☆ 4.4 Review

A Review of Fe-Based Amorphous and Nanocrystalline Alloys: Preparations, Applications, and Effects of Alloying Elements

PHYSICA STATUS SOLIDI A-APPLICATIONS AND MATERIALS SCIENCE (2023)

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Article Chemistry, Physical

Nanocrystalline (Fe,Co,Ni)86B14 soft magnetic alloys prepared by ultra-rapid annealing

Z. Li et al.

Summary: This study investigated the glass-forming range, microstructural features, and soft magnetic properties of (Fe(1-x-)yCo(x)Ni(y))(86)B-14 alloys. It was found that Fe-rich compositions have the largest glass-forming range and exhibit nano-scale grains with bcc and fcc structures after ultra-rapid annealing. The coercivity and saturation magnetic polarization of the nanocrystalline alloys are affected by Co and Ni content, with Co addition generally increasing coercivity and saturation magnetic polarization, while Ni addition has the opposite effect.

JOURNAL OF ALLOYS AND COMPOUNDS (2022)

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Article Materials Science, Ceramics

Optimization of crystallization, microstructure and soft magnetic properties of (Fe0.83B0.11Si0.02P0.03C0.01)99.5Cu0.5 alloy by rapid annealing

Min Zhao et al.

Summary: A (Fe0.83B0.11Si0.02P0.03C0.01)(99.5)Cu-0.5 glass former was developed based on Fe83B11Si2P3C1 alloy. A new rapid annealing method was used to investigate the effect of temperature and time on the improvement of soft magnetic properties. The results show that the addition of Cu expands the interval between the first and second crystallization temperature. The alloy ribbon annealed by the new method exhibits higher saturation magnetization and lower coercivity compared to other nanocrystalline alloys with similar Fe content.

JOURNAL OF NON-CRYSTALLINE SOLIDS (2022)

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Article Materials Science, Multidisciplinary

Formation and crystallization behavior of Fe-based amorphous precursors with pre-existing α-Fe nanoparticles-Structure and magnetic properties of high-Cu-content Fe-Si-B-Cu-Nb nanocrystalline alloys

Yanhui Li et al.

Summary: The structure, crystallization behavior, and magnetic properties of Fe81.3Si4B13Cu1.7 alloy ribbons were studied, as well as the effects of Nb alloying. High-density Cu-clusters and Pre-existing Nano-sized alpha-Fe Particles were found in the amorphous matrix, and the number densities of these clusters were gradually reduced with Nb enrichment. Nb alloying also affected the average size of alpha-Fe grains after annealing, with 4 at.% Nb refining the grains to 8.9 nm. Mechanisms of alpha-Fe nucleation and growth during quenching and annealing were discussed, and a coercivity correlation with alpha-Fe was found, with permeability inversely related to coercivity.

JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY (2021)

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Article Chemistry, Physical

Nano-crystallization behavior and magnetic domain evolution in commercial Fe-Si-B metallic glass

Hyunjong Lee et al.

Summary: The soft ferromagnetic properties of nano-crystalline metallic glass are significantly influenced by microstructure and magnetic domain structure. Controlling the grain size can have a significant impact on coercivity and saturation flux density, leading to the production of soft ferromagnetic metallic glass.

JOURNAL OF ALLOYS AND COMPOUNDS (2021)

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Article Engineering, Electrical & Electronic

Effect of P microalloying on magnetic properties and structure of FeSiBNbCu nanocrystalline alloy

Changjiu Wang et al.

Summary: The study shows that substituting 1% of P for B has little effect on the crystallization behavior, saturation magnetic flux density, and permeability of the alloy, but effectively reduces the coercivity over a wide annealing temperature range.

JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS (2021)

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Article Chemistry, Physical

Nanocrystallization, magnetic properties and bending ductility of antiferromagnetic Mn-doped FeSiBCuPC alloys induced by micro-compressive stress annealing

Jia Xu et al.

Summary: This study demonstrates that Mn doping can improve the amorphous forming ability and thermal stability of the alloy, reduce coercivity, and appropriate MCSA can inhibit grain growth and improve grain size, resulting in nanocrystalline alloys with good comprehensive soft magnetic and mechanical properties.

JOURNAL OF ALLOYS AND COMPOUNDS (2021)

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Article Materials Science, Multidisciplinary

Rapid Annealing Optimizing Magnetic Softness and Thermal Stability of Mn-Substituted Fe-Based Nanocrystalline Alloys

Bojun Zhang et al.

