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Article
Chemistry, Physical
Babneet Kaur et al.
Summary: A non-aqueous zinc ion battery with a wide operational voltage window and high Coulombic efficiency was successfully fabricated. The battery overcomes structural instability and low electrical conductivity issues in both the cathode and the anode by using a conducting polymer layer. The cathode consists of VS4 nanoflowers and carbon nanotubes, outperforming pristine VS4 nanoflowers due to enhanced electrical conductivity, easy electron and ion transfer and transport, effective buffering of volume changes, and better accessibility of active sites. This work lays the foundation for developing zinc ion batteries with ultra-long lifespan and high energy density as advanced energy storage systems.
APPLIED SURFACE SCIENCE
(2023)
Article
Electrochemistry
Shuo Kong et al.
Summary: Fiber-shaped energy storage devices are lightweight, flexible, and can be woven, making them ideal for wearable and portable electronics. The development of fiber-shaped aqueous rechargeable zinc ion batteries (FARZIBs) has enabled the production of safe, cost-effective, and environmentally friendly wearable electronic products. However, achieving high rate capability, energy density, and cycling performance simultaneously for FARZIBs is a challenge. This study demonstrates a high-performance FARZIB using vanadium-based metal-organic frameworks (MOFs) derived vanadic oxide (V2O5) nanowire-bundle arrays (NBAs) grown on conductive carbon nanotube fibers (CNTFs) as the binder-free cathode, showing promising prospects for the next generation of wearable electronics.
ELECTROCHIMICA ACTA
(2023)
Article
Multidisciplinary Sciences
Giorgia Zampardi et al.
Summary: Aqueous zinc-ion batteries have potential as stationary storage systems for power-grid applications, but certain challenges need to be addressed and experimental practices need to be aligned with industrial working conditions to promote their commercialization.
NATURE COMMUNICATIONS
(2022)
Article
Electrochemistry
Kruti K. Halankar et al.
Summary: In this study, a high-performance anode material for sodium ion batteries, Mo2C/C/rGO, was synthesized by a simple and inexpensive method. The composite exhibited improved electrochemical performance, conductivity, and capacity retention. The addition of carbon and rGO nanosheets enhanced electronic conductivity and minimized the adverse effects of volume expansion during charging and discharging. Theoretical studies revealed that the interaction between Mo2C and graphene facilitated the movement of sodium ions in the composite.
Article
Multidisciplinary Sciences
Bingyao Zhang et al.
Summary: This study effectively addresses the issues of dendrite growth and side reactions in zinc-ion batteries by using a highly-confined tannic acid modified sodium alginate composite gel electrolyte. The modified electrolyte guides and regulates zinc deposition, resulting in steady zinc plating/stripping behavior and high cycle stability.
Article
Chemistry, Physical
Rong Luo et al.
Summary: A reduced graphene oxide aerogel with a multi-scale hierarchical cellular structure was successfully prepared using a facile hydrothermal self-assembling strategy. The aerogel exhibited remarkable flexibility, toughness, compressive strength, and electrical conductivity, making it a promising candidate for piezoresistive sensors.
Article
Chemistry, Physical
Hua Li et al.
Summary: Balancing the energy density and power density of supercapacitors is crucial for expanding their application range. This study demonstrates a feasible approach to achieve this balance through the design and synthesis of hierarchically porous graphene aerogels containing doped-heteroatoms and matching with ionic liquid electrolyte.
JOURNAL OF PHYSICAL CHEMISTRY C
(2022)
Article
Chemistry, Physical
Zeyi Wu et al.
Summary: In this study, a novel cathode material Na4VMn(PO4)3@Graphene for aqueous Zn-ion battery (AZIB) was developed, which exhibited high energy density and long lifespan. The compound utilized V and Mn elements to achieve a two-step electron transfer mechanism, resulting in improved capacity and working voltage.
ADVANCED ENERGY MATERIALS
(2022)
Article
Chemistry, Physical
Yan Tan et al.
