Emerging silk fibroin materials and their applications: New functionality arising from innovations in silk crosslinking

Review Chemistry, Multidisciplinary

Silk Fibroin as Sustainable Advanced Material: Material Properties and Characteristics, Processing, and Applications

Ander Reizabal et al.

Summary: In this review, the molecular structure, original properties, available modifications, and processing methods of silk fibroin are presented, providing a wide overview for custom structural and functional variations.

ADVANCED FUNCTIONAL MATERIALS (2023)

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Article Engineering, Biomedical

Injection-Free Delivery of MSC-Derived Extracellular Vesicles for Myocardial Infarction Therapeutics

Junnan Tang et al.

Summary: This study proposes a non-injection method for delivering EVs onto the heart surface to treat MI by spraying a mixture of EVs, GelMA precursors, and photoinitiators. The physically entrapped EVs within the GelMA hydrogel network have an enhanced retention rate and are gradually released through diffusion and/or enzymatic degradation to exert a therapeutic effect in the heart tissue.

ADVANCED HEALTHCARE MATERIALS (2022)

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Article Materials Science, Biomaterials

One-Step FRESH Bioprinting of Low-Viscosity Silk Fibroin Inks

Shinji Sakai et al.

Summary: Silk fibroin (SF) is an attractive material for 3D bioprinting, and this study developed a method to bioprint low-viscosity SF solutions without additives. The printing process was cell-friendly, and the printed SF hydrogel constructs maintained high cell viability for a prolonged period of time, showcasing the potential of this technique in tissue engineering and regenerative medicine.

ACS BIOMATERIALS SCIENCE & ENGINEERING (2022)

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Article Nanoscience & Nanotechnology

Robust Silk Protein Hydrogels Made by a Facile One-Step Method and Their Multiple Applications

Ling Chen et al.

Summary: This article introduces a simple method to prepare tough silk fibroin hydrogels and compares their mechanical properties and biocompatibility with other silk fibroin hydrogels. It also discusses the possibility of using these hydrogels as a multi-functional platform.

ACS APPLIED BIO MATERIALS (2022)

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Article Polymer Science

Self-adhesive plasticized regenerated silk on poly(3-hydroxybutyrate-co-3-hydroxyvalerate) for bio-piezoelectric force sensor and microwave circuit design

Silvia Bittolo Bon et al.

Summary: The study demonstrates that regenerated silk (RS) can act as a self-adhesive thermoplastic material with multifunctional properties, such as piezoelectricity. Specifically, RS hybrids with gold nanorods and Ca ions were produced, forming tough self-adhesive materials on PHBV substrates. These RS/PHBV composites show promise for applications in tissue engineering and as dielectric substrates in microwave circuit design.

JOURNAL OF APPLIED POLYMER SCIENCE (2021)

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Article Biochemistry & Molecular Biology

Hydrogel-Based Bioinks for Cell Electrowriting of Well-Organized Living Structures with Micrometer-Scale Resolution

Miguel Castilho et al.

Summary: Novel hydrogel-based bioinks for cell electrowriting (CEW) have been developed to fabricate well-organized cell-laden fiber structures with diameters ranging from 5 to 40 μm, opening up exciting opportunities for the manufacture of microstructured constructs in regenerative medicine and in vitro models.

BIOMACROMOLECULES (2021)

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Article Biochemistry & Molecular Biology

Spinning Regenerated Silk Fibers with Improved Toughness by Plasticizing with Low Molecular Weight Silk

Ya Yao et al.

Summary: Utilizing low-molecular weight silk as a plasticizer enhances physical crosslinks between high-molecular weight silk chains, improving fiber extensibility and toughness. The regenerated silk fibers produced have high molecular chain orientation and crystallinity, approaching the properties of natural silk fibers.

BIOMACROMOLECULES (2021)

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Article Biochemistry & Molecular Biology

Silk Hydrogels with Controllable Formation of Dityrosine, 3,4-Dihydroxyphenylalanine, and 3,4-Dihydroxyphenylalanine-Fe3+ Complexes through Chitosan Particle-Assisted Fenton Reactions

Jaewon Choi et al.

