☆ 4.8 Review

Recent developments on iron and nickel-based transition metal nitrides for overall water splitting: A critical review

COORDINATION CHEMISTRY REVIEWS (2023)

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Article Chemistry, Physical

Coupling of ruthenium with hybrid metal nitrides heterostructure as bifunctional electrocatalyst for water electrolysis

Huijie Wang et al.

Summary: This study proposes a simple nitridation route to design a hybrid material, Ru-NiWNx, which contains both ruthenium species and mixed metal nitride matrices. The Ru-NiWNx catalyst exhibits excellent bifunctional activity in alkaline electrolytes, with high catalytic activity and conductivity, making it suitable for overall water splitting for hydrogen production.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2023)

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Review Chemistry, Multidisciplinary

In Situ Investigation on Life-Time Dynamic Structure-Performance Correlation Toward Electrocatalyst Service Behavior in Water Splitting

Yong Xie et al.

Summary: Efforts have been focused on high-performance electrocatalysts for water splitting to address the issue of fossil fuel scarcity. With the development of in situ techniques, understanding the dynamic service behaviors of electrocatalysts has become crucial for establishing lifetime structure-performance correlations. Critical challenges and prospects are discussed for establishing these correlations.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Review Chemistry, Multidisciplinary

Critical Review, Recent Updates on Zeolitic Imidazolate Framework-67 (ZIF-67) and Its Derivatives for Electrochemical Water Splitting

Harsharaj S. Jadhav et al.

Summary: Designing and constructing low-cost electrocatalysts with high activity and stability is challenging. This review focuses on metal-organic frameworks (MOFs) as precursor materials for efficient electrocatalysis. Different synthesis approaches and strategies to enhance activity and stability are discussed. The review also provides insights into the applications of MOFs in oxygen and hydrogen evolution reactions and overall water splitting.

ADVANCED MATERIALS (2022)

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Review Chemistry, Multidisciplinary

Single-Atom Engineering to Ignite 2D Transition Metal Dichalcogenide Based Catalysis: Fundamentals, Progress, and Beyond

Xin Wang et al.

Summary: Single-atom catalysis is a pivotal milestone in heterogeneous catalysis, with superior performance and atomic utilization. Recent developments have expanded the single-atom family through different motifs and substrates. This review aims to summarize and discuss the development and applications of 2D TMD-based single-atom catalysis, highlighting the importance of in situ characterization techniques.

CHEMICAL REVIEWS (2022)

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Article Electrochemistry

Integration of heterointerface and porosity engineering to achieve efficient hydrogen evolution of 2D porous NiMoN nanob elts coupled with Ni particles

Zhihui Li et al.

Summary: The design of 2D Ni/Ni0.2Mo0.8N porous heterojunction nanobelts as effective catalyst for the HER is presented, with the intimate combination of Ni and Ni0.2Mo0.8N forming plentiful active sites at the heterojuctional interface. The 2D porous structure provides large accessible surface and promotes mass/charge transfer. The optimized catalysts exhibit excellent HER activity and long-term durability.

ELECTROCHIMICA ACTA (2022)

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Article Chemistry, Multidisciplinary

Phase reconfiguration of multivalent nickel sulfides in hydrogen evolution

Yu Sun et al.

Summary: Deciphering the dynamic evolution of a catalyst's atomic and electronic structure under operating conditions is crucial for understanding its activity origin and improving catalyst design. The study revealed the dynamic reconstruction process from surface to bulk, mediated by sulfur vacancies, with partial Fe substitution enhancing HER performance. The research also uncovered the tendency of transition metals towards lower valence states in the catalytically terminated phase during the HER, highlighting the dynamic correlation between structure and activity.

ENERGY & ENVIRONMENTAL SCIENCE (2022)

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Article Engineering, Chemical

Nickel-Rich Ni3N Particles Stimulated by Defective Graphitic Carbon Nitrides for the Effective Oxygen Evolution Reaction

Xinyue Luo et al.