Summary: This study develops distinctive hierarchitectures of 1T-VS2 nanospheres assembled by nanosheets, which feature abundant active sites, superior electron/ion transport property, and robust structure. The reinforcement of the layered structure of VS2 through Zn2+ pillars residing in VS2 interlayers is proven to be effective. The rapid and highly reversible Zn-ion intercalation behavior within the VS2 nanospheres is verified, and exceptional rate performance and ultralong cycling life are achieved. This work provides new perspectives for prolonging the lifespan of layered Zn-storage materials by modulating the charge/discharge processes.
ADVANCED ENERGY MATERIALS
(2022)
Article
Nanoscience & Nanotechnology
Qi Li et al.
Summary: This study demonstrates the successful development of ultrathin microwave absorbent using VS4/rGO heterostructure. The results show that by regulating the heterointerface, impedance matching and attenuation constant can be effectively improved, leading to enhanced microwave absorption performance.
NANO-MICRO LETTERS
(2022)
Article
Chemistry, Physical
Shiqi Ding et al.
Summary: In this study, PVP was innovatively incorporated with VS4 to improve the kinetic performance, cycling life, and specific capacities of magnesium-ion batteries. The novel design of PVP-VS4 exhibited long-term cycling stability and exceptional high-rate capability. The reaction kinetics and energy storage mechanism were further analyzed using experimental techniques and computational calculations.
ENERGY STORAGE MATERIALS
(2022)
Article
Chemistry, Physical
Jie Yang et al.
Summary: To satisfy the growing demand for power in wearable and portable devices, the design of flexible electrodes is crucial for improving the performance of quasi-solid-state zinc-ion batteries (QAZIBs). This study demonstrates the use of electrospinning and atomic-layer-deposition to enhance the electrochemical properties of flexible film cathodes. The results show that the QAZIBs exhibit high energy density, excellent rate capability, and good cycling performance. The integration of the flexible QAZIBs into a soft inchworm robot further demonstrates their potential applications in soft robotics.
ENERGY STORAGE MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Zixiong Shi et al.
Summary: This topical review highlights the significant role of direct chemical vapor deposition (CVD) technique in the growth of graphene, and summarizes its versatile roles as a modificator, cultivator, defender, and decider. The effects on performance optimization and underlying mechanisms are discussed, with a focus on fundamental properties. The perspectives on material production and device fabrication are also provided for the future development of direct-CVD-enabled graphene in energy applications and beyond.
Article
Engineering, Environmental
Shiqi Ding et al.
Summary: VS4 modified with cation/anion co-doping (MVSO) shows enhanced electrical conductivity and improved cycle and rate performance. MVSO exhibits excellent electrochemical properties, including high specific capacity, ultralong cycling life, superior rate capability, and low self-discharge ratio. The fast reaction kinetics and high capacitive process contribution of MVSO are highlighted.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Chemistry, Physical
Ivette Aguilar et al.
Summary: In this study, the chemistry of rechargeable zinc-manganese dioxide batteries was revisited through a combination of solution chemistry considerations and analytical techniques. The role of electrolyte and its pH in the electrochemical response of the system was confirmed. Experimental evidence for the occurrence of electrodissolution and electrodeposition of MnO2, as well as the formation of soluble zinc hydroxides and chemical precipitation, was provided. The presence of a specific phase was shown to be essential in buffering the system's pH and enhancing the capacity retention.
ENERGY STORAGE MATERIALS
(2022)
Article
Multidisciplinary Sciences
Mingmao Wu et al.
Summary: This paper presents a laser-engraving strategy for producing graphene meta-aerogels with unusual characters. By reinforcing the graphene walls with nanofiber networks and using laser engraving, the macro-configurations of the graphene meta-aerogels can be arbitrarily regulated, resulting in highly elastic, robust, and stiff materials with large reversible elongation, light specific weight, and a wide range of Poisson's ratio.
