☆ 4.8 Review

Status and Prospects of MXene-Based Lithium-Oxygen Batteries: Theoretical Prediction and Experimental Modulation

ADVANCED ENERGY MATERIALS (2023)

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In situ decoration of CoP/Ti 3 C 2 T x composite as efficient electrocatalyst for Li-oxygen battery

Xingzi Zheng et al.

Summary: This paper introduces a novel Li-O2 battery electrocatalyst, a surface-functionalized CoP/Ti3C2Tx composite. The composite exhibits optimized electronic structure and active electrons, which enhance the efficiency of electrochemical reactions. The accordion shaped Ti3C2Tx with large specific surface area and excellent electronic conductivity enables sufficient exposure of active sites and Li2O2 deposition. Transition metal phosphides provide more active catalytic sites and exhibit good electrocatalytic performance. As an electrocatalyst in Li-O2 battery, the CoP/Ti3C2Tx composite achieves high specific discharge capacity and low overpotential, outperforming CoP and Ti3C2Tx individually. The application of transition metal phosphides and MXene in Li-O2 battery not only demonstrates higher cycling stability of the prepared composite, but also points out the direction for improving their electrochemical performance.

CHINESE CHEMICAL LETTERS (2023)

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Article Materials Science, Multidisciplinary

Self-Catalyzed Rechargeable Lithium-Air Battery by in situ Metal Ion Doping of Discharge Products: A Combined Theoretical and Experimental Study

Mengwei Yuan et al.

Summary: The insulating nature of Li2O2 and the limited activity of solid-solid/-liquid interfaces hinder the performance of lithium-air battery, but in-situ doping of Li2O2 with select metal ions can greatly enhance the battery performance.

ENERGY & ENVIRONMENTAL MATERIALS (2023)

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Article Chemistry, Multidisciplinary

New Conceptual Catalyst on Spatial High-Entropy Alloy Heterostructures for High-Performance Li-O2 Batteries

Peng Zhang et al.

Summary: The researchers successfully constructed a unique high-entropy alloy spatial heterostructure electrocatalyst that enhances the electrocatalytic activity of high-entropy alloy catalysts by manipulating electron distribution and the d-band center of interfacial metal atoms for oxygen reduction and evolution reactions in Li-O-2 batteries. The resulting electrocatalyst exhibited minimal polarization potential and long-term cyclability, surpassing most previously reported noble metal-based catalysts.

SMALL (2023)

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Review Chemistry, Physical

Air-Stable Protective Layers for Lithium Anode Achieving Safe Lithium Metal Batteries

Runjing Li et al.

Summary: This review discusses the application of lithium metal as a promising anode material in lithium metal batteries, as well as the corrosion and safety hazards of lithium metal in air. It proposes the solution of constructing stable air-stable protective layers and summarizes the current research progress and development prospects.

SMALL METHODS (2023)

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Article Chemistry, Multidisciplinary

Bimetal Organic Framework-Ti3C2Tx MXene with Metalloporphyrin Electrocatalyst for Lithium-Oxygen Batteries

Sanghee Nam et al.

Summary: This study reports a new method of growing bimetallic cobalt-manganese organic framework on the MXene surface, which achieves high stability in open structured applications by enhancing oxidation resistance and electrocatalytic properties.

ADVANCED FUNCTIONAL MATERIALS (2023)

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Article Chemistry, Multidisciplinary

Highly Stable Garnet Fe2Mo3O12 Cathode Boosts the Lithium-Air Battery Performance Featuring a Polyhedral Framework and Cationic Vacancy Concentrated Surface

Yang Qiu et al.

Summary: This article reports a highly active Fe2Mo3O12 (FeMoO) garnet cathode catalyst for lithium-air batteries (LABs) with high energy density. The experimental and theoretical analysis demonstrates that the catalyst has highly effective air catalytic activity and long-term stability while maintaining good structural stability. The catalyst delivers a cycle life of over 1800 h under a simple half-sealed condition in ambient air.

ADVANCED SCIENCE (2023)

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Article Engineering, Environmental

Tailoring mixed geometrical configurations in amorphous catalysts to activate oxygen electrode reactions of lithium-oxygen batteries

Runjing Li et al.

