期刊
PETROLEUM CHEMISTRY
卷 63, 期 2, 页码 167-175出版社
MAIK NAUKA/INTERPERIODICA/SPRINGER
DOI: 10.1134/S0965544123020020
关键词
zeolite synthesis; MFI; zeolite catalysis; interzeolite transformations
A series of experiments were conducted to investigate the interzeolite transformations of FAU into MFI. The study focused on the effects of various parameters, such as the parent zeolite's composition, presence and type of seed crystals, and recrystallization method, on the resulting MFI zeolites' physicochemical properties and catalytic performance. The researchers were able to optimize the transformation conditions and propose efficient methods for targeted template-free synthesis of MFI zeolites with specific physicochemical properties and active sites.
A series of experiments on interzeolite transformations of FAU into MFI was carried out. The study investigated the effects of various parameters, such as the chemical composition of parent zeolite, presence and type of seed crystals, and recrystallization method, on the physicochemical properties and catalytic performance of the MFI zeolites produced by interzeolite transformation from FAU. This enabled the researchers to optimize the transformation conditions and to propose highly efficient methods for targeted template-free synthesis of MFI zeolites with specific physicochemical properties and specific types of active sites. Based on a comprehensive analysis of the above-mentioned parameters governing the properties of target zeolites, a number of high-performance catalysts for methanol-to-hydrocarbon conversion were synthesized without templates, their catalytic performance being effectively controlled within a wide range.
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