期刊
CHEMCATCHEM
卷 8, 期 3, 页码 527-531出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cctc.201501055
关键词
activated carbon; copper; dimethyl oxalate; hydrogenation; methyl glycolate
资金
- Major State Basic Resource Development Program [2012CB224804]
- NSFC [21373054, 21173052]
- Natural Science Foundation of Shanghai Science and Technology Committee [08DZ2270500]
Copper-based activated-carbon (AC)-supported catalysts were synthesized by a facile ammonia evaporation-impregnation method. Unlike the conventional Cu/SiO2 catalyst, which showed highly catalytic selectivity towards ethylene glycol (EG) or EtOH, Cu/AC catalysts display unique selectivity to methyl glycolate (MG). The catalytic performance relies on the high content of surface Cu+ species and the relatively large copper particles with moderate hydrogenation activity.
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