☆ 4.7 Review

A tutorial review on bimetallic nanoparticles loaded in smart organic polymer microgels/hydrogels

JOURNAL OF MOLECULAR LIQUIDS (2023)

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Article Chemistry, Multidisciplinary

Catalytic degradation of azo dyes by bimetallic nanoparticles loaded in smart polymer microgels

Muhammad Arif

Summary: The contamination of water by azo dyes used in textile industries is increasing rapidly, posing a significant threat to living organisms. Therefore, it is crucial to find efficient methods to remove these dyes from water. In this study, a bimetallic nanoparticle smart polymer microgel system was developed, which demonstrated excellent catalytic efficiency for degradation of various dyes in aqueous medium. The system also showed pH and temperature responsive behavior, and it was found to be a recyclable catalyst.

RSC ADVANCES (2023)

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Article Engineering, Environmental

Extraction of iron (III) ions by core-shell microgel for in situ formation of iron nanoparticles to reduce harmful pollutants from water

Muhammad Arif

Summary: This paper introduces a new system suitable for simultaneous removal of metal ions and organic dyes. Silica microgels surrounded by poly(N-vinylcaprolactam-acrylic acid) were created using the free radical precipitation polymerization method. The system was used to extract iron (III) ions from water and was characterized using various techniques. The resulting iron nanoparticles loaded in the microgels were found to efficiently catalyze the reduction of organic pollutants and toxic transition metal ions.

JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING (2023)

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Article Chemistry, Multidisciplinary

Polymer microgels for the stabilization of gold nanoparticles and their application in the catalytic reduction of nitroarenes in aqueous media

Muhammad Arif et al.

Summary: Polymer microgels with a polystyrene core and poly(N-isopropylmethacrylamide) shell were synthesized, and gold nanoparticles were successfully incorporated into the shell region. The Au-P(STY@NIPM) system was found to be an efficient and recyclable catalyst for the conversion of nitroarenes to aminoarenes using NaBH4 as a reductant.

RSC ADVANCES (2022)

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Article Chemistry, Physical

Multi-functional organic-inorganic hydrogel microspheres as efficient catalytic system for reduction of toxic dyes in aqueous medium

Muhammad Shahid et al.

Summary: In this study, p(NAM) colloidal particles were synthesized and an Ag-p(NAM) organic-inorganic hybrid with fascinating catalytic properties was fabricated. The catalytic system showed efficient reduction of toxic dyes from aqueous medium and could be recycled and reused with almost the same catalytic activity.

ZEITSCHRIFT FUR PHYSIKALISCHE CHEMIE-INTERNATIONAL JOURNAL OF RESEARCH IN PHYSICAL CHEMISTRY & CHEMICAL PHYSICS (2022)

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Article Chemistry, Applied

Chitosan hydrogel wrapped bimetallic nanoparticles based efficient catalysts for the catalytic removal of organic pollutants and hydrogen production

Esraa M. Bakhsh et al.

Summary: A novel catalytic system based on bimetallic nanoparticles entrapped chitosan hydrogel container (Cu-Ag/CH, Cu-Co/CH, Cu-Ni/CH) was prepared for efficient water treatment and H-2 generation, as well as reduction of organic pollutants. Among the catalysts, Cu-Co/CH showed superior performance in catalytic H-2 generation, while Cu-Ni/CH exhibited better efficiency in catalytic reduction of toxic contaminants.

APPLIED ORGANOMETALLIC CHEMISTRY (2022)

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Article Engineering, Chemical

Highly selective recovery of perfluorooctanoic acid from semiconductor wastewater via adsorption on pH-stimulated poly (dimethyl amino) ethyl methacrylate microgels

Yueping Bao et al.

Summary: This study reported a novel water gel material for the selective recovery of high concentration PFOA. The results showed that the water gel had a high adsorption capacity and selectivity for PFOA under specific conditions. Additionally, the water gel exhibited pH responsiveness, allowing for easy release of PFOA. Incorporating the water gel into a dense membrane enabled effective separation of colloidal particles in a water system.

SEPARATION AND PURIFICATION TECHNOLOGY (2022)

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Article Chemistry, Physical

Extraction of copper ions from aqueous medium by microgel particles for in-situ fabrication of copper nanoparticles to degrade toxic dyes

Muhammad Arif et al.