Summary: In this study, an electrocatalyst composed of nickel-rich nickel nitride (NR-Ni3N) and graphitic carbon nitrides (GCNs) was developed for efficient oxygen evolution reaction (OER). The composite exhibited a low overpotential, small Tafel slope, and minimal activity loss after long-term testing, outperforming pure Ni3N and even the noble catalyst RuO2. The excellent OER performance of NR-Ni3N/GCNs can be attributed to the generation of a Ni-rich region and the strong synergistic effect between Ni-Ni3N heterojunction and GCNs.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2022)

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Article Chemistry, Physical

Heterostructured nickel/vanadium nitrides composites for efficient electrocatalytic hydrogen evolution in neutral medium

Yuanman Ni et al.

Summary: This study reports on heterostructured nitrides composites made of Ni3N and VN, which exhibit remarkable hydrogen evolution activity and durability in a neutral medium. The Ni3N-VN composite rivals the state-of-the-art Pt/C electrocatalyst, with lower overpotential and higher current densities, attributed to its tailored electronic structures and promoted water adsorption and dissociation.

JOURNAL OF POWER SOURCES (2022)

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Article Chemistry, Multidisciplinary

Boosting Alkaline Hydrogen and Oxygen Evolution Kinetic Process of Tungsten Disulfide-Based Heterostructures by Multi-Site Engineering

Jinsong Zeng et al.

Summary: This study introduces a multi-site engineering strategy for developing robust WS2-based hybrid electrocatalysts on mesoporous bimetallic nitride nanoarrays for efficient water splitting. The hybrid catalyst exhibits exceptional bifunctional properties for hydrogen and oxygen evolution reactions in base with excellent large-current durability, showcasing promising potential for designing WS2-based heterogeneous electrocatalysts for water electrolysis.

SMALL (2022)

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Article Chemistry, Multidisciplinary

Surface Phase Engineering Modulated Iron-Nickel Nitrides/Alloy Nanospheres with Tailored d-Band Center for Efficient Oxygen Evolution Reaction

Qiming Chen et al.

Summary: The study presents a surface phase engineering strategy to enhance the OER performance of transition metal nitrides, with the synthesized FeNi3-N catalyst showing excellent OER performance in alkaline media. The dual-phase nitrides induced by atom migration on the surface of the catalyst are favorable for decreasing the energy barrier, balancing the absorption and desorption of intermediates, and promoting the OER electrochemical performance.

SMALL (2022)

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Article Chemistry, Applied

Remarkable synergistic effect in cobalt-iron nitride/alloy nanosheets for robust electrochemical water splitting

Mingpeng Chen et al.

Summary: A novel three-step strategy is reported to construct cobalt-iron nitride/alloy nanosheets on nickel foam as a bifunctional catalyst for efficient electrochemical water splitting. The optimized composition of the catalyst can achieve ultra-low overpotentials for both hydrogen and oxygen evolution reactions, boosting overall water splitting with stable performance.

JOURNAL OF ENERGY CHEMISTRY (2022)

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Article Chemistry, Physical

Highly efficient electrocatalytic hydrogen evolution coupled with upcycling of microplastics in seawater enabled via Ni3N/W5N4 janus nanostructures

Fahao Ma et al.

Summary: In this study, a Ni3N/W5N4 nanostructure was designed to achieve efficient electrochemical hydrogen evolution reaction (HER) and microplastics reforming. The new material exhibits Pt-like HER performance and excellent stability, enabling the upgrading of plastic wastes and energy-saving hydrogen production in seawater.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Chemistry, Physical

Bifunctional Ni-Fe/NiMoNx nanosheets on Ni foam for high-efficiency and durable overall water splitting

Yu Qiu et al.

Summary: An efficient and durable bifunctional Ni-Fe/NiMoNx electrocatalyst has been synthesized, exhibiting significant performances in both hydrogen and oxygen evolution reactions. It requires low energy input for overall water splitting.

CATALYSIS COMMUNICATIONS (2022)

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Article Energy & Fuels

Enhanced Oxygen Evolution Catalytic Activity of Ni3Mo3N-MoO2-NiO Nanoparticles via Synergistic Effect

Bin Peng et al.

Summary: This study reports the synthesis of ternary Ni3Mo3N-MoO2-NiO nanoparticles catalyst and its derivatives through pyrolysis method. The catalyst exhibits superior performance in the oxygen evolution reaction, with favorable activity, low overpotential and Tafel slope, as well as excellent stability.

ENERGY & FUELS (2022)

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Article Chemistry, Physical

Pronounced effect of phosphidization on the performance of CoOx encapsulated N-doped carbon nanotubes towards oxygen evolution reaction

Faiza Zulfiqar et al.

