Recent Development of Aqueous Multivalent-Ion Batteries Based on Conversion Chemistry

Article Multidisciplinary Sciences

Constructing robust heterostructured interface for anode-free zinc batteries with ultrahigh capacities

Xinhua Zheng et al.

Summary: The design of a two-dimensional antimony/antimony-zinc alloy heterostructured interface enables dendrite-free Zn deposition with high areal capacity and energy density.

NATURE COMMUNICATIONS (2023)

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Article Chemistry, Physical

Tuning Ion Transport at the Anode-Electrolyte Interface via a Sulfonate-Rich Ion-Exchange Layer for Durable Zinc-Iodine Batteries

Leiqian Zhang et al.

Summary: By constructing a sulfonate-rich ion-exchange layer (SC-PSS) to modulate the transport and reaction of polyiodide and Zn2+, the corrosion and dendritic growth issues on the anode of zinc-iodine batteries can be addressed. The resulting batteries exhibit proper performance over 6000 cycles with high-capacity retention (90.2%) and reversibility (99.89%). The SC-PSS layer blocks polyiodide permeation through electrostatic repulsion and restricts undesirable 2D diffusion of Zn2+ by facilitating desolvation and chemisorption.

ADVANCED ENERGY MATERIALS (2023)

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Article Chemistry, Multidisciplinary

Toward Forty Thousand-Cycle Aqueous Zinc-Iodine Battery: Simultaneously Inhibiting Polyiodides Shuttle and Stabilizing Zinc Anode through a Suspension Electrolyte

Guanhong Chen et al.

Summary: By designing a suspension electrolyte with vermiculite nanosheets (VS), the movement of polyiodides and the stability of the zinc anode in zinc-iodine (Zn-I-2) batteries can be simultaneously controlled. The dissolved polyiodides are effectively anchored on the surface of VS, suppressing the shuttle effect. The VS interfacial layer inhibits side reactions induced by polyiodides, and compensates for the negative charges on the VS surface, enabling dendrite-free Zn plating/stripping behavior. As a result, the Zn-I-2 battery with VS electrolyte achieves an ultra-long lifespan of 40000 cycles with negligible capacity decay at 20 C.

ADVANCED FUNCTIONAL MATERIALS (2023)

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Article Chemistry, Multidisciplinary

A Universal Strategy Toward Low-Cost Aqueous Sulfur-Iodine Batteries

Chuanlong Wei et al.

Summary: Researchers demonstrate an aqueous sulfur-iodine chemistry that can be used in rechargeable aqueous batteries, offering a new possibility for practical applications.

ADVANCED FUNCTIONAL MATERIALS (2023)

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Article Chemistry, Multidisciplinary

2D Mesoporous Zincophilic Sieve for High-Rate Sulfur-Based Aqueous Zinc Batteries

Jiahao Liu et al.

Summary: In this study, an acid-assisted confined self-assembly method (ACSA) was developed to prepare a two-dimensional mesoporous zincophilic sieve (2DZS) as the kinetic interface. The 2DZS interface effectively reduces the anodic polarization of sulfur-based aqueous zinc batteries (SZBs) at high current density, leading to improved lifespan and energy density.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2023)

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Article Chemistry, Multidisciplinary

A Mesoporous Tungsten Oxynitride Nanofibers/Graphite Felt Composite Electrode with High Catalytic Activity for the Cathode in Zn-Br Flow Battery

HyunJin Jung et al.

Summary: This study presents a composite electrode that reduces the electrochemical polarization in aqueous zinc-bromine flow batteries by providing a higher number of catalytically-active sites for faster bromine reaction. The composite electrode consists of conductive graphite felt and highly active tungsten oxynitride nanofibers. The addition of these nanofibers significantly improves reaction kinetics and ion diffusion.

SMALL (2023)

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Article Multidisciplinary Sciences

An asymmetric electrolyte to simultaneously meet contradictory requirements of anode and cathode

Shengmei Chen et al.

Summary: The authors address the contradictory demands from zinc metal anode and cathodes in zinc metal batteries by designing an asymmetric electrolyte composed of an inorganic solid-state electrolyte and a hydrogel electrolyte.

NATURE COMMUNICATIONS (2023)

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Article Multidisciplinary Sciences

Development of rechargeable high-energy hybrid zinc-iodine aqueous batteries exploiting reversible chlorine-based redox reaction

Guojin Liang et al.

Summary: The use of an iodine-based cathode in combination with a Zn anode and a Cl-containing aqueous electrolyte solution demonstrates reversible high-energy interhalogen reactions. This approach allows for a specific discharge capacity of 612.5 mAh g(I2)(-1) and a discharge capacity retention of about 74% after 300 cycles. The efficient and reversible ClRR is achieved by utilizing interhalogen coordinating chemistry and redox-active halogen atoms.

NATURE COMMUNICATIONS (2023)

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Article Engineering, Environmental

Encapsulating selenium into mesoporous carbon for high-performance aqueous Cu-Se battery

Zhouxiang Wu et al.

Summary: A novel aqueous Cu-Se battery with Se encapsulated in ordered mesoporous carbon as cathode is designed. The battery shows high specific capacity and favorable long-span cycling capability due to the synergistic effects of four-electron conversion and robust mesoporous carbon host.

CHEMICAL ENGINEERING JOURNAL (2023)

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Article Engineering, Environmental

A high-performance COF-based aqueous zinc-bromine battery

You Zhang et al.

Summary: Aqueous zinc-bromine batteries integrated with COF-bromine cathode and COF-coated zinc metal anode can effectively solve the problems of zinc dendrite growth and bromine species shuttle effect, achieving stable and efficient energy storage. The COF exhibits strong adsorption towards Br species, immobilizing them and facilitating bidirectional conversion of polybromide. The COF artificial layer on the zinc metal anode regulates zinc flux and prevents dendrite growth. The COF-Zn||Br-2-exCOF full cell delivers a remarkable capacity of approximately 183 mAh g(-1) (approximately 0.61 mAh cm(-2)) after 1000 cycles, with capacity retention of about 83% at 2 A g(-1) and high Coulombic efficiency of -99%. This work inspires insights into developing high-performance aqueous zinc-bromine battery systems.

