☆ 4.2 Review

Utilization of ionic liquids as compatibilizing agents for polymer blends - preparations and properties

POLYMER-PLASTICS TECHNOLOGY AND MATERIALS (2023)

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Effect of PCL-b-PEG Oligomer Containing Ionic Elements on Phase Interfacial Properties and Aggregated Structure of PLA/PCL Blends

Ping Wang et al.

Summary: This study investigates the effects of adding polycaprolactone-polyethylene glycol oligomers and their derivative containing ionic elements on the properties of polylactic acid/polycaprolactone blends. The results show that the blends with added ionic elements have improved compatibility and mechanical properties.

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Nanocellulose Extraction Using Ionic Liquids: Syntheses, Processes, and Properties

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Summary: Increased environmental awareness has led researchers to explore alternatives to hazardous chemicals for extracting nanocellulose. Ionic liquids, which are recyclable and reusable, have been used as a medium for processing cellulose and other biopolymers. This short review provides examples of ionic liquids used for nanocellulose extraction, discusses the sources of cellulose used as raw materials, describes the synthesis of ionic liquids, and reviews the properties of nanocellulose extracted using different ionic liquids. The knowledge gained from this review enhances understanding of the nanocellulose extraction process and the important properties of the extracted nanocellulose.

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Article Chemistry, Multidisciplinary

Structure and Properties of PVDF/PA6 Blends Compatibilized by Ionic Liquid-Grafted PA6

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Summary: In this work, a grafted polyamide 6 with quasi-block structure was used as a compatibilizer for an immiscible PVDF/PA6 blend, and its effects on the morphology, crystallization behavior, mechanical properties, and surface resistance of the blend were systematically investigated. It was found that the compatibilizer had a favorable effect on the blend, improving its morphology and mechanical properties, and providing surface conductivity. Differential scanning calorimetry and wide-angle X-ray diffractometry results revealed different effects of the compatibilizer on the crystallization behavior of PVDF and PA6.

ACS OMEGA (2022)

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Article Materials Science, Multidisciplinary

Cellulose blends with polylactic acid or polyamide 6 from solution blending: Microstructure and polymer interactions

Kerstin Mueller et al.

Summary: This study uses a solvent-based rapid precipitation method to address the limitations of using cellulose in polymer blends. It found that cellulose forms single-phase amorphous blends with intense intermolecular hydrogen bonding with polylactic acid, while forming a two-phase morphological structure with polyamide 6. Homogeneous blend formation between polylactic acid and cellulose shows promise for further material developments.

MATERIALS TODAY COMMUNICATIONS (2022)

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Article Polymer Science

Cellulose blends from gel extrusion and compounding with polylactic acid

Kerstin Mueller et al.

Summary: This study reports the preparation and investigation of cellulose and polylactic acid (PLA) blends using an extrusion process with an ionic liquid and co-solvent for intermediate compatibilization. The obtained transparent films show a homogeneous morphology without phase separation. The blend shows thermal stability and comparable mechanical properties to a multiphase composite.

JOURNAL OF APPLIED POLYMER SCIENCE (2022)

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Review Polymer Science

Preparations and Properties of Ionic Liquid-Assisted Electrospun Biodegradable Polymer Fibers

Ahmad Adlie Shamsuri et al.

Summary: The enhanced awareness of environmental conservation has led researchers to search for alternatives to volatile organic compounds in polymer processing. Ionic liquids have emerged as non-volatile, recyclable, and non-flammable solvents for biodegradable polymers, as well as for the preparation of electrospun fibers. This concise review provides examples of natural and synthetic biodegradable polymers commonly used in electrospinning, and showcases the utilization of ionic liquids in the process. It also demonstrates the preparation of electrospinning solutions using ionic liquids, and presents a concise review of the properties of electrospun biodegradable polymer fibers assisted by different ionic liquids.

POLYMERS (2022)

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Ionic Liquid-Cured Epoxy/PCL Blends with Improved Toughness and Adhesive Properties

Lidia Orduna et al.

