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Article
Chemistry, Physical
Huangwei Zhang et al.
Summary: Using 1-butyl-3-methylimidazolium cation (BMIm(+) ion) as an electrolyte additive can effectively induce the preferential growth of (002) plane and inhibit the formation of Zn dendrites.
ADVANCED ENERGY MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Yuhang Zhou et al.
Summary: The challenges of high Zn ion desolvation energy, sluggish Zn deposition kinetics, and top Zn plating pattern in practical Zn anodes are addressed by introducing zinc pyrovanadate (ZVO) as a solid zinc-ion conductor interface. The ZVO interface boosts desolvation and deposition kinetics and improves uniformity. It also enhances the anti-corrosion ability of Zn anodes, rendering fast rechargeability and durable life. This work provides insights into the design of solid zinc-ion conductor interface to enhance the interface stability and kinetics of Zn metal anodes.
Article
Chemistry, Physical
Ping Xiao et al.
Summary: By utilizing γ-butyrolactone (GBL) as an organic solvent, the deposition behavior and performance of Zn anodes can be regulated, allowing for improved electrochemical performance under high current densities and large areal capacities due to reduced dendrite growth and enhanced reaction reversibility. The strong interactions between GBL molecules and Zn2+ and Zn slab were confirmed by DFT calculations, and the preferential adsorption of GBL at the Zn/electrolyte interface was highlighted through Raman spectra analysis. Electrochemical tests demonstrated the effectiveness of this strategy, achieving a supporting current density of 30 mA cm(-1) and a cycle life of 5000 h for the Zn anode using GBL.
ACS ENERGY LETTERS
(2023)
Article
Chemistry, Multidisciplinary
A-Re Jeon et al.
Summary: Rechargeable magnesium batteries with higher energy density and safety have practical potential, but they face obstacles due to passivation or corrosion issues. However, a chemical activation strategy using simple salt electrolytes has been developed, which successfully improves the performance of the magnesium anode and enables stable cycling over 990 cycles. This activation strategy opens up possibilities for the practical implementation of magnesium batteries using commercially available electrolytes.
Article
Chemistry, Multidisciplinary
Xunzhu Zhou et al.
Summary: In this study, tris(pentafluorophenyl)borane was used as an electrolyte additive to build a stable NaF-rich cathode-electrolyte interphase (CEI) in sodium-ion batteries. The strong interactions between the anion and TPFPB improved the oxidative stability and long-term stability of Na3V2(PO4)3 cathode at high temperatures.
ADVANCED FUNCTIONAL MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Zixiang Liu et al.
Summary: Tripropylene glycol (TG) is used as an organic electrolyte additive to significantly improve the reversibility of aqueous zinc ion batteries (AZIBs). TG participates in the solvation sheath of Zn2+, regulating overpotential and inhibiting side reactions, while also inhibiting the deterioration of dendrites and modifying the direction of zinc deposition. This method can result in dendrite-free, high-performance, and low-cost energy storage systems.
ADVANCED FUNCTIONAL MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Jiandong Wan et al.
Summary: Sodium tartrate is used as a dual-functional electrolyte additive to improve the reversibility of aqueous zinc-ion batteries. The additive preferentially adsorbs on the zinc surface, coordinates with zinc ions, and promotes uniform zinc deposition on the (002) plane, inhibiting side reactions and dendrite growth. This leads to long-term cycling stability and improved performance of zinc||MnO2 full cells.
Article
Chemistry, Multidisciplinary
Longhai Zhang et al.
Summary: We designed and synthesized a porous organic polymer (POP) with a conjugated and hierarchical structure, which exhibited excellent electrochemical properties as an anode material for sodium-ion batteries (SIBs). Through combined experiments and theoretical computation, we revealed the Na-storage mechanism and dynamic evolution processes of the POP, including a 12-electron reaction process with Na and stable composition and structure evolution during repeating sodiation/de-sodiation processes. This quantitative design for ultrafast and highly durable sodium storage in the POP could benefit the rational design of organic electrode materials with ideal electrochemical properties.
ADVANCED MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Wei Zhang et al.
Summary: In this study, a multifunctional additive NHP was introduced to regulate zinc deposition and suppress side reactions in aqueous electrolyte. The results showed that the NHP additive enabled highly reversible Zn plating/stripping behaviors, and improved the electrochemical performances of zinc-ion batteries and zinc-based capacitors.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2023)
Article
Chemistry, Multidisciplinary
Sailin Liu et al.
