期刊
CHEMCATCHEM
卷 7, 期 6, 页码 925-927出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cctc.201403040
关键词
gold; hydrogen peroxide; palladium; selective oxidation; tandem reactions
Alcohol oxidation with 100% selectivity to the aldehyde product (versus acid formation) is achieved at mild conditions by a tandem-type system where the intermediate species of hydrogen peroxide formation from an O-2/H-2 mixture are formed and utilised directly over Au-Pd/Ti-NT catalysts. Insitu reaction of the intermediate species minimises the parallel decomposition of hydrogen peroxide into water, overcoming one of the limitations on the use of hydrogen peroxide as a green oxidant.
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