☆ 4.8 Review

Enabling fast-charging capability for all-solid-state lithium-ion batteries

JOURNAL OF POWER SOURCES (2023)

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Zhe Li et al.

Summary: This study demonstrates a bipolar solid-state battery pouch cell with solid electrolytes and the introduction of a nonflammable ionogel for improved power capability and tolerance to abusive conditions. The in-situ-formed ionogel ensures better solid-solid interfacial contact, leading to higher cell energy and power density. This strategy holds promise for advancing the next-generation high-performance solid-state batteries.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Chemistry, Physical

Effects of porosity and ionic liquid impregnation on ionic conductivity of garnet-based flexible sheet electrolytes

Eric Jianfeng Cheng et al.

Summary: This study discusses the potential application of a flexible sheet electrolyte based on Al-doped LLZO to address the challenges of garnet-type ceramic. The research shows that the ionic conductivity of the electrolyte is influenced by porosity and ionic liquid impregnation, with promising electrochemical performance.

JOURNAL OF POWER SOURCES (2022)

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Article Chemistry, Physical

Hydrogen bonding enhanced SiO2/PEO composite electrolytes for solid-state lithium batteries

Cheng Wang et al.

Summary: The researchers designed hydrogen-bonded polyethylene oxide composite solid electrolytes that can enhance both the ionic conductivity and mechanical strength through the formation of an interconnected network. By adjusting the composition ratio, they overcame the issues of poor film forming and low mechanical strength.

JOURNAL OF MATERIALS CHEMISTRY A (2022)

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Article Chemistry, Physical

Hard Carbon Anode with a Sodium Carborane Electrolyte for Fast-Charging All-Solid-State Sodium-Ion Batteries

Keita Niitani et al.

Summary: All-solid-state sodium-ion batteries have the potential for fast charging, but are often limited by poor contact area and incompatibility between the active material and solid electrolyte. A fast-charging ASIB utilizing a hard carbon anode and a sodium carborane solid electrolyte exhibited excellent performance, showcasing the importance of intimate contact and compatibility between components.

ACS ENERGY LETTERS (2022)

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Article Chemistry, Physical

Sb-doped Li10GeP2S12-type electrolyte Li10SnP2-xSbxS12 with enhanced ionic conductivity and lower lithium-ion migration barrier

Qingtao Wang et al.

Summary: In this study, the P sites of Li10SnP2S12 solid electrolyte were partially substituted with Sb, resulting in an increase in ionic conductivity and improved air stability. Through experimental and computational analysis, it was found that the substitution of P with Sb reduced the activation energy and energy barrier, leading to enhanced ionic conductivity. The assembled all-solid-state battery showed superior performance in specific capacity and cycling stability.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2022)

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Article Materials Science, Multidisciplinary

A Nanoscale Design Approach for Enhancing the Li-Ion Conductivity of the Li10GeP2S12 Solid Electrolyte

James A. Dawson et al.

Summary: This research discovered the significant impact of nanoscaling on the lithium ion conductivity of the lithium superionic conductor Li10GeP2S12 (LGPS). By reducing the particle volume of LGPS, the lithium ion conductivity can be greatly enhanced, suggesting that nanosizing LGPS and other solid electrolytes could improve their lithium ion conductivity.

ACS MATERIALS LETTERS (2022)

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Article Chemistry, Applied

Manipulating interfacial stability of LiNi0.5Co0.3Mn0.2O2 cathode with sulfide electrolyte by nanosized LLTO coating to achieve high-performance all-solid-state lithium batterie

Jingguang Yi et al.

Summary: A core-shell cathode design with nanosized LLTO electrolyte coating on NCM532 cathode is proposed to enhance the interfacial stability in ASSLBs, improving lithium ion migration and suppressing electrolyte decomposition. The nanosized LLTO coating layer provides a facile and effective strategy for constructing high-performance ASSLBs with superior interfacial stability.

JOURNAL OF ENERGY CHEMISTRY (2021)

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Article Chemistry, Physical

Visualizing Lithium Dendrite Formation within Solid-State Electrolytes

Minghao Sun et al.

Summary: The study provides important insights into the growth mechanisms of lithium dendrites within a working lithium battery through in situ microscopic observation of lithium deposition inside the solid-state electrolyte (SSE). It revealed the direct nucleation and propagation of Li within the SSE, leading to structural cracking, possibly caused by crystalline defects present in the SSE.