Summary: The study demonstrates the controlled formation of dityrosine and DOPA in silk hydrogels by manipulating the interaction between Fe3+ ions and silk fibroin using chitosan particles. The addition of EDTA further enhances the selectivity towards DOPA formation.

BIOMACROMOLECULES (2021)

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Article Chemistry, Multidisciplinary

Silk fibroin microneedles fabricated by digital light processing 3D printing

Donghyeok Shin et al.

Summary: This report introduces a method for one-step 3D structuring of protein-based microneedles using digital light processing (DLP) 3D printing. By using riboflavin as a photoinitiator, the printing of silk fibroin (SF) microneedles and the delivery of molecules to the skin in biomedical applications are achieved successfully.

JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY (2021)

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Article Biochemical Research Methods

3D bioprinted silk fibroin hydrogels for tissue engineering

Soon Hee Kim et al.

Summary: The development of biocompatible and precisely printable bioink addresses the growing demand for three-dimensional bioprinting applications in tissue engineering. The versatile bioink, with high mechanical stability and biocompatibility, can be broadly used in nerve tissue engineering and wound healing, among other applications.

NATURE PROTOCOLS (2021)

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Review Biotechnology & Applied Microbiology

Dissolution and processing of silk fibroin for materials science

Hai-Yan Wang et al.

Summary: Silk fibroin from silkworm Bombyx mori has been extensively researched and applied in various fields in recent decades, including cosmetics, biomedicine, and biomaterials. Dissolution and regeneration of SF fibers is crucial for the application of silk protein-based materials, and the process directly impacts the characteristics and mechanical properties of resulting silk biomaterials. This review summarizes common solvents and dissolution methods for silk protein, properties of resulting SF protein, suitable uses of SF dissolved in corresponding solvents, and recent applications of SF in various biomaterials.

CRITICAL REVIEWS IN BIOTECHNOLOGY (2021)

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Review Polymer Science

Recent advances in 3D printing with protein-based inks

Xuan Mu et al.

Summary: Protein-based inks for 3D printing offer unique material characteristics that match specific tissue properties, promote implant-host integration, and serve as an interface between technology and biology. Despite challenges like concentration and structural hierarchy, exploiting the biological, chemical, and physical features of protein-based inks holds key opportunities for tissue engineering and regenerative medicine. Advances in photo-crosslinking mechanisms and rheological principles are enhancing the design and development of protein-based inks for a promising spectrum of biomedical research.

PROGRESS IN POLYMER SCIENCE (2021)

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Article Chemistry, Multidisciplinary

Highly Thermal-Wet Comfortable and Conformal Silk-Based Electrodes for On-Skin Sensors with Sweat Tolerance

Qingsong Li et al.

Summary: A highly thermal-wet comfortable and conformal silk-based electrode has been developed for on-skin electrophysiological measurement under sweaty conditions. The electrode shows high stretchability, low thermal insulation, low evaporative resistance, and high water-vapor transmission rate, enabling better electrocardiography signal quality and the possibility for textile integration to monitor muscle activities under large deformation. This glycerol-plasticized silk-based electrode may further advance on-skin electronics with sweat tolerance.

ACS NANO (2021)

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Article Chemistry, Multidisciplinary

Shape-Engineerable Silk Fibroin Papers for Ideal Substrate Alternatives of Plastic Electronics

Haitao Liu et al.

Summary: Plastic-based electronics are being used to bridge the gap in soft interface applications, but their environmental impact should be considered. Silk fibroin offers a green alternative for electronics development, but brittleness of silk films remains a challenge. The development of trace-ion-assisted plasticization strategy has led to the creation of shape-engineerable pure silk fibroin paper (PSFP), overcoming the brittleness of pure silk films and enabling new possibilities for electronic prototypes and devices.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

The Manufacture of Unbreakable Bionics via Multifunctional and Self-Healing Silk-Graphene Hydrogels

Firoz Babu Kadumudi et al.

