☆ 4.6 Review

Recent Advances in the Structural Design of Silicon/Carbon Anodes for Lithium Ion Batteries: A Review

COATINGS (2023)

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Review Chemistry, Applied

Interfacial design of silicon/carbon anodes for rechargeable batteries: A review

Quanyan Man et al.

Summary: This review provides an overview of the research progress on Si/C anodes in lithium-ion batteries. It highlights the lithiation mechanism, solid electrolyte interface formation, and various carbon sources used in Si/C anodes. The review also summarizes and prospects the selection of carbonaceous materials, structural design, and interface control of Si/C anodes, as well as their application in all-solid-state lithium-ion batteries and sodium-ion batteries.

JOURNAL OF ENERGY CHEMISTRY (2023)

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Article Chemistry, Multidisciplinary

Adjustable Dimensionality of Microaggregates of Silicon in Hollow Carbon Nanospheres: An Efficient Pathway for High-Performance Lithium-Ion Batteries

Ruiyu Zhu et al.

Summary: By utilizing microaggregates derived from cogenetic Si/C nano-building blocks, constructing silicon-carbon hybrid materials can enhance lithium storage performance.

ACS NANO (2022)

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Article Chemistry, Physical

Suitable thickness of carbon coating layers for silicon anode

Chuanlei Qi et al.

Summary: In this study, core-shell nanostructured Si@C materials with different thickness of carbon coating were prepared using chemical vapor deposition. The Si@C composite with 2-3 carbon coating layers exhibited excellent electrical conductivity and strong mechanical strength, which helped to buffer the volume expansion of silicon nanoparticles.

CARBON (2022)

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Article Chemistry, Physical

Architecture and performance of Si/C microspheres assembled by nano- Si via electro-spray technology as stability-enhanced anodes for lithium- ion batteries

Wangwu Li et al.

Summary: This study presents a solution to the poor conductivity and volume changes of Si-based anodes in lithium-ion batteries by designing Si/nitrogen doped carbon layer/carbon framework microspheres (SCM). The SCM anode exhibits a high initial columbic efficiency, a high specific capacity, and good electrochemical performance, providing inspiration for the fabrication of high-performance Si/C anode materials.

JOURNAL OF ALLOYS AND COMPOUNDS (2022)

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Article Chemistry, Physical

Reversible Mg metal anode in conventional electrolyte enabled by durable heterogeneous SEI with low surface diffusion barrier

Yajie Li et al.

Summary: A durable and heterogeneous solid electrolyte interphase (SEI) is proposed using a solvent-assisted additive displacement strategy to protect Mg anode from passivation in conventional electrolytes. This SEI has a low surface diffusion barrier and can tolerate long-term cycling without compromising Mg-ion diffusion. This work opens up new possibilities for the application of simple salt electrolytes in magnesium metal batteries.

ENERGY STORAGE MATERIALS (2022)

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Review Chemistry, Physical

Strategies for Controlling or Releasing the Influence Due to the Volume Expansion of Silicon inside Si-C Composite Anode for High-Performance Lithium-Ion Batteries

Xian Zhang et al.

Summary: Silicon is a promising anode material due to its advantages, but its volume expansion causes short cycle life. Silicon/carbon composites can alleviate this issue by forming carbon layers, cavities, and chemical bonds.

MATERIALS (2022)

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Article Nanoscience & Nanotechnology

Electrolyte Design Enabling Stable Solid Electrolyte Interface for High-Performance Silicon/Carbon Anodes

Ziyue Wen et al.

Summary: Silicon-based materials have shown promise as anodes in high-energy-density lithium-ion batteries (LIBs), but interfacial stability and structural degradation remain challenges. In this study, a novel electrolyte cosolvent with high reduction potential and film-forming ability is introduced to overcome the deterioration of the electrode structure. By analyzing the solid electrolyte interface (SEI) layer on the Si/C anode, it is found that a stable SEI with an organic and inorganic bilayer structure is formed, leading to excellent mechanical properties and ionic conductivity. In situ Raman characterization reveals the Li intercalation mechanism. The Si/C-based batteries exhibit impressive cycling and rate performance, showcasing the potential of this electrolyte design for high-performance LIBs.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Materials Science, Multidisciplinary

A Hollow Silicon Nanosphere/Carbon Nanotube Composite as an Anode Material for Lithium-Ion Batteries

Hao Tang et al.

