Coupling Single-Ni-Atom with Ni-Co Alloy Nanoparticle for Synergistically Enhanced Oxygen Reduction Reaction

Article Chemistry, Multidisciplinary

Decorating Single-Atomic Mn Sites with FeMn Clusters to Boost Oxygen Reduction Reaction

Heng Liu et al.

Summary: By utilizing post-adsorption and secondary pyrolysis, we have successfully constructed single-atomic Mn sites decorated with atomic clusters, which exhibit excellent performance in oxygen reduction reaction (ORR).

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2023)

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Article Chemistry, Multidisciplinary

Clusters Induced Electron Redistribution to Tune Oxygen Reduction Activity of Transition Metal Single-Atom for Metal-Air Batteries

Hongjiao Huang et al.

Summary: By coating and etching metal clusters, the activity of metal single-atoms can be optimized through electron redistribution and modulation of M-N bond lengths, resulting in enhanced ORR activity. This strategy shows great potential in energy storage devices.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Chemistry, Multidisciplinary

Strategic Modulation of Target-Specific Isolated Fe,Co Single-Atom Active Sites for Oxygen Electrocatalysis Impacting High Power Zn-Air Battery

Subhajit Sarkar et al.

Summary: In this study, a bifunctional electrocatalyst with target-specific Fe-N-4/C and Co-N-4/C isolated active sites was developed, showing a symbiotic effect on overall oxygen electrocatalysis performances. The dualism of N-dopants and binary metals lowered the d-band centers of Fe and Co in the catalyst, improving the overpotential of the catalytic processes. The Fe, Co, N-C catalyst demonstrated a high areal power density in both liquid and solid-state Zn-air batteries, making it a suitable candidate for air cathode material in ZABs.

ACS NANO (2022)

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Article Chemistry, Multidisciplinary

Metal-Organic Framework-Derived Graphene Mesh: a Robust Scaffold for Highly Exposed Fe-N4 Active Sites toward an Excellent Oxygen Reduction Catalyst in Acid Media

Jingjing Li et al.

Summary: This study demonstrates the use of a special ultrathin nitrogen-doped graphene nanomesh as a scaffold for highly exposed Fe-N-4 active sites. By adjusting the pore sizes of the nanomesh, highly loaded single-atom catalysts can be synthesized, which exhibit superior performance in oxygen reduction reactions and fuel cell tests. This work provides a novel strategy for constructing highly exposed transition metals and nitrogen co-doped carbon materials catalysts.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2022)

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Article Multidisciplinary Sciences

Iron atom-cluster interactions increase activity and improve durability in Fe-N-C fuel cells

Xin Wan et al.

Summary: This study demonstrates the high activity and stability of an Fe-N-C catalyst for oxygen reduction reaction in acidic fuel cells by introducing nitrogen-coordinated iron clusters and closely surrounding Fe-N-4 active sites. The strong electronic interaction between the iron clusters and the Fe-N-4 sites optimizes the adsorption strength of reaction intermediates and enhances the catalyst's turnover frequency and demetalation resistance.

NATURE COMMUNICATIONS (2022)

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Article Chemistry, Physical

Atomically dispersed Pt and Fe sites and Pt-Fe nanoparticles for durable proton exchange membrane fuel cells

Fei Xiao et al.

Summary: Researchers have designed a hybrid electrocatalyst consisting of atomically dispersed platinum and iron single atoms, as well as platinum-iron alloy nanoparticles. This electrocatalyst exhibits higher activity and durability in proton exchange membrane fuel cells.

NATURE CATALYSIS (2022)

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Article Nanoscience & Nanotechnology

Graphene-nanopocket-encaged PtCo nanocatalysts for highly durable fuel cell operation under demanding ultralow-Pt-loading conditions

Zipeng Zhao et al.

Summary: The authors report the design and development of ultrathin PtCo nanocatalysts encased in graphene nanopockets, which exhibit excellent electrochemical accessibility and durability under low loading conditions. These catalysts show promising fuel cell performance, making them ideal for reducing fuel cell costs.

NATURE NANOTECHNOLOGY (2022)

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Article Nanoscience & Nanotechnology

Anchoring Bimetal Single Atoms and Alloys on N-Doping-Carbon Nanofiber Networks for an Efficient Oxygen Reduction Reaction and Zinc-Air Batteries

Bowen Liu et al.

