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Perovskite/Silicon Tandem Solar Cells: Choice of Bottom Devices and Recombination Layers

ACS ENERGY LETTERS (2023)

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Silicon-based passivating contacts: The TOPCon route

Stefan W. Glunz et al.

Summary: This paper provides an overview of the potential of passivating contacts based on poly-Si/SiOx structures known as TOPCon in improving the efficiency of crystalline silicon solar cells. It discusses the historical development of such contact structures and describes the current state-of-the-art in laboratory and industry. The paper also addresses four different research topics related to TOPCon technology, including re-parametrization of recombination in silicon, control of dopant diffusion, single-sided deposition of the poly-Si layer, and the fabrication of silicon-based tunnel junctions for perovskite-silicon tandem cells.

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Techno-economic analysis of the use of atomic layer deposited transition metal oxides in silicon heterojunction solar cells

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Summary: The production cost of using atomic layer deposition (ALD) to form transition metal oxide (TMO) layers as alternatives to commonly used layers in HJT solar cells (p-doped, n-doped, and indium tin oxide) is likely to be lower than the standard HJT. The main cost driver is the cost of the ALD precursors. This study motivates further development of ALD TMO processes to increase their efficiency and take advantage of the cost advantage.

PROGRESS IN PHOTOVOLTAICS (2023)

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Article Chemistry, Multidisciplinary

One-year outdoor operation of monolithic perovskite/silicon tandem solar cells

Maxime Babics et al.

Summary: Perovskite/silicon tandem solar cells have been recognized as a feasible commercial solution for highly efficient photovoltaics. However, their performance in outdoor environments has not been extensively studied. This research presents the performance of these cells over a full year in a hot and humid location. The study highlights the potential of perovskite/silicon tandem solar cells, but also identifies important factors that affect their efficiency in real-world conditions.

CELL REPORTS PHYSICAL SCIENCE (2023)

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Article Materials Science, Multidisciplinary

Four-terminal perovskite/silicon tandem solar cells based on large-area perovskite solar cells utilizing low-cost copper semi-transparent electrode

Manas R. Samantaray et al.

Summary: This paper presents the fabrication of large-area four-terminal perovskite-Si solar cells and discusses their efficiencies. Large-area semi-transparent perovskite solar cells were fabricated using a thin copper layer as a transparent electrode, and a carrier selective contact-based Si solar cell was also fabricated. The efficiencies of these cells and a commercially available monocrystalline-Si solar cell were evaluated under different illumination conditions, and the combined efficiencies of the 4 T configurations were calculated.

APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING (2022)

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Article Energy & Fuels

Potential of NiOx/Nickel Silicide/n+ Poly-Si Contact for Perovskite/TOPCon Tandem Solar Cells

Jiryang Kim et al.

Summary: In this study, nickel silicide was used as an interlayer in tandem solar cells. The process of thermal evaporation and annealing formed nickel silicide, which showed ohmic contact and low contact resistivity with the poly-Si layer. Compared to other structures, this structure is advantageous for electrical connection and can improve the fill factor.

ENERGIES (2022)

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Article Energy & Fuels

How to make PERC suitable for perovskite-silicon tandem solar cells: A simulation study

Christoph Messmer et al.

Summary: Low-cost and high-efficiency tandem solar cells show great potential for future industrial mass production. The passivated emitter and rear cell (PERC) technology, which currently dominates the market, can be used as the bottom cell concept for perovskite-silicon tandem devices. By reevaluating the current PERC technology and considering different front-side concepts, both full-area and locally contacted front-side designs are promising candidates for achieving tandem cell efficiencies of about 30%.

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Article Energy & Fuels

Light management of PERC solar cell with the front and back dielectric multilayers

Jianming Ding et al.

Summary: Light management is an important method to increase the efficiency of PERC solar cells. By integrating SiOxNy and SiNx dielectric films on the front and rear surfaces, the short circuit current and internal reflection of the cells were improved, resulting in a significant increase of about 80 mA in the champion samples compared to the baseline group.