Summary: This study found that Mn-doping and rapid annealing in Fe-based nanocrystalline alloys can lead to superior magnetic softness, high-saturation magnetic induction, and large permeability. This is attributed to the superb nano-structural stability and the formation of regular magnetic domains.

METALS (2021)

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Article Materials Science, Ceramics

Effect of primary α-Fe on soft magnetic properties of FeCuNbSiB amorphous/nanocrystalline alloy

Jili Ding et al.

Summary: The influence of primary alpha-Fe precipitation on thermal and magnetic properties was investigated by producing Fe76.5-xCu1NbxSi13.5B9 (x=0, 1, 2 and 3) amorphous/nanocrystalline ribbons through melt-spinning. It was found that rapid quenching and heat treatment had similar effects on alpha-Fe precipitation. By optimizing components and heat treatment, magnetic properties of the ribbons could be significantly improved.

JOURNAL OF NON-CRYSTALLINE SOLIDS (2021)

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Article Materials Science, Multidisciplinary

Effect of Fe content on crystallization behavior and soft magnetic properties in FINEMET-type alloys

Ningning Shen et al.

Summary: The study found that as the iron content increases, the glass forming ability of the alloy decreases, and the non-uniform structure and high iron content are beneficial to the rapid precipitation of α-Fe, but weaken the ability of Nb to suppress the growth of α-Fe grains, resulting in the coercivity of the magnet being highly sensitive to annealing temperature.

MATERIALS LETTERS (2021)

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Article Materials Science, Ceramics

Fe-B-Si-C-Cu amorphous and nanocrystalline alloys with ultrahigh hardness and enhanced soft magnetic properties

C. Liu et al.

Summary: Soft magnetic Fe-B-Si-C-Cu amorphous alloys demonstrate high saturation magnetization, low coercivity, high permeability, and hardness. By designing the microstructure carefully, even higher hardness and stability can be achieved.

JOURNAL OF NON-CRYSTALLINE SOLIDS (2021)

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Article Engineering, Electrical & Electronic

Enhanced Magnetic Properties of Hot-Pressed Fe-Based Nanocrystalline Powder Cores With Low-Melted Glass-Modified Insulating

Peng Cao et al.

Summary: Low-melted nano-sized LBSCA glasses have been used to modify resin-based insulating for preparing Fe-based nanocrystalline soft magnetic composites (SMCs) by hot-pressing followed by annealing. The phase transition of the ferromagnetic particles and evolution of the insulating matrix of the SMCs at various annealing temperatures have been investigated, and their magnetic properties have been improved with increased annealing temperature. Internal stresses induced by compaction have been gradually released with increased annealing temperature, leading to lower power losses and enhanced frequency stability of the real part of permeability below 450 degrees C.

IEEE TRANSACTIONS ON MAGNETICS (2021)

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Article Chemistry, Physical

The complementary effects of Fe and metalloids on the saturation magnetization of Fe-based amorphous alloys

Lingxiang Shi et al.

Summary: Developing Fe-based amorphous alloys with high saturation flux density has been a challenging topic, with metalloid elements playing a key role. Fe83-85(B, C, Si)(14-16)P(1) amorphous alloys with high B-s and low H-c were successfully developed, with Fe content and metalloids having strong interrelated effects on the magnetic properties. The effects of metalloids on B-s are shown to be more significant than that of Fe in Fe-rich amorphous alloys, with the effects depending largely on Fe content.

INTERMETALLICS (2021)

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Article Chemistry, Physical

Crystallization behavior, soft magnetic properties and good bending ductility of high Fe content FeSiBCuPC alloys induced by composition design

Jia Xu et al.

Summary: In this study, the effects of adding different ferromagnetic elements, metallic elements with strong non-metallic properties, and transition metal elements with large atomic radius on the crystallization behavior, magnetic properties, and ductility of Fe85Si0.5B9P4Cu0.5C0.1M0.9 alloys were systematically investigated. Through optimal heat treatments, nanocrystalline alloys exhibited excellent soft magnetic properties but further understanding of the microscopic mechanism of plastic deformation and achieving high toughness in amorphous alloys is crucial.

JOURNAL OF ALLOYS AND COMPOUNDS (2021)

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Article Chemistry, Physical

Identifying the optimal amorphous precursor alloy system for dual-phase nanostructure formation according to the impurity tolerance and crystallization mechanism

Fengyu Kong et al.

