☆ 4.8 Review

In Situ and Operando Characterizations of Metal Halide Perovskite and Solar Cells: Insights from Lab-Sized Devices to Upscaling Processes

CHEMICAL REVIEWS (2023)

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Revealing the Transient Formation Dynamics and Optoelectronic Properties of 2D Ruddlesden-Popper Phases on 3D Perovskites

Tim Kodalle et al.

Summary: This study examines the formation of 2D layers on 3D triple cation perovskite films using in situ photoluminescence measurements during the spin-coating and annealing steps. The results reveal two formation regimes and different compositions of the 2D/3D interface for different cations. The study also shows that a higher ratio of quasi-2D phases benefits device performance.

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Summary: In this study, new insights into the halide-segregation process in mixed halide perovskites were obtained through in situ X-ray diffraction measurements. The photoinduced halide segregation leads to the formation of iodide-rich and bromide-rich perovskite compositions with the same Br:I ratios, which can reversely transform back to the mixed halide perovskite under dark conditions. The results help to understand the kinetics and mechanisms of halide-segregation process in mixed-halide perovskites.

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Review Chemistry, Multidisciplinary

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Summary: Metal halide perovskites, particularly tin-based compounds, show promise for optoelectronic applications, with lead-based compounds being toxic and harmful to the environment. Although tin-based perovskites offer advantages such as near-optimal bandgap and good charge carrier mobilities, their efficiency is currently limited by low defect tolerance, fast crystallization, and oxidative instability. Efforts are being made to improve tin-based perovskite solar cells, focusing on strategies to enhance device performances and address existing challenges in a concerted manner.

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Article Chemistry, Multidisciplinary

A finely regulated quantum well structure in quasi-2D Ruddlesden-Popper perovskite solar cells with efficiency exceeding 20%

Jianghu Liang et al.

Summary: Introducing a quantum well reversely graded structure through isopropanol washing into FA-MA mixed 2D perovskite films reduces the quantum confinement effect inside the film, extends the external quantum efficiency response wavelength, and results in out-of-plane orientation, significant grain size, and long carrier lifetime. An unprecedented power conversion efficiency of 20.12% was achieved, with high stability demonstrated through aging tests under different conditions.

ENERGY & ENVIRONMENTAL SCIENCE (2022)

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Thermodynamic Analyses on Nanoarchitectonics of Perovskite from Lead Iodide: Arrhenius Activation Energy

Nelson F. Borrero et al.

Summary: This study measured the activation energy of the formation process of methylammonium lead iodide MAPbI(3) using the Arrhenius equation, with controlled reactions at high temperatures using MAI vapor. The results showed that MAPbI(3) is easily formed at low temperatures, but this also contributes to its instability in environmental conditions.

JOURNAL OF INORGANIC AND ORGANOMETALLIC POLYMERS AND MATERIALS (2022)

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Article Chemistry, Physical

Dual Passivation of Point Defects at Perovskite Grain Boundaries with Ammonium Salts Greatly Inhibits Nonradiative Charge Recombination

Lu Qiao et al.

Summary: Experiments and simulations demonstrate that grain boundaries (GBs) have a detrimental effect on carrier lifetimes in MAPbI(3). It is also found that NH4Cl can passivate common point defects at GBs and accelerate electron-hole recombination. This study shows that the negative role of GBs can be removed by dual passivation with NH4Cl, extending the carrier lifetime.

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Nanoscale chemical heterogeneity dominates the optoelectronic response of alloyed perovskite solar cells

Kyle Frohna et al.

Summary: By combining quantitative optical spectroscopic techniques and synchrotron nanoprobe measurements, we can visualize the nanoscale chemical, structural, and optoelectronic landscape in halide perovskite devices. Compositional disorder plays a dominant role in the optoelectronic response, while the influence of nanoscale strain variations is weaker.

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Light-activated interlayer contraction in two-dimensional perovskites for high-efficiency solar cells

Wenbin Li et al.

Summary: Continuous light illumination causes over 1% contraction in the out-of-plane direction in two-dimensional hybrid perovskites, which is reversible and strongly dependent on specific superlattice packing. Positive charge accumulation enhances the bonding character of inter-slab I-I interactions and activates out-of-plane contraction.

NATURE NANOTECHNOLOGY (2022)

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Article Energy & Fuels

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Martin A. Green et al.