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Article Chemistry, Physical

Inverted perovskite/silicon V-shaped tandem solar cells with 27.6% efficiency via self-assembled monolayer-modified nickel oxide layer

Likai Zheng et al.

Summary: A novel inverted perovskite/silicon V-shaped tandem solar cell was proposed in this work, achieving efficient photon utilization and optimized energy allocation through an elaborate design. The tandem cell demonstrated a high power-conversion efficiency of 27.6%, offering promising potential for reducing carbon emissions in the silicon cell industrial chain.

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Article Energy & Fuels

Monolithic Perovskite/Silicon Tandem Solar Cells Fabricated Using Industrial p-Type Polycrystalline Silicon on Oxide/Passivated Emitter and Rear Cell Silicon Bottom Cell Technology

Silvia Mariotti et al.

Summary: Combining perovskite and silicon solar cells can enhance the power conversion efficiency of silicon single-junction technology.

SOLAR RRL (2022)

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A Brief Review of Passivation Materials and Process for High Efficiency PERC Solar Cell

Jaeun Kim et al.

Summary: PERC technology has dominated the global photovoltaic market over the past decade due to its lower cost and higher efficiency. Research continues to focus on reducing recombination loss and improving efficiency by optimizing passivating contact properties and deposition techniques, particularly with the introduction of HfOx material. Analysis confirms that HfOx deposited using ALD shows low interface trap density and can be adjusted to different fixed charge levels, leading to an efficiency of 22.01% in simulations. Further optimization of HfOx as a passivation layer is expected to enable the fabrication of solar cells with even higher efficiency.

TRANSACTIONS ON ELECTRICAL AND ELECTRONIC MATERIALS (2022)

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Article Nanoscience & Nanotechnology

Developing the Next-Generation Perovskite/Si Tandems: Toward Efficient, Stable, and Commercially Viable Photovoltaics

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Summary: This article discusses the development history, efficiency improvement, and commercialization challenges of perovskite/silicon tandem solar cell technology, emphasizing the importance of improving efficiency and accelerating commercialization.

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Unleashing the Full Power of Perovskite/Silicon Tandem Modules with Solar Trackers

Maxime Babics et al.

Summary: Research shows that combining perovskite/silicon tandem solar cells with solar trackers can achieve higher power generation efficiency and significant economic advantages.

ACS ENERGY LETTERS (2022)

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Article Multidisciplinary Sciences

Efficient and stable perovskite-silicon tandem solar cells through contact displacement by MgFx

Jiang Liu et al.

Summary: The performance of perovskite solar cells with inverted polarity can be improved by adding a MgFx interlayer at the perovskite/C-60 interface. This interlayer facilitates efficient electron extraction, reduces nonradiative recombination, and exhibits good stability under damp-heat conditions.

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Editorial Material Chemistry, Physical

Monolithic Perovskite/Silicon Tandem Photovoltaics with Minimized Cell-to-Module Losses by Refractive-Index Engineering

Lujia Xu et al.

Summary: We report a highly efficient monolithic perovskite/silicon tandem single-cell solar module, achieving a short-circuit current density of 18.6 mA/cm2 through enhanced optical design.

ACS ENERGY LETTERS (2022)

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Nano-optical designs for high-efficiency monolithic perovskite-silicon tandem solar cells

Philipp Tockhorn et al.

Summary: Gentle sinusoidal nanotextures were designed to achieve high-efficiency perovskite-silicon solar cells, offering advantages such as reduced reflection losses, increased fabrication yield, and improved open-circuit voltage.

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Stable pure-iodide wide-band-gap perovskites for efficient Si tandem cells via kinetically controlled phase evolution

Su Geun Ji et al.