Summary: Constructing well-designed catalysts by manipulating geometrical and electrical structures is an effective strategy for high-performance lithium-oxygen chemistry. However, achieving high activity and stability in catalysts simultaneously is challenging. In this study, researchers constructed an amorphous oxide/hydroxide with mixed geometrical configurations, which exhibited good catalytic activity and excellent stability. The catalyst's disordered structure provided numerous active sites and facilitated electron transport, resulting in enhanced oxygen evolution reaction and oxygen reduction reaction. The introduction of certain metal ions further improved the catalytic performance by reducing reaction paths and inducing strong electrostatic interactions. The catalyst demonstrated high specific discharge capacity and cycling stability in lithium-oxygen batteries.

CHEMICAL ENGINEERING JOURNAL (2023)

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Article Chemistry, Multidisciplinary

Theoretical Design and Structural Modulation of a Surface-Functionalized Ti3C2Tx MXene-Based Heterojunction Electrocatalyst for a Li-Oxygen Battery

Xingzi Zheng et al.

Summary: A surface-functionalized nitrogen-doped two-dimensional N-TiO2/Ti3C2Tx heterojunction with high conductivity and optimized electrocatalytic active sites was fabricated. It exhibited high specific capacity and superior cyclability in Li-oxygen batteries, along with reduced overpotential. Through experiments and tests, its high stability and reduced side reaction were verified.

ACS NANO (2022)

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Uniformly distributed reaction by 3D host-lithium composite anode for high rate capability and reversibility of Li-O2 batteries

Min-Gi Jeong et al.

Summary: This study utilized a 3D porous Cu scaffold as a conductive host in Li-O-2 batteries to optimize the composite anode structure, and quantitatively investigated the influences of HLC on Li2O2 formation and decomposition, which provides a theoretical basis for improving the rate capability and reversibility of the batteries.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Materials Science, Multidisciplinary

First-principle study on catalytic activity of functionalized Ti3C2 MXene as cathode catalyst for Li-O2 batteries

Yingying Yang et al.

Summary: In this study, the catalytic activity of Ti3C2 MXene in Li-O-2 batteries was investigated using theoretical calculations. It was found that Ti3C2 MXene with O-terminated groups showed better performance and potential in catalyzing ORR and OER. This research provides guidance for accelerating ORR and OER reactions in Li-O-2 batteries.

CURRENT APPLIED PHYSICS (2022)

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Tuning the oxygen vacancy of mixed multiple oxidation states nanowires for improving Li-air battery performance

Mengwei Yuan et al.

Summary: By tuning the surface oxygen vacancies of CoMoO4 nanowires, highly efficient electrocatalysts were designed to improve the performance of Li-air batteries, enhancing oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) activities.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2022)

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Nonvolatile and Nonflammable Sulfolane-Based Electrolyte Achieving Effective and Safe Operation of the Li-O2 Battery in Open O2 Environment

Zhengang Li et al.

Summary: This paper reports for the first time a highly electrochemical reversible Li-O-2 battery operated in an open O-2 environment. By using a nonvolatile and nonflammable solvent, the limitation of electrolyte for open O-2 environment is addressed. The stable solid electrolyte interface and reversible O-2 generation were achieved through the tuning of electrolyte composition.

NANO LETTERS (2022)

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Long-cycling lithium-oxygen batteries enabled by tailoring Li nucleation and deposition via lithiophilic oxygen vacancy in Vo-TiO2/Ti3C2Tx composite anodes

Yu Yan et al.

Summary: The study presents a composite anode with oxygen vacancy-rich TiO2 nanoparticles uniformly dispersed on Ti3C2Tx, which effectively guides and modulates lithium growth behavior, leading to improved performance in lithium-oxygen batteries.

JOURNAL OF ENERGY CHEMISTRY (2022)

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High areal capacity, long cycle life 4 V ceramic all-solid-state Li-ion batteries enabled by chloride solid electrolytes

Laidong Zhou et al.

Summary: A series of new lithium mixed-metal chlorospinels are reported as solid electrolytes for all-solid-state lithium batteries, which exhibit high ionic conductivity and low electronic conductivity, showing potential for high-performance all-solid-state lithium batteries.

NATURE ENERGY (2022)

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Review Electrochemistry

Recent Progress in MXene-Based Materials for Metal-Sulfur and Metal-Air Batteries: Potential High-Performance Electrodes

Anmin Liu et al.

Summary: MXenes, as an impressive family of two-dimensional transition metal carbides/carbonitrides, show great potential for energy storage due to their ideal specific surface area, excellent electrical conductivity, and superior chemical durability in batteries.

