期刊
OPTICS LETTERS
卷 48, 期 8, 页码 2054-2057出版社
Optica Publishing Group
DOI: 10.1364/OL.485966
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The dynamic control of magnetization by short laser pulses has attracted recent interest. The transient magnetization at the metallic magnetic interface has been investigated using second-harmonic generation and the time-resolved magneto-optical effect. However, the ultrafast light-driven magneto-optical nonlinearity in ferromagnetic heterostructures for terahertz (THz) radiation remains unclear. In this study, we demonstrate THz generation from a metallic heterostructure, Pt/CoFeB/Ta, with contributions from magnetization-induced optical rectification and spin-to-charge current conversion.
The dynamic control of magnetization by short laser pulses has recently attracted interest. The transient magnetization at the metallic magnetic interface has been investigated through second-harmonic generation and the time-resolved magneto-optical effect. However, the ultrafast light-driven magneto-optical nonlinearity in ferromagnetic heterostructures for terahertz (THz) radiation remains unclear. Here, we present THz generation from a metallic heterostructure, Pt/CoFeB/Ta, which is ascribed to an -6-8% contribution from the magnetization-induced optical rectification and an -94-92% contribution from both spin-to-charge current conversion and ultrafast demagnetization. Our results show that THz-emission spectroscopy is a powerful tool to study the picosecond-time-scale nonlinear magneto-optical effect in ferromagnetic heterostructures.
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