Summary: This study reports a pure-iodide wide-band-gap perovskite top cell that is almost free from halide segregation. Cs and dimethylammonium cations were simultaneously incorporated into the A-site of the perovskite to increase the band gap while maintaining the tolerance factor. However, the incorporation of dual cations resulted in the formation of orthorhombic and hexagonal phases instead of the pure perovskite phase.

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Summary: This article discusses the goals of solar cell technology, the unique characteristics and technical parameters of TOPCon solar cells, as well as different deposition methods for the SiOx tunnel oxide layer. It also briefly touches on the impact of deposition conditions on cell parameters and the development of alternative tunnel oxide materials for TOPCon solar cells.

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Perovskite tandem solar cells with improved efficiency and stability

Zhengjie Zhu et al.

Summary: Tandem solar cells offer an attractive approach to increasing power-conversion-efficiency and achieving industry goals, by pairing wide-bandgap metal halide perovskites with complementary bandgap photovoltaic technologies. Comparative studies of 2-terminal and 4-terminal tandems, along with collective efforts to enhance performance, processing, and stability, have led to significant progress in the field. However, further research on mobile ion character and stability testing is crucial for improving perovskite tandems towards long-term outdoor operation.

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Amorphous Silicon Thin Film Deposition for Poly-Si/SiO2 Contact Cells to Minimize Parasitic Absorption in the Near-Infrared Region

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Summary: The research proposes using a thin layer of amorphous silicon in TOPCon solar cells to reduce parasitic absorption, and improving solar cell performance by modifying the timing and temperature of the annealing step. In tandem cell applications, a semitransparent perovskite cell can be used as a filter for absorption in the NIR region.

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The race for the best silicon bottom cell: Efficiency and cost evaluation of perovskite-silicon tandem solar cells

Christoph Messmer et al.

Summary: Perovskite-silicon tandem solar cells have shown rapid progress in the past 5 years and are being investigated as candidates for the next generation of industrial PV devices. Silicon heterojunction technology currently dominates tandem research, but transferring these results to industrial production remains a challenge.

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Article Energy & Fuels

Microcrystalline Silicon Tunnel Junction for Monolithic Tandem Solar Cells Using Silicon Heterojunction Technology

Apolline Puaud et al.

Summary: A microcrystalline silicon tunnel junction was developed to be used as a tunnel recombination junction in a monolithic tandem integration between a large-gap top cell and a silicon heterojunction bottom cell. The addition of this junction on top of silicon heterojunction solar cells improved field effect and passivation, showing promising results for complete integration on the tandem device.

IEEE JOURNAL OF PHOTOVOLTAICS (2021)

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Review Chemistry, Physical

Wide-Bandgap Metal Halide Perovskites for Tandem Solar Cells

Jinhui Tong et al.

Summary: Metal halide perovskite solar cells have emerged as the most promising new-generation solar cell technology, especially for wide-bandgap solar cells. Research progress on developing wide-bandgap PSCs and utilizing them in tandem configurations has been highlighted, emphasizing on efficiency improvement and stability challenges.

ACS ENERGY LETTERS (2021)

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Article Energy & Fuels

Efficient bifacial monolithic perovskite/silicon tandem solar cells via bandgap engineering

Michele De Bastiani et al.

Summary: This study presents bifacial monolithic perovskite/silicon tandem solar cells with high efficiency under various illumination conditions, and demonstrates the advantages of bifaciality in practical environments with relevant albedo. The performance of the bifacial tandems is superior to monofacial tandems, offering increased energy generation potential for locations with specific albedo conditions.

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Progress on the intrinsic a-Si:H films for interface passivation of silicon heterojunction solar cells: A review

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Summary: Amorphous/crystalline silicon heterojunction (SHJ) solar cells are known for their high VOC potential, good bifaciality, simple fabrication process, and low thermal-budget manufacturing. Despite their high efficiency, achieving exceptional passivation and efficiency remains a challenge for researchers.

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Stability Improvement of Perovskite Solar Cells by Compositional and Interfacial Engineering

Weiguang Chi et al.