ELECTROCHEMICAL ENERGY REVIEWS (2022)

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The controllable construction of nanochannel in two-dimensional lamellar film for efficient oxygen reduction reaction and lithium-oxygen batteries

Weixin Zhang et al.

Summary: In this study, a flexible Co-MOF/MXene hybrid film was prepared by inserting two-dimensional Co-MOF nanosheets for efficient Oxygen reduction reaction in Li-O2 batteries, showing high capacity, excellent cycle stability, and outstanding rate performance. Moreover, the capacity and cycle performance of Li-O2 batteries can be controlled by adjusting the loading of 2D Co-MOF and the thickness of Co-MOF/MXene hybrid film.

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Ultrathin Two-Dimensional Bimetal-Organic FrameworkNanosheets as High-Performance Electrocatalysts for Benzyl Alcohol Oxidation

Yujing Song et al.

Summary: Ultrathin two-dimensional metal-organic frameworks (2DMOFs) synthesized through a moderate solvothermal method, with NiCo-61-MOF/NF as the main catalyst, achieved high-efficiency electrocatalysts for the oxidation of benzyl alcohol.

INORGANIC CHEMISTRY (2022)

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Crystal Phase Conversion on Cobalt Oxide: Stable Adsorption toward LiO2 for Film-Like Discharge Products Generation in Li-O2 Battery

Shuting Zhang et al.

Summary: By regulating the crystallization process of cobalt oxide, the reaction mechanism of Li-O-2 batteries can be controlled, leading to improved battery performance. This work provides an important method for tuning the intermediate and constructing high-performance battery systems.

SMALL (2022)

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Article Chemistry, Physical

2D SnSe Cathode Catalyst Featuring an Efficient Facet-Dependent Selective Li2O2 Growth/Decomposition for Li-Oxygen Batteries

Guoliang Zhang et al.

Summary: 2D materials with layered structure, unique electronic properties, and high stability have attracted much attention in the field of cathode catalysts for lithium-oxygen batteries (LOBs). In this study, tin selenide nanosheets with a black phosphorus-like 2D structure were synthesized and used as the cathode catalyst for LOBs. The exposed stack (200) facets and stack edge facets of SnSe nanosheets exhibited superior specific capacity and ultralong cycle stability in LOBs. Experimental and theoretical studies revealed that the 2D surface facets promoted the formation and stabilization of discharge products through the confined adsorption of Li2O2, leading to efficient formation/decomposition of discharge products.

ADVANCED ENERGY MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Composite NiCo2O4@CeO2 Microsphere as Cathode Catalyst for High-Performance Lithium-Oxygen Battery

Yuanhui Wu et al.

Summary: A composite microsphere material composed of NiCo2O4@CeO2 is synthesized and used as an electrocatalyst for lithium-oxygen batteries (LOBs) to address the challenges of high overpotential and poor cycle stability. The unique microstructured catalyst provides sufficient catalytic surface for barrier-free oxygen and lithium ion transport. The introduction of CeO2 increases oxygen vacancies and optimizes the electronic structure of NiCo2O4, thereby enhancing electron transport in the electrode. The catalytic cathode material reduces overpotential to 1.07 V and exhibits stable cycling performance.

ADVANCED SCIENCE (2022)

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Cationic vanadium vacancy-enriched V2-xO5 on V2C MXene as superior bifunctional electrocatalysts for Li-O2 batteries

Haoyang Xu et al.

Summary: This study investigates the bifunctional catalytic activity of V2-xO5@V2C MXene on the oxygen electrode reaction in Li-O-2 batteries. The results demonstrate excellent performance of the V2-xO5@V2C MXene-based Li-O-2 battery, with high energy efficiency and over 500 cycles of excellent cycling performance. Density functional theory calculations confirm that cationic vanadium vacancies can enhance the electrocatalytic activity of transition metal oxides by providing abundant active sites and optimizing reactant adsorption.

SCIENCE CHINA-MATERIALS (2022)

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V 2 C MXene enriched with -O termination as high-efficiency electrocatalyst for lithium-oxygen battery

Haoyang Xu et al.

Summary: This study finds that by regulating the surface functional groups of MXene, the electrocatalytic activity of MXene towards oxygen redox reactions in Li-O2 batteries can be enhanced, thereby improving the energy efficiency and stability of the batteries.

APPLIED MATERIALS TODAY (2022)

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Electronic Bridge Construction via Ag Intercalation to Diminish Catalytic Anisotropy for 2D Tin Diselenide Cathode Catalyst in Lithium-Oxygen Batteries

Guoliang Zhang et al.

