4.7 Article

The interfacial stability of single crystal superalloy affected by the phase structure of the Ni-Al coating

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SCRIPTA MATERIALIA
卷 227, 期 -, 页码 -

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PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.scriptamat.2023.115297

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Ni-Al coating; Single crystal superalloy; Interfacial stability; Nudged elastic band calculation

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The interfacial stability between the bond coating and single crystal superalloy substrate is crucial for their long-term performance. Through experiments and atomistic simulations, coatings with various phase structures were designed, and the intrinsic mechanism underlying recrystallization was investigated. Experimental results showed that recrystallization occurred in the specimen with coatings of medium Al content, while there was no secondary reaction zone in the specimen with coatings of the highest Al content. Simulation results demonstrated that a higher energy barrier was required for new grain nucleation in the substrate under beta-NiAl grains. These findings provide a fundamental understanding of interfacial stability and benefit the design of bond coatings for superalloys.
Interfacial stability between the bond coating and single crystal superalloy substrate is crucial for their long-term performance at elevated temperatures. Herein, we designed coatings with various phase structures and used the typical single crystal superalloy Rene ' N5 as the substrate to investigate the intrinsic mechanism underpinning recrystallization using experiments combined with atomistic simulations. Experimentally, recrystallization occurred in the specimen with coatings of medium Al content (CA-25 specimen); in contrast, there was no secondary reaction zone in the CA-30 specimen with coatings of the highest Al content. From simulations, the nudged elastic band calculation demonstrated that a higher energy barrier (Delta E0) was required for new grain nucleation in the substrate under beta-NiAl grains, which existed in the CA-30 coating. Our findings provide a fundamental understanding of interfacial stability and benefit the design of bond coatings for superalloys.

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