Summary: Solar cells based on metal halide perovskites are approaching their theoretical efficiency limits with global research efforts, but facing challenges in degradation caused by external factors and the improvement of materials and interfaces for stability enhancement.

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Summary: By introducing an interlayer between the electron-transporting and perovskite layers in perovskite solar cells, researchers have successfully enhanced charge extraction and transport from the perovskite, leading to higher power conversion efficiency and fewer interfacial defects. The coherent interlayer allowed the fabrication of devices with a certified efficiency of 25.5%, which maintained about 90% of its initial efficiency even after continuous light exposure for 500 hours. The findings provide guidelines for designing defect-minimizing interfaces in metal halide perovskites and electron-transporting layers.

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Optimization of Tunnel-Junction for Perovskite/Tunnel Oxide Passivated Contact (TOPCon) Tandem Solar Cells

Chunhui Shou et al.

Summary: This study systematically investigated the formation of the tunnel-junction for perovskite/TOPCon tandem solar cells and successfully optimized the process to achieve the minimal contact resistivity at 700 degrees C. The findings provide a simple and useful method for making the tunnel-junction in these tandem solar cells.

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Atomic-layer-deposited Al-doped zinc oxide as a passivating conductive contacting layer for n plus -doped surfaces in silicon solar cells

Bart Macco et al.

Summary: Research has shown that stacks consisting of ultrathin SiO2 coated with ALD ZnO and Al2O3 provide state-of-the-art passivation for n-type crystalline silicon surfaces and additional functionalities for silicon solar cells. The Al2O3 capping layer is crucial in the passivation mechanism, while annealing can significantly improve the transparency and lateral conductivity of ZnO.

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IEEE JOURNAL OF PHOTOVOLTAICS (2021)

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Wide Bandgap Interface Layer Induced Stabilized Perovskite/Silicon Tandem Solar Cells with Stability over Ten Thousand Hours

Yucheng Li et al.

Summary: The perovskite/silicon tandem solar cell can break through the efficiency limitations of silicon cells by optimizing energy level alignment, achieving high efficiency and stability for long-term operation.

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Summary: This study presents a comprehensive subcell diagnosis methodology to identify efficiency limitations in state-of-the-art perovskite/silicon tandem photovoltaics. By analyzing selective intensity-dependent photoluminescence and injection-dependent electroluminescence measurements, it reveals significant losses in perovskite subcells and proposes strategies to minimize these losses.

ACS ENERGY LETTERS (2021)

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Summary: Researchers in the field of perovskite solar cells have been striving to achieve high efficiency and long-term stability. While breakthroughs have been made in efficiency, the challenge of degradation and instability remains a bottleneck. Significant progress has been made in device performance through approaches such as encapsulation, interfacial layer engineering, process engineering, ion engineering, and dopant and alternative engineering.

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Summary: Formamidinium iodide (FAI) based perovskite absorbers have shown to be ideal candidates for highly efficient and stable perovskite solar cells. By co-evaporating FAPbI(3) and controlling the composition, stability of the black perovskite phase at room temperature is achieved. The addition of methylammonium iodide (MAI) during the co-evaporation process leads to good absorption properties and high PSC efficiencies, maintaining stability over long periods of operation.

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Summary: Perovskite/silicon tandem solar cells have shown great potential in surpassing the efficiency limits of single-junction solar cells. By engineering the interface of N-I-P type monolithic PSTSCs, a composite electron transport layer was developed to achieve higher efficiency and open-circuit voltage than before.

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Emitter saturation current densities of 22fA/cm2 applied to industrial PERC solar cells approaching 22% conversion efficiency

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Investigation of positive roles of hydrogen plasma treatment for interface passivation based on silicon heterojunction solar cells

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Inductively coupled plasma chemical vapour deposited AlOx/SiNy layer stacks for applications in high-efficiency industrial-type silicon solar cells

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Effect of hydrogen dilution on intrinsic a-Si:H layer between emitter and Si wafer in silicon heterojunction solar cell

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