Summary: The novel biomaterial CareGum exhibits unique properties such as high mechanical toughness, record-breaking elongation capacity, good conformability, increased electrical conductivity and Young's modulus, as well as self-healing capabilities. By leveraging these characteristics, a durable and self-healing bionic glove is developed for hand gesture sensing and sign translation. CareGum shows promise for applications in fields like cyborganics, bionics, soft robotics, human-machine interfaces, 3D-printed electronics, and flexible bioelectronics.

ADVANCED MATERIALS (2021)

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Article Biochemistry & Molecular Biology

3D Printable Soy/Silk Hybrid Hydrogels for Tissue Engineering Applications

Pramod Dorishetty et al.

Summary: The development of protein-based 3D printable hydrogel systems with tunable structure and properties is crucial in biomedical applications. Hybrid hydrogels co-cross-linked between globular soy protein isolate (SPI) and fibrous silk fibroin (SF) were successfully 3D printed for the first time, showing tunable mechanical properties and increased printing accuracy with higher SF content. The fabricated hybrid hydrogels exhibited larger micropores and good cell attachment and proliferation, demonstrating their potential for tissue engineering applications.

BIOMACROMOLECULES (2021)

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Article Materials Science, Biomaterials

Highly Absorbent Silk Fibroin Protein Xerogel

Kang Cheng et al.

Summary: In this study, a highly absorbent hydrogel was prepared using silk fibroin protein and riboflavin, with covalent bond crosslinking hindering the crystallization of the silk fibroin, resulting in an amorphous xerogel. This xerogel showed promising hemostatic properties and water absorption capacity, indicating its potential for rapid wound hemostasis and fluid absorption.

ACS BIOMATERIALS SCIENCE & ENGINEERING (2021)

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Review Materials Science, Biomaterials

Functional silk fibroin hydrogels: preparation, properties and applications

Haiyan Zheng et al.

Summary: Traditional silk protein hydrogels have limitations in terms of structure and functionality, but the development of functional silk protein hydrogels presents opportunities to overcome these limitations, attracting attention from scholars worldwide.

JOURNAL OF MATERIALS CHEMISTRY B (2021)

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Article Materials Science, Biomaterials

Optimization of hyaluronic acid-tyramine/silk-fibroin composite hydrogels for cartilage tissue engineering and delivery of anti-inflammatory and anabolic drugs

Reihane Ziadlou et al.

Summary: This study aimed to formulate injectable hydrogels for drug delivery and cartilage tissue engineering by combining hyaluronic acid-tyramine (HA-Tyr) with regenerated silk-fibroin (SF) solutions. The HA20/SF80 hydrogel showed superior chondrogenic effects and mechanical properties for cartilage tissue engineering applications, making it a promising biomaterial for osteoarthritis treatment.

MATERIALS SCIENCE & ENGINEERING C-MATERIALS FOR BIOLOGICAL APPLICATIONS (2021)

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Article Nanoscience & Nanotechnology

Biofunctional Silk Kirigami With Engineered Properties

Sayantan Pradhan et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Engineering, Biomedical

Digital light processing 3D printed silk fibroin hydrogel for cartilage tissue engineering

Heesun Hong et al.

BIOMATERIALS (2020)

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Article Engineering, Biomedical

Enzymatically crosslinked silk and silk-gelatin hydrogels with tunable gelation kinetics, mechanical properties and bioactivity for cell culture and encapsulation

Onur Hasturk et al.

BIOMATERIALS (2020)

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Review Biochemistry & Molecular Biology

Spider Silk for Tissue Engineering Applications

Sahar Salehi et al.

MOLECULES (2020)

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Article Chemistry, Multidisciplinary

Tuning the Rigidity of Silk Fibroin for the Transfer of Highly Stretchable Electronics

Jun Huang et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Engineering, Biomedical

Rapid Photocrosslinking of Silk Hydrogels with High Cell Density and Enhanced Shape Fidelity

Xiaolin Cui et al.