Summary: Research on water splitting reaction is important for exploring a low carbon emission alternative energy source. A novel electrocatalyst, CoOx-CoP/N-CNTs, was prepared via phosphidization process and showed improved oxygen evolution reaction (OER) activity compared to unphosphidized material, CoOx/N-CNTs. The phosphidized material exhibited lower overpotential and higher current density.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2022)

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Article Chemistry, Physical

Ru-doped 3D porous Ni3N sphere as efficient Bi- functional electrocatalysts toward urea assisted water-splitting

Yibing Liu et al.

Summary: In this study, Ru-doped 3D porous Ni3N spheres were synthesized as urea oxide electrocatalyst. The catalyst exhibited good bifunctional catalytic performance for hydrogen evolution and oxygen evolution reactions with low overpotentials. It also showed good electrocatalytic performance in neutral and alkaline seawater electrolytes. Furthermore, the catalyst demonstrated extraordinary catalytic activity and stability toward urea oxide. It can be powered by sustainable energy sources such as wind, solar, and thermal energies.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2022)

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Article Chemistry, Physical

Heterostructure engineering of iridium species on nickel/molybdenum nitride for highly-efficient anion exchange membrane water electrolyzer

Huijie Wang et al.

Summary: This study successfully developed a novel catalyst for water electrolysis systems, which exhibits high activity and bifunctional characteristics, presenting excellent reaction kinetics in both hydrogen evolution and oxygen evolution reactions. By applying this catalyst to anion-exchange membrane water electrolyzers, superior performance was achieved.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2022)

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Article Chemistry, Multidisciplinary

Phase-Controlled Synthesis of Nickel-Iron Nitride Nanocrystals Armored with Amorphous N-Doped Carbon Nanoparticles Nanocubes for Enhanced Overall Water Splitting

Mingyu Chen et al.

Summary: Transition metal nitrides (TMNs) nanostructures show great potential in clean energy and catalysis fields. This study successfully synthesized pure-phase Ni2+xFe2-xN/NC nanocubes and demonstrated their excellent electrocatalytic water splitting performance and durability.

SMALL (2022)

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Review Chemistry, Multidisciplinary

Transition Metal Non-Oxides as Electrocatalysts: Advantages and Challenges

Chandni Das et al.

Summary: The identification of hydrogen as a green fuel has sparked interest in sustainable development and research in water electrolysis. Transition metal non-oxides (TMNOs) have emerged as efficient electrocatalysts, outperforming transition metal oxides (TMOs). TMNOs can effectively catalyze the oxygen evolution reaction (OER), hydrogen evolution reaction (HER), and oxygen reduction reaction (ORR), making them potential replacements for conventional noble metal electrocatalysts. This review discusses the crystal structure, synthesis strategies, and properties of nanostructured TMNOs, as well as the challenges and future prospects of energy conversion and storage materials in advancing the hydrogen economy.

SMALL (2022)

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Article Energy & Fuels

Underpotential deposition promoting low Pt loading on MoO2/MoS2 heterostructure towards wide pH green hydrogen evolution

Bin Dong et al.

Summary: In this study, a Pt@MoO2/MoS2 catalyst was prepared using an underpotential deposition (UPD)-replacement route, showing enhanced hydrogen evolution reaction (HER) activity and long-term stability compared to the Pt/C benchmark. The synergistic regulation of water dissociation and hydrogen adsorption/desorption by Pt and MoO2/MoS2, along with strong electron interaction due to the metal-support effect, contribute to the improved performance of the catalyst.

FUEL (2022)

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Article Chemistry, Physical

Interface engineering of bimetallic nitrides nanowires as a highly efficient bifunctional electrocatalyst for water splitting

Ruijie Dai et al.

Summary: In this study, nickel molybdenum nitride heterostructure nanowire arrays were successfully synthesized on nickel foam to achieve high-performance self-supporting electrodes. These electrodes exhibited low overpotentials in water splitting reactions, providing a new approach for the design of non-precious metal-based transition metal nitride catalysts.

JOURNAL OF ALLOYS AND COMPOUNDS (2022)

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Review Chemistry, Physical

Layered Double Hydroxide-Derived Nanomaterials for Efficient Electrocatalytic Water Splitting: Recent Progress and Future Perspective

Arslan Hameed et al.