Summary: This article presents consolidated tables showing the highest independently confirmed efficiencies for solar cells and modules, with guidelines outlined for inclusion of results into these tables and a review of new entries since June 2021.

PROGRESS IN PHOTOVOLTAICS (2022)

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Conformal quantum dot-SnO2 layers as electron transporters for efficient perovskite solar cells

Minjin Kim et al.

Summary: The study replaced the commonly used mesoporous titanium dioxide electron transport layer with a thin layer of polyacrylic acid-stabilized tin(IV) oxide quantum dots, which improved the efficiency and stability of perovskite solar cells and enabled successful scaling up of PSCs production.

SCIENCE (2022)

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Impedance spectroscopy for perovskite solar cells: characterisation, analysis, and diagnosis

Elizabeth von Hauff et al.

Summary: Impedance spectroscopy (IS) has great potential for characterising and diagnosing perovskite solar cells (PSC), but interpretation of the data is challenging due to the many dynamic processes involved. This study proposes a universal framework for IS analysis on PSC, which includes reviewing timescales for electrical and electrochemical dynamics and guidelines for obtaining high quality impedance spectra. The study also introduces a universal equivalent circuit model (ECM) that can be used to parameterise material properties and monitor loss mechanisms in PSC.

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Zhenhua Xu et al.

Summary: This study presents a two-step phase transition process to deposit high-quality photovoltaic alpha-FAPbI(3) films using a printing method. By carefully selecting a Lewis base and acid, the energy barrier in the intermediary phase is reduced, resulting in phase-pure and stable films with high efficiency solar devices. This work provides new insights in alpha-FAPbI(3) crystallization for constructing efficient and stable printed photovoltaic devices.

NANO ENERGY (2022)

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Article Chemistry, Multidisciplinary

Exploration of the Defect Passivation in Perovskite Materials Using Organic Spacer Cations

Kongchao Shen et al.

Summary: This study investigates the defect passivation mechanism in quasi-2D metal halide perovskite light emitting diodes. The results reveal that the electrostatic interaction between proper organic spacer cations and defective PbBr64- octahedrons plays a crucial role in defect passivation, particularly at grain boundaries. The thermal stability of perovskite films and device performance are improved after the defect passivation process.

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All-Slot-Die-Coated Inverted Perovskite Solar Cells in Ambient Conditions with Chlorine Additives

Thai Son Le et al.

Summary: This study demonstrates the successful application of slot-die coating for large-scale production of perovskite solar cells, achieving high power conversion efficiency. The use of Cl-containing additives and vacuum quenching is essential for reproducible crystallization of perovskite films, leading to improved performance of the devices. Additionally, the methodology is successfully upscaled for minimodule fabrication, showing great potential for sheet-to-sheet production of perovskite solar cells.

SOLAR RRL (2022)

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Jianhong Zhao et al.

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Summary: Lab-scale perovskite solar cells have achieved efficiencies comparable to the best monocrystalline silicon cells, and efforts are now focused on production. The use of frontal metal grids is crucial for large-area perovskite cells and modules, but a trade-off between reduced resistive losses and increased shadowed area must be considered. Evaluation of grid parameters is essential for the assembly of viable large-scale cells and modules, although specific grid designs for perovskite cells are currently limited in the literature.

SOLAR RRL (2022)

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In Operando, Photovoltaic, and Microscopic Evaluation of Recombination Centers in Halide Perovskite-Based Solar Cells

Arava Zohar et al.

Summary: We present a powerful approach to assess the defect densities in lead halide perovskite materials based on electric field mapping. By measuring the electric field profile using electron beam-induced current, we deduced the defect densities and found that they mainly exist at the interfaces with selective contacts rather than in the perovskite film. These results are highly relevant for improving the efficiency of photovoltaic devices.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Unveiling the Interaction Mechanisms of Electron and X-ray Radiation with Halide Perovskite Semiconductors using Scanning Nanoprobe Diffraction

Jordi Ferrer Orri et al.

Summary: The interaction of high-energy electrons and X-ray photons with beam-sensitive semiconductors is investigated using nanoprobe diffraction techniques. The changes in the local crystal structure of hybrid halide perovskite films are tracked as a function of fluence, revealing the formation of PbBr2 and PbI2 crystallites, as well as the presence of pinholes. This study emphasizes the importance of addressing high-angle grain boundaries for improving the stability of halide polycrystalline films, especially for applications vulnerable to high-energy radiation.