NATURE COMMUNICATIONS
(2022)
Article
Chemistry, Physical
Louis Godeffroy et al.
Summary: This study uses optical reflectometry to analyze the charge and discharge of MnO2 electrodes in aqueous Zn-MnO2 batteries, highlighting the significant role of solid-phase zinc hydroxide sulfate in these processes.
ADVANCED ENERGY MATERIALS
(2022)
Review
Chemistry, Multidisciplinary
Yi Lin et al.
Summary: Holey graphene is a derivative of graphene with through-thickness holes, and it has various advantages in energy storage applications, including high electrical conductivity, high surface area, mechanical robustness, and chemical inertness. The presence of holes enhances mass transport and allows dry pressing of robust electrodes without the need for toxic solvents or binders. This unique property broadens the application horizon in energy storage.
ACCOUNTS OF CHEMICAL RESEARCH
(2022)
Article
Nanoscience & Nanotechnology
Hongran Sun et al.
Summary: In this study, rose-like VS2 nanosheets were prepared and incorporated into a SWCNT network to form a C-VS2 composite. The composites showed rapid electron transfer and ion diffusion due to the chemical bonding between layers. The reversible Zn/C-VS2 system exhibited high specific capacity, excellent cyclic stability, and remarkable rate capability. The flexible C-VS2 films also served as a cathode for soft-packaged ZIBs, which showed good electrochemical stability even under bending conditions.
ACS APPLIED MATERIALS & INTERFACES
(2022)
Article
Engineering, Environmental
Saiful Islam et al.
Summary: In this study, polypyrrole-coated Na(1.1)V3O(7.9) nanorods were synthesized through microwave-assisted hydrothermal process for aqueous rechargeable zinc-ion batteries. The PPy coating enhances electronic conductivity and Zn(2+) diffusion kinetics, leading to improved discharge capacity, power capability, and cycling stability. The P-NVO cathode demonstrates superior energy density and cycling stability.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Energy & Fuels
Xiaoyang Zhang et al.
Summary: In this study, a Fe7SC sorbent was prepared via hydrothermal impregnation for the removal of Hg-0 from simulated syngas. The introduction of oxygen enhanced the capture of Hg-0 by inducing targeted H2S oxidation. The effects of oxygen, temperature, and syngas composition on Hg-0 adsorption performance were investigated. Fe7SC exhibited superior Hg-0 removal performance in the presence of H2S + O2. The interaction between H2S and oxygen was responsible for its enhanced Hg-0 capture capacity. CO and H2 suppressed Hg-0 adsorption, while H2O inhibited Hg-0 removal due to competitive adsorption. The kinetic analysis suggested that Hg-0 surface chemisorption was the rate-controlling step.
Article
Chemistry, Physical
Yamin Feng et al.
Summary: A novel VS2/MXene cathode material is fabricated in this study, which exhibits improved ionic transfer and electronic diffusion kinetics. The VS2/MXene cathode shows excellent cycle life and high capacity, while the assembly of flexible zinc-ion microbattery (ZIMB) also demonstrates high capacity and long cycle life.
JOURNAL OF POWER SOURCES
(2022)
Article
Engineering, Environmental
Feng Wei et al.
Summary: N, P codoped foamy-like carbons (NPFC) with abundant defect sites were prepared from osmanthus flowers using a simply and confined pyrolysis method. NPFC exhibited high electrical conductivity and porous structures, providing abundant defects and active sites for ion adsorption and electron transfer. As a cathode material for hybrid capacitors, NPFC showed large energy density and long cycle life in aqueous electrolyte.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Chemistry, Multidisciplinary
Yan Wang et al.
Summary: In this study, a hierarchical VS2@VS4 structure was developed as a cathode, which exhibited good electrochemical performance with high capacity retention rates at both low temperature and room temperature, indicating the potential for developing high-performance energy-storage composites.