Summary: Layered double hydroxides (LDHs) have attracted intense interest as active electrocatalysts for water splitting due to their diverse compositions and layered structure. However, limitations such as structure collapse and poor conductivity hinder their application. Therefore, the development of LDH-derived nanomaterials as high-performance electrocatalysts is of great importance.

ACS ENERGY LETTERS (2022)

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Article Materials Science, Multidisciplinary

Substitutional Doping Engineering toward W2N Nanorod for Hydrogen Evolution Reaction at High Current Density

Zixuan Dan et al.

Summary: Ni-W2N@NF catalyst was synthesized to achieve excellent HER performance in an alkaline environment. Experimental analyses confirmed that Ni enters the W2N lattice by substitutional doping, optimizing the free energy of hydrogen adsorption and hydroxide adsorption. This work offers a feasible idea for designing an effective catalyst for HER reaction under industrial large current in an alkaline solution.

ACS MATERIALS LETTERS (2022)

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Article Chemistry, Multidisciplinary

Bimetallic Ni-Mo nitride@N-doped C as highly active and stable bifunctional electrocatalysts for full water splitting

Yu Zhang et al.

Summary: Designing low-cost, highly active and stable electrocatalysts is crucial for renewable energy storage and conversion devices. A NiMoN nanosheet hybrid catalyst was fabricated through a reduction reaction, showing high activity and stability, with promising potential in large-scale water splitting.

NEW JOURNAL OF CHEMISTRY (2022)

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Article Nanoscience & Nanotechnology

Regulating the Interfacial Electron Density of La0.8Sr0.2Mn0.5Co0.5O3/RuOx for Efficient and Low-Cost Bifunctional Oxygen Electrocatalysts and Rechargeable Zn-Air Batteries

Yawen Dai et al.

Summary: A new bifunctional electrocatalyst LSMC-Ru, with outstanding activity and low potential gap, was fabricated by anchoring RuOx to the LSMC perovskite. The strong electronic interaction between RuOx and LSMC promotes oxygen evolution reaction (OER) and oxygen reduction reaction (ORR), enabling high performance in a Zn-air battery with low cost. The strategy of anchoring a low dosage noble metal catalyst to perovskite shows potential for other noble metal-non-noble metal composite electrocatalysts to achieve competitive performance and low cost.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Physical

Experimental and theoretical investigation of reconstruction and active phases on honeycombed Ni3N-Co3N/C in water splitting

Chao Huang et al.

Summary: Decorated with carbon speckles, the honeycombed Ni3N-Co3N catalyst shows excellent performance in both oxygen evolution reaction (OER) and hydrogen evolution reaction (HER), with low overpotentials, small Tafel slopes, and high stability. A water-splitting cell composed of this bifunctional catalyst can be driven by a standard 1.5 V battery, demonstrating its commercial practicality. Experimental and theoretical results provide insights into the active sites, conductivity, roles of Ni3N, Co3N, and C, as well as the reaction mechanism in HER and OER.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Chemistry, Physical

Nickel-Iron nitrides and alloy heterojunction with amorphous N-doped carbon Shell: High-efficiency synergistic electrocatalysts for oxygen evolution reaction

Hyung Wook Choi et al.

Summary: Nickel-Iron nitrides and alloys show superior OER performance with improved catalytic properties and durability through morphological control strategies.

APPLIED SURFACE SCIENCE (2021)

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Article Chemistry, Physical

A highly efficient and robust hybrid structure of CoNiN@NiFe LDH for overall water splitting by accelerating hydrogen evolution kinetics on NiFe LDH

Jie Wang et al.

Summary: The hybrid nano-architecture of CoNiN@NiFe LDH as a bifunctional electrocatalyst for overall water splitting exhibits excellent OER activities and stability, attributed to abundant active sites and strong electronic interactions.

APPLIED SURFACE SCIENCE (2021)

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Article Chemistry, Physical

Iron-doped cobalt nitride nanoparticles (Fe-Co3N): An efficient electrocatalyst for water oxidation

Liqian Wu et al.

