☆ 4.6 Review

Recent Progress of Metal-Oxide-Based Catalysts for Non-Oxidative Coupling of Methane to Ethane and Hydrogen

CATALYSTS (2023)

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Summary: This study proposes a heteroatom engineering strategy for photocatalytic nonoxidative coupling of methane (NOCM) using Pd single atoms loaded onto TiO2 catalyst. By reducing the contribution of oxygen sites to the valence band with the construction of Pd-O-4 structure, high selectivity for C2H6 production is achieved. The photocatalytic system shows high activity, selectivity, and durability, approaching the level of thermocatalysis under mild conditions.

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