Summary: Silicon has a high theoretical specific capacity as a lithium-ion battery anode material, but suffers from poor cycling performance due to volume expansion. The use of hollow structure and template method, such as polystyrene microspheres, can improve silicon's cycling performance. Hollow silicon spheres with a pore diameter of around 50 nm are obtained and used in carbon nanotubes to create lithium-ion battery anode material, which exhibits excellent cycling performance and rate capability.

COATINGS (2022)

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Article Chemistry, Physical

Facile fabrication of Si-embedded amorphous carbon@graphitic carbon composite microspheres via spray drying as high-performance lithium-ion battery anodes

Su Hyun Yang et al.

Summary: In this study, silicon-nanoparticle-embedded amorphous carbon-graphitic carbon composite microspheres were synthesized using a spray drying process. The resulting microspheres exhibit superior electrochemical properties compared to bare silicon nanopowders and silicon/amorphous carbon composite microspheres, thanks to their unique structure and the presence of empty voids. The composite-based electrode shows excellent long-term cycling stability and stable reversible discharge capacity even at high current density.

APPLIED SURFACE SCIENCE (2022)

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Review Chemistry, Multidisciplinary

Biomass-Based Silicon and Carbon for Lithium-Ion Battery Anodes

Manoj Muraleedharan Pillai et al.

Summary: This review paper focuses on the development of Si and carbon anodes derived from various types of biogenic sources, particularly from plant-derived biomass resources. The biomass precursors, process/extraction methods for producing Si and carbon, the critical physicochemical properties influencing the lithium storage in LIBs, and how they affect the electrochemical performance are highlighted. The review paper also discusses the current research challenges and prospects of biomass-derived materials in developing advanced battery materials.

FRONTIERS IN CHEMISTRY (2022)

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Article Chemistry, Physical

Distinctive conductivity improvement by embedding Cu nanoparticles in the carbon shell of submicron Si@C anode materials for LIBs

Si Chen et al.

Summary: In this study, a Si@C-Cu core shell structure was fabricated by embedding Cu nanoparticles in the carbon shell of submicron Si waste. The resulting Si@C-Cu anode showed improved conductivity and enhanced strength, enabling it to withstand the expansion stress from lithium intercalation in Si. It exhibited high specific discharge capacity and coulombic efficiency, indicating its promising potential as an anode material for lithium-ion batteries.

SUSTAINABLE ENERGY & FUELS (2022)

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Article Materials Science, Multidisciplinary

A comparison of core-shell Si/C and embedded structure Si/C composites as negative materials for lithium-ion batteries

Shuai-Jin Wu et al.

Summary: This study investigated and compared silicon-based negative materials with different microstructures, focusing on their electrochemical performance and electrode morphology evolution during cycling. The embedded structure Si/C material showed superior cycling performance and electrode structure maintenance compared to core-shell Si/C material, with a higher capacity retention ratio after 100 cycles. These findings can provide guidance for the design and application of nano/micro-structured silicon-based negative materials.

RARE METALS (2021)

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Article Nanoscience & Nanotechnology

Reversible Silicon Anodes with Long Cycles by Multifunctional Volumetric Buffer Layers

Tiansheng Mu et al.

Summary: By structurally manipulating the silicon composite anode T-Si@C, a stable configuration has been achieved to enhance the energy storage performance of lithium-ion batteries. The anode exhibits outstanding long-term cycling reversibility and good rate capability, as well as superior electrochemical reversibility in full cells.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Directly conversion the biomass-waste to Si/C composite anode materials for advanced lithium ion batteries

Qiang Ma et al.

Summary: A strategy for converting rice husks into Si/C composite structure anodes was established, resulting in batteries with superior electrochemical stability.