CHEMICAL ENGINEERING JOURNAL (2023)

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Article Chemistry, Multidisciplinary

Redox Catalysis Promoted Activation of Sulfur Redox Chemistry for Energy-Dense Flexible Solid-State Zn-S Battery

Hong Zhang et al.

Summary: In this study, a high-energy Zn-S system was designed with a high-capacity cathode and fast redox mediators, allowing for highly reversible conversion between sulfur and ZnS. The proposed redox electrocatalysis effect provides reliable insights into the tunable Zn-S chemistry, leading to improved performance in Zn-S cells.

ACS NANO (2022)

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Review Chemistry, Multidisciplinary

Recent Advances of Aqueous Rechargeable Zinc-Iodine Batteries: Challenges, Solutions, and Prospects

Dun Lin et al.

Summary: Aqueous rechargeable zinc-iodine batteries (ZIBs) are considered as promising candidates for grid-scale electrochemical energy storage due to their safety, high theoretical capacity, and energy density. However, challenges such as self-discharge, sluggish kinetics, low energy density, and unstable Zn metal anodes need to be addressed. This article reviews the electrochemistry of ZIBs, discusses the fundamental questions, and highlights the key strategies and recent accomplishments in overcoming these challenges.

ADVANCED MATERIALS (2022)

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Article Chemistry, Physical

Multifunctional porous carbon strategy assisting high-performance aqueous zinc-iodine battery

Lijing Yan et al.

Summary: The study proposes a strategy of using porous carbon to modify the zinc anode and immobilize the iodine active materials in order to address the performance degradation issues of aqueous zinc-iodine batteries. The optimized battery demonstrates satisfactory capacity retention and fast charging speed at high rates.

CARBON (2022)

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Article Engineering, Environmental

Electrode and electrolyte regulation to promote coulombic efficiency and cycling stability of aqueous zinc-iodine batteries

Wanlong Wu et al.

Summary: The study achieves excellent rate capability and cycling stability by synergistically regulating the electrode and electrolyte to confine the charged products. The use of conducting polymer polyaniline (PANI) as the polyiodide binder leads to high coulombic efficiency and capacity retention in aqueous zinc-iodine batteries.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Chemistry, Physical

A renewable biomass-based lignin film as an effective protective layer to stabilize zinc metal anodes for high-performance zinc-iodine batteries

Ke Wang et al.

Summary: This study demonstrates the use of renewable polymers as a surface coating layer to protect zinc anodes in zinc-iodine batteries, effectively suppressing triiodide ion shuttling and zinc dendrite formation. The results show that the introduction of renewable polymers significantly improves the stability and cycle life of the batteries.

JOURNAL OF MATERIALS CHEMISTRY A (2022)

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Article Chemistry, Physical

A High Energy Density Bromine-Based Flow Battery with Two-Electron Transfer

Yue Xu et al.

Summary: Bromine-based flow batteries with BrCl2-/Br- as a redox couple demonstrate high capacity and long cycle life by inhibiting side reactions, showing great potential for large-scale energy storage applications.

ACS ENERGY LETTERS (2022)

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Article Chemistry, Physical

High performance and long cycle life neutral zinc-iron flow batteries enabled by zinc-bromide complexation

Minghui Yang et al.

Summary: Zinc-based flow batteries with bromide ions as stabilizers show improved redox reversibility between Zn and Zn2+. The addition of ZnBr2 as an electrolyte additive promotes the coordination interactions between Zn2+ and Br-, enhancing the efficiency and cycling stability of neutral Zn/Fe flow batteries for large-scale energy storage.

ENERGY STORAGE MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Unlocking the Reversible Selenium Electrode for Non-Aqueous and Aqueous Calcium-Ion Batteries

Rui Zhou et al.

Summary: Calcium-ion batteries have promising potential as multivalent ion battery systems, and selenium has been explored as a reliable electrode material. Selenium demonstrates high energy density and long-term cyclic stability, making it suitable for both non-aqueous and aqueous electrolytes.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Polyiodide Confinement by Starch Enables Shuttle-Free Zn-Iodine Batteries

Shao-Jian Zhang et al.

Summary: This study proposes a structure confinement strategy using starch to suppress polyiodide shuttling in Zn-I-2 batteries, resulting in a highly reversible and long-cycling Zn-I-2 battery with high Coulombic efficiency. The starch effectively inhibits Zn corrosion triggered by polyiodide, providing a cheap yet effective strategy for high-cyclability Zn-I-2 batteries.

ADVANCED MATERIALS (2022)

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Article Engineering, Environmental

Regulating the electro-deposition behavior of Fe metal anode and the applications in rechargeable aqueous iron-iodine batteries

Wanlong Wu et al.

Summary: In this study, the deposition behavior of iron metal electrodes was regulated by zinc doping, resulting in the formation of homogeneous small particles and achieving high coulombic efficiency and stability. This research has potential implications for the development of high-performance aqueous iron-metal batteries.

CHEMICAL ENGINEERING JOURNAL (2022)

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Review Materials Science, Multidisciplinary

Ion migration and defect effect of electrode materials in multivalent-ion batteries

Zhexuan Liu et al.

Summary: This review highlights the fundamental scientific understanding of ion migration and defect chemistry in electrode materials of multivalent-ion batteries (MVIBs). The basic principles and key factors affecting ion diffusion are discussed, and the influence of defect engineering on multivalent-ion diffusion behavior is explained. The application of defective electrodes in MVIBs with advanced functions is also explored.