Summary: The Fe83B12Si4Cu1 and Fe83P12Si4Cu1 alloys allow for easy preparation of fully amorphous ribbons, showing potential for industrial production with high impurity tolerance. Different alloy systems exhibit varying degrees of surface crystallization, with Fe83B12Si4Cu1 alloy showing a wide crystallization temperature interval. Further research is needed to develop impurity purification processes for Fe83B12-xPxSi4Cu1 alloys to improve their impurity tolerance.

INTERMETALLICS (2021)

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Article Materials Science, Ceramics

Combinatorial synthesis of nanocrystalline FeSiBPCuC-Ni-(Nb,Mo) soft magnetic alloys with high corrosion resistance

Takahiro Yamazaki et al.

Summary: The study fabricated FeSiBPCuC amorphous thin films with enhanced corrosion resistance through a new technique. The addition of Ni and Mo elements promoted the improvement of the corrosion resistance of the alloys.

JOURNAL OF NON-CRYSTALLINE SOLIDS (2021)

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Article Materials Science, Multidisciplinary

Improvement of saturation magnetic flux density in Fe-Si-B-Nb-Cu nanocomposite alloys by magnetic field annealing

Seoyeon Kwon et al.

CURRENT APPLIED PHYSICS (2020)

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Article Chemistry, Physical

Effects of the substitution of Si by P on crystallization behavior, soft magnetic properties and bending ductility of FeSiBCuPC alloys

Jia Xu et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2020)

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Article Materials Science, Multidisciplinary

Optimization of the structure and soft magnetic properties of a Fe87B13 nanocrystalline alloy by additions of Cu and Nb

Licheng Wu et al.

JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS (2020)

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Article Materials Science, Multidisciplinary

Influence of Co substitution for Fe on magnetic properties and crystal structure of soft magnetic Fe81.3Mo0.2Cu0.5Si4B14 alloy

L. Hawelek et al.

JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS (2020)

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Article Materials Science, Ceramics

High Bs of FePBCCu nanocrystalline alloys with excellent soft-magnetic properties

Long Hou et al.

JOURNAL OF NON-CRYSTALLINE SOLIDS (2020)

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Article Chemistry, Physical

A study on the role of Ni content on structure and properties of Fe-Ni-Si-B-P-Cu nanocrystalline alloys

Xingjie Jia et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2020)

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Review Materials Science, Multidisciplinary

Recent progress in Fe-based amorphous and nanocrystalline soft magnetic materials

Daichi Azuma et al.

JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS (2020)

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Article Materials Science, Multidisciplinary

Si microalloying optimizes the thermal stability, crystallization behaviors and magnetic properties of Fe-rich Fe-B-Cu-Hf alloys

H. Yuan et al.

JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS (2020)

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Article Materials Science, Multidisciplinary

Composition design for Fe-based soft magnetic amorphous and nanocrystalline alloys with high Fe content

Lingxiang Shi et al.

MATERIALS & DESIGN (2020)

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Article Materials Science, Multidisciplinary

Composition dependence of amorphous forming, crystallization behavior, magnetic and electronic properties of silicon-rich FeSiBCuNb alloys

Ting Luo et al.

JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS (2020)

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Article Materials Science, Ceramics

Comparative study of V and Mo on the glass formation and magnetic properties of Fe-Si-B-Cu-Nb-M (M = V, Mo) nanocrystalline for high frequency applications

Meng Xiao et al.

JOURNAL OF NON-CRYSTALLINE SOLIDS (2020)

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Article Physics, Multidisciplinary

Effect of chemical composition and Cu addition on crystallization and magnetic characteristics of FeZrB alloys

Wanqiu Yu et al.

PHYSICS LETTERS A (2020)

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Article Chemistry, Physical

Improving the amorphous forming ability and magnetic properties of FeSiBPCu amorphous and nanocrystalline alloys by utilizing carbon

Y. L. Li et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2020)

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Article Materials Science, Multidisciplinary

Significant improvement of soft magnetic properties for Fe-based nanocrystalline alloys by inhibiting surface crystallization via a magnetic field assisted melt-spinning process

Lei Xie et al.

JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS (2019)

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Article Materials Science, Multidisciplinary

Al addition effect on structure and magnetic properties in high Bs Fe-Cu-Si-B alloys

Hongjun Duan et al.