ADVANCED HEALTHCARE MATERIALS (2020)

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Review Chemistry, Multidisciplinary

Fundamentals and Applications of Photo-Cross-Linking in Bioprinting

Khoon S. Lim et al.

CHEMICAL REVIEWS (2020)

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Article Materials Science, Biomaterials

Enhancing Resistance of Silk Fibroin Material to Enzymatic Degradation by Cross-Linking Both Crystalline and Amorphous Domains

Filippo Valente et al.

ACS BIOMATERIALS SCIENCE & ENGINEERING (2020)

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Review Polymer Science

Tuning the conformation and mechanical properties of silk fibroin hydrogels

Narges Johari et al.

EUROPEAN POLYMER JOURNAL (2020)

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Article Materials Science, Multidisciplinary

Intelligent Silk Fibroin Ionotronic Skin for Temperature Sensing

Jialin Liu et al.

ADVANCED MATERIALS TECHNOLOGIES (2020)

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Article Chemistry, Physical

3D Bioprinted Highly Elastic Hybrid Constructs for Advanced Fibrocartilaginous Tissue Regeneration

Joao B. Costa et al.

CHEMISTRY OF MATERIALS (2020)

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Article Materials Science, Multidisciplinary

Rapidly photocurable silk fibroin sealant for clinical applications

Soon Hee Kim et al.

NPG ASIA MATERIALS (2020)

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Article Biochemistry & Molecular Biology

Visible-light-induced hyaluronate hydrogel for soft tissue fillers

Bo Min Hong et al.

INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES (2020)

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Article Biochemistry & Molecular Biology

Laccase-mediated construction of flexible double-network hydrogels based on silk fibroin and tyramine-modified hyaluronic acid

Lin Wang et al.

INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES (2020)

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Article Materials Science, Biomaterials

Tubular Silk Fibroin/Gelatin-Tyramine Hydrogel with Controllable Layer Structure and Its Potential Application for Tissue Engineering

Sheng Xu et al.

ACS BIOMATERIALS SCIENCE & ENGINEERING (2020)

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Article Materials Science, Biomaterials

Silk fibroin nanofibrous mats for visible sensing of oxidative stress in cutaneous wounds

Sushant Singh et al.

BIOMATERIALS SCIENCE (2020)

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Article Materials Science, Biomaterials

Rapid and cytocompatible cell-laden silk hydrogel formation via riboflavin-mediated crosslinking

Susanna Piluso et al.

JOURNAL OF MATERIALS CHEMISTRY B (2020)

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Article Materials Science, Biomaterials

Dynamic Photo-cross-linking of Native Silk Enables Macroscale Patterning at a Microscale Resolution

Anastasia Brif et al.

ACS BIOMATERIALS SCIENCE & ENGINEERING (2020)

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Article Materials Science, Biomaterials

Silk degumming time controls horseradish peroxidase-catalyzed hydrogel properties

Jugal Kishore Sahoo et al.

BIOMATERIALS SCIENCE (2020)

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Article Biochemistry & Molecular Biology

High-strength and self-recoverable silk fibroin cryogels with anisotropic swelling and mechanical properties

Berkant Yetiskin et al.

INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES (2019)

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Article Biochemistry & Molecular Biology

Changes in Silk Feedstock Rheology during Cocoon Construction: The Role of Calcium and Potassium Ions

Peter R. Laity et al.

MACROMOLECULAR BIOSCIENCE (2019)

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Article Multidisciplinary Sciences

Sutureless repair of corneal injuries using naturally derived bioadhesive hydrogels

Ehsan Shirzaei Sani et al.

SCIENCE ADVANCES (2019)

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Article Multidisciplinary Sciences

3D bioprinting of collagen to rebuild components of the human heart

A. Lee et al.

SCIENCE (2019)

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Article Engineering, Biomedical

Silk Hydrogels Crosslinked by the Fenton Reaction

Jaewon Choi et al.