Summary: In this study, monodisperse core shell microgel particles with a diameter of 88 +/- 3 nm were synthesized and characterized. The adsorption of copper ions and catalytic reduction of organic pollutants by the microgel particles were investigated.

ZEITSCHRIFT FUR PHYSIKALISCHE CHEMIE-INTERNATIONAL JOURNAL OF RESEARCH IN PHYSICAL CHEMISTRY & CHEMICAL PHYSICS (2022)

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Article Chemistry, Inorganic & Nuclear

Catalytic degradation of organic dyes using Au-poly (styrene@N-isopropylmethacrylamide) hybrid microgels

Muhammad Arif et al.

Summary: Poly(styrene@N-isopropylmethacrylamide) microgel particles were prepared using seed facilitated free radical precipitation polymerization technique, and gold nanoparticles were integrated into the shell of the microgel particles to form a gold-P(ST@NPM) hybrid microgel system with excellent catalytic activity.

INORGANIC CHEMISTRY COMMUNICATIONS (2022)

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Article Chemistry, Applied

Efficient reduction of organic pollutants and H2 generation using bimetallic nanoparticles coated alginate hydrogel beads

Shahid Ahmad et al.

Summary: A simple method was used to prepare calcium alginate-activated carbon composite beads (Alg-ACBDs) and decorate them with different metal nanoparticles. The Fe-0-Cu-0/Alg-ACBDs catalyst showed efficient reduction reaction for 4-NP and MO.

MICROPOROUS AND MESOPOROUS MATERIALS (2022)

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Article Materials Science, Multidisciplinary

Catalytic degradation of methyl orange using bimetallic nanoparticles loaded into poly(N-isopropylmethacrylamide) microgels

Muhammad Arif et al.

Summary: A catalytic system containing bimetallic nanoparticles loaded in polymer microgels was designed to degrade organic dyes in water. The system showed remarkable catalytic efficiency, even after recycling, with a degradation rate of 90%.

MATERIALS TODAY COMMUNICATIONS (2022)

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Review Chemistry, Multidisciplinary

Recent Advances in Microgels: From Biomolecules to Functionality

Yufan Xu et al.

Summary: This review discusses the applications and potential of microgels in various fields, including biomedical research, materials science, and bioengineering. The synthesis of microgels using microfluidic technologies is a key enabling technology for tailoring their properties. Microgels play important roles in liquid-liquid phase separation, micromechanics, biosensors, and regenerative medicine.

SMALL (2022)

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Article Chemistry, Applied

CuAu bimetallic plasmonic-enhanced catalysts supported on alginate biohydrogels

Oscar Ramirez et al.

Summary: In this study, a series of hybrid materials composed of inorganic plasmonic mono- and bimetallic nanoparticles supported on organic bio-based hydrogel beads were synthesized and characterized. The bimetallic materials exhibited a localized surface plasmon resonance in the visible region and showed higher catalytic activity compared to the monometallic counterparts. Furthermore, the materials also demonstrated enhanced photocatalytic properties.

CARBOHYDRATE POLYMERS (2022)

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Review Chemistry, Multidisciplinary

Complete life of cobalt nanoparticles loaded into cross-linked organic polymers: a review

Muhammad Arif

Summary: The unique combination of cobalt nanoparticles and smart polymer microgels has attracted great interest in the production of hydrogen gas and removal of toxic dyes from water. The responsive behavior of microgels makes cobalt nanoparticle-loaded microgels most suitable for these applications. Various types of cobalt nanoparticle microgels have been reported in the literature, with hybrid microgel formations playing an important role. This report provides a comprehensive review of the synthesis, classification, characterization, and applications of cobalt nanoparticle microgels, with a focus on their catalytic generation of hydrogen and reduction of pollutants.

RSC ADVANCES (2022)

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Article Chemistry, Multidisciplinary

Enhanced catalytic activity in hydrogen production from hydrolysis of sodium borohydride using starch hydrogel-CoNi bimetallic alloys

Sanoe Chairam et al.