Summary: This study proposes an ion-intercalation strategy to diminish the catalytic anisotropy of 2D materials for better lithium-oxygen battery performance. The results demonstrate that intercalated Ag ions can regulate the electronic states between stack edge planes, significantly enhancing the catalytic capability of 2D materials. It can efficiently accelerate charge transfer and suppress passivation during the oxygen reduction/evolution reaction process.

ADVANCED ENERGY MATERIALS (2022)

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Nb2CTx MXene Cathode for High-Capacity Rechargeable Aluminum Batteries with Prolonged Cycle Lifetime

Xingjun Liu et al.

Summary: This study demonstrates that rechargeable aluminum batteries with 2D Nb2CTx MXene as a cathode material exhibit excellent capacity and long cyclic performance. After proper treatment, aluminum batteries embedded with calcined Nb2CTx MXene cathodes retain high capacity and significantly extended cyclic lifetime. The controllable d-spacing of Nb2CTx nanosheets promotes ion migration, leading to enhanced charge storage. The formation of niobium oxides and amorphous carbon after calcination benefits the electrochemical performance of Nb2CTx MXene electrode in aluminum batteries.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Review Chemistry, Physical

Ion Transport Kinetics in Low-Temperature Lithium Metal Batteries

Anjun Hu et al.

Summary: This review systematically reviews and discusses the critical limiting factors and challenges for low-temperature ion transport behaviors, and comprehensively summarizes the strategies to enhance Li+ transport kinetics. Finally, perspectives on future research directions of low-temperature LMBs towards practical applications are proposed.

ADVANCED ENERGY MATERIALS (2022)

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Highly efficient two-dimensional Ag2Te cathode catalyst featuring a layer structure derived catalytic anisotropy in lithium-oxygen batteries

Liang Guo et al.

Summary: In this study, chemically bonded silver telluride nanowires were used as a highly efficient catalyst for lithium-oxygen batteries (LOBs), exhibiting outstanding performance and stability. Experimental and computational results revealed the superior catalytic activity and weak structure-derived catalytic anisotropy of the two-dimensional layer structure of silver telluride in LOBs.

ENERGY STORAGE MATERIALS (2022)

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Review Chemistry, Physical

Recent Advances in Titanium Carbide MXene (Ti3C2TX) Cathode Material for Lithium-Air Battery

Samra Asad et al.

Summary: As fossil fuels are becoming depleted, the world is shifting towards renewable energy sources and energy storage technologies. Metal-air batteries, specifically lithium-air batteries, are gaining attention due to their high energy density. MXenes, with their high electrical conductivity and catalytic activity, have emerged as promising materials for energy storage applications.

ACS APPLIED ENERGY MATERIALS (2022)

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Article Chemistry, Physical

Stacking surface derived catalytic capability and by-product prevention for high efficient two dimensional Bi2Te3 cathode catalyst in Li-oxygen batteries

Juanjuan Feng et al.

Summary: In this study, the catalytic performance of 2D structured Bi2Te3 in Li-oxygen batteries was investigated. The stack surface (001) plane of Bi2Te3 was found to provide outstanding catalytic capability and high conductivity, leading to high specific capacity and cycling stability.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Review Chemistry, Multidisciplinary

Evolving aprotic Li-air batteries

Zhenzhen Wu et al.

Summary: Lithium-air batteries have attracted significant attention due to their high energy density and renewable features. However, the lack of critical electrode materials and a thorough understanding of the chemistry has hindered their development. Recent research has focused on systematic electrode design, fabrication, and modification, as well as comprehensive electrolyte selection. Future development requires further exploration and optimization.

CHEMICAL SOCIETY REVIEWS (2022)

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Article Chemistry, Physical

Accelerating the reaction kinetics of lithium-oxygen chemistry by modulating electron acceptance-donation interaction in electrocatalysts

Chuan Zhao et al.

Summary: This study demonstrates the improved performance of lithium-oxygen batteries by using Co-doped Zn-based zeolite imidazole framework nanosheets as catalysts. The incorporation of Co allows for the regulation of electronic structure and the formation of unique product morphology, resulting in efficient mass and charge transfer.

JOURNAL OF MATERIALS CHEMISTRY A (2022)

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Article Chemistry, Multidisciplinary

Mildly Oxidized MXene (Ti3C2, Nb2C, and V2C) Electrocatalyst via a Generic Strategy Enables Longevous Li-O2 Battery under a High Rate

Yongxiang Jiang et al.