ADVANCED HEALTHCARE MATERIALS (2019)

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Article Engineering, Biomedical

The Biomedical Use of Silk: Past, Present, Future

Chris Holland et al.

ADVANCED HEALTHCARE MATERIALS (2019)

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Article Biochemistry & Molecular Biology

Highly elastomeric photocurable silk hydrogels

Dajiang Kuang et al.

INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES (2019)

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Article Materials Science, Biomaterials

Preparation and Statistical Characterization of Tunable Porous Sponge Scaffolds using UV Cross-linking of Methacrylate-Modified Silk Fibroin

Alessio Bucciarelli et al.

ACS BIOMATERIALS SCIENCE & ENGINEERING (2019)

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Review Chemistry, Multidisciplinary

Tyrosine-Rich Peptides as a Platform for Assembly and Material Synthesis

Jaehun Lee et al.

ADVANCED SCIENCE (2019)

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Article Chemistry, Multidisciplinary

Self-Healable Multifunctional Electronic Tattoos Based on Silk and Graphene

Qi Wang et al.

ADVANCED FUNCTIONAL MATERIALS (2019)

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Review Materials Science, Multidisciplinary

Chemically Modified Silk Proteins

Jianming Chen et al.

ADVANCED ENGINEERING MATERIALS (2018)

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Article Chemistry, Multidisciplinary

Plasticizing Silk Protein for On-Skin Stretchable Electrodes

Geng Chen et al.

ADVANCED MATERIALS (2018)

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Review Chemistry, Multidisciplinary

Engineering the Future of Silk Materials through Advanced Manufacturing

Zhitao Zhou et al.

ADVANCED MATERIALS (2018)

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Review Chemistry, Multidisciplinary

Silkworm silk-based materials and devices generated using bio-nanotechnology

Wenwen Huang et al.

CHEMICAL SOCIETY REVIEWS (2018)

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Article Dentistry, Oral Surgery & Medicine

Shining a light on high volume photocurable materials

William M. Palin et al.

DENTAL MATERIALS (2018)

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Article Biochemistry & Molecular Biology

Preparation of a multifunctional fibroin-based biomaterial via laccase-assisted grafting of chitooligosaccharide

Qian Zhou et al.

INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES (2018)

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Article Biochemistry & Molecular Biology

Photopolymerized maleilated chitosan/methacrylated silk fibroin micro/nanocomposite hydrogels as potential scaffolds for cartilage tissue engineering

Yingshan Zhou et al.

INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES (2018)

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Article Biochemistry & Molecular Biology

Enzymatically crosslinked and mechanically tunable silk fibroin/pullulan hydrogels for mesenchymal stem cells delivery

Tao Li et al.

INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES (2018)

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Review Engineering, Biomedical

Polymerization shrinkage stress of resin-based dental materials: A systematic review and meta-analyses of technique protocol and photo- activation strategies

Eliseu Aldrighi Munchow et al.

JOURNAL OF THE MECHANICAL BEHAVIOR OF BIOMEDICAL MATERIALS (2018)

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Article Chemistry, Multidisciplinary

Tough Photocrosslinked Silk Fibroin/Graphene Oxide Nanocomposite Hydrogels

Rajkamal Balu et al.

LANGMUIR (2018)

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Article Multidisciplinary Sciences

Rapidly responsive silk fibroin hydrogels as an artificial matrix for the programmed tumor cells death

Viviana P. Ribeiro et al.

PLOS ONE (2018)

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Article Cell & Tissue Engineering

UV-Assisted 3D Bioprinting of Nanoreinforced Hybrid Cardiac Patch for Myocardial Tissue Engineering

Mohammad Izadifar et al.

TISSUE ENGINEERING PART C-METHODS (2018)

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Article Multidisciplinary Sciences

Precisely printable and biocompatible silk fibroin bioink for digital light processing 3D printing

Soon Hee Kim et al.

NATURE COMMUNICATIONS (2018)

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Article Engineering, Biomedical

Peroxidase-immobilized porous silica particles for in situ formation of peroxidase-free hydrogels with attenuated immune responses

Li Li et al.