Summary: In this study, the phase behavior, microstructure, mechanical and adhesive properties of ionic liquid (IL)-cured epoxy resins modified with poly(epsilon-caprolactone) (PCL) were investigated. The results showed that the addition of PCL plasticized the network blends, reducing the glass transition temperature and crosslinking density. Low PCL contents had little impact on the mechanical properties, but significantly improved the adhesive properties. However, higher PCL contents, especially using imidazolium-based IL, greatly increased the toughness. Overall, the balance achieved between mechanical and adhesive properties of IL-cured epoxy/PCL blends is an important step towards sustainability, with the use of a biodegradable polymer and non-volatile ILs as curing agents.

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Summary: The increasing concern for the environment has led to a focus on fabricating polymer biocomposites. Ionic liquids have been utilized for the pretreatment of natural fillers, improving the physicomechanical properties of polymer biocomposites.

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Article Polymer Science

Ionic liquids as dispersing agents of graphene nanoplatelets in poly(methyl methacrylate) composites with microwave absorbing properties

Camila Mouta Caldas et al.

Summary: By modifying PMMA nanocomposites and incorporating GNP with different fluorinated ionic liquids, composites with high thermal stability and conductivity can be obtained, showing excellent absorption properties in terms of microwave absorption.

JOURNAL OF APPLIED POLYMER SCIENCE (2021)

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Article Polymer Science

Effect of ionic liquid segments of copolymer on compatibilization process and dielectric behavior of polylactide/polyvinylidene fluoride blends

Ping Wang et al.

Summary: The effects of PMI on the compatibility of PLA and PVDF were investigated, showing significant improvement compared to PMV. The compatibility of PLA and PVDF was related to the relaxation behavior of the blends, identified with MWS interfacial polarization. The higher epsilon' of PLA/PVDF/PMI blends was attributed to the stimulation of MWS interfacial polarization by the ion mobility of PMI.

JOURNAL OF APPLIED POLYMER SCIENCE (2021)

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Article Biochemistry & Molecular Biology

Effect of ionic liquid 1-buyl-3-methylimidazolium halide on the structure and tensile property of PBS/corn starch blends

Jin Xu et al.

Summary: This study successfully prepared a poly (butylene succinate) / corn starch blend material with good tensile properties by adding ionic liquid-modified corn starch. The ionic liquid acted as a plasticizer and a compatibilizer in the blend, significantly reducing the crystallinity of the material and improving the morphology of the blend.

INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES (2021)

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Article Polymer Science

Thermoset-thermoplastic-ionic liquid ternary hybrids as novel functional polymer materials

Nour Halawani et al.

Summary: This study demonstrates the synergistic use of PEI and IL in epoxy networks, improving hydrophobic behavior and thermal stability while introducing shape memory behavior. The complex interphase generated by the thermoplastic-IL combination enhances the multifunctionality of the polymer blends.

POLYMER (2021)

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Review Chemistry, Multidisciplinary

Application of Quaternary Ammonium Compounds as Compatibilizers for Polymer Blends and Polymer Composites-A Concise Review

Ahmad Adlie Shamsuri et al.

Summary: This review focuses on the application of two types of QACs as compatibilizers for polymer blends and polymer composites, specifically quaternary ammonium surfactants (QASs) and quaternary ammonium ionic liquids (QAILs), due to their unique chemical structure and interaction capabilities with polymer components. The influence of QASs and QAILs on the thermo-mechanical properties of the polymer blends and composites is also discussed, aiming to provide insights for researchers in this field.

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Review Polymer Science

A Brief Review on the Influence of Ionic Liquids on the Mechanical, Thermal, and Chemical Properties of Biodegradable Polymer Composites

Ahmad Adlie Shamsuri et al.

Summary: Biodegradable polymers can be decomposed by bacteria and can be incorporated with fillers to fabricate biodegradable polymer composites. Ionic liquids are increasingly used in the fabrication of polymer composites in this field.

