Photoelectrochemical Selective Oxidation of Glycerol to Glyceraldehyde with Bi-Based Metal-Organic-Framework-Decorated WO3 Photoanode

Article Chemistry, Physical

Electrochemical oxidation of glycerol to hydroxypyruvic acid on cobalt (oxy)hydroxide by high-valent cobalt redox centers

Xin Huang et al.

Summary: Substoichiometric cobalt (oxy)hydroxide has been demonstrated as an effective electrocatalyst for selective glycerol oxidation to hydroxypyruvic acid, offering a new perspective for glycerol valorization.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Chemistry, Physical

Enhancing the photocatalytic activity of Ruddlesden-Popper Sr2TiO4 for hydrogen evolution through synergistic silver doping and moderate reducing pretreatment

Hongbo Xiao et al.

Summary: In this study, silver-doped and moderately reduced Sr2TiO4 photocatalysts were synthesized, showing improved morphological characteristics and enhanced hydrogen generation performance.

MATERIALS TODAY ENERGY (2022)

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Article Chemistry, Physical

Non-metal fluorine doping in Ruddlesden-Popper perovskite oxide enables high-efficiency photocatalytic water splitting for hydrogen production

Xiao Han et al.

Summary: In this study, a non-metal fluorine (F-) doping strategy was utilized to enhance the photocatalytic activity of Ruddlesden-Popper Sr2TiO4 perovskites for H-2 evolution reaction (HER). By optimizing the F- doping amount, the highest H2 generation rate was achieved by Sr2TiO3.97F0.03, which showed a 44% enhancement compared to Sr2TiO4. The improved photocatalytic activity of Sr2TiO3.97F0.03 can be attributed to the effects of F- doping on surface oxygen vacancies, charge carrier recombination, conduction band position, band gap energy, particle size, and specific surface area.

MATERIALS TODAY ENERGY (2022)

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Article Chemistry, Physical

Selective oxidation of glycerol over different shaped WO3 supported Pt NPs

Lihua Yang et al.

Summary: In this study, Pt catalysts supported on different shaped WO3 (rod-like, lamellar and cuboid) were prepared and tested for the selective oxidation of glycerol in base-free aqueous solution. The Pt/R-WO3 catalyst with rod-like WO3 support showed higher surface area and activity, as well as enhanced selectivity towards glyceric acid.

MOLECULAR CATALYSIS (2022)

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Article Nanoscience & Nanotechnology

WO3 Photoanode with Predominant Exposure of {202} Facets for Enhanced Selective Oxidation of Glycerol to Glyceraldehyde

Jie Ouyang et al.

Summary: Controlling facet exposure can modulate the activity and selectivity of a photoanode. This study demonstrates that a WO3 photoanode with predominant exposure of {202} facets exhibits superior photoelectrocatalytic oxidation efficiency for glycerol, achieving high selectivity and Faraday efficiency for the valuable C3 products.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Chemistry, Physical

Fluorine-doped iron oxyhydroxide cocatalyst: promotion on the WO3 photoanode conducted photoelectrochemical water splitting

Yan Li et al.

Summary: In this study, the performance of WO3 as a photoanode was improved by doping with F and preparing F:FeOOH/BiVO4/WO3 composite photoanodes. The composite photoanodes exhibited significantly enhanced photocurrent and showed good stability and electron lifetime. Additionally, F-doped FeOOH showed better catalytic performance than FeOOH. This work may have important implications for the application of photocatalysts in PEC water splitting.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Engineering, Chemical

Glycerin to Acrolein: Can Renewable Processes Challenge Traditional Processes?

Jingfeng Yang et al.

Summary: The production of acrolein was compared using the FAA, PO, and GTA processes, and it was found that the PO process is the most economical. However, the renewable process performed better if certain conditions were met.

CHEMICAL ENGINEERING & TECHNOLOGY (2022)

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Article Chemistry, Multidisciplinary

Selective Photoelectrocatalytic Glycerol Oxidation to Dihydroxyacetone via Enhanced Middle Hydroxyl Adsorption over aBi2O3-Incorporated Catalyst

Lan Luo et al.