ACTA BIOMATERIALIA (2018)

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Article Chemistry, Multidisciplinary

Calcium-Modified Silk as a Biocompatible and Strong Adhesive for Epidermal Electronics

Ji-Won Seo et al.

ADVANCED FUNCTIONAL MATERIALS (2018)

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Article Engineering, Multidisciplinary

Flexible nanofibers-reinforced silk fibroin films plasticized by glycerol

Xiufang Li et al.

COMPOSITES PART B-ENGINEERING (2018)

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Review Pharmacology & Pharmacy

Reverse-engineered silk hydrogels for cell and drug delivery

F. Philipp Seib

THERAPEUTIC DELIVERY (2018)

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Article Nanoscience & Nanotechnology

Directed assembly of bio-inspired hierarchical materials with controlled nanofibrillar architectures

Peter Tseng et al.

NATURE NANOTECHNOLOGY (2017)

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Article Polymer Science

Cryogelation within cryogels: Silk fibroin scaffolds with single-, double- and triple-network structures

Berkant Yetiskin et al.

POLYMER (2017)

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Article Multidisciplinary Sciences

Deformable and conformal silk hydrogel inverse opal

Kyungtaek Min et al.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2017)

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Article Cell Biology

Engineering a highly elastic human protein-based sealant for surgical applications

Nasim Annabi et al.

SCIENCE TRANSLATIONAL MEDICINE (2017)

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Article Multidisciplinary Sciences

Silk-hydrogel Lenses for Light-emitting Diodes

Rustamzhon Melikov et al.

SCIENTIFIC REPORTS (2017)

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Article Engineering, Biomedical

Molecular and macro-scale analysis of enzyme-crosslinked silk hydrogels for rational biomaterial design

Meghan McGill et al.

ACTA BIOMATERIALIA (2017)

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Article Materials Science, Multidisciplinary

A bioinspired dual-crosslinked tough silk protein hydrogel as a protective biocatalytic matrix for carbon sequestration

Chang Sup Kim et al.

NPG ASIA MATERIALS (2017)

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Article Engineering, Biomedical

Enzymatically crosslinked silk-hyaluronic acid hydrogels

Nicole R. Raia et al.

BIOMATERIALS (2017)

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Article Nanoscience & Nanotechnology

Enhancing Mechanical Properties of Silk Fibroin Hydrogel through Restricting the Growth of β-Sheet Domains

Dihan Su et al.

ACS APPLIED MATERIALS & INTERFACES (2017)

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Article Chemistry, Multidisciplinary

Photolithographic Micropatterning of Conducting Polymers on Flexible Silk Matrices

Ramendra K. Pal et al.

ADVANCED MATERIALS (2016)

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Article Biochemistry & Molecular Biology

Preparation of antibacterial silk fibroin membranes via tyrosinase-catalyzed coupling of ε-polylysine

Ping Wang et al.

BIOTECHNOLOGY AND APPLIED BIOCHEMISTRY (2016)

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Article Engineering, Biomedical

Phenol red-silk tyrosine cross-linked hydrogels

Aswin Sundarakrishnan et al.

ACTA BIOMATERIALIA (2016)

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Review Engineering, Biomedical

Silk protein-based hydrogels: Promising advanced materials for biomedical applications

Sonia Kapoor et al.

ACTA BIOMATERIALIA (2016)

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Article Chemistry, Multidisciplinary

Design of Multistimuli Responsive Hydrogels Using Integrated Modeling and Genetically Engineered Silk-Elastin-Like Proteins

Wenwen Huang et al.

ADVANCED FUNCTIONAL MATERIALS (2016)

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Article Chemistry, Multidisciplinary

Photocrosslinking of Silk Fibroin Using Riboflavin for Ocular Prostheses

Matthew B. Applegate et al.

ADVANCED MATERIALS (2016)

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Article Biochemistry & Molecular Biology

Thermal and Structural Properties of Silk Biomaterials Plasticized by Glycerol

Joseph E. Brown et al.