CHEMICAL COMMUNICATIONS
(2022)
Article
Chemistry, Physical
Tzu-Chun Huang et al.
Summary: This study reports the synthesis of VTe2 by a hydrothermal method and demonstrates its potential as a cathode material for AZIBs. The morphology of VTe2 can be controlled by adjusting the pH value. Nanosheet VTe2 shows excellent battery performance and offers a promising approach for electrode design in metal-ion batteries.
SUSTAINABLE ENERGY & FUELS
(2022)
Article
Energy & Fuels
Xiaoyang Zhang et al.
Summary: In this study, a Fe7SC sorbent was prepared for the removal of Hg0 from simulated syngas by introducing oxygen to induce H2S oxidation for enhanced capture of Hg0. Fe7SC demonstrated superior Hg0 removal performance in the presence of H2S + O2. CO and H2 suppressed Hg0 adsorption, while H2O inhibited Hg0 removal due to competitive adsorption.
Article
Chemistry, Physical
Qiulong Li et al.
Summary: This study successfully utilized metallic Zn-Co3O4 nanowire arrays as the cathode to fabricate an all-solid-state fiber-shaped aqueous rechargeable Co//Zn battery, which exhibits remarkable capacity, rate capability, and energy density.
Article
Chemistry, Physical
Meenu Sharma et al.
Summary: The temperature dependent Raman spectroscopy of reduced graphene oxide (rGO) reveals the combined effect of anharmonicity, crystallite size, and defects on the peak positions and line widths of G- and D- modes. The dominance of true-anharmonic part in shifting the peak positions is indicated by theoretical models. The contributions of electron-phonon coupling, anharmonicity, and defects to the temperature dependent variation of line width are discussed.
Article
Chemistry, Physical
Lingli Xing et al.
Summary: Transition metal sulfides, as promising electrode materials for aluminum-ion batteries, have been hindered by their low energy density and poor rate property. This study successfully synthesized channels-rich VS4 nanowire clusters, demonstrating superior electrochemical performances as a cathode for rechargeable AIBs. The stable channels-rich structures of the VS4 nanowire clusters and proposed intercalation mechanism provide new insights into the chemistry of AIBs for electrochemical energy storage.
Article
Chemistry, Multidisciplinary
Zhiyu Wang et al.
Summary: The study found that intercalating TFSI- anions into VS4 can enhance sulfur evolution during charging, resulting in improved cycling reversibility and capacity retention in the composite electrode.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Nanoscience & Nanotechnology
Youcun Bai et al.
Summary: In this study, VSe2 nanosheets supported on stainless-steel with defects were synthesized through a hydrothermal reduction strategy, resulting in improved conductivity and activity. The Se defect was found to adjust the adsorption energy of Zn2+ ions, leading to enhanced reversibility and electrochemical performance of the Zn// VSe2-x-SS battery. The VSe2-x-SS electrode exhibited good specific capacity, rate performance, and cyclic stability, providing insights into the energy-storage mechanism of Zn2+ ions in this material for future electrode design.
ACS APPLIED MATERIALS & INTERFACES
(2021)
Article
Chemistry, Physical
Youcun Bai et al.
Summary: The study successfully designs an advanced stainless steel-supported oxygen-rich vacancy cistern-like nanobelt cathode with broadened interlayer spacings and ultrafast reaction kinetic, showing high capacity, excellent rate performance, and cyclic stability as the cathode of an aqueous zinc-ion battery. The research also demonstrates the cathode's excellent performance under various harsh conditions and reveals the Zn2+ storage mechanism.
Article
Chemistry, Physical
Zhiguo Ren et al.
Summary: Rechargeable aqueous zinc-ion batteries (AZIBs) have strong competitiveness in terms of cost and safety, but the lack of stable cathode materials has hindered their development. This study reveals that V5S8 can serve as a superior intercalated cathode material for AZIBs, delivering high capacity and record capacity retention, driven by its metallic characteristic and optimal zinc-ion diffusion path. In-situ synchrotron X-ray diffraction, ex-situ X-ray photoelectron spectroscopy, and DFT calculations provide significant insights into the reaction mechanism of V5S8 cathode, highlighting its self-adaptive multistage ion storage properties.