Summary: This study reports a photoelectrocatalytic (PEC) glycerol oxidation method for the production of dihydroxyacetone (DHA) with enhanced selectivity. A heterogeneous photoanode consisting of Bi2O3 nanoparticles on TiO2 nanorod arrays was used, and the selectivity of DHA was increased. Experimental and theoretical studies revealed the interaction between the catalyst and glycerol, as well as the parallel pathways of the reaction. Furthermore, a self-powered PEC system was designed, achieving high productivity of DHA and H2.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2022)

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Article Chemistry, Physical

Mediating the Oxidizing Capability of Surface-Bound Hydroxyl Radicals Produced by Photoelectrochemical Water Oxidation to Convert Glycerol into Dihydroxyacetone

Yang Liu et al.

Summary: In this study, a ternary photoanode material was developed for the selective oxidation of glycerol to 1,3-dihydroxyacetone. The photoanode showed high selectivity and kinetic response, with hydroxyl radicals generated by water oxidation playing a dominant role as active oxygen species. The oxidation product obtained mainly came from water. The role of different components in enhancing the selectivity and catalyzing the reaction was revealed through spectroscopic and computational studies.

ACS CATALYSIS (2022)

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Article Chemistry, Physical

Enhancing glycerol electrooxidation from synergistic interactions of platinum and transition metal carbides

Hansen Mou et al.

Summary: This study demonstrates the synergistic interactions between platinum and transition metal carbide substrates, which leads to higher activity and selectivity for glycerol oxidation in electrochemical fuel cells. The insights gained from in-situ FTIR analysis, X-ray absorption fine structure characterization, and density functional theory calculations provide a deeper understanding of the catalysts' performance.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Chemistry, Physical

CeO2 nanoarray decorated Ce-doped ZnO nanowire photoanode for efficient hydrogen production with glycerol as a sacrificial agent

Seungkyu Kim et al.

Summary: A novel CeO2-decorated Ce-doped ZnO nanowire photoanode has been reported for efficient PEC glycerol oxidation and hydrogen production, with improved charge separation, light-harvesting, and glycerol adsorption. The Ce-doped ZnO array shows enhanced operation stability and doubled hydrogen evolution compared to a bare ZnO electrode.

CATALYSIS SCIENCE & TECHNOLOGY (2022)

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Article Engineering, Environmental

Selective photoelectrocatalytic oxidation of glycerol by nanotube, nanobelt and nanosponge structured TiO2 on Ti plates

Sidika Cetinkaya et al.

Summary: The photoelectrocatalytic oxidation of glycerol to commercially valuable compounds using TiO2 photoanodes was investigated. The effects of various factors on the oxidation activity and product selectivity were studied. The results showed that TiO2 nanotubes exhibited the best catalytic activity under certain conditions.

JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING (2022)

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Review Chemistry, Physical

Single-atom catalysts for high-efficiency photocatalytic and photoelectrochemical water splitting: distinctive roles, unique fabrication methods and specific design strategies

Jingsheng He et al.

Summary: This article presents a comprehensive review of recent advances in single-atom catalysts (SACs) for photocatalytic and photoelectrochemical water splitting. The distinctive roles of SACs and unique fabrication methods are highlighted. Additionally, several specific design strategies to enhance the photo(electro)catalytic activity of SACs are discussed, along with prospects for future applications in efficient solar energy utilization.

JOURNAL OF MATERIALS CHEMISTRY A (2022)

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Review Chemistry, Applied

Surface-Modified Co-doped ZnO Photoanode for Photoelectrochemical Oxidation of Glycerol

Yubin Lee et al.

Summary: By fabricating a photoanode with cobalt-doped zinc oxide nanoparticles, researchers have enhanced the efficiency and selectivity of glycerol oxidation to glyceric acid, providing a new approach to improve the photocatalytic properties of ZnO.

CATALYSIS TODAY (2021)

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Article Chemistry, Physical

Glyceraldehyde production by photocatalytic oxidation of glycerol on WO3-based materials

Jie Yu et al.

Summary: The valorization of glycerol into high added-value products by photocatalysis not only creates good economic benefits, but also meets global low-carbon and energy-saving environmental protection needs. This study found that WO3-based materials exhibit outstanding selectivity towards valuable oxidation products like glyceraldehyde, establishing a new starting point for the development of advanced materials for efficient glycerol valorization.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Chemistry, Physical

Co-catalytic effects of Bi-based metal-organic framework on BiVO4 photoanodes for photoelectrochemical water oxidation

Seungkyu Kim et al.