PROGRESS IN MATERIALS SCIENCE (2022)

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Article Chemistry, Multidisciplinary

Bio-Derived and Cost-Effective Membranes with High Selectivity for Redox Flow Batteries Based on Host-Guest Chemistry

Li Gao et al.

Summary: Redox flow batteries (RFBs) are a promising energy storage system for renewable energy, with membranes playing a critical role in regulating their performance. This study reports a membrane composed of abundant natural materials, which achieves high selectivity through host-guest interactions. The membrane shows promise for zinc-iodine RFBs, with high selectivity towards triiodide.

SMALL (2022)

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Article Chemistry, Physical

Four-Electron Transfer Reaction Endows High Capacity for Aqueous Cu-Se Battery

Junwei Zhang et al.

Summary: In this study, a novel Cu-Se conversion battery was constructed based on the quantitative analysis of chemical thermodynamic properties. The synergism between the variable-valence charge carrier and copper selenides enables the battery to exhibit a high initial reversible capacity, exceptional long-span cycling stability, and outstanding rate performance.

ADVANCED ENERGY MATERIALS (2022)

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Article Chemistry, Applied

Non-layer-transformed Mn3O4 cathode unlocks optimal aqueous magnesium-ion storage via synergizing amorphous ion channels and grain refinement

Zhongyu Pan et al.

Summary: In this study, a pre-treated Mn3O4 cathode was chosen for aqueous Mg2+ storage, and the surface was decorated with tortuous amorphous ion diffusion channels, resulting in optimal performances.

JOURNAL OF ENERGY CHEMISTRY (2022)

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Article Chemistry, Physical

Controllable C-N site assisting observable potential difference for homogeneous copper deposition in aqueous Cu-S batteries

Huihui Yan et al.

Summary: Aqueous Cu-S battery with four-electron sulfur reaction has been developed, achieving high capacity discharge and recyclability by protecting the copper metal anode from dendrite formation.

ENERGY STORAGE MATERIALS (2022)

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Article Chemistry, Physical

A Highly Reversible Low-Cost Aqueous Sulfur-Manganese Redox Flow Battery

Jiafeng Lei et al.

Summary: This study presents an ultra-low-cost sulfur-manganese redox flow battery, which solves the dendrite issue of metal-manganese batteries and achieves improved cycling stability. The low cost of sulfur and manganese species enables a significantly low electrolyte cost.

ACS ENERGY LETTERS (2022)

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Article Chemistry, Physical

Spreading the full spectrum of layer-structured compounds for kinetics-enhanced aqueous multivalent metal-ion batteries

Jingjuan Li et al.

Summary: Aqueous rechargeable multivalent metal-ion batteries have great potential due to their high ionic diffusivity and safety. However, challenges such as active materials dissolution, structural collapse, and low electrical conductivity still need to be addressed.

ENERGY STORAGE MATERIALS (2022)

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Article Chemistry, Physical

Suppressed Layered-to-Spinel Phase Transition in δ-MnO2 via van der Waals Interaction for Highly Stable Zn/MnO2 Batteries

Ce Qiu et al.

Summary: Coupling delta-MnO2 nanosheets with reduced graphene oxide (rGO) through vdW self-assembly can effectively suppress the phase transition issue and achieve excellent cycling performance in the hybrid cathode.

SMALL METHODS (2022)

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Article Chemistry, Multidisciplinary

Boosting Cathode Activity and Anode Stability of Zn-S Batteries in Aqueous Media Through Cosolvent-Catalyst Synergy

Min Yang et al.

Summary: In this study, we developed an optimized electrolyte for aqueous Zn-S battery using a mixture of tetraglyme (G4), water, and I2. The synergistic effect of G4-I2 improved the conversion kinetics of S and stabilized the Zn anode, leading to enhanced reversibility and cycling stability of the battery. The improved Zn-S cell delivered a high capacity at high current density and retained over 70% capacity after 600 cycles at 4A g(-1). The findings of this study can be applied to other ethers/water hybrid electrolytes, demonstrating the universality of the optimized electrolyte design strategy.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Multidisciplinary Sciences

Development of long lifespan high-energy aqueous organic∥iodine rechargeable batteries

Zishuai Zhang et al.

Summary: Rechargeable aqueous metal parallel to I-2 electrochemical energy storage systems offer a cost-effective alternative for grid energy storage. The use of 3,4,9,10-perylenetetracarboxylic diimide (PTCDI) as a negative electrode active material and a KCl/I-2 aqueous electrolyte solution can overcome the drawbacks of metallic deposition and the formation of electrochemically inactive by-products. The proposed system shows promising performance with high discharge capacity and voltage.

NATURE COMMUNICATIONS (2022)

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Article Chemistry, Physical

A durable ZnS cathode for aqueous Zn-S batteries

Dongdong Liu et al.

Summary: By using a carbon-sheathed ZnS cathode and introducing iodinated thiourea as a redox mediator, the activation barrier was effectively reduced, leading to a high-performance Zn-S battery.

NANO ENERGY (2022)

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Article Chemistry, Multidisciplinary

A High-Performance Quasi-Solid-State Aqueous Zinc-Dual Halogen Battery

Shuyao Lv et al.

Summary: This article introduces a quasi-solid aqueous zinc-dual halogen battery with high capacity and energy density. By constructing a freestanding carbon cloth-iodine cathode and a concentrated aqueous gel electrolyte, as well as adding LiNO3 and acrylamide-based polymer matrix, efficient battery reactions and stable anode/electrolyte interface are achieved.

ACS NANO (2022)

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Review Chemistry, Multidisciplinary

Iodine Redox Chemistry in Rechargeable Batteries

Jizhen Ma et al.