Summary: To stabilize the zinc anode in zinc metal batteries, researchers have developed a controlled electrolytic method using a high dipole moment solvent dimethyl methylphosphonate (DMMP) to create a monolithic solid electrolyte interphase (SEI). This DMMP-based electrolyte generates a homogeneous and robust phosphate SEI (Zn-3(PO4)(2) and ZnP2O6). With the protection provided by this in situ monolithic SEI, the zinc electrode exhibits long-term cycling performance and high Coulombic efficiency in both zinc|zinc and zinc|copper cells. The use of a DMMP-H2O hybrid electrolyte in a full V2O5|zinc battery also results in high capacity retention following a large number of cycles.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2023)
Article
Chemistry, Physical
Shangqing Jiao et al.
Summary: An effective Helmholtz plane (HP) reconstruction mechanism on zinc metal anodes (ZMAs) in ZnSO4 electrolyte activated by zinc pyrrolidone carboxylate (PCA-Zn) additive is proposed to weaken dendrites proliferation and parasitic side reactions. The PCA-Zn additive activates a self-repairing HP with carboxyls serving as anchors and bis-zincophilic-terminal preferentially adhering to the ZMAs surface, reshaping an H2O/SO42--repellent HP and suppressing in-plane diffusion of Zn2+. The HP enables stable ZMAs/electrolyte interphasial chemistry and significantly boosts the cyclic durability of the AZMBs.
ENERGY STORAGE MATERIALS
(2023)
Article
Chemistry, Physical
Tianjiang Sun et al.
Summary: To address the issue of organic cathode dissolution in aqueous zinc-organic batteries (AZOBs), a solubility-limited dibenzo[a,c]dibenzo[5,6:7,8]quinoxalino[2,3-i]phenazine-10,21-dione (TABQ-PQ) molecule was successfully designed and synthesized. The extended pi-conjugated plane improved the p conjugation effect of TABQ-PQ and enhanced its pi-pi stacked interaction, leading to low solubility and good structural stability. The TABQ-PQ cathode exhibited an H+-coordination charge-storage mechanism, high capacitance-controlling behavior, and demonstrated a superlong cycling life of over 30,000 cycles and a high discharge capacity of 140.7 mAh g(-1) at 20 A g(-1). This work provides insights into the design of solubility-limited organic electrodes for high-performance AZOBs.
ENERGY STORAGE MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Tianjiang Sun et al.
Summary: In this study, a small organic molecule PTONQ with extended pi-conjugated plane was designed and a partial charge regulation strategy was adopted. The Zn//PTONQ battery showed good cycling stability, fast charge transfer kinetics, and anti-freeze performance. Ex situ characterizations confirmed that the capacity mainly comes from Zn2+ insertion/removal of PTONQ and explained the formation mechanism of the by-products.
ADVANCED FUNCTIONAL MATERIALS
(2023)
Review
Chemistry, Multidisciplinary
Peng Xiong et al.
Summary: Compared to inorganic electrode materials, organic electrode materials have advantages such as lightweight, customizable structure, high specific capacity, wide availability of natural resources, and recyclability. However, they also have drawbacks including low ionic conductivity and susceptibility to degradation over time. Covalent triazine frameworks (CTFs) have emerged as a promising strategy for organic electrodes, offering customizability, stability, and versatility. This review provides an overview of CTFs, their synthesis, and their performance in energy storage devices.
ENERGY & ENVIRONMENTAL SCIENCE
(2023)
Article
Chemistry, Physical
Yichun Wang et al.
Summary: The development of highly safe and low-cost aqueous batteries is of great significance in achieving carbon neutrality. This study proposes a unique conversion electrochemistry of copper selenides for robust and energetic aqueous charge storage, demonstrating remarkable rate capability and electrochemical durability.
Article
Chemistry, Multidisciplinary
Shangqing Jiao et al.
Summary: This study presents an ion sieve coating that effectively inhibits dendrite growth on metallic zinc anodes, improving the rechargeability of aqueous zinc metal batteries. Experimental and theoretical analyses demonstrate that the coating facilitates the desolvation of zinc clusters, weakens hydrogen evolution reaction, and homogenizes ion flux, resulting in dendrite-free zinc deposition. The symmetric cell with the ion sieve coating shows a lifespan of up to 3000 hours, highlighting the enhanced performance of zinc metal batteries.