Summary: Metal-organic frameworks (MOFs) show promise as co-catalysts for enhancing PEC water splitting, with the decoration of the BiVO4 photoanode surface with a Bi-based MOF leading to increased photocurrent density and improved operational stability.

APPLIED SURFACE SCIENCE (2021)

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Review Chemistry, Physical

Metal organic frameworks as electrocatalysts: Hydrogen evolution reactions and overall water splitting

Meena Nemiwal et al.

Summary: This review summarizes the recent advances in heterogeneous catalysis using metal organic frameworks (MOFs) as electrocatalysts for hydrogen evolution reaction (HER) and water splitting, including the enhancement of performance with composites of MOFs and bifunctional electrocatalysts derived from MOFs using different synthetic approaches.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2021)

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Review Engineering, Environmental

Recent progress on metal-organic frameworks based- and derived-photocatalysts for water splitting

Hanzhuo Luo et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Review Energy & Fuels

A review on feedstocks, production processes, and yield for different generations of biodiesel

Digambar Singh et al.

FUEL (2020)

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Article Chemistry, Applied

Microwave-Assisted Solvothermal Synthesis and Photocatalytic Activity of Bismuth(III) Based Metal-Organic Framework

Vinh Huu Nguyen et al.

TOPICS IN CATALYSIS (2020)

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Article Chemistry, Physical

3D core-shell WO3@α-Fe2O3 photoanode modified by ultrathin FeOOH layer for enhanced photoelectrochemical performances

Jin Zhang et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2020)

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Article Chemistry, Physical

Unveiling the crystallographic facet dependence of the photoelectrochemical glycerol oxidation on bismuth vanadate

Truong-Giang Vo et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Article Chemistry, Physical

Ultrathin 2D/2D WO3/g-C3N4 step-scheme H2-production photocatalyst

Junwei Fu et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2019)

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Article Multidisciplinary Sciences

Selective photoelectrochemical oxidation of glycerol to high value-added dihydroxyacetone

Dong Liu et al.

NATURE COMMUNICATIONS (2019)

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Article Electrochemistry

Converting glycerol aqueous solution to hydrogen energy and dihydroxyacetone by the BiVO4 photoelectrochemical cell

Lu-Wei Huang et al.

ELECTROCHIMICA ACTA (2019)

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Article Chemistry, Multidisciplinary

Bi-metal-organic frameworks type II heterostructures for enhanced photocatalytic styrene oxidation

Lulu Liu et al.

NANOSCALE (2019)

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Review Chemistry, Physical

Study on catalyst selection for electrochemical valorization of glycerol

Mohamed S. E. Houache et al.

SUSTAINABLE ENERGY & FUELS (2019)

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Review Chemistry, Applied

Selective oxidation of glycerol in a base-free aqueous solution: A short review

Lihua Yang et al.

CHINESE JOURNAL OF CATALYSIS (2019)

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Article Chemistry, Physical

Preparation and characterization of metals supported on nanostructured TiO2 hollow spheres for production of hydrogen via photocatalytic reforming of glycerol

Tumelo W. P. Seadira et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2018)

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Article Materials Science, Multidisciplinary

Facile and one step synthesis of WO3 nanorods and nanosheets as an efficient photocatalyst and humidity sensing material

M. Parthibavarman et al.

VACUUM (2018)

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Review Chemistry, Physical

Recent Advances in Thermo-, Photo-, and Electrocatalytic Glycerol Oxidation

Georgios Dodekatos et al.

ACS CATALYSIS (2018)

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Article Chemistry, Multidisciplinary

Photocatalytic Reforming of Biomass Derived Crude Glycerol in Water: A Sustainable Approach for Improved Hydrogen Generation Using Ni(OH)(2) Decorated TiO2 Nanotubes under Solar Light Irradiation

Nagappagari Lakshmana Reddy et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2018)

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Review Chemistry, Inorganic & Nuclear

Metal-organic frameworks for electrocatalysis

Pei-Qin Liao et al.

COORDINATION CHEMISTRY REVIEWS (2018)

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Article Materials Science, Ceramics

Molecularly imprinted photocatalyst for glyceraldehyde production

Cicero Coelho de Escobar et al.