Summary: This study reports a bimetal single-atom-based nanofiber network for efficient ORR electrocatalysis and zinc-air batteries. The versatile process developed in this study allows for mass production of efficient composite electrocatalysts. The bimetal SAC-based nanofiber networks show superior catalytic performance and device performance, attributed to the appealing intrinsic activity, the carbon shielding effect, and the hierarchical porous structure.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Nanoscience & Nanotechnology

MOF-Derived Bimetallic Pd-Co Alkaline ORR Electrocatalysts

Weixuan Xu et al.

Summary: Developing highly active, durable, and low-cost electrocatalysts for the oxygen reduction reaction (ORR) is crucial for advancing and commercializing fuel cell technologies. This study reports a novel family of Pd-Co binary alloys embedded in bimetallic organic framework-derived polyhedral carbon supports. Among the materials studied, annealed BMOF-derived Pd3Co exhibits the most promising ORR activity and stability. The strategies developed in this research provide promising insights into the rational design and synthesis of ORR electrocatalysts for alkaline fuel cells.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Chemistry, Multidisciplinary

Synergistic Hybrid Electrocatalysts of Platinum Alloy and Single-Atom Platinum for an Efficient and Durable Oxygen Reduction Reaction

Bowen Liu et al.

Summary: By anchoring platinum alloys on single-atom Pt-decorated carbon, the inherent deficiencies of Pt single-atom materials and platinum alloys are overcome, enabling efficient and durable catalysis in the ORR reaction.

ACS NANO (2022)

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Article Chemistry, Multidisciplinary

The Progress and Outlook of Metal Single-Atom-Site Catalysis

Xiao Liang et al.

Summary: Single-atom-site catalysts are a highly prosperous branch of catalysis research that have made tremendous progress in recent years. The major goal of research is to establish feasible synthetic strategies for preparing high-performance catalysts, understand the active-site structures and catalytic mechanisms, and develop practical catalysts with industrial value.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2022)

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Article Chemistry, Multidisciplinary

Fe-N-C Boosts the Stability of Supported Platinum Nanoparticles for Fuel Cells

Fei Xiao et al.

Summary: This study found that Pt/Fe-N-C has better electrochemical surface area retention compared to conventional high-surface-area carbon. In situ studies revealed that the Pt dissolution rate of Pt/Fe-N-C is 3 times smaller than that of Pt/C during cycling. Density functional theory calculations further demonstrated that Fe-N-C can provide stable support and alleviate oxide formation. This finding emphasizes the importance of carbon support selection for achieving a more durable Pt-based electrocatalyst.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2022)

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Review Chemistry, Multidisciplinary

Intrinsic Electrocatalytic Activity Regulation of M-N-C Single-Atom Catalysts for the Oxygen Reduction Reaction

Chang-Xin Zhao et al.

Summary: This Review summarizes the regulation strategies for promoting the intrinsic electrocatalytic ORR activity of M-N-C SACs by modulation of the center metal atoms, the coordinated atoms, the environmental atoms, and the guest groups. The study includes both theoretical calculations and experimental investigations to provide a comprehensive understanding of the structure-performance relationship. Proposed future directions involve developing advanced M-N-C SACs for electrocatalytic ORR and other analogous reactions.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Simultaneously Crafting Single-Atomic Fe Sites and Graphitic Layer-Wrapped Fe3C Nanoparticles Encapsulated within Mesoporous Carbon Tubes for Oxygen Reduction

Xun Cui et al.

Summary: A simple and robust approach was employed to synthesize one-dimensional hollow tubular carbon-based materials with highly efficient oxygen reduction reaction performance. By simultaneously crafting single-atomic Fe sites and graphitic layer-wrapped Fe3C nanoparticles, the Fe-N-doped hollow mesoporous carbon tubes were successfully prepared and used as the ORR electrocatalyst. The impressive ORR performances of the Fe-N-HMCTs are attributed to the favorable configuration of active sites in conjunction with the advantageous 1D hollow tubular architecture.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Non-Bonding Interaction of Neighboring Fe and Ni Single-Atom Pairs on MOF-Derived N-Doped Carbon for Enhanced CO2 Electroreduction

Long Jiao et al.