CHINESE CHEMICAL LETTERS (2021)

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Review Energy & Fuels

Recent advances of silicon, carbon composites and tin oxide as new anode materials for lithium-ion battery: A comprehensive review

Mohd Asyadi Azam et al.

Summary: The performance of lithium-ion batteries is influenced by the efficient electrochemical reactions between anode and cathode. New anode materials such as silicon, carbon composites, and tin oxide are being studied as potential substitutes for graphite, with a focus on their impact on battery performance. Recent progress in anode materials in lithium-ion batteries from 2016 to 2020 is discussed in this review, presenting an overview of design, recent developments, and challenges.

JOURNAL OF ENERGY STORAGE (2021)

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Article Chemistry, Physical

Coral-like porous composite material of silicon and carbon synthesized by using diatomite as self-template and precursor with a good performance as anode of lithium-ions battery

Fang Di et al.

Summary: Utilizing low-cost natural diatomite as both precursor and template, a coral-like porous Si/C (CLP-Si/C) material with stable cycling performance as LIB anode has been successfully synthesized in this study, providing a promising strategy for producing porous Si/C anode materials with high-performance.

JOURNAL OF ALLOYS AND COMPOUNDS (2021)

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Article Chemistry, Applied

N-doped porous carbon nanofibers sheathed pumpkin-like Si/C composites as free-standing anodes for lithium-ion batteries

Yanfei Zeng et al.

Summary: The use of free-standing Si/C-ZIF-8/CNFs electrodes can achieve high capacity and good cycling performance. This study provides a new pathway for the development of high-performance silicon-based anodes.

JOURNAL OF ENERGY CHEMISTRY (2021)

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Editorial Material Energy & Fuels

Silicon anodes

Yi Cui

NATURE ENERGY (2021)

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Article Chemistry, Physical

Scalable synthesis of interconnected hollow Si/C nanospheres enabled by carbon dioxide in magnesiothermic reduction for high-performance lithium energy storage

Jian Zhang et al.

Summary: The study demonstrates a novel interconnected hollow Si/C nanospheres with thin shells consisting of Si crystals and highly wrinkled amorphous carbon layers, synthesized by introducing CO2 as a green carbon source in magnesiotherimic reduction to accelerate commercial application. The interconnected carbon networks and MgO cores are simultaneously generated via the reaction between CO2 and excess Mg vapor, with the hollow structure realized after removing in-situ generated MgO templates through acid etching. The unique interconnected Si/C hybrid delivers high capacity, impressive cycling performance, and good Coulombic efficiency, benefiting from improved Li+ ion transportation and electron transfer kinetics, as well as the volume buffering effects of the hollow architecture.

JOURNAL OF POWER SOURCES (2021)

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Article Chemistry, Physical

Solid-state batteries designed with high ion conductive composite polymer electrolyte and silicon anode

Jun Pan et al.

Summary: A three-dimensional porous composite polymer electrolyte with high ionic conductivity was successfully fabricated to address low ionic conductivity in polymer solid-state batteries, along with controlled Li dendrite growth. This design, along with the adoption of micro-sized Si@Li3PO4@C, has significantly improved the performance of SSBs, paving a new way to construct practical solid-state batteries.

ENERGY STORAGE MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Binary Network of Conductive Elastic Polymer Constraining Nanosilicon for a High-Performance Lithium-Ion Battery

Yongxiang Su et al.

Summary: A multifunctional polymeric binder synthesized from conducting polymer and stretchable polymer is capable of forming a three-dimensional network beneficial for electron transfer and mechanical stability, while also being elastic and adhesive to accommodate the huge volume change of silicon. This binder, with high conductivity, elasticity, and self-healing properties, shows enhanced cycling stability and rate performance for nanosilicon anode, making it a promising option for high performance lithium-ion batteries.

ACS NANO (2021)

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Article Chemistry, Multidisciplinary

A Micrometer-Sized Silicon/Carbon Composite Anode Synthesized by Impregnation of Petroleum Pitch in Nanoporous Silicon

Sujong Chae et al.