Article
Chemistry, Multidisciplinary
Wenyong Chen et al.
Summary: In this study, a maltose-based hybrid electrolyte with hydrogen bond-functionalized massive solvation modules is constructed to address the poor cyclic stability of zinc-ion batteries. The solvation modules promote uniform deposition of zinc at the anode interface and hinder parasitic reactions through hydrogen bond confinement. Meanwhile, they prevent structural collapse at the cathode interface and maintain low interfacial activation energy during cycling. The resultant full batteries retain 84.2% of their initial specific capacity after 400 continuous cycles at a low current density of 50 mA g(-1).
ADVANCED FUNCTIONAL MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Kefeng Ouyang et al.
Summary: A strategy to build an indium metal interphase on the zinc anode surface is proposed, preventing hydrogen evolution reaction and zinc corrosion, guiding smooth zinc deposition. This approach achieves ultrahigh cumulative capacities and stable plating/stripping behavior, with encouraging rate performance and cyclic stability for Zn-V2O5 batteries.
ADVANCED FUNCTIONAL MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Zhaodong Huang et al.
Summary: This study presents three types of small dipole molecules for developing aqueous electrolytes with high safety and wide electrochemical stability window, expanding the potential of aqueous rechargeable batteries. Ab initio molecular dynamics simulations were used to explore the solvation-sheath structures, demonstrating how these small molecules affect the hydrogen bond network between water molecules, enhancing the performance of the electrolyte.
ADVANCED MATERIALS
(2022)
Article
Chemistry, Physical
Rui Yao et al.
Summary: This study introduces a dual-function electrolyte additive to address severe side reactions over zinc metal anodes in aqueous zinc metal batteries, resulting in stable cycling for over 2145 hours. The strategy also enhances the reversibility of energy storage devices based on manganese dioxide and activated carbon.
ADVANCED ENERGY MATERIALS
(2022)
Review
Multidisciplinary Sciences
Sailin Liu et al.
Summary: This review examines the failure mechanism of rechargeable zinc metal batteries under temperature influence, presents current electrolyte strategies for improving battery performance in harsh temperatures, and offers perspectives on their industrial application.
Article
Nanoscience & Nanotechnology
Yang Song et al.
Summary: In this study, a metal-organic framework modified separator is proposed for robust aqueous zinc-ion batteries. The modified separator enhances the transport ability of charge carriers and corrosion resistance, resulting in dendrite-free zinc deposition. Experimental results show excellent performance in terms of cycle life and capacity retention.
NANO-MICRO LETTERS
(2022)
Article
Chemistry, Multidisciplinary
Dong Han et al.
Summary: A new eutectic electrolyte is developed to enhance the stability of aqueous zinc-ion battery. The electrolyte effectively inhibits hydrogen evolution reaction, corrosion, dendrite formation, and by-products, enabling stable cycling of the zinc anode.
ADVANCED FUNCTIONAL MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Hongyu Qin et al.
Summary: This study introduces a thiourea additive to improve the performance of aqueous zinc ion batteries (AZIBs) by constructing a unique metal-molecule interface, which regulates the interface chemistry of the zinc electrode and the electrolyte environment. The metal-molecule interface acts as a corrosion inhibitor to alleviate water-induced side reactions and as a regulator for promoting homogeneous zinc deposition, resulting in a corrosion-free and dendrite-free zinc anode. The zinc|zinc symmetric cell exhibits an extended lifespan and high cumulative capacity, while the zinc|V2O5 full cell shows a high capacity retention after cycles.
ADVANCED FUNCTIONAL MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Rui Wang et al.
Summary: Rechargeable aqueous zinc-ion batteries are considered ideal for large-scale energy storage due to their high safety, eco-friendliness, and low cost. However, the growth of dendrites and parasitic reactions at the anode-electrolyte interface hinder their practical realization. This study proposes that the electrochemical performance of the Zn-metal anode can be improved by using a 3D ZnTe semiconductor substrate, which leads to long cycle life and small voltage hysteresis.
ADVANCED FUNCTIONAL MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Junnan Hao et al.