Summary: This article discusses the potential and challenges of combining halogens with metal anodes in a single cell to develop novel rechargeable batteries, emphasizing the importance of understanding the fundamental reactions of iodine/polyiodide for designing high-performance cathodes. Special focus is placed on the basic principles of iodine redox chemistry and its correlation with structure-function relationships.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Nanoscience & Nanotechnology

Carbon Nanotube Scaffolds Entrapped in a Gel Matrix for Realizing the Improved Cycle Life of Zinc Bromine Redox Flow Batteries

Raghu Pandiyan Naresh et al.

Summary: In this study, a nanofiller (such as multiwalled carbon nanotubes) dispersed in a polymer matrix effectively inhibited bromine diffusion in zinc bromine redox flow batteries. The MWCNT/PAN composite Daramic membrane showed remarkable electrochemical performance with high Coulombic efficiency compared to traditional microporous membranes. This novel membrane also displayed exceptional long cycling performance and reduced self-discharge rate in the flow battery system, showcasing its potential as an alternative to existing membranes in this application.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Conversion-Type Nonmetal Elemental Tellurium Anode with High Utilization for Mild/Alkaline Zinc Batteries

Ze Chen et al.

Summary: A conversion-type Te-based ZIB that can work in both mild and alkaline electrolytes is reported in this study, delivering remarkable capacities with high anode utilization. The system achieves ultralong cycling life and high gravimetric energy density, shedding light on the development of advanced conversion-type anode for high-performance batteries with superior stability.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Confining Aqueous Zn-Br Halide Redox Chemistry by Ti3C2Tx MXene

Xinliang Li et al.

Summary: This study introduces an advanced aqueous zinc redox battery by incorporating an electrochemically active parasite Br-2 into the Ti3C2Tx MXene host. The battery delivers efficient output capability in the high-voltage region and shows excellent cycling performance at low temperatures.

ACS NANO (2021)

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Article Chemistry, Multidisciplinary

Halogenated Ti3C2 MXenes with Electrochemically Active Terminals for High-Performance Zinc Ion Batteries

Mian Li et al.

Summary: Experimental exploration of various halogen terminals on the surface of Ti3C2 MXenes showed that the presence of Br and I elements resulted in improved electrochemical performance for aqueous zinc ion batteries. The Lewis-acidic-melt etching route proved to be effective in tuning the surface chemistry of MXenes for expanding their potential applications.

ACS NANO (2021)

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Article Chemistry, Multidisciplinary

Enhanced Redox Kinetics and Duration of Aqueous I2/I- Conversion Chemistry by MXene Confinement

Xinliang Li et al.

Summary: The study introduced a Nb2CTX host and achieved electro-oxidation of I- ions in MXene through electrodeposition strategy, thereby improving redox kinetics and duration. The aqueous Zn battery based on a Zn metal anode and ZnSO4 electrolyte showed outstanding performance, surpassing other aqueous MXenes and I-2-metal batteries.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Electrocatalytic Iodine Reduction Reaction Enabled by Aqueous Zinc-Iodine Battery with Improved Power and Energy Densities

Longtao Ma et al.

Summary: In this study, Prussian blue analogue hosts with continuous channels were proposed to enhance I2 utilization efficiency and reaction kinetics, leading to the release of 1/3 I-. The Co[Co1/4Fe3/4(CN)(6)]/I-2//Zn battery showed high energy density and power density, with promising rate performance.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

A Single-Flow Battery with Multiphase Flow

Lihi Amit et al.

Summary: The article introduces a potentially inexpensive Zn-Br-2 RFB that is membraneless and requires only a single flow. The study explores the effects of polybromide-phase volume fraction and Br-2 concentration on cell performance and plating efficiencies.

CHEMSUSCHEM (2021)

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Article Multidisciplinary Sciences

A four-electron Zn-I2 aqueous battery enabled by reversible I-/I2/I+ conversion

Yiping Zou et al.

Summary: In this study, a four-electron aqueous zinc-iodine battery was developed by enhancing the iodine electrochemistry using a specially designed electrolyte. Experimental characterization and modeling showed that limited water activity and sufficient free chloride ions in the electrolyte are crucial for the four-electron process. The advantages of the electrolyte also help stabilize the zinc anode, leading to a high energy density and reliable cycling performance for the Zn-I-2 aqueous battery.

NATURE COMMUNICATIONS (2021)

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Article Chemistry, Physical

Reversible Insertion of I-Cl Interhalogen in a Graphite Cathode for Aqueous Dual-Ion Batteries

Qiubo Guo et al.

Summary: This study introduces a novel aqueous deep eutectic solvent gel electrolyte that enables reversible chloride storage in a graphite cathode through the formation of iodine-chloride interhalogens. The results demonstrate three reversible steps in the process, including iodine plating, oxidation to form I-Cl interhalides, and intercalation into graphite.

ACS ENERGY LETTERS (2021)

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Article Chemistry, Multidisciplinary

An Energetic CuS-Cu Battery System Based on CuS Nanosheet Arrays

Yichun Wang et al.

Summary: In this study, a high-energy aqueous copper ion system based on CuS nanosheet arrays was developed, showing high capacity, robust rate capability, and ultra-stable cycling. The charge-storage mechanism involving the reversible transition from CuS to Cu2S was systematically investigated. Additionally, a hybrid ion battery consisting of CuS positive electrode and Zn negative electrode was demonstrated, providing high energy and power performance.

ACS NANO (2021)

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Article Chemistry, Multidisciplinary

Synergistic Effect between S and Se Enhancing the Electrochemical Behavior of SexSy in Aqueous Zn Metal Batteries

Wei Li et al.

Summary: By introducing selenium and its synergistic effect with sulfur, high-performance conversional cathode materials have been successfully designed in this study, with optimized selenium content achieving excellent electrochemical properties to enhance the energy density and stability of aqueous Zn batteries.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Water-Salt Oligomers Enable Supersoluble Electrolytes for High-Performance Aqueous Batteries

Shengying Cai et al.

