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Article
Chemistry, Multidisciplinary
Dengyi Xiong et al.
Summary: Aqueous zinc anode has been re-evaluated for its advantages in safety and cost concerns. However, the limited lifespan caused by Zn dendritic and side reactions hampers its commercial development. In this study, a high-dense TiO2-x solid electrolyte interphase (HDSEI) with rich oxygen vacancies is successfully constructed in an aqueous electrolyte, which significantly enhances the performance and lifespan of zinc anodes. This in-situ approach provides a feasible solution to implement dendrite-free metal anodes.
ADVANCED FUNCTIONAL MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Siwei Zhao et al.
Summary: In order to enhance the zinc ion conductivity and suppress dendrite growth, researchers have designed a heteroanionic zinc ion conductor (ZnyO1-xFx) as a protective layer. By tuning the F content and thickness, the coated anode shows a low overpotential of 20.4 mV for 1000 h cycle life and high stability for 1000 cycles. This work sheds light on the development of high-performance Zn-based energy storage devices.
ADVANCED MATERIALS
(2023)
Article
Chemistry, Physical
Zhilin Jiang et al.
Summary: A high-entropy oxide with abundant surface defects and narrow bandgap was designed and synthesized for photocatalytic CO2 conversion. The oxide exhibited excellent activity and stability for CO2 reduction under visible light without any co-catalyst, thanks to its ultra-narrow bandgap, abundant structural defects, uniform dispersion of metal elements, and suitable band structure.
APPLIED SURFACE SCIENCE
(2023)
Article
Chemistry, Physical
Haoran Du et al.
Summary: By designing a polyelectrolyte coating that is rich in hydrophobic and anion-blocking groups, undesired side reactions at the zinc electrode|electrolyte interface can be suppressed, leading to a prolonged cycling life of the zinc electrodes.
ENERGY STORAGE MATERIALS
(2023)
Article
Chemistry, Physical
Xiaomei Huo et al.
Summary: A versatile Zn-based laponite (Zn-LT) interface is constructed for uniform and rapid Zn deposition in aqueous zinc-ion batteries (AZIBs), resulting in high Coulombic efficiency and long lifespan.
ADVANCED ENERGY MATERIALS
(2023)
Article
Engineering, Environmental
Xin Qi et al.
Summary: This study designs an organic molecule as an artificial layer to address the issues of dendrite growth and uneven zinc deposition in aqueous zinc ion batteries, which demonstrates promising prospects with long-term cycling stability and excellent rate performance. The sulfur-containing functional groups in the organic materials also successfully resolve the problems of zinc anodes.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Engineering, Environmental
Shan Cai et al.
Summary: Constructing an artificial interfacial layer on the zinc anode using dithio-bridged chelate network can improve the thermos-kinetics properties and suppress dendrite growth, leading to an extended electrode lifetime.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Chemistry, Multidisciplinary
Yahan Meng et al.
Summary: This study proposes a new principle of regulating the p-band center of metal oxide protective coating to balance the adsorption energy and migration energy barrier of zinc for effective deposition and stripping. The experiments and calculations show that a highly stable and reversible zinc anode can be achieved using indium tin oxide (ITO) as the substrate. This work provides a general strategy and new insight for improving the efficiency of zinc anode protection.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2023)
Article
Chemistry, Multidisciplinary
Yahan Meng et al.
Summary: This study proposes a new principle for regulating the p-band center of a metal oxide protective coating to achieve effective control over zinc deposition and stripping. Experimental and theoretical results show that by using indium tin oxide as the nucleation site, highly stable and reversible zinc anode can be achieved. The research provides a general strategy and new insight for the construction of efficient zinc anode protection layers.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2023)
Article
Nanoscience & Nanotechnology
Ying Zhang et al.
Summary: The researchers improve the cycling lifespan and electrochemical performance of aqueous zinc-ion batteries (AZIBs) by constructing an artificial protective interface layer on the zinc metal. A dense and uniform complex coating layer of phytic acid (PA) and zinc is formed on the zinc anodes, effectively inhibiting corrosion reactions and enhancing the deposition and stripping of zinc. Under experimental conditions, the PA-Zn metal anode exhibits low overpotential and long lifespan.