Summary: This study reveals the challenges in aqueous Zn-ion batteries and proposes a new electrolyte strategy to address these issues. Experimental results demonstrate that the strategy can achieve high reversibility and long lifespan for Zn-ion batteries.
ADVANCED MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Fuhua Yang et al.
Summary: It is demonstrated that H-2 evolution in aqueous zinc-ion batteries primarily originates from solvated water and can be suppressed by additives, leading to improved cycle stability and electrochemical performance.
ADVANCED MATERIALS
(2022)
Article
Engineering, Environmental
Yiqin Liu et al.
Summary: In this study, a functional double-network hydrogel electrolyte (FDHE) is designed to enhance the reversibility of zinc in wearable zinc-ion batteries (ZIBs). The results show that FDHE has robust mechanical properties and excellent reversibility in ZIBs.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Multidisciplinary Sciences
Wenyao Zhang et al.
Summary: This study reports a highly reversible aqueous zinc battery with a dynamic and self-repairing protective interphase formed by the addition of graphitic carbon nitride quantum dots. The system exhibits single Zn2+ conduction, dendrite-free Zn plating/stripping, and impressive cyclability, making it a promising alternative to lithium batteries in low-cost, large-scale applications.
NATURE COMMUNICATIONS
(2022)
Article
Chemistry, Physical
Chaofeng Zhang et al.
Summary: This paper reports a template-assisted strategy to obtain a bimetallic telluride heterostructure supported on an N-doped carbon shell, which promotes the diffusion of K+ ions for rapid charge transfer. It is shown that the electron-rich telluride sites and built-in electric fields in the heterostructure provide abundant cation adsorption sites and facilitate interfacial electron transport during potassiation/depotassiation. The heterostructure exhibits high structural stability and a highly reversible capacity up to 5000 cycles at 5 A g(-1).
ADVANCED ENERGY MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Yizhao Chai et al.
Summary: By preparing a ZnIn alloy anode, reversibility and stability of Zn metal in aqueous Zn-ion batteries are achieved. The bulk phase structure of the ZnIn alloy and the evenly dispersed indium nucleation enable stable Zn deposition and prevent further nucleation. This method improves the Zn stripping process and effectively inhibits Zn dendrite growth.
Article
Chemistry, Physical
Tianjiang Sun et al.
Summary: This study proposes a mild perchlorate-based electrolyte without strong acid addition to improve the efficiency of the Mn2+/MnO2 redox reaction. The results show that this novel aqueous proton battery exhibits excellent rate capability and cycle life, even under low-temperature conditions.
JOURNAL OF MATERIALS CHEMISTRY A
(2022)
Article
Chemistry, Physical
Yujin Ren et al.
Summary: Flexible zinc-ion batteries have rapidly developed in recent years as an essential branch of flexible energy storage devices. This study successfully utilized 3D printing technology to create flexible aqueous micro-ZIBs, demonstrating their stability and potential.
Article
Chemistry, Multidisciplinary
Shuanggui Zhang et al.
Summary: By embedding high-density and high-performance active materials in ZnTe@C nanowires, fast charge transfer paths are provided while maintaining the structural and electrical integrity of ZnTe. This strategy represents an effective way to achieve electrode materials with excellent gravimetric and volumetric capacities in energy storage systems.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Chemistry, Physical
Runzhi Qin et al.
Summary: The addition of ethylene glycol as an additive in aqueous electrolyte effectively inhibits the short-circuit issue induced by zinc dendrite growth in zinc-ion batteries, leading to longer cycling lifespan. By modifying the solvation sheath of zinc ions, the diffusion rate of zinc ions is reduced, promoting a uniform deposition morphology.
Article
Nanoscience & Nanotechnology
Lu Yue et al.
Summary: In this study, a dual enhancement of SnS2/graphene composite anodes for sodium-ion batteries was achieved through S-compositing and Co doping via a one-step hydrothermal reaction. The composite showed superior cycling stability and rate capability, with high reversible specific capacities at different current densities. The enhancement mechanism was attributed to the composite's favorable three-dimensional structure, Co doping, and S-composition inducing a synergistic effect.
ACS APPLIED MATERIALS & INTERFACES
(2021)
Article
Chemistry, Multidisciplinary
Junnan Hao et al.
