucleation of perovskite nanocrystals is shown to occur on preexisting silver seeds, with evidence of charge transfer between the perovskite and silver nanoparticles leading to modified optical properties. Understanding and controlling the reduction of Ag+ at all synthetic stages is critical for achieving stability and functionality in silver-based lead-free perovskite nanocrystals.
CHEMISTRY OF MATERIALS
(2021)
Article
Multidisciplinary Sciences
Changjiu Sun et al.
Summary: The performance of perovskite light-emitting diodes tends to decline as the active area increases, with severe phase-segregation identified as the cause. The introduction of L-Norvaline to construct an intermediate phase has successfully suppressed the phase-segregation, resulting in highly-efficient large-area quasi-2D films.
NATURE COMMUNICATIONS
(2021)
Article
Chemistry, Physical
Bo Zhou et al.
Summary: By doping Sb3+ and Bi3+ ions into Cs2NaInCl6 single crystals, blue and yellow emissions were achieved, leading to white light emission with a quantum yield of 77%. This dual emission is attributed to self-trapped excitons (STEs) related to different [SbCl6]3- octahedra, with the blue emission resulting from limited Jahn-Teller deformation from Sb3+ doping and the yellow STE emission enhanced by Bi3+ induced lattice distortion and sub-band level formation. Tuning between warm and cold white light can be achieved by adjusting the Sb3+/Bi3+ doping ratio.
ACS ENERGY LETTERS
(2021)
Article
Chemistry, Multidisciplinary
Ying Liu et al.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2020)
Article
Chemistry, Multidisciplinary
Peigeng Han et al.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2020)
Article
Multidisciplinary Sciences
Muyu Cong et al.
Article
Chemistry, Physical
Rui Sun et al.
ACS ENERGY LETTERS
(2020)
Article
Multidisciplinary Sciences
Leimeng Xu et al.
NATURE COMMUNICATIONS
(2020)
Article
Chemistry, Physical
Ying Liu et al.
CHEMISTRY OF MATERIALS
(2019)
Article
Chemistry, Multidisciplinary
Yehonadav Bekenstein et al.
Article
Chemistry, Multidisciplinary
Jizhong Song et al.
ADVANCED MATERIALS
(2018)
Article
Chemistry, Multidisciplinary
Bin Yang et al.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2018)
Article
Multidisciplinary Sciences
Jiajun Luo et al.
Article
Chemistry, Multidisciplinary
Gencai Pan et al.
Article
Optics
Weicheng Pan et al.
Review
Chemistry, Multidisciplinary
Pablo Docampo et al.
ACCOUNTS OF CHEMICAL RESEARCH
(2016)
Article
Chemistry, Physical
Aslihan Babayigit et al.
Review
Chemistry, Multidisciplinary
Guogang Li et al.
CHEMICAL SOCIETY REVIEWS
(2015)
Article
Multidisciplinary Sciences
Qingfeng Dong et al.
Article
Chemistry, Physical
Philipp Pust et al.