ACS APPLIED MATERIALS & INTERFACES
(2022)
Review
Nanoscience & Nanotechnology
Bin Li et al.
Summary: This article reviews the role of interfacial engineering in inhibiting the growth of Zn dendrites and the occurrence of side reactions. Researchers have regulated the deposition behavior of Zn ions through surface modification and the addition of electrolyte additives to achieve uniform Zn nucleation and flat Zn deposition, improving the cycling stability of Zn anodes.
NANO-MICRO LETTERS
(2022)
Article
Chemistry, Physical
Jiaxian Zheng et al.
Summary: This study demonstrates that a TiN protective coating with preferential (200) orientation can effectively suppress Zn dendritic growth and side reactions, while regulating the growth pattern of the byproduct. This provides a new pathway for achieving high-efficiency reversible Zn plating/stripping.
ACS ENERGY LETTERS
(2022)
Article
Chemistry, Physical
He Gan et al.
Summary: In this study, a multi-functional protective layer was constructed to improve the performance of aqueous energy storage devices by regulating the deposition behavior of zinc, overcoming the limitations of uncontrollable dendrites growth and side reactions. The well-designed zinc anode achieved high Coulombic efficiency and long lifespan.
ENERGY STORAGE MATERIALS
(2022)
Review
Chemistry, Physical
Ahmad Naveed et al.
Summary: Zinc batteries are praised for their safety, environmental friendliness, and low toxicity, but the poor rechargeability of the zinc anode hinders their applications. By studying the zinc electrochemistry in different electrolyte systems and suggesting methods to improve the reversibility and stability of the zinc anode, the potential of organic electrolytes with safe organic solvents for high-performance zinc ion batteries is highlighted.
ENERGY STORAGE MATERIALS
(2022)
Article
Chemistry, Physical
Aosai Chen et al.
Summary: In this study, a uniform ridge-like ZnMoO4 layer was directly formed on the zinc anode within 20 seconds by chemical deposition, improving the issues of uneven zinc deposition and hydrogen evolution in aqueous zinc-ion batteries. Zn@ZnMoO4 demonstrates strong hydrogen suppression capability, excellent cycling stability, and high capacity retention rate.
ENERGY STORAGE MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Huaming Yu et al.
Summary: A highly antiwater interface layer is designed on Zn metal to address the corrosion and dendrite growth problems in aqueous Zn metal batteries. The experimental results show that this interface layer can prevent water damage to the Zn anode surface and facilitate fast zinc-ion adsorption and migration. The modified anode exhibits long cycling lifespan and low polarization voltage, demonstrating its potential for high-performance aqueous zinc-metal batteries.
Article
Chemistry, Multidisciplinary
Pan He et al.
Summary: This study proposes a simple and rapid surface passivation strategy to significantly improve the cycling stability and corrosion resistance of aqueous zinc ion batteries.
ADVANCED MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Ming Zhao et al.
Summary: This study proposes a strategy to fabricate a semi-immobilized ionic liquid interface layer in order to address the issues of irregular dendrite growth and side reactions in aqueous zinc ion batteries (ZIBs). By using immobilized SiO2@cation and free anions, the Zn anode is protected and achieves stable cycling performance over a wide temperature range.
ADVANCED MATERIALS
(2022)
Article
Engineering, Environmental
Jianping Yan et al.
Summary: Spraying a versatile zirconium phosphate (ZrP)-based artificial solid electrolyte interface (ASEI) onto the zinc anode can effectively solve the dendrites growth and side reactions in aqueous zinc-ion batteries (ZIBs), leading to improved performance and cycling stability.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Chemistry, Applied
Hao Fu et al.
Summary: This study presents a simple and applicable immersion method to address the challenges faced by zinc metal anodes, such as dendrite formation and corrosion. A zinc phytate (PAZ) coating is formed on the surface of commercial zinc flakes through a substitution reaction, which mitigates corrosion, reduces interfacial impedance, and accelerates zinc ion migration kinetics. The method also selectively exposes the (002) crystal plane with strong atomic bonding, improving corrosion resistance and suppressing dendrite formation.