Summary: This study presents a universal synthesis approach to fabricate mildly oxidized MXenes as cathode catalysts for Lithium-oxygen batteries (LOBs), achieving high specific capacity and long lifespan. The mo-V2CTx shows excellent electrocatalytic performance and stability, operating continuously for 90 cycles under a high current density.

ACS NANO (2021)

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Article Chemistry, Multidisciplinary

Halogenated Ti3C2 MXenes with Electrochemically Active Terminals for High-Performance Zinc Ion Batteries

Mian Li et al.

Summary: Experimental exploration of various halogen terminals on the surface of Ti3C2 MXenes showed that the presence of Br and I elements resulted in improved electrochemical performance for aqueous zinc ion batteries. The Lewis-acidic-melt etching route proved to be effective in tuning the surface chemistry of MXenes for expanding their potential applications.

ACS NANO (2021)

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Article Chemistry, Multidisciplinary

Ambient-Stable Two-Dimensional Titanium Carbide (MXene) Enabled by Iodine Etching

Huanhuan Shi et al.

Summary: The study demonstrated a fluoride-free, iodine-assisted etching route for preparing oxygen-rich two-dimensional MXene with intact lattice structure. These MXene sheets exhibit excellent thin-film conductivity and great ambient stability in water, showing promise for practical applications.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Halogen Etch of Ti3AlC2 MAX Phase for MXene Fabrication

Ali Jawaid et al.

Summary: A new room-temperature etching method using halogens in anhydrous media can synthesize MXenes from Ti3AlC2, providing opportunities for controlled surface chemistries to modulate MXene properties. The radical-mediated process strongly depends on various factors, such as the molar ratio of halogen to MAX phase, concentration of halogen, solvent, and temperature.

ACS NANO (2021)

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Article Chemistry, Multidisciplinary

Ultrafast, One-Step, Salt-Solution-Based Acoustic Synthesis of Ti3C2 MXene

Ahmed El Ghazaly et al.

Summary: This study presents a one-step synthesis method for the conversion from Ti3AlC2 MAX to Ti3C2Tz MXene on the order of milliseconds, facilitated by the combination of protons and fluorine ions to selectively etch the MAX phase. The results demonstrate that flexible electrodes fabricated using this method exhibit comparable electrochemical performance to previously reported ones.

ACS NANO (2021)

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Editorial Material Chemistry, Physical

Polarized nucleation and efficient decomposition of Li2O2 for Ti2C MXene cathode catalyst under a mixed surface condition in lithium-oxygen batteries

Jiajia Li et al.

ENERGY STORAGE MATERIALS (2021)

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Article Chemistry, Physical

Surface defect engineering of metal oxides photocatalyst for energy application and water treatment

Pankaj Raizada et al.

Summary: Despite the excellent characteristics of metal oxides in photocatalysis, they often suffer from charge carrier recombination and limited visible response, leading to reduced photocatalytic output. This study provides a comprehensive overview of recent developments in classifying metal oxide defects based on host crystal lattice dimensions, focusing on surface modifications through various types of defects and their impacts on photocatalytic performance. By modifying the morphology and electronic structure of metal oxide photocatalysts through defect engineering, their activity can be significantly improved for applications such as H-2 evolution, CO2 reduction, pollutant degradation, and bacterial disinfection.

JOURNAL OF MATERIOMICS (2021)

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Article Chemistry, Multidisciplinary

Carbon-Reinforced Nb2CTx MXene/MoS2 Nanosheets as a Superior Rate and High-Capacity Anode for Sodium-Ion Batteries

Zeyu Yuan et al.

Summary: The development of sodium-ion battery anode materials with excellent performance has improved cycling stability and rate capabilities, potentially expanding the practical applications of sodium-ion batteries.

ACS NANO (2021)

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Article Chemistry, Multidisciplinary

Single Semi-Metallic Selenium Atoms on Ti3C2 MXene Nanosheets as Excellent Cathode for Lithium-Oxygen Batteries

Danyang Zhao et al.

Summary: A CO2-assisted thermal-reaction strategy was developed to fabricate isolated semi-metallic selenium single-atom-doped Ti3C2 MXene catalysts for high-performance Li-O-2 batteries, significantly enhancing the oxygen reduction kinetics, improving overpotentials, and promoting the absorption ability of lithium peroxide, leading to improved redox kinetics and reduced overpotentials.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Reversed Charge Transfer and Enhanced Hydrogen Spillover in Platinum Nanoclusters Anchored on Titanium Oxide with Rich Oxygen Vacancies Boost Hydrogen Evolution Reaction

Zhen-Wei Wei et al.