Summary: Through the direct pyrolysis of MOFs assembled with Fe and Ni-doped ZnO nanoparticles, a novel Fe-1-Ni-1-N-C catalyst with neighboring Fe and Ni single-atom pairs on nitrogen-doped carbon support has been precisely constructed. The synergism of neighboring Fe and Ni single-atom pairs significantly boosts the electrocatalytic reduction of CO2, surpassing catalysts with separate Fe or Ni single atoms. The study reveals the importance of the communicative effect between adjacent single atoms for improved catalysis in single-atom catalysts containing multiple metal species.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Chemistry, Physical

Electronically Modified Atomic Sites Within a Multicomponent Co/Cu Composite for Efficient Oxygen Electroreduction

Qingran Zhang et al.

Summary: The novel ORR catalyst, SA-CoCu@Cu/CoNP, exhibits remarkable catalytic activity, exceptional stability, and excellent methanol tolerance in alkaline media, outperforming commercial platinum carbon under identical testing conditions and being active in acidic media. The improved ORR catalytic performance is attributed to the modified electronic structure of Co-N-x active sites due to an electron donating effect from the embedded nanoparticles and nearby Cu-N-x species.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Promoting Atomically Dispersed MnN4 Sites via Sulfur Doping for Oxygen Reduction: Unveiling Intrinsic Activity and Degradation in Fuel Cells

Lin Guo et al.

Summary: A sulfur-doped Mn-N-C catalyst was synthesized through an effective adsorption-pyrolysis process, exhibiting favorable oxygen reduction reaction (ORR) activity in acidic media. The catalyst showed enhanced performance and stability in comparison to the S-free catalyst, with insights provided into catalyst degradation associated with Mn oxidation and agglomeration. The promoted ORR activity was mainly attributed to the spatial effect from the repulsive interaction between the ORR intermediates and adjacent S dopants.

ACS NANO (2021)

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Review Chemistry, Multidisciplinary

Recent Advances in Electrocatalysts for Proton Exchange Membrane Fuel Cells and Alkaline Membrane Fuel Cells

Fei Xiao et al.

Summary: The article summarizes the current development status of PEMFCs and AMFCs, including electrocatalyst design, catalyst layer optimization, and cell performance. It discusses and compares the activity, stability, and fuel cell performance of different types of electrocatalysts for the oxygen reduction and hydrogen oxidation reactions, while also exploring research directions for further development.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

MIL-101-Derived Mesoporous Carbon Supporting Highly Exposed Fe Single-Atom Sites as Efficient Oxygen Reduction Reaction Catalysts

Xiaoying Xie et al.

Summary: Fe single-atom catalysts with atomic FeNx active sites show great promise as alternatives to platinum-based catalysts for the oxygen reduction reaction. This study utilized a mesoporous MOF NH2-MIL-101(Al) as a precursor to prepare a series of N-doped carbon supports with well-defined mesoporous structure at different pyrolysis temperatures. The resulting Fe SAC-MIL101-T catalysts showed outstanding ORR activity in alkaline media and excellent performance in zinc-air batteries.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Exceptional Electrochemical HER Performance with Enhanced Electron Transfer between Ru Nanoparticles and Single Atoms Dispersed on a Carbon Substrate

Panpan Su et al.

Summary: The study introduces a new method to control the electrocatalytic behavior of supported metal nanoparticles by dispersing single metal atoms on O-doped graphene, showing improved performance for the hydrogen evolution reaction. This approach offers a new strategy for modulating the activity and stability of metal nanoparticles in electrocatalysis processes.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Understanding the Synergistic Effects of Cobalt Single Atoms and Small Nanoparticles: Enhancing Oxygen Reduction Reaction Catalytic Activity and Stability for Zinc-Air Batteries

Zhe Wang et al.

Summary: A highly efficient and durable oxygen reduction reaction (ORR) catalyst consisting of atomically dispersed Co single atoms and small Co nanoparticles co-anchored on nitrogen-doped porous carbon nanocage was reported. The catalyst exhibited outstanding ORR activity and remarkable stability in alkaline media, outperforming Pt/C catalyst. Practical zinc-air battery assembled with this catalyst showed high power density, specific capacity, and cycling stability.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Analytical

Modulating Oxygen Reduction Behaviors on Nickel Single-Atom Catalysts to Probe the Electrochemiluminescence Mechanism at the Atomic Level

Wenling Gu et al.