MATERIALS RESEARCH BULLETIN (2019)

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Article Physics, Condensed Matter

Crystallization behavior and magnetic properties for the Fe73(Si0.64B0.27P0.09)23+xCu1Nb3-x (x=0, 1 and 2) alloys

Luo Ting et al.

PHYSICA B-CONDENSED MATTER (2019)

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Article Chemistry, Physical

Nanocrystallization, good soft magnetic properties and ultrahigh mechanical strength for Fe82-85B13-16Si1Cu1 amorphous alloys

L. L. Pang et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2019)

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Article Materials Science, Multidisciplinary

Nanocrystalline soft magnetic materials with a saturation magnetization greater than 2 T

R. Parsons et al.

JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS (2019)

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Review Materials Science, Multidisciplinary

Amorphous-nanocrystalline alloys: fabrication, properties, and applications

F. C. Li et al.

MATERIALS TODAY ADVANCES (2019)

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Article Engineering, Electrical & Electronic

Effect of Mo on nanocrystallization and magnetic properties of Fe83-x B10C6Cu1Mox (x=0-1.25) soft magnetic alloys

L. Zhu et al.

JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS (2018)

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Article Chemistry, Physical

First principle study on the Si effect in the Fe-based soft magnetic nano-crystalline alloys

Yaocen Wang et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2018)

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Article Chemistry, Physical

Effect of Nb, Si and Cu on the crystallization process and magnetic properties of FeNbBP alloys

Weide Lin et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2018)

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Article Chemistry, Physical

Nano-crystallization of amorphous alloys by ultra-rapid annealing: An effective approach to magnetic softening

K. Suzuki et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2018)

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Article Chemistry, Physical

The effect of Co addition on magnetic and structural properties of nanocrystalline (Fe, Co)-Si-B-P-Cu alloys

Markus Kuhnt et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2018)

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Article Metallurgy & Metallurgical Engineering

Microstructure and magnetic properties of Fe81.3Si4B13Cu1.7 nanocrystalline alloys with minor Nb addition

Xiang-cheng Ren et al.

JOURNAL OF IRON AND STEEL RESEARCH INTERNATIONAL (2018)

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Influence of Al addition on structural, crystallization and soft magnetic properties of DC Joule annealed FeCo based nanocrystalline alloys

Premkumar Murugaiyan et al.

JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS (2018)

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Role of Mo addition on structure and magnetic properties of the Fe85Si2B8P4Cu1 nanocrystalline alloy

Xingjie Jia et al.

JOURNAL OF NON-CRYSTALLINE SOLIDS (2018)

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Article Chemistry, Physical

Optimization of crystallization, microstructure and soft magnetic properties of Fe-B-Cu alloys by rapid cyclic annealing

X. B. Zhai et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2018)

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Article Engineering, Chemical

Soft magnetic properties of Fe-based amorphous/nanocrystalline hybrid materials

Yeonjoo Lee et al.

POWDER TECHNOLOGY (2018)

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Article Chemistry, Physical

Effects of Cu cluster evolution on soft magnetic properties of Fe83B10C6Cu1 metallic glass in two-step annealing

G. T. Xia et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2017)

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Article Chemistry, Physical

Soft magnetic Fe-Si-B-Cu nanocrystalline alloys with high Cu concentrations

Yanhui Li et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2017)

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Article Materials Science, Multidisciplinary

Fe(Co)SiBPCCu nanocrystalline alloys with high Bs above 1.83 T

Tao Liu et al.

JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS (2017)

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Article Nanoscience & Nanotechnology

Effect of heating rate during primary crystallization on soft magnetic properties of melt-spun Fe-B alloys

B. Zang et al.

SCRIPTA MATERIALIA (2017)

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Article Green & Sustainable Science & Technology

Energy-efficient distribution transformers in Europe: impact of Ecodesign regulation

Anibal De Almeida et al.

ENERGY EFFICIENCY (2016)

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Article Chemistry, Physical

Composition design of high Bs Fe-based amorphous alloys with good amorphous-forming ability

Anding Wang et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2016)

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Industrialization of nanocrystalline Fe-Si-B-P-Cu alloys for high magnetic flux density cores

Kana Takenaka et al.

JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS (2016)

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Article Chemistry, Physical

Optimization of thermal stability and soft-magnetic properties of FeSiBPCuNb alloys by Nb content tuning

Zhen Xiang et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2015)

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Article Physics, Applied

An amorphous alloy core medium frequency magnetic-link for medium voltage photovoltaic inverters

Md Rabiul Islam et al.