Summary: The study demonstrates that Pt nanoclusters supported on porous TiO2 nanosheets with rich oxygen vacancies exhibit significantly higher catalytic activity for the HER compared to those supported on TiO2 with deficient oxygen vacancies. This is attributed to the ability of the TiO2 support with rich oxygen vacancies to facilitate reversed charge transfer and enhanced hydrogen spillover, promoting proton reduction and hydrogen desorption at Pt catalytic sites. This work provides a new strategy for the rational design of highly efficient HER catalysts.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

MnCo2S4-CoS1.097 Heterostructure Nanotubes as High Efficiency Cathode Catalysts for Stable and Long-Life Lithium-Oxygen Batteries Under High Current Conditions

Qing Xia et al.

Summary: Constructing heterostructures is an effective method to improve the electrical conductivity and electrocatalytic properties of metal sulfide catalysts. In this study, MnCo2S4-CoS1.097 nanotubes were successfully prepared and demonstrated high specific capacities and good cycling stability under high current conditions. The superior electrochemical performance is attributed to fast ion and electron transmission, multiple active sites, and the nanotube architecture with large specific surface area.

ADVANCED SCIENCE (2021)

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Article Chemistry, Physical

Research progress of MXene-based catalysts for electrochemical water-splitting and metal-air batteries

Jingyuan Qiao et al.

Summary: MXenes, a rising family of 2D materials, show great potential in electrocatalysis due to their unique combination of properties such as high electrical conductivities and adjustable surface properties. This review summarizes the preparation methods, properties, and applications of MXenes in important reactions like HER, OER, and ORR. Strategies for improving their performance and discussing the challenges and prospects in the field are also highlighted.

ENERGY STORAGE MATERIALS (2021)

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Article Chemistry, Physical

A-site cationic defects induced electronic structure regulation of LaMnO3 perovskite boosts oxygen electrode reactions in aprotic lithium-oxygen batteries

Dayue Du et al.

Summary: This study presents a facile strategy to fabricate LaMnO3-δ perovskite with abundant defects, which exhibits superior electrocatalytic performance in Li-O-2 batteries by modulating the local coordination state of active Mn atoms and optimizing the electronic structure. The abundant crystal defects not only enhance the covalency of Mn-O bonds but also promote lattice oxygen participated redox reaction, accelerating electron transport and regulating Li2O2 formation and decomposition mechanism.

ENERGY STORAGE MATERIALS (2021)

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Article Multidisciplinary Sciences

A highly stable and flexible zeolite electrolyte solid-state Li-air battery

Xiwen Chi et al.

Summary: Solid-state lithium-air batteries with integrated ultrathin, high-ion-conductive zeolite X membrane as the sole solid electrolyte exhibit excellent electrochemical performance, flexibility, and stability. These batteries have a high capacity and cycle life, outperforming batteries based on other materials under the same conditions, and show potential for practical applicability in various energy-storage systems.

NATURE (2021)

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Article Chemistry, Physical

MoSe2@CNT Core-Shell Nanostructures as Grain Promoters Featuring a Direct Li2O2 Formation/Decomposition Catalytic Capability in Lithium-Oxygen Batteries

Biao He et al.

Summary: This study investigates the use of MoSe2@CNT to improve the performance of lithium-oxygen batteries, with the MoSe2 layers acting as grain promoters and preventing the formation of byproducts. The cathode demonstrated superior specific capacity, excellent rate capabilities, and long cycle life.

ADVANCED ENERGY MATERIALS (2021)

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Article Nanoscience & Nanotechnology

Suppressing Redox Shuttle with MXene-Modified Separators for Li-O2 Batteries

Lei Shi et al.

Summary: A chemical binding strategy based on a MXene-modified separator with a 3D porous hierarchical structure has been developed to suppress the I-3(-) shuttling in LiI-involved Li-O-2 battery. The abundant -OH terminal groups on the MXene surface act as effective binding sites for suppressing the migration of I-3(-), while the 3D porous structure ensures fast transfer of lithium ions, resulting in improved battery performance.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Rational Design of Highly Stable and Active MXene-Based Bifunctional ORR/OER Double-Atom Catalysts

Bo Wei et al.