JOURNAL OF SOL-GEL SCIENCE AND TECHNOLOGY (2018)

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Review Chemistry, Multidisciplinary

WO3-based photocatalysts: morphology control, activity enhancement and multifunctional applications

Pengyu Dong et al.

ENVIRONMENTAL SCIENCE-NANO (2017)

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Review Chemistry, Multidisciplinary

Earth-abundant catalysts for electrochemical and photoelectrochemical water splitting

Isolda Roger et al.

NATURE REVIEWS CHEMISTRY (2017)

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Review Chemistry, Multidisciplinary

Electrocatalysis for the oxygen evolution reaction: recent development and future perspectives

Nian-Tzu Suen et al.

CHEMICAL SOCIETY REVIEWS (2017)

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Article Chemistry, Multidisciplinary

Carbon coated porous nickel phosphides nanoplates for highly efficient oxygen evolution reaction

Xin-Yao Yu et al.

ENERGY & ENVIRONMENTAL SCIENCE (2016)

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Review Chemistry, Physical

Review: Biofuel production from plant and algal biomass

Roman A. Voloshin et al.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2016)

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Article Chemistry, Multidisciplinary

Effect of the morphology and phases of WO3 nanocrystals on their photocatalytic efficiency

Davidne Nagy et al.

RSC ADVANCES (2016)

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Article Chemistry, Physical

One-Step Hydrothermal Deposition of Ni:FeOOH onto Photoanodes for Enhanced Water Oxidation

Lili Cai et al.

ACS ENERGY LETTERS (2016)

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Review Chemistry, Multidisciplinary

Noble metal-free hydrogen evolution catalysts for water splitting

Xiaoxin Zou et al.

CHEMICAL SOCIETY REVIEWS (2015)

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Article Chemistry, Multidisciplinary

Non-precious alloy encapsulated in nitrogen-doped graphene layers derived from MOFs as an active and durable hydrogen evolution reaction catalyst

Yang Yang et al.

ENERGY & ENVIRONMENTAL SCIENCE (2015)

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Article Chemistry, Multidisciplinary

A Bismuth-Based Metal-Organic Framework as an Efficient Visible-Light-Driven Photocatalyst

Guanzhi Wang et al.

CHEMISTRY-A EUROPEAN JOURNAL (2015)

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Article Chemistry, Physical

Crude glycerol as a raw material for the liquid phase oxidation reaction

Elzbieta Skrzynska et al.

APPLIED CATALYSIS A-GENERAL (2014)

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Review Chemistry, Multidisciplinary

Photoelectrochemical hydrogen production from biomass derivatives and water

Xihong Lu et al.

CHEMICAL SOCIETY REVIEWS (2014)

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Water adsorption in MOFs: fundamentals and applications

Jerome Canivet et al.

CHEMICAL SOCIETY REVIEWS (2014)

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Editorial Material Chemistry, Multidisciplinary

Metal-Organic Frameworks (MOFs)

Hong-Cai ''Joe'' Zhou et al.

CHEMICAL SOCIETY REVIEWS (2014)

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Review Chemistry, Multidisciplinary

Green and sustainable manufacture of chemicals from biomass: state of the art

Roger A. Sheldon

GREEN CHEMISTRY (2014)

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Article Chemistry, Physical

Photoelectrochemical performance of graphene-modified TiO2 photoanodes in the presence of glycerol as a hole scavenger

Muhammad Ibadurrohman et al.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2014)

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Synthesis and Electrocatalytic Activity Evaluation of Nanoflower Shaped Ni-Pd on Alcohol Oxidation Reaction

Mohammad Shamsuddin Ahmed et al.

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Benchmarking Heterogeneous Electrocatalysts for the Oxygen Evolution Reaction

Charles C. L. McCrory et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2013)

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The Chemistry and Applications of Metal-Organic Frameworks

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SCIENCE (2013)

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Etherification of biodiesel-derived glycerol with ethanol for fuel formulation over sulfonic modified catalysts

Juan A. Melero et al.

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Glycerol Carboxylation to Glycerol Carbonate in the Presence of Rhodium Complexes with Phosphine Ligands

N. N. Ezhova et al.

PETROLEUM CHEMISTRY (2012)

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Large-Pore Apertures in a Series of Metal-Organic Frameworks

Hexiang Deng et al.