Summary: This study reports a highly soluble ZnCl2/ZnBr2/Zn(OAc)(2) aqueous electrolyte, which breaks through the physical solubility limit by forming acetate-capped water-salt oligomers, enabling high-performance aqueous dual-ion batteries.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Electrolyte Design for In Situ Construction of Highly Zn 2+ ‐Conductive Solid Electrolyte Interphase to Enable High‐Performance Aqueous Zn‐Ion Batteries under Practical Conditions

Xiaohui Zeng et al.

ADVANCED MATERIALS (2021)

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Article Chemistry, Physical

Unraveling H+/Zn2+ Sequential Conversion Reactions in Tellurium Cathodes for Rechargeable Aqueous Zinc Batteries

Jinzhi Wang et al.

Summary: The study revealed a sequential conversion reaction involving H+/Zn2+ with 6e(-) transfer for tellurium-based cathodes, achieving outstanding capacity in aqueous zinc electrolytes. Two distinct redox processes of TeO2 <-> Te and Te <-> ZnTe were explicitly revealed within the electrochemical window of routine aqueous Zn electrolytes.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2021)

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Article Chemistry, Physical

A trifunctional electrolyte for high-performance zinc-iodine flow batteries

Q. P. Jian et al.

Summary: The NH4Br improved electrolyte for zinc-iodine flow battery enhances ionic conductivity, reduces iodine precipitation and zinc dendrite growth, improves kinetics and reversibility of redox couples, and provides high energy efficiency, charge capacity, and cycle life compared to conventional electrolyte.

JOURNAL OF POWER SOURCES (2021)

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Article Chemistry, Physical

A defect-free MOF composite membrane prepared via in-situ binder-controlled restrained second-growth method for energy storage device

Jine Wu et al.

Summary: This study presents a method to introduce continuous and uniform metal organic framework selective layers on porous polymer substrates via controlling MOF nucleation and growth, creating highly selective composite membranes. The well-ordered pores of MOF play a key role in controlling selectivities on different ions, leading to improved coulombic efficiency in batteries.

ENERGY STORAGE MATERIALS (2021)

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Article Nanoscience & Nanotechnology

Establishing High-Performance Quasi-Solid Zn/I2 Batteries with Alginate-Based Hydrogel Electrolytes

Wenshuo Shang et al.

Summary: By designing and synthesizing alginate-based hydrogel electrolyte, the cycling stability and performance of Zinc-iodine batteries are significantly improved. The hydrogel effectively blocks the shuttle of triiodide ions, mitigates Zn dendritic growth and corrosion reactions, leading to higher capacity and cycling durability of the battery.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Prototypical Study of Double-Layered Cathodes for Aqueous Rechargeable Static Zn-I2 Batteries

Dun Lin et al.

Summary: By utilizing a double-layered cathode structure, the undesired shuttling of triiodide ions has been successfully suppressed, resulting in outstanding Coulombic efficiency and voltage efficiency for ZIBs. These findings offer new insights for the design and fabrication of ZIBs and other batteries based on conversion reactions.

NANO LETTERS (2021)

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Article Multidisciplinary Sciences

A universal strategy towards high-energy aqueous multivalent-ion batteries

Xiao Tang et al.

Summary: Rechargeable multivalent-ion batteries, such as those using calcium, magnesium or aluminum, are promising candidates for large-scale electrochemical energy storage. Researchers have developed various aqueous multivalent-ion cells utilizing concentrated aqueous gel electrolytes, sulfur-containing anodes, and high-voltage metal oxide cathodes, showing satisfactory performance and potential for future energy storage technologies.

NATURE COMMUNICATIONS (2021)

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Article Energy & Fuels

Polysulfide-based redox flow batteries with long life and low levelized cost enabled by charge-reinforced ion-selective membranes

Zhejun Li et al.

Summary: The study introduces a membrane design to reduce capacity decay in polysulfide-based ARFBs over long cycles and durations, enhancing cost-effectiveness. By developing a charge-reinforced ion-selective membrane, the polysulfide flow battery demonstrates stable cycling with low capacity decay rate. Small-angle X-ray scattering and in-situ attenuated total reflectance-Fourier transform infrared/solid-state NMR indicate improved membrane properties compared to commercial Nafion membrane.

NATURE ENERGY (2021)

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Article Chemistry, Physical

Materials design and fundamental understanding of tellurium-based electrochemistry for rechargeable batteries

Yue Zhang et al.

Summary: Rechargeable tellurium (Te)-based batteries are promising energy storage devices with high volumetric energy density, but face challenges in terms of electrochemistry and overall performance. Research focuses on understanding the role of Te structure, carbon host chemistry, electrolytes, and addressing issues like Te pulverization and parasitic effects to achieve reversible Te phase transitions. Additional studies are conducted on novel metal-Te based batteries to compare performance data and explore potential research directions for the future.

ENERGY STORAGE MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Laser-Induced Graphene Assisting Self-Conversion Reaction for Sulfur-Free Aqueous Cu-S Battery

Zhengwei Yang et al.

Summary: A novel redox couple of CuS/Cu2S is proposed for high reversible capacity in aqueous metal-sulfur batteries, with the commercially viable laser-induced graphene (LIG) successfully applied for the first time. The synergism between the novel redox couple and LIG leads to good cycling stability and high reversible capacity in the battery performance.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

A Cascade Battery: Coupling Two Sequential Electrochemical Reactions in a Single Battery

Chunlong Dai et al.

Summary: The cascade battery proposed in this study couples two sequential electrochemical reactions in a single battery, showing many advantages compared to traditional batteries. It integrates two batteries internally, eliminating the need for additional inactive connecting materials, can more fully utilize the inactive reaction chamber, and achieve a higher areal capacity even at low solid cathode loading.