Summary: Designing highly active and bifunctional oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) catalysts with non-noble metals such as Fe/Co/Ni on MXene surfaces has shown superior performance compared to traditional unifunctional catalysts, providing a novel pathway for tunable catalytic behavior in MXenes. The electronic structure analyses revealed that the excellent catalytic activities in MXene-based DACs are attributed to the electron-capturing capability and synergistic interactions between Fe/Co/Ni adsorbents and MXene substrate. These findings not only suggest promising candidates for MXene-based bifunctional ORR/OER catalysts but also offer new theoretical insights into rationally designing noble-metal-free bifunctional DACs.

ADVANCED MATERIALS (2021)

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Review Chemistry, Multidisciplinary

Advances in the Synthesis of 2D MXenes

Yi Wei et al.

Summary: MXenes, versatile materials with adjustable structures and rich surface chemistry, have been recognized as potential 2D materials for various applications. Recent research has focused on synthetic routes, etching methods, and delamination strategies for large-scale preparation and stable storage. Antioxidation strategies for MXenes have also been summarized for future developments and practical applications.

ADVANCED MATERIALS (2021)

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Editorial Material Materials Science, Ceramics

A decade of discovery: A review of MXenes, the family of 2D transition metal carbides and nitrides

Yury Gogotsi

AMERICAN CERAMIC SOCIETY BULLETIN (2021)

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Bifunctional Catalytic Activity Guided by Rich Crystal Defects in Ti3C2 MXene Quantum Dot Clusters for Li-O2 Batteries

Peng Wang et al.

Summary: The study demonstrates that the Ti3C2 QDC/N-C material, with abundant crystal defects and well-defined grain boundaries and edge defects, enhances catalytic activity and cycling stability for lithium-oxygen batteries. Furthermore, density functional theory calculations reveal the significant role of crystal defects in catalytic centers.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Physical

Unique intermediate adsorption enabled by anion vacancies in metal sulfide embedded MXene nanosheets overcoming kinetic barriers of oxygen electrode reactions in lithium-oxygen batteries

Ruixin Zheng et al.

Summary: Designing electrode materials with sulfur vacancy-rich Ni3S2 on two-dimensional MXene as a bifunctional catalyst for lithium-oxygen batteries (LOBs) significantly reduces overpotentials, improves long-term cyclic stability, and modifies the deposition mechanism of Li2O2 by exposing coordination unsaturated sites on the surface.

ENERGY STORAGE MATERIALS (2021)

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Review Chemistry, Physical

Defective Structures in Metal Compounds for Energy-Related Electrocatalysis

Xuecheng Yan et al.

Summary: This article focuses on the manipulation of electronic structures and surface properties of electrocatalysts, as well as the introduction of defects to enhance their activity. It summarizes the commonly used methods for creating anion and cation vacancies, and emphasizes the control of defect density and filling heteroatoms to improve catalytic performance.

SMALL STRUCTURES (2021)

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Review Multidisciplinary Sciences

The world of two-dimensional carbides and nitrides (MXenes)

Armin Vahid Mohammadi et al.

Summary: MXenes, a family of two-dimensional materials, have diverse properties and wide-ranging applications in areas such as optics, catalysis, sensing, and medicine. Future research directions will focus on deepening the fundamental understanding of MXenes properties and exploring their potential for hybridization with other 2D materials.

SCIENCE (2021)

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Article Chemistry, Multidisciplinary

An artificial hybrid interphase for an ultrahigh-rate and practical lithium metal anode

Anjun Hu et al.

Summary: An artificial hybrid SEI layer composed of lithium-antimony alloy and lithium fluoride was constructed to reduce electron tunneling between the Li anode and SEI, resulting in uniform Li deposition and stable Li plating/stripping behaviors at an ultrahigh rate. This work uncovers the internal mechanism of Li+ transport within the SEI component, providing a pathway to stabilize the Li anode under practical high-rate conditions.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Highly Efficient Nb2C MXene Cathode Catalyst with Uniform O-Terminated Surface for Lithium-Oxygen Batteries

Gaoyang Li et al.

Summary: The study demonstrates the catalytic capability of Nb2C MXene as a cathode material for LOBs, highlighting its superior electrocatalytic performance and high-rate cycle stability.