JOURNAL OF ENERGY CHEMISTRY
(2022)
Review
Materials Science, Multidisciplinary
Courtney-Elyce M. Lewis et al.
Summary: The global competition to find new technologies for clean and effective renewable energy sources is driven by the climate crisis. Vanadium-containing materials, such as vanadium phosphates, are being used in zinc-ion batteries as a cheap, safe, and eco-friendly alternative.
ADVANCED MATERIALS TECHNOLOGIES
(2022)
Article
Chemistry, Physical
Minghui Qiu et al.
Summary: In this study, an intermediate layer of sulfonate group modified boron nitride nanosheets was designed to regulate the electrochemical behavior of zinc, effectively suppressing dendrite growth and side reactions. The resulting zinc anode showed enhanced performance in aqueous zinc-ion batteries.
ENERGY STORAGE MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Pinji Wang et al.
Summary: Multifunctional interfacial engineering on the Zn anode, through the spontaneous construction of a carbonyl-containing layer (Zn@ZCO), effectively suppresses dendrite growth, hydrogen evolution, and sluggish kinetics associated with Zn deposition. The Zn@ZCO anode exhibits a long cycling lifespan, dendrite-free surface, and excellent rate performance in aqueous zinc-ion batteries.
ADVANCED MATERIALS
(2022)
Article
Chemistry, Physical
Donghong Wang et al.
Summary: By selecting a stable cathode framework and suitable tunnels, high energy efficiency for the storage of Zn2+ ions can be achieved. The use of K+ ions as charge carriers also contributes to the reduction of overpotential. This research demonstrates the potential for improving energy efficiency of aqueous zinc batteries and suggests further research directions.
Article
Chemistry, Physical
Mao-Cheng Liu et al.
Summary: This study demonstrates the inhibition of dendrite growth and side reactions on the zinc anode through the use of a hydrophobic organic-inorganic surface modification layer, which provides a solid foundation for the realization of ultra-stable zinc ion batteries.
Article
Chemistry, Physical
Ning Dong et al.
Summary: A novel Zn anode structure with porous indium coating layer and polyacrylamide polymer layer is proposed in this study, which significantly enhances the cycling stability and long-term lifespan of Zn batteries through synergistic effects.
Article
Chemistry, Multidisciplinary
Xiaofeng He et al.
Summary: The study introduces a concept of constructing an anion concentration gradient-assisted solid-electrolyte interphase for metal anodes, which enhances ionic conductivity and suppresses dendritic growth and side reactions. This new approach enables stable plating/stripping of zinc metal and shows improved cycling stability in various types of batteries and supercapacitors.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2022)
Article
Chemistry, Physical
Jian Yin et al.
Summary: This study demonstrates an indium-coated carbon-zinc composite (ICZ) anode with outstanding cyclic stability in aqueous zinc batteries. By reducing the overpotential required for zinc nucleation and preventing parasitic reactions, the ICZ anode enhances the cyclic stability of zinc ion batteries and zinc ion capacitors.
Article
Chemistry, Multidisciplinary
Qianyi Ma et al.
Summary: The addition of 2-propanol is shown to regulate the outer solvation shell structure of Zn2+ in aqueous Zn-ion batteries, resulting in uniform Zn deposition and dendrite-free growth.
ADVANCED MATERIALS
(2022)
Review
Chemistry, Multidisciplinary
Qihui Zhang et al.
Summary: This review focuses on the latest research progress in the design of artificial interphase layers (AIL) for zinc anode protection, including the classification of functional materials, preparation methods, mechanism investigations, and device performances. The origins of zinc instability are explained from the perspectives of electrical field, mass transfer, and nucleation process, followed by a comprehensive summary of the functions and design criteria of AIL. Finally, current challenges and future outlooks are discussed based on theoretical and experimental considerations.
Article
Chemistry, Multidisciplinary
Yu Liu et al.
Summary: In this study, a Prussian blue analog of copper hexacyanoferrate (CuHCF) was used as a solid-state electrolyte protection layer to coat the zinc anode surface, effectively inhibiting dendrite growth and side reactions, and improving the cycling stability and capacity retention of zinc-ion batteries.