ACS ENERGY LETTERS (2021)

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Article Chemistry, Physical

High Ionic Conductivity Achieved in Li3Y(Br3Cl3) Mixed Halide Solid Electrolyte via Promoted Diffusion Pathways and Enhanced Grain Boundary

Zhantao Liu et al.

Summary: A new halide compound Li3Y(Br3Cl3) with high Li+ conductivity and good stability was synthesized and characterized, showing improved grain boundary contact and overall conductivity after hot-pressing. MI all-solid-state batteries using this electrolyte demonstrated high capacity and good rate performance at room temperature, opening up opportunities for the design of halide ionic conductors and the development of all-solid-state batteries.

ACS ENERGY LETTERS (2021)

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Article Chemistry, Physical

Predicting Charge Transfer Stability between Sulfide Solid Electrolytes and Li Metal Anodes

Haesun Park et al.

Summary: The research investigates the reduction or oxidation of solid electrolytes by battery electrodes, finding that most solid electrolytes are susceptible to electron injection, except for Li3BS3 which shows resistance to reduction. Comparing charge transfer stability with chemical stability allows for a comprehensive assessment of interfacial stability. This approach is demonstrated through experiments on the Li/Li2H2PO4/LGPS interface system.

ACS ENERGY LETTERS (2021)

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Article Multidisciplinary Sciences

A mechanistic investigation of the Li10GeP2S12|LiNi1-x-yCoxMnyO2 interface stability in all-solid-state lithium batteries

Tong-Tong Zuo et al.

Summary: Researchers investigated the degradation mechanisms at the LGPS/NCM622 interface and found that electronic transport limits the growth of the degradation layer at the electrode|electrolyte interface. Additionally, they demonstrated the presence of two oxidation mechanisms at medium (3.7 V vs. Li+/Li < E < 4.2 V vs. Li+/Li) and high (E > = 4.2 V vs. Li+/Li) potentials.

NATURE COMMUNICATIONS (2021)

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Review Energy & Fuels

Moving beyond 99.9% Coulombic efficiency for lithium anodes in liquid electrolytes

Gustavo M. Hobold et al.

Summary: This review examines the trends and key descriptors of Coulombic efficiency in Li-metal batteries over the past five decades, as well as strategies to improve CE. While advancements have been made in cost and energy density of Li-ion batteries, achieving high Coulombic efficiency consistently remains a challenge.

NATURE ENERGY (2021)

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Article Chemistry, Physical

Self-Stabilized LiNi0.8Mn0.1Co0.1O2 in thiophosphate-based all-solid-state batteries through extra LiOH

Yubin Zhang et al.

Summary: NMC 811 as a potential cathode material for next generation high-energy all-solid-state lithium batteries faces compatibility issues with thiophosphate-based electrolytes. Researchers have developed a LiOH-based surface stabilization strategy to address this issue, providing optimized cycling stability and capacity for the battery. This coating method is simple and cost-effective, offering a promising solution for improving the performance of NMC 811 in solid-state electrolytes.

ENERGY STORAGE MATERIALS (2021)

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Article Multidisciplinary Sciences

A dynamic stability design strategy for lithium metal solid state batteries

Luhan Ye et al.

Summary: A multi-layered electrolyte design can inhibit the growth of lithium dendrites in solid-state lithium metal batteries, improving their performance. However, practical challenges remain in realizing a lithium metal anode for batteries.

NATURE (2021)

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Article Chemistry, Physical

Visualizing plating-induced cracking in lithium-anode solid-electrolyte cells

Ziyang Ning et al.

Summary: The propagation of lithium dendrites and cracks through ceramic electrolytes can lead to short circuits in batteries. The cracks initiate near the surface of the lithium electrode and propagate transversely across the electrolyte, driven by lithium ingress.

NATURE MATERIALS (2021)

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Article Nanoscience & Nanotechnology

Ultrastable Anode/Electrolyte Interface in Solid-State Lithium-Metal Batteries Using LiCux Nanowire Network Host

Qiushi Dai et al.