ADVANCED MATERIALS (2021)

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Article Engineering, Environmental

Phosphorus-doped carbon sheets decorated with SeS2 as a cathode for aqueous Zn-SeS2 battery

Wei Li et al.

Summary: In this study, phosphorus-doped carbon sheets encapsulated SeS2 was proposed as a conversional cathode for aqueous Zn-based batteries, achieving high energy density and long cycle life. The reaction mechanisms were explored, and experimental and theoretical calculations suggested that I2 additive acted as a redox mediator to enhance battery performance.

CHEMICAL ENGINEERING JOURNAL (2021)

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Review Chemistry, Multidisciplinary

Sulfur-Based Aqueous Batteries: Electrochemistry and Strategies

Jiahao Liu et al.

Summary: This article focuses on constructing a theory-to-application methodology for aqueous sulfur-based batteries. Research reveals the complexity in the electrochemistry of aqueous sulfur-based batteries, which poses challenges and potential for future development. Further exploration in both theory and practice is needed for the future development direction.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Chemistry, Multidisciplinary

Stabilizing Zinc Electrodeposition in a Battery Anode by Controlling Crystal Growth

Shuo Jin et al.

Summary: A method of crystal growth stabilization using polymer-salt complexes has been proposed to reshape the deposition of crystalline metals, allowing for exceptional morphological control and unprecedented cycle life in rechargeable batteries utilizing zinc as an anode material. Preliminary studies have demonstrated the practical benefits of this approach in Zn-I2 full battery cells.

SMALL (2021)

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Review Chemistry, Multidisciplinary

The Emerging of Aqueous Zinc-Based Dual Electrolytic Batteries

Chunlong Dai et al.

Summary: Aqueous zinc-based batteries face limitations due to intercalation reactions and strict cathode requirements, while zinc-based dual electrolytic batteries utilize reversible electrolytic reactions for high performance and safety. Various types of zinc-based DEBs have been systematically studied, and opportunities and challenges for the future have been identified.

SMALL (2021)

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Article Chemistry, Physical

High-Rate Aqueous Aluminum-ton Batteries Enabled by Confined Iodine Conversion Chemistry

Shuo Yang et al.

Summary: A new conversion-type cathode material for rechargeable aqueous aluminum-ion batteries, based on iodine embedded in N-doped microporous carbon polyhedrons derived from MOF, shows high reversibility, superior specific capacity, and high rate performance. The reversible reaction mechanism between I-2 and I- in the battery has been confirmed through experimental analysis. Additionally, a flexible Al-I-2 battery using solid-state hydrogel electrolyte demonstrates comparable performance to those using liquid electrolyte and is suitable for powering wearable devices.

SMALL METHODS (2021)

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Article Chemistry, Physical

Rechargeable aqueous zinc-bromine batteries: an overview and future perspectives

Yanbin Yin et al.

Summary: Zinc-bromine batteries are receiving attention for their high theoretical energy density and low cost, yet face obstacles in large-scale applications. Therefore, in-depth research and advancement on the battery's structure, electrolyte, anode, cathode, and membrane are significant. This review of past and current investigations provides insights for future development, focusing on materials and chemistry.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2021)

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Article Chemistry, Physical

Highly reversible aqueous zinc metal batteries enabled by fluorinated interphases in localized high concentration electrolytes

Shunqiang Chen et al.

Summary: In this study, a localized high concentration electrolyte (LHCE) using 1,4-dioxane as the diluent and hydrogen-bond modulator is reported for aqueous zinc (Zn) metal batteries. The unique solvation structure in LHCE greatly boosts anion chemistries to induce fluorinated interphases on Zn anode and V2O5 cathode, achieving higher rate capabilities and Zn coulombic efficiencies without dendrite formation. This approach can be applied to adjust electrolyte physical properties and control interphase formation in other aqueous battery systems for practical applications.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Multidisciplinary

A Zn-S aqueous primary battery with high energy and flat discharge plateau

Lian-Wei Luo et al.

Summary: This disposable aqueous primary battery chemistry utilizes environmentally benign sulfur cathode and Zn anode, showcasing high energy density and areal capacity under high mass loading conditions.

CHEMICAL COMMUNICATIONS (2021)

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Article Chemistry, Multidisciplinary

Zinc/selenium conversion battery: a system highly compatible with both organic and aqueous electrolytes†

Ze Chen et al.

Summary: A new conversion-type Zn-Se battery has been developed, showing superior performance in both organic and aqueous electrolytes with extraordinary capacities, rate capability, and cycling performance. The battery also exhibits very low voltage plateau slopes, allowing for high energy densities and compatibility with various electrolytes, opening new possibilities for zinc batteries.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Article Chemistry, Multidisciplinary

Activating the I0/I+ redox couple in an aqueous I2-Zn battery to achieve a high voltage plateau

Xinliang Li et al.

Summary: This study demonstrates the activation of reversible redox behavior in iodine conversion batteries through electrolyte adjustment, achieving significant performance enhancements.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Article Chemistry, Multidisciplinary

A Stimulus-Responsive Zinc-Iodine Battery with Smart Overcharge Self-Protection Function

Wang Faxing et al.

ADVANCED MATERIALS (2020)

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Article Engineering, Environmental

Low-cost MgFexMn2-xO4 cathode materials for high-performance aqueous rechargeable magnesium-ion batteries

Yongquan Zhang et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Review Nanoscience & Nanotechnology

Design strategies for nonaqueous multivalent-ion and monovalent-ion battery anodes

Matthew Li et al.

NATURE REVIEWS MATERIALS (2020)

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Article Nanoscience & Nanotechnology

High-Performance Rechargeable Aluminum-Selenium Battery with a New Deep Eutectic Solvent Electrolyte: Thiourea-AlCl3

Shu-Chi Wu et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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An Aqueous Hybrid Zinc-Bromine Battery with High Voltage and Energy Density

Xinhai Yuan et al.