Summary: In this study, Fe-doping Co3N catalysts with low overpotential and small Tafel slope were successfully synthesized, and the enhancement of OER performance was attributed to the electronic modulation induced by Fe incorporation. The introduction of heterogeneous element is shown to be a simple and effective strategy to regulate the OER property of cobalt nitrides catalysts.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2021)

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Article Materials Science, Multidisciplinary

Tailoring the d-band center of N-doped carbon nanotube arrays with Co4N nanoparticles and single-atom Co for a superior hydrogen evolution reaction

Bo Cao et al.

Summary: A 3D self-supported integrated electrode with Co4N nanoparticles and single-atom Co exhibits robust performance for the hydrogen evolution reaction due to its abundance of active sites and synergistic effects among components, optimizing the d-band center for efficient electrocatalysis.

NPG ASIA MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Stable and Highly Efficient Hydrogen Evolution from Seawater Enabled by an Unsaturated Nickel Surface Nitride

Huanyu Jin et al.

Summary: A novel unsaturated nickel surface nitride catalyst has been developed for efficient and stable hydrogen electrocatalytic production in alkaline seawater. The catalyst shows lower overpotential compared to traditional metal nitrides and can effectively generate hydronium ions in high-pH electrolyte.

ADVANCED MATERIALS (2021)

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Article Chemistry, Physical

Interface engineered NiMoN/Ni3N heterostructures for enhanced alkaline hydrogen evolution reaction

Wei Hua et al.

Summary: By constructing NiMoN/Ni3N heterostructures through interface engineering, the alkaline HER electrocatalyst shows enhanced activity with lower overpotential and smaller Tafel slope, indicating a promising approach for developing superior catalysts for alkaline electrolysis.

APPLIED SURFACE SCIENCE (2021)

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Article Materials Science, Multidisciplinary

Plasma mediated preparation of NiFeNx nanoparticles anchored on nickel foam for efficient oxygen evolution in alkaline solution

Yan Pan et al.

Summary: This paper presents a plasma mediated nitriding method for preparing transition metal nitrides for efficient oxygen evolution reaction. The obtained NiFeNx/NF composite structure shows excellent performance, with low overpotential and good stability attributed to the synergistic effect of NiFe bimetallic nitrides.

MATERIALS LETTERS (2021)

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Article Chemistry, Physical

A-Site Management Prompts the Dynamic Reconstructed Active Phase of Perovskite Oxide OER Catalysts

Yu Sun et al.

Summary: Perovskite oxides, with a refined A-site management strategy, can enhance OER performance through promoting the surface reconstruction of the active phase. The A-site Ce doping in particular shows a strong correlation with the dynamic structure-activity relationship during OER, providing insights for accurate design of high-efficiency perovskite OER electrocatalysts.

ADVANCED ENERGY MATERIALS (2021)

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Article Materials Science, Multidisciplinary

Nickel-doped Co4N nanowire bundles as efficient electrocatalysts for oxygen evolution reaction

Dan Li et al.

Summary: In this study, nickel doping was introduced into one-dimensional hierarchical Co4N structures to enhance OER performance, resulting in increased amount of Co3+ and improved electrocatalytic kinetics. The optimal Ni-doped Co4N with Ni/Co molar ratio of 0.25 exhibited excellent OER performance, with low overpotential and Tafel slope, as well as high long-term stability. Doping with Fe and Cu further enhanced the OER activity of Co4N nanowire bundles.

SCIENCE CHINA-MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Single-Atom Co-Decorated MoS2 Nanosheets Assembled on Metal Nitride Nanorod Arrays as an Efficient Bifunctional Electrocatalyst for pH-Universal Water Splitting

Thi Luu Luyen Doan et al.

Summary: The study developed an advanced bifunctional electrocatalyst based on single-atom Co-decorated MoS2 nanosheets grown on 3D titanium nitride nanorod arrays for overall water splitting in pH-universal electrolytes, showing superior efficiency and stability compared to previous non-noble metal catalysts.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Physical

Boosting the electrocatalytic HER performance of Ni3N-V2O3 via the interface coupling effect

Peng Zhou et al.