ADVANCED MATERIALS (2022)

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Article Materials Science, Multidisciplinary

Time-Resolved Grazing Incidence X-Ray Absorption Spectroscopy for the In Situ Investigation of the Initial Stages of Sputter-Deposited Copper Thin Films

Dirk Luetzenkirchen-Hecht et al.

Summary: The growth of thin copper films on float glass substrates using sputter deposition was studied in situ with X-ray absorption fine structure spectroscopy, showing different stages of film growth from the formation of copper clusters to 3D growth of Cu crystallites. The method provides detailed analysis of film thickness and surface roughness, offering further prospects for research in this field.

PHYSICA STATUS SOLIDI A-APPLICATIONS AND MATERIALS SCIENCE (2022)

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Local nanoscale phase impurities are degradation sites in halide perovskites

Stuart Macpherson et al.

Summary: Understanding the nanoscopic chemical and structural changes is crucial for mitigating device degradation in emerging energy materials. Researchers have developed a multimodal microscopy toolkit to investigate the impact of phase impurities on the performance and longevity of formamidinium-rich perovskite absorbers. The study also demonstrates that manipulating these impurities can alleviate performance losses and intrinsic degradation processes.

NATURE (2022)

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Article Multidisciplinary Sciences

Damp heat-stable perovskite solar cells with tailored-dimensionality 2D/3D heterojunctions

Randi Azmi et al.

Summary: By tailoring the dimensional fragments of two-dimensional perovskite layers, damp-heat stable perovskite solar cells with high power conversion efficiencies were successfully fabricated. These cells retain over 95% of their initial value after more than 1000 hours under damp-heat test conditions, meeting one of the critical industrial stability standards for photovoltaic modules.

SCIENCE (2022)

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Article Chemistry, Physical

Microstructure of Methylammonium Lead iodide Perovskite Thin Films: A Comprehensive Study of the Strain and Texture

Asma A. Medjahed et al.

Summary: This study investigates the mechanisms of strain and texture observed in MAPbI(3) thin films deposited on various oxide substrates. The results show that the strain of the perovskite layers is essentially relaxed behavior, contradicting the commonly accepted hypothesis. The texture in the perovskite layers is studied using synchrotron full-field diffraction X-ray microscopy, and the stability of different orientations is analyzed by DFT calculations.

ADVANCED ENERGY MATERIALS (2022)

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Article Chemistry, Applied

Extended X-ray absorption fine structure (EXAFS) of FAPbI3 for understanding local structure-stability relation in perovskite solar cells

Dong-Ho Kang et al.

Summary: In this study, EXAFS was used to investigate the local structural changes of FAPbI(3) and found that perovskite films prepared from precursor solution with excess PbI2 showed better stability compared to those from excess FAI, despite similar power conversion efficiency. Excess FAI resulted in a rapid phase transition and poor device stability, as confirmed by the increased (Pb-I) bond distance evaluated by the Pb L-III-edge EXAFS study. This work provides important insights into the local structure-stability relation in FAPbI(3)-based PSCs.

JOURNAL OF ENERGY CHEMISTRY (2022)

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Article Energy & Fuels

Correlative In Situ Multichannel Imaging for Large-Area Monitoring of Morphology Formation in Solution-Processed Perovskite Layers

Simon Ternes et al.

Summary: This study demonstrates the use of in situ multichannel imaging (IMI) for real-time monitoring and feedback control in the large-scale production of perovskite photovoltaics. IMI can detect characteristic changes in perovskite formation dynamics and coating inhomogeneities, making it valuable for industrial-scale fabrication processes such as roll-to-roll printing.

SOLAR RRL (2022)

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Editorial Material Chemistry, Physical

Why it is important to determine and report the impact of probe radiation

Emma N. Antonio et al.

Summary: This study investigates the use of X-ray radiation for in situ research on Li-sulfur batteries, finding that X-ray radiation can cause severe damage to the batteries and emphasizes the importance of determining beam damage for meaningful measurements.

JOULE (2022)

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Article Physics, Applied

A step-by-step guide to perform x-ray photoelectron spectroscopy

Grzegorz Greczynski et al.

Summary: There is a growing concern within the surface science community regarding the decline in work quality and meaningless chemical bond assignment in XPS articles. This trend could have disastrous consequences for scientific research. To address this, a comprehensive tutorial is offered, providing a step-by-step guide for experimental planning, data acquisition, spectra analysis, and results presentation, with a focus on improving the quality and reliability of XPS data analysis. The tutorial aims to broaden the application of XPS and enhance practitioners' ability to draw meaningful insights from XPS analysis.

