期刊
SCIENCE OF THE TOTAL ENVIRONMENT
卷 872, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.scitotenv.2023.162214
关键词
Nitrogen -containing biomass; Pyrolysis; Biofuels; Nitrogen -doped carbon materials; Chemicals
This article summarizes the research on the pyrolysis of nitrogen-containing biomass, focusing on the effect of biomass composition on pyrolysis products and the characteristics of high and low nitrogen biomass. It discusses the biofuel characteristics, nitrogen migration, application prospects, and unique advantages of nitrogen-doped carbon materials for catalysis, adsorption, and energy storage. The feasibility of producing nitrogen-containing chemicals is also reviewed. The future outlook for denitrification and upgrading of bio-oil, performance improvement of nitrogen-doped carbon materials, and separation and purification of nitrogen-containing chemicals is addressed.
Pyrolysis of nitrogen-containing biomass holds tremendous potential for producing varieties of high value-added products, alleviating energy depletion. Based on the research status about nitrogen-containing biomass pyrolysis, the effect of biomass feedstock composition on pyrolysis products is first introduced from the aspects of elemental analysis, proximate analysis, and biochemical composition. The properties of biomass with high and low nitrogen used in pyrolysis are briefly summarized. Then, with the pyrolysis of nitrogen-containing biomass as the core, biofuel characteristics, nitrogen migration during pyrolysis, the application prospects, unique advantages of nitrogen-doped carbon materials for catalysis, adsorption and energy storage are introduced, as well as their feasibility in producing nitrogen-containing chemicals (acetonitrile and nitrogen heterocyclic) are reviewed. The future outlook for the application of the pyrolysis of nitrogen-containing biomass, specifically, how to realize the denitrification and upgrading of bio-oil, performance improvement of nitrogen-doped carbon materials, as well as separation and purification of nitrogen-containing chemicals, are addressed.
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