Summary: The construction of a suitable coupling interface is essential for improving the performance of high-efficient electrocatalysts. In this study, a Ni3N-V2O3 composite was designed and synthesized, showing excellent electrocatalytic hydrogen evolution reaction (HER) performance. The introduction of V2O3 led to a confinement effect and interface coupling effect, which greatly increased catalytic sites and improved performance.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Engineering, Environmental

Hierarchical Ni3N/Ni0.2Mo0.8N heterostructure nanorods arrays as efficient electrocatalysts for overall water and urea electrolysis

Rui-Qing Li et al.

Summary: The new Ni3N/Ni0.2Mo0.8N/NF catalyst demonstrates multifunctional superior performance for overall water and urea electrolysis, requiring low overpotentials and ultrasmall potentials for hydrogen generation.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Chemistry, Physical

Computational screening of bifunctional single atom electrocatalyst based on boron nitride nanoribbon for water splitting

Guohong Fan et al.

Summary: Designing bifunctional single atom catalyst is a promising strategy for developing efficient and low-cost electrocatalyst for overall water splitting. FeN4-BNNR and RhN4-BNNR are identified as the most efficient catalysts for both HER and OER, with low HER/OER overpotential. The activity of TMN4-BNNR depends on the binding strength toward intermediates and the electron-donating ability and d band center of the catalyst.

APPLIED CATALYSIS A-GENERAL (2021)

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Article Chemistry, Physical

One-step plasma nitriding synthesis of NixN/NF (x=3, 4) for efficient hydrogen evolution

Guanshui Ma et al.

Summary: In this study, a simple plasma-enhanced discharge nitridation method was utilized to fabricate NixN/NF cathode, which showed excellent HER electrocatalytic performance and long-term durability in alkaline conditions. Density functional calculations revealed that the introduction of N atoms in NF reduced the values of Gibbs free energy, particularly at the Ni4N-Ni interfacial sites, resulting in the lowest value for H adsorption-desorption.

APPLIED SURFACE SCIENCE (2021)

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Article Chemistry, Physical

Self-supported Ni3N nanoarray as an efficient nonnoble-metal catalyst for alkaline hydrogen evolution reaction

Wenna Liu et al.

Summary: A simple one-step nitridation method was used to fabricate Ni3N nanorod arrays on nickel foam for electrocatalytic water splitting. The obtained Ni3N/NF electrode showed extremely low overpotential and excellent cycle stability for the hydrogen evolution reaction.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2021)

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Article Chemistry, Physical

Carbon supported Ni3N/Ni heterostructure for hydrogen evolution reaction in both acid and alkaline media

Dhandapani Balaji et al.

Summary: The study introduced a special route to construct carbon-supported Ni3N/Ni as an effective electrocatalyst for the hydrogen evolution reaction, showing superior electrical conductivity and charge transfer rate. By enhancing the electronic structure through intrinsic active sites, the Ni3N/Ni@C750 degrees C composite demonstrated enhanced electrocatalytic behavior in both acid and alkaline electrolytes.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2021)

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Article Chemistry, Physical

Synergizing aliovalent doping and interface in heterostructured NiV nitride@oxyhydroxide core-shell nanosheet arrays enables efficient oxygen evolution

Xiaorui Gao et al.

Summary: In this study, a novel NiV nitride@oxyhydroxide (NiVN@OOH) heterostructured nanosheet was successfully developed for efficient oxygen evolution reaction (OER) with superior activity and long-term stability. This nanosheet, featuring abundant core-shell interfaces, vertically aligned nanosheet arrays, and purposely-chosen V-doping, exhibits significantly enhanced OER activity through synergistic effects of aliovalent doping and interface engineering.

NANO ENERGY (2021)

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Review Chemistry, Multidisciplinary

Perfecting electrocatalysts via imperfections: towards the large-scale deployment of water electrolysis technology

Shilong Jiao et al.

Summary: Hydrogen is increasingly seen as a key energy carrier in decarbonization efforts and strategies for clean energy economies. Improving the efficiency of electrocatalytic water splitting is crucial for reducing energy consumption and increasing conversion efficiency. The incorporation of multidimensional imperfections has shown promise in modulating electron distribution and speeding up electrocatalysis kinetics.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Review Chemistry, Multidisciplinary

Transition metal nitrides for electrochemical energy applications

Hao Wang et al.

Summary: Researchers have shown that by designing nanostructured TMNs with tailored morphology, it is possible to address issues such as limited active sites and sluggish ionic kinetics in bulk TMNs, ultimately improving electrochemical performance. Recent progress in TMN-based nanomaterials has focused on geometric-structure design, electronic-structure engineering, and applications in electrochemical energy conversion and storage.