SCIENCE (2012)

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Palladium-Tin Alloyed Catalysts for the Ethanol Oxidation Reaction in an Alkaline Medium

Wenxin Du et al.

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Heterojunction BiVO4/WO3 electrodes for enhanced photoactivity of water oxidation

Suk Joon Hong et al.

ENERGY & ENVIRONMENTAL SCIENCE (2011)

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Article Food Science & Technology

Oligomerization of glycerol - a critical review

Andreas Martin et al.

EUROPEAN JOURNAL OF LIPID SCIENCE AND TECHNOLOGY (2011)

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Review Chemistry, Multidisciplinary

Selective catalytic oxidation of glycerol: perspectives for high value chemicals

Benjamin Katryniok et al.

GREEN CHEMISTRY (2011)

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Review Chemistry, Multidisciplinary

Glycerol dehydration to acrolein in the context of new uses of glycerol

Benjamin Katryniok et al.

GREEN CHEMISTRY (2010)

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Cs-Modified WO3 Photocatalyst Showing Efficient Solar Energy Conversion for O2 Production and Fe (III) Ion Reduction under Visible Light

Yugo Miseki et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2010)

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Article Chemistry, Physical

Synthesis of glycerol carbonate from glycerol and dimethyl carbonate by transesterification: Catalyst screening and reaction optimization

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Virtual High Throughput Screening Confirmed Experimentally: Porous Coordination Polymer Hydration

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Review Chemistry, Multidisciplinary

Chemoselective catalytic conversion of glycerol as a biorenewable source to valuable commodity chemicals

Chun-Hui (Clayton) Zhou et al.

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Efficient photoelectrolysis of water using TiO2 nanotube arrays by minimizing recombination losses with organic additives

S. K. Mohapatra et al.

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Evaluation of nitrogen doping of tungsten oxide for photoelectrochemical water splitting

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JOURNAL OF PHYSICAL CHEMISTRY C (2008)

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UV-generated free radicals (FR) in skin: Their prevention by sunscreens and their induction by self-tanning agents

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SPECTROCHIMICA ACTA PART A-MOLECULAR AND BIOMOLECULAR SPECTROSCOPY (2008)

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Dimitris I. Kondarides et al.

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Impact of preparation and handling on the hydrogen storage properties of Zn4O(1,4-benzenedicarboxylate)3 (MOF-5)

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Etherification of glycerol and ethylene glycol by isobutylene

Katarina Klepacova et al.

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Hydrogenolysis of glycerol over carbon-supported Ru and Pt catalysts

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Anaerobic fermentation of glycerol: a path to economic viability for the biofuels industry

Syed Shams Yazdani et al.

CURRENT OPINION IN BIOTECHNOLOGY (2007)

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Photoelectrochemical behavior of nanostructured WO3 thin-film electrodes:: The oxidation of formic acid

Damian Monllor-Satoca et al.

CHEMPHYSCHEM (2006)

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A study on the carboxylation of glycerol to glycerol carbonate with carbon dioxide: The role of the catalyst, solvent and reaction conditions

Michele Aresta et al.

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The interaction of water with MOF-5 simulated by molecular dynamics

Jeffery A. Greathouse et al.

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Selective oligomerization of glycerol over mesoporous catalysts

J Barrault et al.

TOPICS IN CATALYSIS (2004)

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The structure and electrical conductivity of vacuum-annealed WO3 thin films

M Gillet et al.

THIN SOLID FILMS (2004)

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Article Chemistry, Multidisciplinary

Glycerol hydrogenolysis on heterogeneous catalysts

J Chaminand et al.

GREEN CHEMISTRY (2004)

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Mg-doped WO3 as a novel photocatalyst for visible light-induced water splitting

DW Hwang et al.

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Gelatin microspheres crosslinked with D,L-glyceraldehyde as a potential drug delivery system: preparation, characterisation, in vitro and in vivo studies

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INTERNATIONAL JOURNAL OF PHARMACEUTICS (2001)

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Photoelectrochemical Selective Oxidation of Glycerol to Glyceraldehyde with Bi-Based Metal-Organic-Framework-Decorated WO3 Photoanode

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