Tendency Regulation of Competing Reactions Toward Highly Reversible Tin Anode for Aqueous Alkaline Batteries

Article Chemistry, Physical

A dendrite-free Ga-In-Sn-Zn solid-liquid composite anode for rechargeable zinc batteries

Wei Wang et al.

Summary: By using the Ga-In-Sn-Zn solid-liquid composite (SLC) to construct the SLC-2 electrode, stable and dendrite-free zinc deposition can be achieved, improving the cycle stability of zinc batteries.

ENERGY STORAGE MATERIALS (2023)

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Article Chemistry, Multidisciplinary

Sn Alloying to Inhibit Hydrogen Evolution of Zn Metal Anode in Rechargeable Aqueous Batteries

Luyao Wang et al.

Summary: Alloying with Sn is an effective strategy to inhibit hydrogen evolution and dendrite growth of Zn metal anodes in rechargeable aqueous batteries. In-situ monitoring shows that Sn alloy electrodes have significantly lower hydrogen evolution compared to pure Zn electrodes, while also providing favorable Zn nucleation sites for more uniform Zn deposition. The Zn-Sn alloy electrodes demonstrate improved cycling performance in terms of plating/stripping cycles and depth of discharge, making them a practical solution for stabilizing Zn metal electrodes in rechargeable aqueous batteries.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Regulating Interfacial Desolvation and Deposition Kinetics Enables Durable Zn Anodes with Ultrahigh Utilization of 80%

Hongrun Jin et al.

Summary: This study introduces an aluminum-doped zinc oxide (AZO) interphase to improve the cycling stability and utilization of zinc anodes in aqueous zinc ion batteries (ZIBs), showing promising durability and stability in the AZO-coated zinc (AZO@Zn) anode. The V2O5/AZO@Zn full cell exhibits high capacity retention at high rates.

SMALL (2022)

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Article Green & Sustainable Science & Technology

A non-flammable hydrous organic electrolyte for sustainable zinc batteries

Daliang Han et al.

Summary: Aqueous zinc batteries are safer than lithium-ion batteries, but their anodes are susceptible to dendrite failure and side reactions. The authors demonstrate a low-cost electrolyte that involves hydrate salt and organic solvent, proving to be non-flammable. The zinc battery cell delivers excellent performance even at low temperatures of -30 degrees Celsius.

NATURE SUSTAINABILITY (2022)

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Article Chemistry, Multidisciplinary

Intrinsic Carbon Defects Induced Reversible Antimony Chemistry for High-Energy Aqueous Alkaline Batteries

Fuxin Wang et al.

Summary: This study designs a new defect-modified carbon skeleton (D-CS) for developing high-capacity, dendrite-free, and stable anode materials for aqueous alkaline batteries (AABs). The Sb/D-CS electrode demonstrates excellent reversibility and cycling stability at practical capacity and high depth of discharge. Furthermore, the electrode remains stable even under high-capacity operation.

ADVANCED MATERIALS (2022)

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Article Chemistry, Physical

A simple way to induce anode-electrolyte interface engineering through a functional composite separator for zinc-nickel batteries

Zequan Zhao et al.

Summary: By developing a solid-state functionalized composite (FC) separator, the anode-electrolyte interface characteristics of Zn-Ni batteries can be regulated to improve their performance and cycling life. The addition of PAAK helps mitigate hydrogen evolution reaction and improve water retention ability, while reducing the negative effects of oxygen from cathodes. The results demonstrate the large potentials of this new generation of Zn-Ni batteries.

NANO ENERGY (2022)

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Editorial Material Green & Sustainable Science & Technology

Charging sustainable batteries comment

Christian Bauer et al.

Summary: Rechargeable batteries are expected to experience exponential growth in the next decade, thanks to the wider adoption of electric vehicles. An international expert panel has proposed a feasible pathway towards sustainable batteries, emphasizing the importance of vision, innovation, and practice.

NATURE SUSTAINABILITY (2022)

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Article Materials Science, Multidisciplinary

Promoting ion adsorption and desolvation kinetics enables high capacity and rate capability of stibium anode for advanced alkaline battery

Peng Zhang et al.

Summary: This study demonstrates the construction of a nitrogen doped carbon cages (NCCs) substrate for high capacity and rate capability anode using antimony (Sb) metal. By enhancing the adsorption and desolvation process of [Sb(OH) 4 ] ??? via increased attraction toward (OH) ???, the Sb/NCCs anode exhibits high capacity, outstanding coulombic efficiency, and impressive lifespan.

JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY (2022)

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Article Chemistry, Multidisciplinary

Hierarchical Heterostructure Engineering of Layered Double Hydroxides on Nickel Sulfides Heteronanowire Arrays as Efficient Cathode for Alkaline Aqueous Zinc Batteries

Kai Zhou et al.