CHEMICAL SOCIETY REVIEWS (2021)

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Article Chemistry, Physical

Highly active and stable nickel-molybdenum nitride (Ni2Mo3N) electrocatalyst for hydrogen evolution

Sang Heon Park et al.

Summary: This study introduces a nonprecious metal electrocatalyst based on bimetallic nanoscale nickel molybdenum nitride for the hydrogen evolution reaction (HER), demonstrating high activity and stability. The Ni2Mo3N/NF catalyst exhibits excellent performance in alkaline media, possibly due to the N sites in Ni2Mo3N with a N-Mo coordination number of four having a hydrogen adsorption energy close to that of Pt.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Physical

Large-current-stable bifunctional nanoporous Fe-rich nitride electrocatalysts for highly efficient overall water and urea splitting

Fengming Cai et al.

Summary: The study introduces a bifunctional nanoporous Fe-rich nitride hybrid electrocatalyst with extraordinary catalytic activities for both oxygen evolution and urea oxidation reactions, showing impressive long-term durability at large current densities. By combining this catalyst with an efficient NiMoO4-H-2 catalyst for hydrogen evolution, the researchers achieved commercially viable current densities for overall water and urea electrolysis with outstanding long-term durability, surpassing most reported electrolyzers. This work presents a novel approach to develop multifunctional electrocatalysts using earth-abundant elements for energy-efficient hydrogen production and pollution treatment in urea-rich wastewater.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Multidisciplinary

The rational design of Cu2-xSe@(Co,Cu)Se2 core-shell structures as bifunctional electrocatalysts for neutral-pH overall water splitting

Li Liu et al.

Summary: By integrating element doping, morphology design, and constructing a complex, a highly efficient bifunctional electrocatalyst was successfully fabricated for H-2 generation from neutral-pH water. The novel Cu2-xSe@(Co,Cu)Se-2 core-shell structure exhibited excellent performance with high current density at low overpotentials.

NANOSCALE (2021)

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Review Chemistry, Physical

Interface engineering of transitional metal sulfide-MoS2 heterostructure composites as effective electrocatalysts for water-splitting

Yanqiang Li et al.

Summary: The construction of transitional metal sulfide-MoS2 heterostructures can enhance the catalytic efficiency for water splitting reactions and potentially lead to bifunctional catalysts.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Nanoscience & Nanotechnology

Regulating the Interfacial Electron Density of La0.8Sr0.2Mn0.5Co0.5O3/RuOx for Efficient and Low-Cost Bifunctional Oxygen Electrocatalysts and Rechargeable Zn-Air Batteries

Yawen Dai et al.

Summary: The bifunctional electrocatalyst LSMC-Ru shows outstanding activity with a low dose of ruthenium, achieving synergy between ORR and OER through electronic interaction. It delivers excellent performance and cycling stability in Zn-air battery applications.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Self-Supported Transition-Metal-Based Electrocatalysts for Hydrogen and Oxygen Evolution

Hongming Sun et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Physical

Plasma-heteroatom-doped Ni-V-Fe trimetallic phospho-nitride as high-performance bifunctional electrocatalyst

Huafeng Fan et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Review Chemistry, Multidisciplinary

Recent Advances in Electrocatalytic Hydrogen Evolution Using Nanoparticles

Jing Zhu et al.

CHEMICAL REVIEWS (2020)

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Article Nanoscience & Nanotechnology

Plasma Transforming Ni(OH)2 Nanosheets into Porous Nickel Nitride Sheets for Alkaline Hydrogen Evolution

Guoling Li et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Chemistry, Multidisciplinary

Spontaneous Synthesis of Silver-Nanoparticle-Decorated Transition-Metal Hydroxides for Enhanced Oxygen Evolution Reaction

Zhao Zhang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Multidisciplinary

Single-Atom Vacancy Defect to Trigger High-Efficiency Hydrogen Evolution of MoS2

Xin Wang et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Review Chemistry, Physical

Recent Advances on Water-Splitting Electrocatalysis Mediated by Noble-Metal-Based Nanostructured Materials

Yingjie Li et al.

ADVANCED ENERGY MATERIALS (2020)

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