期刊
PHOTONICS
卷 10, 期 6, 页码 -出版社
MDPI
DOI: 10.3390/photonics10060654
关键词
scintillator; photoluminescence; radiation detection; 4f-4f transitions; charge transfer; floating zone method
类别
Mg4Ta2O9 single crystals doped with 0.01, 0.1, and 1% Er were grown using the floating zone method. Their photoluminescence and scintillation properties were studied, confirming the presence of a hexagonal structure and emission peaks at 1550 nm due to 4f-4f transitions of Er3+ ions. The samples also exhibited scintillation with a broad emission band at 350 nm and detection limits of 0.06 Gy/h for scintillation detector applications.
Mg4Ta2O9 single crystals doped with 0.01, 0.1, and 1% Er were grown using the floating zone method, and their photoluminescence and scintillation properties were studied. X-ray diffraction analysis confirmed that all samples had a hexagonal structure of Mg4Ta2O9. The samples showed that the emission peak at 1550 nm was due to 4f-4f transitions of Er3+ ions, with quantum yields of 32.9, 46.6, and 18.0% for 0.01, 0.1, and 1% doping concentrations, respectively. All samples showed scintillation with a broad emission band at 350 nm due to charge transfer from Ta5+ to O2- ions and emission peak at 1550 nm due to 4f-4f transition of Er3+ ions. The dose rate response functions showed that the detection limit for all samples was 0.06 Gy/h for scintillation detector applications.
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