Summary: The study reports a method of preserving the porous Si nanostructure by impregnating petroleum pitch inside porous Si before high-temperature treatment, resulting in a Si/C composite with desired porosity and high conductivity. In a Si||Li(Ni0.5Co0.2Mn0.3)O-2 (NMC532) battery, an anode with 80% pitch-derived carbon/nanoporous Si shows very stable cycling performance.

ADVANCED MATERIALS (2021)

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Article Chemistry, Physical

In-situ low-temperature strategy from waste sugarcane leaves towards micro/meso-porous carbon network embedded nano Si-SiOx@C boosting high performances for lithium-ion batteries

Wenyan Chen et al.

Summary: A new strategy for preparing high value-added silicon-based materials from biomass, utilizing molten-salt assisted low-temperature reaction, successfully fabricated nano Si-SiOx@C composites with micro/meso-porous carbon network embedded, exhibiting excellent electrochemical performance and cycling stability. This approach has the potential to advance research on functional materials derived from biomass.

CARBON (2021)

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Article Electrochemistry

Achieving fully reversible conversion in Si anode for lithium-ion batteries by design of pomegranate-like Si@C structure

Chong Han et al.

Summary: Pomegranate-like Si@C microspheres exhibit excellent electrochemical performance, stabilizing the structure of Si particles and improving electrochemical properties. This unique structure enables the sample to achieve high Coulombic efficiency and stable cycling.

ELECTROCHIMICA ACTA (2021)

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Article Energy & Fuels

Interconnected Hollow Si/C Hybrids Engineered by the Carbon Dioxide-Introduced Magnesiothermic Reduction of Biosilica from Reed Plants for Lithium Storage

Jie Wang et al.

Summary: The research reports the fabrication of interconnected hollow Si/C hybrids derived from reed plants using CO2, showing excellent performance potential; the amount of CO2 and HCl concentration during the extraction of SiO2 affected the structure design and composition of the Si/C hybrids in this synthetic system; the Si/C composites demonstrated outstanding cycling performance and rate capability, attributed to their unique structure and high electrical conductivity.

ENERGY & FUELS (2021)

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Article Chemistry, Physical

Mussel-pearl-inspired design of Si/C composite for ultrastable lithium storage anodes

Yu Du et al.

Summary: The study developed a mussel-pearl-inspired silicon-embedded carbon/graphite composite to overcome the obstacles of volume expansion and poor conductivity of silicon in new generation high-performance lithium-ion batteries. The composite showed ultrastable reversible capacity, superior initial Coulombic efficiency, and high capacity retention over cycles, with superior rate capacity at high current density. The excellent electrochemical performances were attributed to the structure stability of mussel pearl design providing effective protection for silicon nanoparticles.

JOURNAL OF ALLOYS AND COMPOUNDS (2021)

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Article Chemistry, Multidisciplinary

Silicon@Natural Nitrogen-Doped Biomass Carbon Composites Derived from Silicon Tofu as Green and Efficient Anode Materials for Lithium-Ion Batteries

Xuejiao Xu et al.

Summary: The use of tofu as a low-cost source of carbon and nitrogen can effectively transform protein structures into a carbon-nitrogen conductive network, maintaining the integrity of the electrode structure during cycling. The Si@natural nitrogen-doped biomass carbon composite shows promising reversible capacity even at high current densities, with an environmentally friendly and sustainable preparation process. This research provides a simple, clean, and scalable solution for green and efficient anode materials for LIBs.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2021)

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Article Chemistry, Physical

Encapsulating Nanoscale Silicon inside Carbon Fiber as Flexible Self-Supporting Anode Material for Lithium-Ion Battery

Wangwu Li et al.

Summary: A flexible freestanding N-doped core-shell Si/C nanofiber anode was prepared in this study, which addresses the issues of volume change and low conductivity of silicon materials, demonstrating good cycling performance.

ACS APPLIED ENERGY MATERIALS (2021)

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Article Chemistry, Physical

Boron-Doped and Carbon-Controlled Porous Si/C Anode for High-Performance Lithium-Ion Batteries

Lei Li et al.

Summary: Silicon, as a promising anode material for next generation lithium-ion batteries, was synthesized using a facile method based on dealloying reaction to create porous boron-doped silicon with low carbon content. This anode showed high initial Coulombic efficiency, excellent rate performance, and long cycle stability.