Article
Chemistry, Physical
Peng-Fang Zhang et al.
Summary: This study proposes a simple and cost-effective method of designing a ZnTA anticorrosive film on Zn anodes. The film demonstrates excellent uniformity and coverage, resulting in remarkable suppression of hydrogen evolution and corrosion. As a result, highly-reversible Zn-I-2 batteries with excellent rate performance and ultra-long lifespan are achieved.
Article
Chemistry, Physical
Hao Fu et al.
Summary: The study presents a method for developing stable thermodynamics and fast kinetics in Zn metal anodes by selectively reacting weak oxidants to crystal planes, leading to the formation of a thermodynamically stable ZnMoO4 passivation layer. The method improves the reaction kinetics and inhibits corrosion and side reactions, making it valuable for constructing metal electrodes with fast kinetics and stable thermodynamics.
ENERGY STORAGE MATERIALS
(2022)
Article
Chemistry, Physical
Wei Ling et al.
Summary: Researchers have developed a lightweight silver nanowire aerogel (AgNWA) to address the issue of zinc-dendrite growth and achieve stable cycling of zinc metal anodes in extreme conditions. The AgNWA guides a uniform zinc plating/stripping process, allowing for dendrite-free deposition at high rates and capacities. The AgNWA anode demonstrates high efficiency and stability in both supercapacitors and batteries, making it a promising material for fast-charging zinc batteries with high zinc utilization.
ENERGY STORAGE MATERIALS
(2022)
Article
Engineering, Environmental
Yanxin Li et al.
Summary: This study reports a facile impregnation treatment for the synthesis of a protective layer composed of ultrafine metallic tin particles on the zinc foil. The use of ultrafine particles improves the electrochemical deposition behavior of aqueous zinc ion batteries by enhancing the electric field and active sites for accelerated transport kinetics. The stability at high areal capacity is achieved through reduced nucleation energy barrier. The practical implementation of this technique has been validated in coin cells and flexible pouch cells.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Chemistry, Physical
Mao-Cheng Liu et al.
Summary: The study designed organic hydrophobic polyvinylidene fluoride and inorganic Santa Barbara Amorphous-15 (PVDF-SBA15) hybrids as a surface modification layer for zinc anode, effectively inhibiting dendrite growth and side reactions, laying a solid foundation for ultra-stable zinc ion batteries.
Article
Chemistry, Physical
Shan Guo et al.
Summary: Electrolyte additive is a key technology in energy storage, especially for aqueous zinc-ion batteries, but there is a lack of systematic research on its features and mechanisms. A comprehensive review on commonly used zinc-ion electrolyte additives is essential for further improvements in this field.
ENERGY STORAGE MATERIALS
(2021)
Article
Nanoscience & Nanotechnology
Kevin Foster et al.
Summary: The study investigated the performance and electrical contact resistance of a trivalent chromium passivation layer and a cobalt-free version on gamma-ZnNi-coated Al 6061-T6. The cobalt-containing passivation layer exhibited higher corrosion resistance and lower resistance, with differing exposure results on the aluminum substrate.
ACS APPLIED MATERIALS & INTERFACES
(2021)
Article
Chemistry, Multidisciplinary
Minshen Zhu et al.
Summary: The study presents a technique using a polyimide coating to solve the capacity loss issue of zinc anodes in an acid electrolyte. The polyimide coordinates with zinc ions to build a zinc blanket, reducing the concentration gradient at the electrode/electrolyte interface for fast kinetics and low plating/stripping overpotential.
ADVANCED MATERIALS
(2021)
Review
Chemistry, Physical
Zhehan Yi et al.
Summary: Zinc-ion batteries are considered promising candidates for next-generation energy storage systems due to their high safety, resource availability, and environmental friendliness. However, the instability of the Zn metal anode has hindered their reliable deployment, and efforts have been made to overcome this through electrode structure design, interface modification, and electrolyte/separator optimization. Understanding and categorizing these strategies based on their intrinsic mechanisms are important for the development of novel Zn metal anodes for ZIBs.