Summary: In this study, starch hydrogel was used as a template to synthesize starch hydrogel-CoNi bimetallic alloys, which showed promising catalytic activity in hydrogen production. Various factors affecting the hydrolysis of NaBH4 were investigated, with the catalyst showing good reusability and stability. This approach demonstrates great potential for large-scale synthesis of bimetallic alloys with starch hydrogel as a biocompatible material for catalysis applications.

JOURNAL OF THE IRANIAN CHEMICAL SOCIETY (2021)

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Review Materials Science, Composites

New Advances and Future Possibilities in Forming Technology of Hybrid Metal-Polymer Composites Used in Aerospace Applications

Tomasz Trzepiecinski et al.

Summary: Fibre metal laminates are advanced composite materials used in the production of high-end products, such as carbon, aramid, and glass reinforced aluminum laminates. This review focuses on the developing technologies and forming methods for hybrid metal-polymer composites, as well as summarizing the progress and future directions of research on HMPCs.

JOURNAL OF COMPOSITES SCIENCE (2021)

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Article Environmental Sciences

Cu-Fe embedded cross-linked 3D hydrogel for enhanced reductive removal of Cr(VI): Characterization, performance, and mechanisms

Yin Wang et al.

Summary: This study demonstrates the innovative fabrication of a three-dimensionally structured Cu-Fe embedded cross-linked cellulose hydrogel (nFeCu-CH) with significantly enhanced adsorption-reduction property towards Cr(VI) wastewater. The superior reductive activity and recyclability of nFeCu-CH make it a potential material for the remediation of Cr(VI) contaminated wastewater.

CHEMOSPHERE (2021)

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Article Materials Science, Multidisciplinary

Anionic hydrogel fabricated with metal nanoparticles: highly efficient and easily recyclable catalysts

Hina Naeem et al.

Summary: Poly(methacrylic acid) hydrogels were synthesized using a free radical polymerization process as templates for the synthesis of silver, cobalt, and bimetallic nanoparticles. The loaded metal ions in the hydrogels were treated with a reducing agent to obtain corresponding metal nanoparticles, which were used as catalysts for degrading organic dyes and nitro compounds in contaminated water. Various parameters of the catalysts and their reusability were investigated.

SOFT MATERIALS (2021)

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Review Chemistry, Physical

Gold nanoparticles and polymer microgels: Last five years of their happy and successful marriage

Muhammad Arif et al.

Summary: The unique combination of gold nanoparticles and smart polymer microgels has shown great potential in biomedical, environmental, and catalytic applications, with various morphologies and architectures available in literature. The structure of hybrid microgels plays a crucial role in their applications, leading to the design of specific assemblies for particular purposes. Recent advancements in the classification, synthesis, properties, characterization, and applications of gold nanostructures loaded into microgels have been reviewed, focusing on their biomedical, catalytic, environmental, and sensing applications in the past five years.

JOURNAL OF MOLECULAR LIQUIDS (2021)

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Article Multidisciplinary Sciences

Synthesis of bimetallic nanoparticles loaded on to PNIPAM hybrid microgel and their catalytic activity

Mohib Ullah Kakar et al.

Summary: This study successfully synthesized carboxyl-functionalized PNIPAM microgels with excellent catalytic properties, incorporating copper, palladium, and Cu/Pd nanoparticles into thiol-functionalized PNIPAM microgels. The prepared Cu/Pd hybrid exhibited remarkable catalytic properties for the degradation of 4-Nitrophenol and methylene blue, outperforming its atomic analogue.

SCIENTIFIC REPORTS (2021)

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Article Engineering, Environmental

Highly porous cryogels loaded with bimetallic nanoparticles as an efficient antimicrobial agent and catalyst for rapid reduction of water-soluble organic contaminants

Abdul Haleem et al.

Summary: The study focused on developing robust materials with antibacterial and catalytic activities for efficient reduction and removal of organic pollutants from wastewater. The materials were characterized using different techniques, including FT-IR, XRD, TGA, SEM, EDX, and TEM, confirming their stability, uniform distribution of nanoparticles, and high antibacterial and catalytic performance. The bimetallic nanoparticle loaded cryogel exhibited excellent stability and significant antibacterial and catalytic activities.

JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING (2021)

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Article Materials Science, Biomaterials

In situ synthesis of superorganism-like Au NPs within microgels with ultra-wide absorption in visible and near-infrared regions for combined cancer therapy

Shengtao Wang et al.

Summary: In this study, a superstructure resembling a superorganism was created by using microgel to densely pack 50 nm Au NPs, allowing for collective plasmon coupling and efficient photothermal conversion. This system also demonstrated the ability to load photosensitive drugs for combined cancer treatments of photothermal therapy and photodynamic therapy.

BIOMATERIALS SCIENCE (2021)

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Review Chemistry, Analytical

Hybrid Microgels for Catalytic and Photocatalytic Removal of Nitroarenes and Organic Dyes From Aqueous Medium: A Review

Muhammad Shahid et al.

CRITICAL REVIEWS IN ANALYTICAL CHEMISTRY (2020)

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Article Polymer Science

Preparation and catalytic properties of modified PGMA-based pH-responsive hydrogel films as a novel template for in situ synthesis of Au, Ag, and Au:Ag nanoparticles

Gokhan Kocak

JOURNAL OF APPLIED POLYMER SCIENCE (2020)

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Article Chemistry, Physical

Extraction of cobalt ions from aqueous solution by microgels for in-situ fabrication of cobalt nanoparticles to degrade toxic dyes: A two fold-environmental application

Muhammad Shahid et al.

CHEMICAL PHYSICS LETTERS (2020)

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Article Chemistry, Analytical

Cu/Au/Pt trimetallic nanoparticles coated with DNA hydrogel as target-responsive and signal-amplification material for sensitive detection of microcystin-LR

Pian Wu et al.

ANALYTICA CHIMICA ACTA (2020)

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Article Environmental Sciences

Silver nanoparticles stabilized in polymer hydrogels for catalytic degradation of azo dyes

Sadia Iqbal et al.

ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY (2020)

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Article Physics, Condensed Matter

Smart microgel-metal hybrid particles of PNIPAM-co-PAA@AgAu: synthesis, characterizations and modulated catalytic activity

Prachi Bhol et al.

JOURNAL OF PHYSICS-CONDENSED MATTER (2020)

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Review Materials Science, Composites

Surfactants: Recent advances and their applications

Samy M. Shaban et al.

COMPOSITES COMMUNICATIONS (2020)

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Article Nanoscience & Nanotechnology

Controlling Size and Morphology in Hybrid Core@Shell and Core@Shell@Satellite Nanostructures for Sensing by Surface-Enhanced Raman Scattering

Carlos Alarcon-Fernandez et al.

ACS APPLIED NANO MATERIALS (2020)

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Article Materials Science, Multidisciplinary

Comparison of Cross-Linked Branched and Linear Poly(ethylene imine) Microgel Microstructures and Their Impact in Antimicrobial Behavior, Copper Chelation, and Carbon Dioxide Capture

Molly E. Payne et al.

ACS APPLIED POLYMER MATERIALS (2020)

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Article Nanoscience & Nanotechnology

Temperature-Controlled Catalysis by Core-Shell-Satellite AuAg@pNIPAM@Ag Hybrid Microgels: A Highly Efficient Catalytic Thermoresponsive Nanoreactor

Lazaros Tzounis et al.

ACS APPLIED MATERIALS & INTERFACES (2019)

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Article Chemistry, Multidisciplinary

Coupling membrane and Fe-Pd bimetallic nanoparticles for trichioroethene removing from water

Bangkai Li et al.

JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY (2019)

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Article Polymer Science

Photocrosslinked hybrid composites with Ag, Au or Au-Ag NPs as visible-light triggered photocatalysts for degradation/reduction of aromatic nitroderivatives

Violeta Melinte et al.

EUROPEAN POLYMER JOURNAL (2019)

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Article Environmental Sciences

Kinetic research on dechlorinating dichlorobenzene in aqueous system by nano-scale nickel/iron loaded with CMC/NFC hydrogel

Xiao-Fang Wan et al.

CHEMOSPHERE (2018)

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Review Pharmacology & Pharmacy

Sterilization of implantable polymer-based medical devices: A review

Namita P. Tipnis et al.