Summary: This study demonstrates the potential application of carbon-supported nickel SACs as coreaction accelerators in enhancing ECL signals; By modulating the surrounding environment of the center metal atoms, control over oxygen reduction behaviors to selectively produce intermediate ROS provides an important opportunity for studying the ECL process; Experimental and calculated results suggest that the superoxide radical (O-2(center dot-)) is the main radical for the ECL reaction, with the Ni-N-4/C catalyst preferred for its four-electron pathway to activate dissolved O-2 and enhance ECL emission.

ANALYTICAL CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Decarboxylation-Induced Defects in MOF-Derived Single Cobalt Atom@Carbon Electrocatalysts for Efficient Oxygen Reduction

Shuai Yuan et al.

Summary: The study focuses on developing transition metal single-atom catalysts (SACs) for the oxygen reduction reaction (ORR) by using a decarboxylation-induced defects strategy to enhance their intrinsic activity. A gas-transport method was used to produce defective Co SACs (Co@DMOF) from carboxylate/amide mixed-linker MOF (DMOF), showing improved ORR activity compared to Co@ZIF-8-900.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Identification of Catalytic Sites for Oxygen Reduction in Metal/Nitrogen-Doped Carbons with Encapsulated Metal Nanoparticles

Ming-Xi Chen et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Multidisciplinary

Construction of Highly Active Metal-Containing Nanoparticles and FeCo-N4Composite Sites for the Acidic Oxygen Reduction Reaction

Shu-Hu Yin et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Review Chemistry, Physical

Electrocatalysis of Single-Atom Sites: Impacts of Atomic Coordination

Bingzhang Lu et al.

ACS CATALYSIS (2020)

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Review Chemistry, Multidisciplinary

Theoretical Understandings of Graphene-based Metal Single-Atom Catalysts: Stability and Catalytic Performance

Hong-Ying Zhuo et al.

CHEMICAL REVIEWS (2020)

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Review Chemistry, Multidisciplinary

Advanced Electrocatalysts with Single-Metal-Atom Active Sites

Yuxuan Wang et al.

CHEMICAL REVIEWS (2020)

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Article Chemistry, Multidisciplinary

Atomically dispersed Fe-N-C decorated with Pt-alloy core-shell nanoparticles for improved activity and durability towards oxygen reduction

Xiang Ao et al.

ENERGY & ENVIRONMENTAL SCIENCE (2020)

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Review Chemistry, Multidisciplinary

From metal-organic frameworks to single/dual-atom and cluster metal catalysts for energy applications

Chun-Chao Hou et al.

ENERGY & ENVIRONMENTAL SCIENCE (2020)

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Article Chemistry, Physical

Atomically Dispersed Cu-N-C as a Promising Support for Low-Pt Loading Cathode Catalysts of Fuel Cells

Liting Cui et al.

ACS APPLIED ENERGY MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Isolated Diatomic Ni-Fe Metal-Nitrogen Sites for Synergistic Electroreduction of CO2

Wenhao Ren et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Article Chemistry, Physical

Nitrogen-coordinated single iron atom catalysts derived from metal organic frameworks for oxygen reduction reaction

Fei Xiao et al.

NANO ENERGY (2019)

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Article Chemistry, Multidisciplinary

Markedly Enhanced Oxygen Reduction Activity of Single-Atom Fe Catalysts via Integration with Fe Nanoclusters

Xiang Ao et al.

ACS NANO (2019)

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Article Chemistry, Multidisciplinary

Atomically Dispersed Binary Co-Ni Sites in Nitrogen-Doped Hollow Carbon Nanocubes for Reversible Oxygen Reduction and Evolution

Xiaopeng Han et al.

ADVANCED MATERIALS (2019)

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Article Chemistry, Multidisciplinary

An Isolated Zinc-Cobalt Atomic Pair for Highly Active and Durable Oxygen Reduction

Ziyang Lu et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Article Chemistry, Multidisciplinary

Single-Atom Fe-Nx-C as an Efficient Electrocatalyst for Zinc-Air Batteries

Junxing Han et al.

ADVANCED FUNCTIONAL MATERIALS (2019)

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Article Chemistry, Multidisciplinary

Atomically Dispersed Transition Metals on Carbon Nanotubes with Ultrahigh Loading for Selective Electrochemical Carbon Dioxide Reduction

Yi Cheng et al.

ADVANCED MATERIALS (2018)

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Article Chemistry, Multidisciplinary

Single Tungsten Atoms Supported on MOF-Derived N-Doped Carbon for Robust Electrochemical Hydrogen Evolution

Wenxing Chen et al.