JOURNAL OF APPLIED PHYSICS (2022)

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Article Multidisciplinary Sciences

Sequential vacuum-evaporated perovskite solar cells with more than 24% efficiency

Hang Li et al.

Summary: Vacuum evaporation is a promising method for the fabrication of perovskite solar cells, with the advantages of precise film thickness control and compatibility with large-scale production. A Cl-containing alloy-mediated sequential vacuum evaporation approach was developed to fabricate perovskite films with high uniformity and few defects, resulting in high power conversion efficiency. The method provides a reproducible approach for scalable fabrication of large-area, high-efficiency perovskite solar cells and other perovskite-based optoelectronics.

SCIENCE ADVANCES (2022)

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Review Energy & Fuels

Advances and challenges in understanding the microscopic structure-property-performance relationship in perovskite solar cells

Yuanyuan Zhou et al.

Summary: The emergence of perovskite photovoltaic technology has greatly advanced our understanding of metal halide perovskite thin-film microstructures and their effects on optoelectronic properties, device efficiency, and stability. This article discusses the morphological characteristics of three key microstructure types in perovskites, explores their impacts on performance and degradation, and calls for more research on hidden microstructures and high-spatiotemporal-resolution characterizations.

NATURE ENERGY (2022)

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Surface stability of ionic-liquid-passivated mixed-cation perovskite probed with in situ photoelectron spectroscopy

Suresh Maniyarasu et al.

Summary: In recent times, the stability of mixed-cation metal halide perovskites has been significantly improved by incorporating ionic liquid additives into the perovskite precursor. The study shows that a small amount of 1-octyl-3-methylimidazolium chloride ionic liquid prevents the out-diffusion of organic ions from the lattice, leading to improved stability. Furthermore, the device fabricated with the ionic liquid additive demonstrates higher power conversion efficiency.

JOURNAL OF MATERIALS CHEMISTRY A (2022)

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Review Chemistry, Multidisciplinary

Strain effects on halide perovskite solar cells

Bowen Yang et al.

Summary: This article reviews the influence of strain on the performance and stability of halide perovskite solar cells, covering the origins, characterization techniques, and control strategies of strain. It also proposes effective strategies for future strain engineering. The comprehensive review is important for researchers to gain a deeper understanding of strain effects and improve performance towards commercialization.

CHEMICAL SOCIETY REVIEWS (2022)

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Article Chemistry, Multidisciplinary

Revealing the Perovskite Film Formation Using the Gas Quenching Method by In Situ GIWAXS: Morphology, Properties, and Device Performance

Rodrigo Szostak et al.

Summary: This study investigates the formation mechanism of MAPbI(3) and Cs(x)FA(1-)(x)Pb(I0.83Br0.17)(3) perovskites during deposition process using X-ray scattering, comparing the influence of DMSO and NMP solvents. The results show that the choice of optimal solvent varies for different Cs content, which is crucial for the final performance of the solar cells.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Review Chemistry, Multidisciplinary

In Situ/Operando Electrocatalyst Characterization by X-ray Absorption Spectroscopy

Janis Timoshenko et al.

Summary: X-ray absorption spectroscopy (XAS) is a crucial method for investigating the structure and composition of heterogeneous catalysts, revealing the nature of active sites and establishing links between structural motifs, local electronic structure, and catalytic properties. Recent advancements in instrumentation and data analysis approaches for deciphering X-ray absorption near edge structure (XANES) and extended X-ray absorption fine structure (EXAFS) spectra have been discussed, with emphasis on applications in the field of heterogeneous catalysis, particularly in electrocatalysis.

CHEMICAL REVIEWS (2021)

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Review Chemistry, Multidisciplinary

A Systematic Review of Metal Halide Perovskite Crystallization and Film Formation Mechanism Unveiled by In Situ GIWAXS

Minchao Qin et al.

Summary: Understanding the film formation mechanisms of metal halide perovskites is crucial for achieving high-quality perovskite films and high-performance devices. However, due to the complexity of perovskite composition, dimensionality, and processing conditions, this remains a great challenge.

ADVANCED MATERIALS (2021)

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Review Chemistry, Multidisciplinary

A Review on Scaling Up Perovskite Solar Cells

Daiyu Li et al.