JOURNAL OF APPLIED PHYSICS (2014)

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Review Chemistry, Multidisciplinary

Recent progress in high Bs and low Hc Fe-based nanocrystalline alloys

Dewei Chu et al.

NANOTECHNOLOGY REVIEWS (2014)

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Article Nuclear Science & Technology

Characterization of Fe-based alloy coating deposited by supersonic plasma spraying

Piao Zhong-yu et al.

FUSION ENGINEERING AND DESIGN (2013)

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Proceedings Paper Materials Science, Characterization & Testing

Phase Structure and Magnetic Properties of Fe-Nb-B-Nd Type of Bulk Nanocrystalline Alloys

Grzegorz Ziolkowski et al.

APPLIED CRYSTALLOGRAPHY XXII (2013)

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Effect of P to B concentration ratio on soft magnetic properties in FeSiBPCu nanocrystalline alloys

Fanli Kong et al.

JOURNAL OF APPLIED PHYSICS (2012)

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Article Physics, Applied

Fe-based nanocrystalline FeBCCu soft magnetic alloys with high magnetic flux density

Xingdu Fan et al.

JOURNAL OF APPLIED PHYSICS (2011)

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Article Nanoscience & Nanotechnology

Ternary Fe-P-C bulk metallic glass with good soft-magnetic and mechanical properties

Jianfeng Wang et al.

SCRIPTA MATERIALIA (2011)

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Article Chemistry, Physical

Effect of Zr on the thermal stability and magnetic properties of Fe78Si9B13 glassy alloy

H. J. Ma et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2010)

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Article Materials Science, Multidisciplinary

Crystallisation progress in Si-rich ultra-soft nanocomposite alloy fabricated by melt spinning

Duc-The Ngo et al.

JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS (2010)

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Article Materials Science, Multidisciplinary

The influence of Al content on glass forming ability and magnetic properties of high Ms nanocrystalline FeSiBPCuAl alloy

B. S. Dong et al.

MATERIALS LETTERS (2010)

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Article Engineering, Electrical & Electronic

New Excellent Soft Magnetic FeSiBPCu Nanocrystallized Alloys With High Bs of 1.9 T From Nanohetero-Amorphous Phase

Akihiro Makino et al.

IEEE TRANSACTIONS ON MAGNETICS (2009)

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Article Physics, Applied

New Fe-metalloids based nanocrystalline alloys with high Bs of 1.9 T and excellent magnetic softness

Akihiro Makino et al.

JOURNAL OF APPLIED PHYSICS (2009)

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Article Materials Science, Multidisciplinary

High Bs nanocrystalline Fe84-x-yCuxNbySi4B12 alloys (x=0.0-1.4, y=0.0-2.5)

Motoki Ohta et al.

JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS (2009)

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Article Physics, Applied

Magnetic properties of nanocrystalline Fe82.65Cu1.35SixB16-x alloys (x=0-7)

Motoki Ohtaa et al.

APPLIED PHYSICS LETTERS (2007)

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Article Physics, Applied

New high-Bs Fe-based nanocrystalline soft magnetic alloys

Motoki Ohta et al.

JAPANESE JOURNAL OF APPLIED PHYSICS PART 2-LETTERS & EXPRESS LETTERS (2007)

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Article Chemistry, Physical

The peculiarity of contraction in the primary crystallization of amorphous Fe73.5Nb3Cu1Si13.5B9 alloy

Y. C. Niu et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2007)

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Article Physics, Applied

Exceptionally high glass-forming ability of an FeCoCrMoCBY alloy

J Shen et al.

APPLIED PHYSICS LETTERS (2005)

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Article Materials Science, Ceramics

Effects of high boron content on crystallization, forming ability and magnetic properties of amorphous Fe91-xZr5BxNb4 alloy

B Yao et al.

JOURNAL OF NON-CRYSTALLINE SOLIDS (2003)

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Article Materials Science, Multidisciplinary

The influence of post-annealing cooling rates on magnetic properties of Fe-based nanocrystalline alloys

A Kolano et al.

JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS (2003)

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Article Materials Science, Multidisciplinary

Comparison and analysis of continuously jetting and discretely jetting method used in rapid ice prototype forming

C Feng et al.

MATERIALS & DESIGN (2002)

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Article Materials Science, Multidisciplinary

Effect of cooling rate on magnetic properties of amorphous and nanocrystalline Fe73.5Cu1Nb3Si15.5B7 alloy

M Hasiak et al.

JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS (2000)

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