期刊
ADVANCED MATERIALS
卷 27, 期 47, 页码 7824-7831出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.201503730
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资金
- Ministry of Science and Technology of China [2014CB239402, 2013CB834505]
- Chinese Academy of Sciences [KGZD-EW-T05]
- National Natural Science Foundation of China [21401206, 51322213, 21301183, 51172245, 91127005]
- Beijing Natural Science Foundation [2152033]
- National Program for Support of Top-Notch Young Professionals
Defect-rich ultrathin ZnAl-layered double hydroxide nanosheets are successfully prepared. Under UV-vis irradiation, these nanosheets are superior effi cient catalysts for the photoreduction of CO2 to CO with water. The formed oxygen vacancies lead to the formation of coordinatively unsaturated Zn+ centers within the nanosheets, responsible for the very high photocatalytic activities.
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