ACS APPLIED ENERGY MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Self-supporting dual-confined porous Si@c-ZIF@carbon nanofibers for high-performance lithium-ion batteries

Jiale Chen et al.

Summary: Dual-confined porous Si@c-ZIF@carbon nanofibers exhibit excellent cycling and rate performance when used as self-supporting anodes for lithium-ion batteries.

CHEMICAL COMMUNICATIONS (2021)

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Review Chemistry, Multidisciplinary

Regulating the carbon distribution of anode materials in lithium-ion batteries

Miaomiao Jiang et al.

Summary: The exploration of electrode materials has a crucial impact on the development of lithium-ion batteries, with challenges in conductivity and volume change hindering commercial application. Carbon-matrix composite anodes have been identified as an effective strategy, with recent advances focusing on regulating carbon distribution. This review provides insights into future trends in carbon-matrix electrode design for LIBs.

NANOSCALE (2021)

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Article Chemistry, Multidisciplinary

Nano/Microstructured Silicon-Carbon Hybrid Composite Particles Fabricated with Corn Starch Biowaste as Anode Materials for Li-Ion Batteries

Hyun Jung Kwon et al.

NANO LETTERS (2020)

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Article Chemistry, Physical

Lithium-conducting covalent-organic-frameworks as artificial solid-electrolyte-interphase on silicon anode for high performance lithium ion batteries

Qing Ai et al.

NANO ENERGY (2020)

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Article Energy & Fuels

Scalable Synthesis of Si/C Microspheres with 3D Conducting Nanosized Porous Channels as High-Performance Anodes in LIBs

Shimin Huang et al.

ENERGY & FUELS (2020)

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Review Electrochemistry

Research Progress of Silicon/Carbon Anode Materials for Lithium-Ion Batteries: Structure Design and Synthesis Method

Xinzhi Li et al.

CHEMELECTROCHEM (2020)

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Article Chemistry, Physical

A novel raspberry-like yolk-shell structured Si/C micro/nano-spheres as high-performance anode materials for lithium-ion batteries

Canliang Ma et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2020)

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Prospects for lithium-ion batteries and beyond-a 2030 vision

Clare P. Grey et al.

NATURE COMMUNICATIONS (2020)

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Graphene bubble film encapsulated Si@C hollow spheres as a durable anode material for lithium storage

Xiaoyu Liu et al.

ELECTROCHIMICA ACTA (2020)

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Nano-silicon embedded in MOFs-derived nitrogen-doped carbon/cobalt/carbon nanotubes hybrid composite for enhanced lithium ion storage

Hang Luo et al.

APPLIED SURFACE SCIENCE (2020)

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A compact silicon-carbon composite with an embedded structure for high cycling coulombic efficiency anode materials in lithium-ion batteries

Wei Zhang et al.

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The influence of compact and ordered carbon coating on solid-state behaviors of silicon during electrochemical processes

Shuo Zhou et al.

CARBON ENERGY (2020)

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Engineering the Distribution of Carbon in Silicon Oxide Nanospheres at the Atomic Level for Highly Stable Anodes

Guanjia Zhu et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Scalable synthesis of ant-nest-like bulk porous silicon for high-performance lithium-ion battery anodes

Weili An et al.

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NANOMATERIALS (2019)

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Morphology-controlled synthesis of hollow Si/C composites based on KI-assisted magnesiothermic reduction for high performance Li-ion batteries

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Nano-Si/C microsphere with hollow double spherical interlayer and submicron porous structure to enhance performance for lithium-ion battery anode

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Effects of nitrogen doping on Si/carbon composite anode derived from Si wastes as potential active materials for Li ion batteries

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Low-Temperature Reduction Strategy Synthesized Si/Ti3C2 MXene Composite Anodes for High-Performance Li-Ion Batteries

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Hollow Triple-Layer Puff-like HCs@Si@C Composites with High Structural Stability for High-Performance Lithium-Ion Battery

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ACS APPLIED ENERGY MATERIALS (2019)

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