INTERNATIONAL JOURNAL OF PHARMACEUTICS (2018)

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Article Chemistry, Multidisciplinary

Preparation and characterization of Ag-Pd bimetallic nano-catalysts in thermosensitive microgel nano-reactor

Tao Zhang et al.

RSC ADVANCES (2018)

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Article Chemistry, Multidisciplinary

Ag-Au bimetallic nanocomposites stabilized with organic-inorganic hybrid microgels: synthesis and their regulated optical and catalytic properties

Lei Li et al.

RSC ADVANCES (2018)

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Article Chemistry, Applied

Au Core-Pd Shell Bimetallic Nanoparticles Immobilized within Hyper-Cross-Linked Polystyrene for Mechanistic Study of Suzuki Cross-Coupling: Homogeneous or Heterogeneous Catalysis?

Nadezhda A. Nemygina et al.

ORGANIC PROCESS RESEARCH & DEVELOPMENT (2018)

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Article Chemistry, Physical

Hydrogel covered bimetallic Co:Ni magnetic nano alloy for protein adsorption in biomedical application

Kausar Rajar et al.

JOURNAL OF MOLECULAR STRUCTURE (2017)

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Article Polymer Science

Green Synthesis of Smart Metal/Polymer Nanocomposite Particles and Their Tuneable Catalytic Activities

Noel Peter Bengzon Tan et al.

POLYMERS (2016)

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Article Materials Science, Multidisciplinary

Self-assembly of monodisperse composite microgels with bimetallic nanorods as core and PNIPAM as shell into close-packed monolayers and SERS efficiency

Xu Dong et al.

MATERIALS & DESIGN (2016)

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Review Polymer Science

Active polymer nanofibers for photonics, electronics, energy generation and micromechanics

Luana Persano et al.

PROGRESS IN POLYMER SCIENCE (2015)

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Article Chemistry, Multidisciplinary

Bimetallic Au/Ag nanoparticle loading on PNIPAAm-VAA-CS8 thermoresponsive hydrogel surfaces using ss-DNA coupling, and their SERS efficiency

Anastasios C. Manikas et al.

RSC ADVANCES (2015)

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Article Chemistry, Multidisciplinary

Antibacterial nanocomposite hydrogels for superior biomedical applications: a Facile eco-friendly approach

Gownolla Malegowd Raghavendra et al.

RSC ADVANCES (2015)

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Article Chemistry, Multidisciplinary

Magnetic Co-Fe bimetallic nanoparticle containing modifiable microgels for the removal of heavy metal ions, organic dyes and herbicides from aqueous media

M. Ajmal et al.

RSC ADVANCES (2015)

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Article Chemistry, Multidisciplinary

Interfacial Assembly of Mussel-Inspired Au@Ag@ Polydopamine Core-Shell Nanoparticles for Recyclable Nanocatalysts

Jiajing Zhou et al.

ADVANCED MATERIALS (2014)

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Article Chemistry, Multidisciplinary

Temperature Controlled Fluorescence on Au@Ag@PNIPAM-PTEBS Microgels: Effect of the Metal Core Size on the MEF Extension

Rafael Contreras-Caceres et al.

LANGMUIR (2014)

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Article Chemistry, Multidisciplinary

Radiation synthesis of hydrogels as carriers for catalytic nanoparticles and their use in hydrogen production from sodium borohydride

Ghada A. Mahmoud

MONATSHEFTE FUR CHEMIE (2014)

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Article Chemistry, Multidisciplinary

A general approach to mono- and bimetallic organometallic nanoparticles

Sudheendran Mavila et al.

CHEMICAL SCIENCE (2014)

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Article Chemistry, Physical

Polymer hydrogel supported Pd-Ni-B nanoclusters as robust catalysts for hydrogen production from hydrolysis of sodium borohydride

Wenyu Liu et al.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2013)

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Article Engineering, Biomedical

Water-dispersible multifunctional hybrid nanogels for combined curcumin and photothermal therapy

Weitai Wu et al.

BIOMATERIALS (2011)

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Article Chemistry, Physical

Synthesis and physicochemical properties of cationic microgels based on poly(N-isopropylmethacrylamide)

Xiaobo Hu et al.