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Article Materials Science, Multidisciplinary

Enhancing the properties of PBAT/PLA composites with novel phosphorus-based ionic liquid compatibilizers

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Summary: In this study, two ionic liquids were successfully synthesized and applied as compatibilizers for PBAT/PLA composites, leading to significant improvements in toughness, flame retardancy, and processability of the materials. The addition of ionic liquids resulted in more uniform dispersion of PLA in the PBAT matrix, contributing to enhanced material properties.

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Summary: The improvement of ecological conscience has led researchers to focus on reducing processing time and cost of solvents for cellulose dissolution, with ionic liquids being widely employed due to their recyclability and nonvolatility. Various biopolymers, such as chitosan, chitin, starch, protein, and cellulose acetate, can also be processed using ionic liquids for diverse applications. The review discusses examples of imidazolium-based ionic liquids commonly used for cellulose dissolution, as well as organic liquids used as co-solvents for ionic liquids. Additionally, it demonstrates the properties and applications of regenerated cellulose and blends from different types of cellulose/ionic liquid/co-solvent solutions, serving as a model basis for novel applications.

E-POLYMERS (2021)

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Article Chemistry, Multidisciplinary

Recovery of Cobalt and Manganese from Spent Lithium-ion Batteries using a Phosphonium-based Ionic Liquid

Mochmad L. Firmansyah et al.

Summary: A novel hydrophobic ionic liquid was developed as an extractant for the recovery of cobalt and manganese from spent lithium-ion batteries. The absence of organic diluent in the extraction process provides an advantage over conventional methods, allowing for a continuous extraction process with the potential for reuse of the IL.

SOLVENT EXTRACTION RESEARCH AND DEVELOPMENT-JAPAN (2021)

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Ionic liquids synthesis and applications: An overview

Sandip K. Singh et al.

JOURNAL OF MOLECULAR LIQUIDS (2020)

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Ionic Liquid-Polymer Composites: A New Platform for Multifunctional Applications

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Absorption of n-butane in imidazolium and phosphonium ionic liquids and application to separation of hydrocarbon gases

Takashi Makino et al.

SEPARATION AND PURIFICATION TECHNOLOGY (2019)

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Article Chemistry, Physical

Effect of P[MPEGMA-IL] on morphological evolution and conductivity behavior of PLA/PCL blends

Ping Wang et al.

IONICS (2019)

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Article Chemistry, Physical

A well-defined biodegradable 1,2,3-triazolium-functionalized PEG-b-PCL block copolymer: facile synthesis and its compatibilization for PLA/PCL blends

Ping Wang et al.

IONICS (2018)

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Article Polymer Science

Effect of block copolymer containing ionic liquid moiety on interfacial polarization in PLA/PCL blends

Ping Wang et al.

JOURNAL OF APPLIED POLYMER SCIENCE (2018)

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Influence of Ionic Liquids on the Morphology of Corn Flour/Polyester Mixtures

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Toughening of Epoxy/Ionic Liquid Networks with Thermoplastics Based on Poly(2,6-dimethy1-1,4-phenylene ether) (PPE)

Thi Khanh Ly Nguyen et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2017)

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Bronsted acidic ionic liquids: New transesterification agents for the compatibilization of polylactide/ethylene-co-vinyl acetate blends

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EUROPEAN POLYMER JOURNAL (2017)

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Ionic liquids as solvents for PPTA oligomers

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Probing nanomechanical properties with AFM to understand the structure and behavior of polymer blends compatibilized with ionic liquids

Benjamin Megevand et al.

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Phosphonium ionic liquids as new compatibilizing agents of biopolymer blends composed of poly(butylene-adipate-co-terephtalate)/poly(lactic acid) (PBAT/PLA)

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Ionic liquids-lignin combination: an innovative way to improve mechanical behaviour and water vapour permeability of eco-designed biodegradable polymer blends

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MACROMOLECULAR CHEMISTRY AND PHYSICS (2015)

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