ENERGY STORAGE MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
By Zeyi Wu et al.
Summary: A bilayer-structured VOPO4.2H(2)O (bilayer-VOP) nanosheet with high-concentration oxygen vacancies was developed through a facile liquid-exfoliation strategy. The nanosheets showed superior properties in zinc-ion transport coefficient and electron conductivity, leading to outstanding performance in rechargeable zinc-ion batteries.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Chemistry, Physical
Pei Yu et al.
Summary: The introduction of multiwalled carbon nanotube significantly improves the conductivity and structural stability of VS4, enhancing its performance in sodium ion batteries. The synthesized VS4/MWCNT composite exhibits good discharge capacity and rate capability at different current densities.
JOURNAL OF POWER SOURCES
(2021)
Review
Chemistry, Multidisciplinary
Jiahao Liu et al.
Summary: This article focuses on constructing a theory-to-application methodology for aqueous sulfur-based batteries. Research reveals the complexity in the electrochemistry of aqueous sulfur-based batteries, which poses challenges and potential for future development. Further exploration in both theory and practice is needed for the future development direction.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2021)
Article
Chemistry, Multidisciplinary
Qiulong Li
Summary: In this study, a NiCoP@NiCoP electrode was designed with metallic characteristics and excellent electrochemical performance, showing significantly improved electrochemical performance in asymmetric supercapacitors. The FASC device assembled with this electrode achieved high areal capacitance and ultrahigh energy density, making it a promising candidate for next-generation wearable and portable energy-storage devices.
Article
Chemistry, Multidisciplinary
Qi Lu et al.
Summary: The study successfully designed and fabricated a high-efficiency bifunctional electrocatalyst using high-temperature shock technology, with high activities for both oxygen reduction and oxygen evolution reactions. The composite structure of the catalyst utilizes the synergistic effect and intrinsic activity of the Co-N-C moiety, as well as the porous structure of carbon nanofibers.
Article
Chemistry, Multidisciplinary
Linfeng Hu et al.
Summary: The study addresses the challenges of sluggish Zn2+ diffusion kinetics and poor cyclic stability in cathode materials for aqueous ZIBs by synthesizing PA-intercalated VOPO4·2H2O materials with different interlayer spacing. The optimized 16.5 angstrom spacing shows enhanced zinc-ion diffusion and cycling stability, leading to improved battery performance.
ENERGY & ENVIRONMENTAL SCIENCE
(2021)
Article
Chemistry, Physical
Dian Zhang et al.
Summary: A nitrogen-doped hierarchical porous carbon material was developed to improve the electrochemical performance and stability of aluminum-sulfur batteries. By utilizing a low-cost electrolyte and a sulfur composite cathode, the battery showed significant improvements in cycling performance and capacity. This study sheds light on the design of composite cathodes for high-reversibility, high-capacity, and low-cost Al-S batteries.
JOURNAL OF MATERIALS CHEMISTRY A
(2021)
Article
Electrochemistry
Fang Tang et al.
ELECTROCHIMICA ACTA
(2020)
Article
Chemistry, Multidisciplinary
Zeyi Wu et al.
Article
Chemistry, Physical
Qiancheng Zhu et al.
JOURNAL OF MATERIALS CHEMISTRY A
(2020)
Article
Multidisciplinary Sciences
Guochun Yan et al.
NATURE COMMUNICATIONS
(2019)
Article
Chemistry, Physical
Qiulong Li et al.
JOURNAL OF MATERIALS CHEMISTRY A
(2019)
Review
Chemistry, Physical
Lin Xu et al.
Article
Chemistry, Multidisciplinary
Lili Wang et al.
Article
Chemistry, Physical
Yanru Fan et al.