COLLOID AND POLYMER SCIENCE (2011)

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Article Chemistry, Physical

The on demand generation of hydrogen from Co-Ni bimetallic nano catalyst prepared by dual use of hydrogel: As template and as reactor

Nurettin Sahiner et al.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2011)

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Article Chemistry, Multidisciplinary

In Situ Growth of Catalytic Active Au - Pt Bimetallic Nanorods in Thermoresponsive Core - Shell Microgels

Yan Lu et al.

ACS NANO (2010)

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Core-shell hybrid nanogels for integration of optical temperature-sensing, targeted tumor cell imaging, and combined chemo-photothermal treatment

Weitai Wu et al.

BIOMATERIALS (2010)

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Review Pharmacology & Pharmacy

Drug release kinetics and transport mechanisms of non-degradable and degradable polymeric delivery systems

Yao Fu et al.

EXPERT OPINION ON DRUG DELIVERY (2010)

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Article Chemistry, Physical

Seeding Growth of Pd/Au Bimetallic Nanoparticles on Highly Cross-Linked Polymer Microspheres with Ionic Liquid and Solvent-Free Hydrogenation

Baoji Hu et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2010)

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Article Chemistry, Multidisciplinary

Synthesis of Multifunctional Composite Microgels via In Situ Ni Growth on pNIPAM-Coated Au Nanoparticles

Ana Sanchez-Iglesias et al.

ACS NANO (2009)

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Review Chemistry, Multidisciplinary

Hyperbranched and Highly Branched Polymer Architectures-Synthetic Strategies and Major Characterization Aspects

Brigitte I. Voit et al.

CHEMICAL REVIEWS (2009)

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Article Chemistry, Physical

Tunable Photolumineseence of Ag Nanocrystals in Multiple-Sensitive Hybrid Microgels

Weitai Wu et al.

CHEMISTRY OF MATERIALS (2009)

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Article Chemistry, Physical

Effects of Temperature and pH on the Contraction and Aggregation of Microgels in Aqueous Suspensions

Nodar Al-Manasir et al.

JOURNAL OF PHYSICAL CHEMISTRY B (2009)

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Article Chemistry, Physical

Zwitterionic Poly(betaine-N-isopropylacrylamide) Microgels: Properties and Applications

Mallika Das et al.

CHEMISTRY OF MATERIALS (2008)

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Article Chemistry, Multidisciplinary

Study of pH-Responsive microgels containing methacrylic acid: Effects of particle composition and added calcium

Helene Dalmont et al.

LANGMUIR (2008)

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Article Polymer Science

Responsive backbones based on alternating triazole-pyridine/benzene copolymers: From helically folding polymers to metallosupramolecularly crosslinked gels

Robert M. Meudtner et al.

MACROMOLECULAR RAPID COMMUNICATIONS (2008)

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Review Polymer Science

Construction of linear polymers, dendrimers, networks, and other polymeric architectures by copper-catalyzed azide-alkyne cycloaddition Click chemistry

Jeremiah A. Johnson et al.

MACROMOLECULAR RAPID COMMUNICATIONS (2008)

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Article Polymer Science

Preparation of novel metallic and bimetallic cross-linked poly(vinyl alcohol) nanocomposites under microwave irradiation

Mallikarjuna N. Nadagouda et al.

MACROMOLECULAR RAPID COMMUNICATIONS (2007)

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Article Chemistry, Physical

Dispersing multi-walled carbon nanotubes with water-soluble block copolymers and their use as supports for metal nanoparticles

Zhimin Wang et al.

CARBON (2007)

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Article Chemistry, Physical

In situ metal particle preparation in cross-linked poly(2-acrylamido-2-methyl-1-propansulfonic acid) hydrogel networks

Nurettin Sahiner

COLLOID AND POLYMER SCIENCE (2006)

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Article Chemistry, Multidisciplinary

Hybrid microgels with reversibly changeable multiple brilliant color

D Suzuki et al.

LANGMUIR (2006)

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Review Chemistry, Multidisciplinary

Dendrimer-encapsulated metal nanoparticles: Synthesis, characterization, and applications to catalysis

RM Crooks et al.

ACCOUNTS OF CHEMICAL RESEARCH (2001)

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