ADVANCED ENERGY MATERIALS
(2021)
Article
Chemistry, Physical
Cheng Liu et al.
Summary: The study introduces an electrochemical-inert liquid gallium-indium alloy coating for zinc anodes in rechargeable metal batteries, addressing interfacial issues such as dendrite growth and electrode corrosion. The unique coating promotes inward deposition of zinc during charging, improving corrosion resistance and enabling a lower polarization. This effective approach shows promising results in terms of extended lifespan and improved capacity retention in full cells, indicating potential for future development of rechargeable metal batteries beyond zinc-storage systems.
ACS ENERGY LETTERS
(2021)
Article
Chemistry, Multidisciplinary
Penghui Cao et al.
Summary: By utilizing a zinc phosphorus solid solution alloy coated on zinc foil as the anode, the study achieved successful cycling at high current density and large areal capacity, demonstrating the potential for large-scale application of aqueous zinc-ion batteries in high-power devices.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Yang Yang et al.
Summary: The study successfully developed a Zn@ZnF2 electrode with a multi-functional protective layer by designing a 3D interconnected ZnF2 matrix on the surface of Zn foil. This electrode exhibits stable zinc deposition kinetics and good plating/stripping reversibility, showing potential for practical application in various battery systems.
ADVANCED MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Longtao Ma et al.
Summary: By using a ZnF2 solid ion conductor to isolate Zn metal, the hydrogen evolution in Zn metal batteries has been significantly reduced, leading to improved performance and stability of the batteries.
ADVANCED MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Long Zhang et al.
Summary: The introduction of a multifunctional ZnSe protective layer effectively addresses the corrosion, hydrogen evolution, and dendrite formation issues in aqueous Zn metal batteries, improving the stability and performance of the batteries.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Canbin Deng et al.
Summary: The surface of the Zn metal anode is reconstructed by a cerium-based conversion film (Zn@CCF), effectively preventing rapid growth of the film near zinc grain boundaries, resulting in long lifespan and low polarization power. This research helps suppress zinc dendrite formation and underscores the importance of surface reconstruction of the Zn metal anode for corrosion inhibition.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Maya Messaykeh et al.
Summary: The study investigates the effect of additives on metal/oxide interfaces in real time, demonstrating that small amounts of additives can dramatically improve the adhesion of films, which is of great practical interest. The findings highlight the potential of using noncontinuous and partially oxidized films of additives to enhance the sticking of films, closer to realistic application scenarios. Additionally, anchoring a functional film by discrete predeposited seeds can help maintain its properties intact.
CRYSTAL GROWTH & DESIGN
(2021)
Article
Chemistry, Multidisciplinary
Tian Chen Li et al.
Summary: A modified Zn foil with a zincophilic ZnSe layer is proposed in this study, showing lower nucleation energy barrier and faster ion diffusion kinetics in aqueous systems. At the same time, detrimental zinc corrosion is effectively mitigated. Experimental results demonstrate exceptional cycling stability for the ZnSe@Zn/MnO2 full cell over 500 cycles.
Article
Chemistry, Physical
Jin Cao et al.
Summary: A functional separator composed of cellulose nanofibers and graphene oxide is developed for dendrite-free and stable zinc ion batteries. This separator promotes uniform zinc deposition and significantly enhances the performance of zinc anodes in various types of batteries.
ADVANCED ENERGY MATERIALS
(2021)
Review
Chemistry, Multidisciplinary
Ming Li et al.
Summary: This study comprehensively summarizes the role of water molecules in rechargeable aqueous zinc-ion batteries, focusing on the influencing mechanisms from various perspectives. It also proposes new insights and actionable methods for the potential future directions in the design of high-performance AZIBs.
ENERGY & ENVIRONMENTAL SCIENCE
(2021)
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Junnan Hao et al.
ADVANCED MATERIALS
(2020)
Review
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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2020)
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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2020)
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(2020)
Review
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(2019)
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(2011)
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SURFACE & COATINGS TECHNOLOGY
(2008)
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SURFACE & COATINGS TECHNOLOGY
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