Summary: This study successfully develops self-supported hierarchical heterostructure composites for nickel-zinc batteries, which greatly improves the capacity and cycle stability. The electrode structure provides abundant reactive sites, rapid ion diffusion channels, and fast electron transfer routes, as well as strong structural stability. Additionally, the strong interfacial charge transfer effectively modifies the electronic structure of the composites, improving the reaction kinetics. The fabricated battery exhibits superior capacity, energy density, power density, and cycling performance.

SMALL (2022)

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Article Chemistry, Multidisciplinary

Triple-Function Electrolyte Regulation toward Advanced Aqueous Zn-Ion Batteries

Junnan Hao et al.

Summary: This study reveals the challenges in aqueous Zn-ion batteries and proposes a new electrolyte strategy to address these issues. Experimental results demonstrate that the strategy can achieve high reversibility and long lifespan for Zn-ion batteries.

ADVANCED MATERIALS (2022)

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Article Nanoscience & Nanotechnology

Root Reason for the Failure of a Practical Zn-Ni Battery: Shape Changing Caused by Uneven Current Distribution and Zn Dissolution

Yuanhao Shen et al.

Summary: Despite the excellent rate performance and environmental friendliness, poor cycling life of aqueous Zn-Ni batteries is mainly attributed to the shape changing of the Zn anode resulting from uneven current distribution and the dissolution of Zn.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Multidisciplinary Sciences

Oxygen-rich interface enables reversible stibium stripping/plating chemistry in aqueous alkaline batteries

Haozhe Zhang et al.

Summary: Aqueous alkaline batteries face challenges due to the unsatisfactory performance of anode materials, but a promising Sb metal anode with fast reaction kinetics and favorable stability is demonstrated through an oxygen-rich interface induced reversible Sb stripping/plating chemistry.

NATURE COMMUNICATIONS (2021)

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Article Chemistry, Physical

Water Invoking Interface Corrosion: An Energy Density Booster for Ni//Zn Battery

Weidong He et al.

Summary: A significant increase in electrode capacity was achieved by manipulating bimetallic sulfide nanointerfaces via water invoking interface corrosion, resulting in a breakthrough in Ni//Zn batteries.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Multidisciplinary

A Dendrite-Free Tin Anode for High-Energy Aqueous Redox Flow Batteries

Yanxin Yao et al.

Summary: This study presents an aqueous metal anode based on tin, which effectively addresses the severe dendrite issues in redox flow batteries. Compared to state-of-the-art zinc metal anodes, the alkaline Sn electrode demonstrates superior performance in cycling life and areal capacity.

ADVANCED MATERIALS (2021)

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News Item Multidisciplinary Sciences

MATERIALS SCIENCE Zinc aims to beat lithium batteries at storing energy

Robert F. Service

SCIENCE (2021)

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Article Chemistry, Physical

Multifunctional tin layer enabled long-life and stable anode for aqueous zinc-ion batteries

W. Guo et al.

Summary: The aqueous zinc-ion battery is a promising energy storage system due to its low-cost, non-toxic, and high-safety attributes. However, the zinc anode faces challenges such as corrosion and dendrite growth, hindering practical applications. By coating zinc with tin, reaction reversibility is enhanced, leading to stable low-voltage hysteresis during charging and discharging cycles.

MATERIALS TODAY ENERGY (2021)

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Article Chemistry, Physical

Constructing nano-channeled tin layer on metal zinc for high-performance zinc-ion batteries anode

Zhenyu Miao et al.

Summary: Rechargeable aqueous zinc-ion batteries have been studied extensively due to the unique properties of zinc. The tin-modified zinc anode, Sn-Zn, was developed to address dendrite formation and side reactions, improving battery performance. Multiscale investigation techniques, including micro-CT, were used to study zinc dendrite inhibition and the induction mechanism of zinc by tin.

ECOMAT (2021)

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Article Chemistry, Physical

Fabrication and theoretical investigation of cobaltosic sulfide nanosheets for flexible aqueous Zn/Co batteries

Si-Wen Zhang et al.

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Preparation of promising anode materials with Sn-MOF as precursors for superior lithium and sodium storage

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NATURE ENERGY (2020)

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Stabilization of Sn Anode through Structural Reconstruction of a Cu-Sn Intermetallic Coating Layer

Guanzhi Wang et al.

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Realizing high zinc reversibility in rechargeable batteries

Lin Ma et al.

NATURE ENERGY (2020)

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A scalable top-down strategy toward practical metrics of Ni-Zn aqueous batteries with total energy densities of 165 W h kg-1 and 506 W h L-1

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Multicomponent Hierarchical Cu-Doped NiCo-LDH/CuO Double Arrays for Ultralong-Life Hybrid Fiber Supercapacitor

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Nickel@Nickel Oxide Core-Shell Electrode with Significantly Boosted Reactivity for Ultrahigh-Energy and Stable Aqueous Ni-Zn Battery

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Tendency Regulation of Competing Reactions Toward Highly Reversible Tin Anode for Aqueous Alkaline Batteries

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