CHEMELECTROCHEM (2020)

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Molecular crowding electrolytes for high-voltage aqueous batteries

Jing Xie et al.

NATURE MATERIALS (2020)

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A High-Potential Anion-Insertion Carbon Cathode for Aqueous Zinc Dual-Ion Battery

Qiubo Guo et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Initiating a Reversible Aqueous Zn/Sulfur Battery through a Liquid Film

Yuwei Zhao et al.

ADVANCED MATERIALS (2020)

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A Perspective toward Practical Lithium-Sulfur Batteries

Meng Zhao et al.

ACS CENTRAL SCIENCE (2020)

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Review Energy & Fuels

Current status and future directions of multivalent metal-ion batteries

Yanliang Liang et al.

NATURE ENERGY (2020)

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Article Chemistry, Physical

Decoupled low-cost ammonium-based electrolyte design for highly stable zinc-iodine redox flow batteries

Mahboubeh Mousavi et al.

ENERGY STORAGE MATERIALS (2020)

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Article Chemistry, Physical

A high-power aqueous rechargeable Fe-I2 battery

Chong Bai et al.

ENERGY STORAGE MATERIALS (2020)

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A High-Performance Aqueous Zinc-Bromine Static Battery

Lujie Gao et al.

ISCIENCE (2020)

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Challenges and Opportunities for Multivalent Metal Anodes in Rechargeable Batteries

Xinyue Zhang et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Chemistry, Multidisciplinary

A Metal-Organic Framework as a Multifunctional Ionic Sieve Membrane for Long-Life Aqueous Zinc-Iodide Batteries

Huijun Yang et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Multidisciplinary

A Zinc-Dual-Halogen Battery with a Molten Hydrate Electrolyte

Hongwen Liu et al.

ADVANCED MATERIALS (2020)

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Aqueous Zinc-Tellurium Batteries with Ultraflat Discharge Plateau and High Volumetric Capacity

Ze Chen et al.

ADVANCED MATERIALS (2020)

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Article Multidisciplinary Sciences

Persistent and reversible solid iodine electrodeposition in nanoporous carbons

Christian Prehal et al.

NATURE COMMUNICATIONS (2020)

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A Low Cost Aqueous Zn-S Battery Realizing Ultrahigh Energy Density

Wei Li et al.

ADVANCED SCIENCE (2020)

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A superior electronic conducting tellurium electrode enabled high rate capability rechargeable Mg batteries

Tao Lu et al.

MATERIALS TODAY ENERGY (2020)

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Article Chemistry, Physical

Self-Assembled Solid-State Gel Catholyte Combating Iodide Diffusion and Self-Discharge for a Stable Flexible Aqueous Zn-I2 Battery

Keval K. Sonigara et al.

ADVANCED ENERGY MATERIALS (2020)

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Review Chemistry, Physical

Metal-Tellurium Batteries: A Rising Energy Storage System

Ze Chen et al.

SMALL STRUCTURES (2020)

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Article Chemistry, Multidisciplinary

A rechargeable aqueous aluminum-sulfur battery through acid activation in water-in-salt electrolyte

Zhiqiu Hu et al.

CHEMICAL COMMUNICATIONS (2020)

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A high energy efficiency and long life aqueous Zn-I2 battery

Wei Li et al.

JOURNAL OF MATERIALS CHEMISTRY A (2020)

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Article Chemistry, Multidisciplinary

Reversible Oxygen Redox Chemistry in Aqueous Zinc-Ion Batteries

Fang Wan et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Article Electrochemistry

Sulfur and nitrogen enriched graphene foam scaffolds for aqueous rechargeable zinc-iodine battery

Ke Lu et al.

ELECTROCHIMICA ACTA (2019)

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Aqueous Li-ion battery enabled by halogen conversion-intercalation chemistry in graphite

Chongyin Yang et al.

NATURE (2019)

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A Four-Electron Sulfur Electrode Hosting a Cu2+/Cu+ Redox Charge Carrier

Xianyong Wu et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Editorial Material Chemistry, Multidisciplinary

Aqueous batteries get energetic

Xianyong Wu et al.

NATURE CHEMISTRY (2019)

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Highly active nanostructured CoS2/CoS heterojunction electrocatalysts for aqueous polysulfide/iodide redox flow batteries

Dui Ma et al.

NATURE COMMUNICATIONS (2019)

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Review Chemistry, Multidisciplinary

Advanced Materials for Zinc-Based Flow Battery: Development and Challenge

Zhizhang Yuan et al.

ADVANCED MATERIALS (2019)

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A TiN Nanorod Array 3D Hierarchical Composite Electrode for Ultrahigh-Power-Density Bromine-Based Flow Batteries

Chenhui Wang et al.

ADVANCED MATERIALS (2019)

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Article Chemistry, Physical

Rechargeable Iron-Sulfur Battery without Polysulfide Shuttling

Xianyong Wu et al.

ADVANCED ENERGY MATERIALS (2019)

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Article Chemistry, Multidisciplinary

High-Energy Efficiency Membraneless Flowless Zn-Br Battery: Utilizing the Electrochemical-Chemical Growth of Polybromides

Ju-Hyuk Lee et al.

ADVANCED MATERIALS (2019)

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Article Chemistry, Multidisciplinary

In Operando Visualization of the Electrochemical Formation of Liquid Polybromide Microdroplets

Yutong Wu et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Article Chemistry, Physical

Activation-free synthesis of microporous carbon from polyvinylidene fluoride as host materials for lithium-selenium batteries

Mohammad Hossein Aboonasr Shiraz et al.

JOURNAL OF POWER SOURCES (2019)

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Article Chemistry, Physical

Realizing highly efficient energy retention of Zn-Br2 redox flow battery using rGO supported 3D carbon network as a superior electrode

Subramanian Suresh et al.

