4.8 Article

Light trapping enhanced broadband photodetection and imaging based on MoSe2/pyramid Si vdW heterojunction

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NANO RESEARCH
卷 -, 期 -, 页码 -

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TSINGHUA UNIV PRESS
DOI: 10.1007/s12274-023-5650-x

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two-dimensional (2D) MoSe2 layers; light trapping; van der Waals (vdW) heterojunction; broadband photodetector; self-powered imaging

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In this study, a MoSe2/pyramid Si mixed-dimensional van der Waals heterojunction array is presented for broadband photodetection and imaging. The photodetector exhibits a wide spectral response range, high responsivity, and ultrafast response time due to enhanced optical absorption and high-quality van der Waals heterojunction. Moreover, the photodetector array demonstrates outstanding broadband image sensing capability. This research provides a novel development route for high-performance and broadband photodetector array by MoSe2/pyramid Si mixed-dimensional heterojunction.
Two-dimensional (2D) layered materials have been considered promising candidates for next-generation optoelectronics. However, the performance of 2D photodetectors still has much room for improvement due to weak light absorption of planar 2D materials and lack of high-quality heterojunction preparation technology. Notably, 2D materials integrating with mature bulk semiconductors are a promising pathway to overcome this limitation and promote the practical application on optoelectronics. In this work, we present the patterned assembly of MoSe2/pyramid Si mixed-dimensional van der Waals (vdW) heterojunction arrays for broadband photodetection and imaging. Benefited from the light trapping effect induced enhanced optical absorption and high-quality vdW heterojunction, the photodetector demonstrates a wide spectral response range from 265 to 1550 nm, large responsivity up to 0.67 A center dot W-1, high specific detectivity of 1.84 x 10(13) Jones, and ultrafast response time of 0.34/5.6 mu s at 0 V. Moreover, the photodetector array exhibits outstanding broadband image sensing capability. This study offers a novel development route for high-performance and broadband photodetector array by MoSe2/pyramid Si mixed-dimensional heterojunction.

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