Summary: A similar antisolvent strategy has been used to enhance Zn reversibility and suppress dendrite growth in Zn plating/stripping, with promising results shown in 50% methanol electrolyte. This low-cost strategy can be easily applied to other solvents, demonstrating practical universality and potential for enhancing performance in electrochemistry and energy storage research.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2021)
Article
Chemistry, Multidisciplinary
Xiaohui Zeng et al.
ADVANCED MATERIALS
(2021)
Article
Multidisciplinary Sciences
Zedong Zhao et al.
Summary: This study developed a fluorinated covalent organic framework film as a protective layer for aqueous zinc anode battery, aiming to reduce zinc dendrite growth and electrolyte corrosion, achieve horizontally arranged zinc deposition, and improve stability and cycling performance.
NATURE COMMUNICATIONS
(2021)
Article
Nanoscience & Nanotechnology
Longsheng Cao et al.
Summary: The study introduces an aqueous zinc battery with a solid-electrolyte interphase that enables excellent performance in various tests, demonstrating its potential for practical applications in energy storage.
NATURE NANOTECHNOLOGY
(2021)
Article
Chemistry, Multidisciplinary
Yuping Liu et al.
Summary: A highly efficient electrocatalyst, consisting of monodisperse molybdenum nanoparticles embedded onto nitrogen-doped graphene, was developed to enhance lithium polysulfide conversion in lithium-sulfur batteries. The electrocatalyst facilitates fast conversion of LiPSs by attracting electrons of LiPS anions. Batteries based on this new cathode showed excellent performance and stability, suggesting the great potential of molybdenum nanoparticles in high-performance Li-S batteries.
Article
Chemistry, Multidisciplinary
Jiming Peng et al.
Summary: A surface-coating strategy using NiFe2O4 was developed to enhance the performance of Li-rich layered oxides in lithium-ion batteries, resulting in improved cycle stability and rate capability. This strategy effectively traps surface lattice oxygen and restrains cation migration, decoupling the surface oxygen redox from cation movement.
Article
Chemistry, Multidisciplinary
Sailin Liu et al.
Summary: By tuning the solvation structure of the electrolyte and using fire-retardant triethyl phosphate as a cosolvent, the challenges of cathode dissolution, water reactivity, and zinc dendrites in aqueous zinc-ion batteries have been successfully addressed. The optimized electrolyte structure leads to high average Coulombic efficiency in Zn/Cu cells and enables over 1000 cycles at high current density.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Shilin Zhang et al.
Summary: A surface-charge-regulating strategy was developed to fabricate microsized 2D non-layered metal sulfides, which can easily modulate the manner of surface charge arrangement during the growth of crystal nuclei. This approach resulted in materials with preferred orientation, atomic thickness, and potential for energy-related applications.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Junnan Hao et al.
Summary: Research findings indicate that Zn2+ storage in CuI cathode involves a direct conversion reaction mechanism, rather than an intercalation mechanism, and this mechanism can also be applied to other high-capacity cathodes effectively.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2021)
Article
Chemistry, Multidisciplinary
Peng Sun et al.
Summary: The addition of glucose in ZnSO4 electrolyte can improve the performance of Zn ion batteries by suppressing Zn dendrite growth and side reactions, enhancing stability.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2021)
Article
Chemistry, Physical
Shao-Jian Zhang et al.
Summary: The study introduces a simple method using ethylene diamine tetraacetic acid tetrasodium salt (Na(4)EDTA) to suppress the poor reversibility of the Zn anode in aqueous Zn-ion batteries, effectively inhibiting dendrite growth and hydrogen evolution. Additionally, the added EDTA promotes desolvation of Zn, prolonging the electrode lifespan.
ADVANCED ENERGY MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Junnan Hao et al.
ADVANCED FUNCTIONAL MATERIALS
(2020)
Article
Chemistry, Multidisciplinary
Junnan Hao et al.
ADVANCED MATERIALS
(2020)
Article
Chemistry, Physical
Xiaohui Zeng et al.
ADVANCED ENERGY MATERIALS
(2020)
Review
Chemistry, Multidisciplinary
Junnan Hao et al.
ENERGY & ENVIRONMENTAL SCIENCE
(2020)
Article
Chemistry, Multidisciplinary
Junnan Hao et al.
ADVANCED FUNCTIONAL MATERIALS
(2019)
Review
Chemistry, Physical
Xiaohui Zeng et al.
ENERGY STORAGE MATERIALS
(2019)