JOURNAL OF POWER SOURCES (2019)

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Review Multidisciplinary Sciences

Recycling lithium-ion batteries from electric vehicles

Gavin Harper et al.

NATURE (2019)

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Formation of Magnesium Dendrites during Electrodeposition

Rachel Davidson et al.

ACS ENERGY LETTERS (2019)

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Metal Oxide Coatings on Carbon Electrodes with Large Mesopores for Deeply Charged Zinc Bromine Redox Flow Batteries

Brian P. Williams et al.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2019)

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Rechargeable ultrahigh-capacity tellurium-aluminum batteries

Xuefeng Zhang et al.

ENERGY & ENVIRONMENTAL SCIENCE (2019)

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Aqueous alkaline-acid hybrid electrolyte for zinc-bromine battery with 3V voltage window

Feng Yu et al.

ENERGY STORAGE MATERIALS (2019)

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Plating and stripping calcium in an organic electrolyte

Da Wang et al.

NATURE MATERIALS (2018)

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Rechargeable Zinc-Aqueous Polysulfide Battery with a Mediator-Ion Solid Electrolyte

Martha M. Gross et al.

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Materials and Device Constructions for Aqueous Lithium-Sulfur Batteries

Sol Yun et al.

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Rechargeable aqueous zinc-iodine batteries: pore confining mechanism and flexible device application

Yixin Li et al.

CHEMICAL COMMUNICATIONS (2018)

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Highly reversible zinc metal anode for aqueous batteries

Fei Wang et al.

NATURE MATERIALS (2018)

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Self-standing sulfur cathodes enabled by 3D hierarchically porous titanium monoxide-graphene composite film for high-performance lithium-sulfur batteries

Yi Chen et al.

NANO ENERGY (2018)

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Fluorine-free water-in-ionomer electrolytes for sustainable lithium-ion batteries

Xin He et al.

NATURE COMMUNICATIONS (2018)

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A Rechargeable Al-Te Battery

Handong Jiao et al.

ACS APPLIED ENERGY MATERIALS (2018)

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Review Chemistry, Multidisciplinary

Redox-Flow Batteries: From Metals to Organic Redox-Active Materials

Jan Winsberg et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2017)

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High-performance zinc bromine flow battery via improved design of electrolyte and electrode

M. C. Wu et al.

JOURNAL OF POWER SOURCES (2017)

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Quantification of the Voltage Losses in the Minimal Architecture Zinc-Bromine Battery Using GITT and EIS

Kevin W. Knehr et al.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2017)

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A high-capacity dual core-shell structured MWCNTs@S@PPy nanocomposite anode for advanced aqueous rechargeable lithium batteries

Xiongwei Wu et al.

NANOSCALE (2017)

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Unique aqueous Li-ion/sulfur chemistry with high energy density and reversibility

Chongyin Yang et al.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2017)

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A rechargeable iodine-carbon battery that exploits ion intercalation and iodine redox chemistry

Ke Lu et al.

NATURE COMMUNICATIONS (2017)

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Aqueous Electrochemical Energy Storage with a Mediator-Ion Solid Electrolyte

Xingwen Yu et al.

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An Aqueous Ca-Ion Battery

Saman Gheytani et al.

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Controlling Solid-Liquid Conversion Reactions for a Highly Reversible Aqueous Zinc-Iodine Battery

Huilin Pan et al.

ACS ENERGY LETTERS (2017)

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Review Nanoscience & Nanotechnology

Lithium battery chemistries enabled by solid-state electrolytes

Arumugam Manthiram et al.

NATURE REVIEWS MATERIALS (2017)

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Tellurium-Impregnated Porous Cobalt-Doped Carbon Polyhedra as Superior Cathodes for Lithium-Tellurium Batteries

Jiarui He et al.

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Cage-Like Porous Carbon with Superhigh Activity and Br2-Complex-Entrapping Capability for Bromine-Based Flow Batteries

Chenhui Wang et al.

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Miniaturisation of Zn/Br redox flow battery cell and investigation of electrode materials influence on its characteristics

Yoshiki Nagai et al.

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Bimodal highly ordered mesostructure carbon with high activity for Br2/Br- redox couple in bromine based batteries

Chenhui Wang et al.

NANO ENERGY (2016)

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A high-energy and low-cost polysulfide/iodide redox flow battery

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NANO ENERGY (2016)

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A Brief Review on Multivalent Intercalation Batteries with Aqueous Electrolytes

Ramesh K. Guduru et al.

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A high-capacity and long-life aqueous rechargeable zinc battery using a metal oxide intercalation cathode

Dipan Kundu et al.

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Water-in-salt electrolyte enables high-voltage aqueous lithium-ion chemistries

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Ambipolar zinc-polyiodide electrolyte for a high-energy density aqueous redox flow battery

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Tellurium@Ordered Macroporous Carbon Composite and Free-Standing Tellurium Nanowire Mat as Cathode Materials for Rechargeable Lithium-Tellurium Batteries

Ning Ding et al.

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Use of ion-selective polymer membranes for an aqueous electrolyte rechargeable Li-ion-polysulphide battery

Rezan Demir-Cakan et al.

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An aqueous electrolyte rechargeable Li-ion/polysulfide battery

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Lithium-tellurium batteries based on tellurium/porous carbon composite

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Confined selenium within porous carbon nanospheres as cathode for advanced Li-Se batteries

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Selenium@Mesoporous Carbon Composite with Superior Lithium and Sodium Storage Capacity

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A novel single flow zinc-bromine battery with improved energy density

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Core-shell sulfur@polypyrrole composites as high-capacity materials for aqueous rechargeable batteries

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Rechargeable lithium/iodine battery with superior high-rate capability by using iodine-carbon composite as cathode

Y. L. Wang et al.

ENERGY & ENVIRONMENTAL SCIENCE (2011)

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Recent Development of Aqueous Multivalent-Ion Batteries Based on Conversion Chemistry

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