Strongly enhanced light-matter coupling of monolayer WS2 from a bound state in the continuum

Combining a tungsten disulfide monolayer and a topologically protected bound state in the continuum formed by a one-dimensional photonic crystal, strong light-matter interaction enhancement and large exciton-polariton nonlinearities at room temperature are demonstrated. Exciton-polaritons derived from the strong light-matter interaction of an optical bound state in the continuum with an excitonic resonance can inherit an ultralong radiative lifetime and significant nonlinearities, but their realization in two-dimensional semiconductors remains challenging at room temperature. Here we show strong light-matter interaction enhancement and large exciton-polariton nonlinearities at room temperature by coupling monolayer tungsten disulfide excitons to a topologically protected bound state in the continuum moulded by a one-dimensional photonic crystal, and optimizing for the electric-field strength at the monolayer position through Bloch surface wave confinement. By a structured optimization approach, the coupling with the active material is maximized here in a fully open architecture, allowing to achieve a 100 meV photonic bandgap with the bound state in the continuum in a local energy minimum and a Rabi splitting of 70 meV, which results in very high cooperativity. Our architecture paves the way to a class of polariton devices based on topologically protected and highly interacting bound states in the continuum.

Automated summary

In this study, strong light-matter interaction enhancement and large exciton-polariton nonlinearities at room temperature were demonstrated by combining a tungsten disulfide monolayer and a topologically protected bound state in the continuum formed by a one-dimensional photonic crystal. By optimizing for the electric-field strength at the monolayer position through Bloch surface wave confinement, a 100 meV photonic bandgap with the bound state in the continuum and a Rabi splitting of 70 meV were achieved in a fully open architecture. This architecture opens up possibilities for polariton devices based on topologically protected and highly interacting bound states in the continuum.