ADVANCED MATERIALS (2018)

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Review Chemistry, Multidisciplinary

Metal Catalysts for Heterogeneous Catalysis: From Single Atoms to Nanoclusters and Nanoparticles

Lichen Liu et al.

CHEMICAL REVIEWS (2018)

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Review Chemistry, Multidisciplinary

Heterogeneous single-atom catalysis

Aiqin Wang et al.

NATURE REVIEWS CHEMISTRY (2018)

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Article Chemistry, Multidisciplinary

Coordination of Atomic Co-Pt Coupling Species at Carbon Defects as Active Sites for Oxygen Reduction Reaction

Longzhou Zhang et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2018)

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Review Chemistry, Multidisciplinary

O-2 Activation by Metal Surfaces: Implications for Bonding and Reactivity on Heterogeneous Catalysts

Matthew M. Montemore et al.

CHEMICAL REVIEWS (2018)

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Article Chemistry, Multidisciplinary

Single Atomic Iron Catalysts for Oxygen Reduction in Acidic Media: Particle Size Control and Thermal Activation

Hanguang Zhang et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2017)

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Review Chemistry, Multidisciplinary

Single-Atom Electrocatalysts

Chengzhou Zhu et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2017)

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Article Chemistry, Multidisciplinary

Pyridinic-Nitrogen-Dominated Graphene Aerogels with Fe-N-C Coordination for Highly Efficient Oxygen Reduction Reaction

Xiaoyang Cui et al.

ADVANCED FUNCTIONAL MATERIALS (2016)

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Article Chemistry, Multidisciplinary

Single Cobalt Atoms with Precise N-Coordination as Superior Oxygen Reduction Reaction Catalysts

Peiqun Yin et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2016)

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Article Chemistry, Multidisciplinary

Understanding the High Activity of Fe-N-C Electrocatalysts in Oxygen Reduction: Fe/Fe3C Nanoparticles Boost the Activity of Fe-Nx

Wen-Jie Jiang et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2016)

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Review Chemistry, Multidisciplinary

On the Role of Metals in Nitrogen-Doped Carbon Electrocatalysts for Oxygen Reduction

Justus Masa et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2015)

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Article Chemistry, Multidisciplinary

Stability of Fe-N-C Catalysts in Acidic Medium Studied by Operando Spectroscopy

Chang Hyuck Choi et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2015)

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Article Chemistry, Multidisciplinary

Integrating NiCo Alloys with Their Oxides as Efficient Bifunctional Cathode Catalysts for Rechargeable Zinc-Air Batteries

Xien Liu et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2015)

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Article Multidisciplinary Sciences

Highly active oxygen reduction non-platinum group metal electrocatalyst without direct metal-nitrogen coordination

Kara Strickland et al.

NATURE COMMUNICATIONS (2015)

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Article Chemistry, Multidisciplinary

ZIF-8 Derived Graphene-Based Nitrogen-Doped Porous Carbon Sheets as Highly Efficient and Durable Oxygen Reduction Electrocatalysts

Hai-xia Zhong et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2014)

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Editorial Material Chemistry, Multidisciplinary

Metal-Organic Frameworks (MOFs)

Hong-Cai ''Joe'' Zhou et al.

CHEMICAL SOCIETY REVIEWS (2014)

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Review Chemistry, Multidisciplinary

Flexible metal-organic frameworks

A. Schneemann et al.

CHEMICAL SOCIETY REVIEWS (2014)

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Article Chemistry, Multidisciplinary

Iron Encapsulated within Pod-like Carbon Nanotubes for Oxygen Reduction Reaction

Dehui Deng et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2013)

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Editorial Material Chemistry, Multidisciplinary

Introduction to Metal-Organic Frameworks

Hong-Cai Zhou et al.

CHEMICAL REVIEWS (2012)

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Review Multidisciplinary Sciences

Electrocatalyst approaches and challenges for automotive fuel cells

Mark K. Debe

NATURE (2012)

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Article Nanoscience & Nanotechnology

Dependence of the blocking temperature in exchange biased ferromagnetic/antiferromagnetic bilayers on the thickness of the antiferromagnetic layer

X. Y. Lang et al.

NANOTECHNOLOGY (2007)

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Coupling Single-Ni-Atom with Ni-Co Alloy Nanoparticle for Synergistically Enhanced Oxygen Reduction Reaction

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