BIOMACROMOLECULES (2016)

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Article Engineering, Biomedical

Bio-functionalized silk hydrogel microfluidic systems

Siwei Zhao et al.

BIOMATERIALS (2016)

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Article Biochemical Research Methods

Printing of stretchable silk membranes for strain measurements

Shengjie Ling et al.

LAB ON A CHIP (2016)

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Article Medicine, Research & Experimental

Reloadable Silk-Hydrogel Hybrid Scaffolds for Sustained and Targeted Delivery of Molecules

Saket Kumar Singh et al.

MOLECULAR PHARMACEUTICS (2016)

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Review Materials Science, Biomaterials

Dityrosine Cross-Linking in Designing Biomaterials

Benjamin P. Partlow et al.

ACS BIOMATERIALS SCIENCE & ENGINEERING (2016)

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Article Materials Science, Biomaterials

New Visible-Light Photoinitiating System for Improved Print Fidelity in Gelatin-Based Bioinks

Khoon S. Lim et al.

ACS BIOMATERIALS SCIENCE & ENGINEERING (2016)

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Review Materials Science, Biomaterials

Dityrosine Cross-Linking in Designing Biomaterials

Benjamin P. Partlow et al.

ACS BIOMATERIALS SCIENCE & ENGINEERING (2016)

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Article Materials Science, Biomaterials

New Visible-Light Photoinitiating System for Improved Print Fidelity in Gelatin-Based Bioinks

Khoon S. Lim et al.

ACS BIOMATERIALS SCIENCE & ENGINEERING (2016)

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Article Multidisciplinary Sciences

Tumor Growth Suppression Induced by Biomimetic Silk Fibroin Hydrogels

Le-Ping Yan et al.

SCIENTIFIC REPORTS (2016)

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Article Engineering, Biomedical

Injectable hydrogel systems crosslinked by horseradish peroxidase

Fan Lee et al.

BIOMEDICAL MATERIALS (2016)

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Review Engineering, Biomedical

Processing Techniques and Applications of Silk Hydrogels in Bioengineering

Michael Floren et al.

JOURNAL OF FUNCTIONAL BIOMATERIALS (2016)

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Article Nanoscience & Nanotechnology

Facile Fabrication of Robust Silk Nanofibril Films via Direct Dissolution of Silk in CaCl2-Formic Acid Solution

Feng Zhang et al.

ACS APPLIED MATERIALS & INTERFACES (2015)

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Article Nanoscience & Nanotechnology

Biopatterning of Silk Proteins for Soft Micro-optics

Ramendra K. Pal et al.

ACS APPLIED MATERIALS & INTERFACES (2015)

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Article Engineering, Biomedical

Bioprintable, cell-laden silk fibroin-gelatin hydrogel supporting multilineage differentiation of stem cells for fabrication of three-dimensional tissue constructs

Sanskrita Das et al.

ACTA BIOMATERIALIA (2015)

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Article Biochemistry & Molecular Biology

Covalent Immobilization of Catalase onto Regenerated Silk Fibroins via Tyrosinase-Catalyzed Cross-Linking

Ping Wang et al.

APPLIED BIOCHEMISTRY AND BIOTECHNOLOGY (2015)

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Article Biochemistry & Molecular Biology

The Effect of Sterilization on Silk Fibroin Biomaterial Properties

Jelena Rnjak-Kovacina et al.

MACROMOLECULAR BIOSCIENCE (2015)

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Article Biotechnology & Applied Microbiology

Electrodeposited gels prepared from protein alloys

Yinan Lin et al.

NANOMEDICINE (2015)

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Review Polymer Science

Structures, mechanical properties and applications of silk fibroin materials

Leng-Duei Koh et al.

PROGRESS IN POLYMER SCIENCE (2015)

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Article Multidisciplinary Sciences

Aqueous multiphoton lithography with multifunctional silk-centred bio-resists

Yun-Lu Sun et al.

NATURE COMMUNICATIONS (2015)

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