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Nanostructured Ni/Ti3C2Tx MXene hybrid as cathode for lithium-oxygen battery

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Iron doped CoP nanowires on carbon cloth: An efficient and stable electrocatalyst for Li-O2 battery

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Single Zinc Atoms Immobilized on MXene (Ti3C2Clx) Layers toward Dendrite-Free Lithium Metal Anodes

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Heterostructured NiS2/ZnIn2S4 Realizing Toroid-like Li2O2 Deposition in Lithium-Oxygen Batteries with Low-Donor-Number Solvents

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Scalable Synthesis of Ti3C2Tx MXene

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Recent Advances of Two-Dimensional (2 D) MXenes and Phosphorene for High-Performance Rechargeable Batteries

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Nickel oxide nanoparticles decorated highly conductive Ti3C2 MXene as cathode catalyst for rechargeable Li-O2 battery

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Spontaneous Atomic Ruthenium Doping in Mo2CTX MXene Defects Enhances Electrocatalytic Activity for the Nitrogen Reduction Reaction

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A general Lewis acidic etching route for preparing MXenes with enhanced electrochemical performance in non-aqueous electrolyte

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3D MXene Architectures for Efficient Energy Storage and Conversion

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In situ decoration of nanosized metal oxide on highly conductive MXene nanosheets as efficient catalyst for Li -O 2 battery

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Excellent electrolyte-electrode interface stability enabled by inhibition of anion mobility in hybrid gel polymer electrolyte based Li-O2 batteries

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Check Interfacial electronic structure design of MXene-based electrocatalyst via vacancy modulation for lithium -oxygen battery

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Challenges and Strategy on Parasitic Reaction for High-Performance Nonaqueous Lithium-Oxygen Batteries

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Highly Reversible O2Conversions by Coupling LiO2Intermediate through a Dual-Site Catalyst in Li-O2Batteries

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Recent Advances in Nanostructured Transition Metal Carbide- and Nitride-Based Cathode Electrocatalysts for Li-O2 Batteries (LOBs): A Brief Review

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Metal-defected spinel MnxCo3-xO4 with octahedral Mn-enriched surface for highly efficient oxygen reduction reaction

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Theoretical Prediction of Catalytic Activity of Ti2C MXene as Cathode for Li-O2 Batteries

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Interfacial Super-Assembled Porous CeO2/C Frameworks Featuring Efficient and Sensitive Decomposing Li2O2 for Smart Li-O2 Batteries

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Ni(OH)2 Nanoflakes Supported on 3D Ni3Se2 Nanowire Array as Highly Efficient Electrodes for Asymmetric Supercapacitor and Ni/MH Battery

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Ultrathin Two-Dimensional Metal Organic Framework Nanosheets with the Inherent Open Active Sites as Electrocatalysts in Aprotic Li-O2 Batteries

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Prediction of Synthesis of 2D Metal Carbides and Nitrides (MXenes) and Their Precursors with Positive and Unlabeled Machine Learning

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Metal-organic frameworks and their derivatives for metal-air batteries

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Perovskite La0.5Sr0.5CoO3-δ Grown on Ti3C2Tx MXene Nanosheets as Bifunctional Efficient Hybrid Catalysts for Li-Oxygen Batteries

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Single-Crystalline Ultrathin Co3O4 Nanosheets with Massive Vacancy Defects for Enhanced Electrocatalysis

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Holey 2D Nanosheets of Low-Valent Manganese Oxides with an Excellent Oxygen Catalytic Activity and a High Functionality as a Catalyst for Li-O-2 Batteries

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Atomic Cobalt Covalently Engineered Interlayers for Superior Lithium-Ion Storage

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W-Based Atomic Laminates and Their 2D Derivative W1.33C MXene with Vacancy Ordering

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Preferential Cation Vacancies in Perovskite Hydroxide for the Oxygen Evolution Reaction

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Porous Co3O4 nanorods anchored on graphene nanosheets as an effective electrocatalysts for aprotic Li-O-2 batteries

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Exploring MXenes as Cathodes for Non-Aqueous Lithium-Oxygen Batteries: Design Rules for Selectively Nucleating Li2O2

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Uniform FexNiy Nanospheres: Cost-Effective Electrocatalysts for Nonaqueous Rechargeable Li-O2` Batteries

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Two-Dimensional Molybdenum Carbide (MXene) as an Efficient Electrocatalyst for Hydrogen Evolution

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Large-scale delamination of multi-layers transition metal carbides and carbonitrides MXenes

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A review of cathode materials and structures for rechargeable lithium-air batteries

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Advanced hydrogen storage alloys for Ni/MH rechargeable batteries

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