Summary: High interfacial resistance and uncontrollable lithium dendrite are common issues in solid-state Li-metal batteries, but the synthesis of a composite anode with a three-dimensional LiCux nanowire network host infiltrated with Li (Li* anode) offers a solution. This Li* anode demonstrates good wettability with LLZTO, high mechanical strength, and the ability to suppress Li dendrites, leading to remarkable electrochemical performance in symmetric cells and full cells with various cathodes.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Editorial Material Materials Science, Ceramics

Lining up for better performance: Researchers tailor interfaces in solid-state batteries

[Anonymous]

AMERICAN CERAMIC SOCIETY BULLETIN (2021)

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Article Chemistry, Physical

Local electronic structure variation resulting in Li 'filament' formation within solid electrolytes

Xiaoming Liu et al.

Summary: Solid electrolytes show promise for Li metal anodes, but Li infiltration along grain boundaries can lead to battery failure due to its association with local electronic band structure. Optimization of grain-boundary electronic conductivity is crucial for future solid-state battery design.

NATURE MATERIALS (2021)

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Review Chemistry, Physical

Fast Charging of Lithium-Ion Batteries: A Review of Materials Aspects

Manuel Weiss et al.

Summary: Fast charging is essential for the economic success of electric vehicles, with lithium-ion batteries facing limitations due to the transport of lithium ions within the electrodes. Understanding these limitations is crucial for optimizing material properties for fast-charging applications.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Physical

Improving Contact Impedance via Electrochemical Pulses Applied to Lithium-Solid Electrolyte Interface in Solid-State Batteries

Anand Parejiya et al.

Summary: The study demonstrates that a facile electrochemical pulse technique can improve the interfacial impedance and contact in SSBs, leading to higher energy density batteries. The application of short duration, high-voltage pulses can lower contact impedance and enhance contact between Li and LALZO through local Joule heating. The pulse technique shows potential to significantly reduce charge-transfer resistance and improve interfacial contacts in solid-state battery configurations.

ACS ENERGY LETTERS (2021)

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Review Chemistry, Multidisciplinary

Establishing a unified framework for ion solvation and transport in liquid and solid electrolytes

Donald J. Siegel et al.

Summary: Researchers have proposed a unified framework to relate atomic and continuum scale phenomena in electrolytes used in batteries. By examining the different solvation structures in liquids and solids, it has been shown that the mobility of entities affects the translation of working ions on different length scales.

TRENDS IN CHEMISTRY (2021)

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Article Materials Science, Multidisciplinary

Progress in thermal stability of all-solid-state-Li-ion-batteries

Yujing Wu et al.

Summary: This review discusses solutions to the thermal issues of lithium-ion batteries, introduces the development prospects of all-solid-state lithium-ion batteries and the current research status of thermal stability of solid-state electrolytes.

INFOMAT (2021)

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Article Materials Science, Multidisciplinary

Operando analysis of the molten Li|LLZO interface: Understanding how the physical properties of Li affect the critical current density

Bryan Kinzer et al.

Summary: Solid-state electrolytes show potential for high-energy-density Li metal batteries, but the penetration of Li at high current densities remains a challenge. Research reveals a significant increase in critical current density for LLZO at the melting point of Li and highlights the critical role of mechanical properties in determining CCD.

MATTER (2021)

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Article Chemistry, Physical

Revealing the role of the cathode-electrolyte interface on solid-state batteries

Beniamin Zahiri et al.

Summary: Interfaces play crucial roles in the performance of secondary solid-state batteries, and the crystallography and morphology of thick cathodes directly impact long-term performance. Minimizing interfacial area is key to understanding interface instabilities and improving cell performance. Dense and thick cathodes are suggested for increasing energy density and stability of solid-state batteries.

NATURE MATERIALS (2021)

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A Highly Efficient All-Solid-State Lithium/Electrolyte Interface Induced by an Energetic Reaction

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Synthesis and electrochemical performance of (100? x )Li 7 P 3 S 11-x Li 2 OHBr composite solid electrolyte for all -solid-state lithium batteries

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NATURE ENERGY (2020)

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ACS APPLIED MATERIALS & INTERFACES (2020)

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Fast Charge Transfer across the Li7La3Zr2O12 Solid Electrolyte/LiCoO2 Cathode Interface Enabled by an Interphase-Engineered All-Thin-Film Architecture

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Zijian Wang et al.

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Interphase Morphology between a Solid-State Electrolyte and Lithium Controls Cell Failure

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ACS ENERGY LETTERS (2019)

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Computational study of lithium nucleation tendency in Li7La3Zr2O12 (LLZO) and rational design of interlayer materials to prevent lithium dendrites

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