Summary: This paper reviews the recent progress on scaling up perovskite solar cells and discusses the design and fabrication of efficient perovskite solar modules. It summarizes various scalable methods for large-area uniform perovskite films, potential charge transport materials, electrode materials, and encapsulation techniques. Additionally, the cost and environmental impact of perovskite solar modules are outlined.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Review Chemistry, Multidisciplinary

Impedance Spectroscopy of Metal Halide Perovskite Solar Cells from the Perspective of Equivalent Circuits

Antonio Guerrero et al.

Summary: Impedance spectroscopy (IS) is widely used in the study of metal halide perovskite materials, solar cells, electrooptic and memory devices, however, the variability of samples and the presence of coupled ionic-electronic effects continue to present complex challenges in this field.

CHEMICAL REVIEWS (2021)

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Article Chemistry, Physical

20.8% Slot-Die Coated MAPbI3 Perovskite Solar Cells by Optimal DMSO-Content and Age of 2-ME Based Precursor Inks

Jinzhao Li et al.

Summary: Efficiency records for solution-processed solar cell devices incorporating metal-halide perovskite semiconductors continue to be broken, with the need for scalable process technology and optimized ink formulations highlighted for large-area prototypes. The study demonstrates the importance of rational insights into ink composition and process control for reproducible manufacturing of MHP-based devices. The addition of a limited amount of DMSO prevents the formation of an intermediate crystalline phase and promotes the formation of the desired perovskite phase, while excess DMSO content negatively impacts thin-film morphology.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Physical

Four-Fold Multi-Modal X-ray Microscopy Measurements of a Cu(In,Ga)Se2 Solar Cell

Christina Ossig et al.

Summary: The research team demonstrated, for the first time, the simultaneous assessment of composition, structure, and performance in thin-film solar cells using sophisticated microscopy techniques. By using scanning X-ray microscopy on a Cu(In,Ga)Se-2 solar cell, they discovered structural features correlated with defects that limit the overall efficiency of the solar cell.

MATERIALS (2021)

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Article Multidisciplinary Sciences

Consequence of aging at Au/HTM/perovskite interface in triple cation 3D and 2D/3D hybrid perovskite solar cells

Zubair Ahmad et al.

Summary: Perovskite solar cells show great promise as an alternative to traditional photovoltaic technologies, with 2D/3D hybrid cells offering improved stability and efficiency. However, further research is needed on the degradation processes and charge dynamics at interfaces to enhance long-term performance. Analysis of the Au/HTM/perovskite interface degradation suggests it significantly impacts charge accumulation and impedance, leading to efficiency loss.

SCIENTIFIC REPORTS (2021)

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Article Chemistry, Analytical

Effect of illumination and applied potential on the electrochemical impedance spectra in triple cation (FA/MA/Cs) 3D and 2D/3D perovskite solar cells

Sumayya M. Abdulrahim et al.

Summary: This research aims to provide a comprehensive understanding of the illumination and voltage dependence of impedence spectra of 3D & 2D/3D PSCs with aging time, revealing complex variations in charge transfer and capacitance features under different operating conditions.

JOURNAL OF ELECTROANALYTICAL CHEMISTRY (2021)

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Article Multidisciplinary Sciences

Crystallization in one-step solution deposition of perovskite films: Upward or downward?

Shangshang Chen et al.

Summary: Research has shown that perovskite films prepared by one-step solution processes grow downward during thermal annealing, starting from an intermediate phase rather than from bottom to top. Understanding this vertical heterogeneity of perovskite films is crucial as it significantly impacts the efficiency and stability of perovskite solar cells.

SCIENCE ADVANCES (2021)

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Article Chemistry, Physical

Elucidating the Full Potential of OPV Materials Utilizing a High-Throughput Robot-Based Platform and Machine Learning

Xiaoyan Du et al.

Summary: The study demonstrates automated characterization of organic photovoltaic materials and devices, with optimization guided by Gaussian process regression. Improving molecular ordering and using thin active layers with medium thermal annealing temperature are identified as effective ways to enhance efficiency and suppress burn-in losses. The research findings enable rapid screening of materials with high efficiency and photostability.

JOULE (2021)

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Article Green & Sustainable Science & Technology

Assessing health and environmental impacts of solvents for producing perovskite solar cells

Rosario Vidal et al.

Summary: The study analyzes the human health toxicity and environmental implications of solvents used in perovskite solar cells, recommending dimethyl sulfoxide (DMSO) as the green choice for large-scale production.

NATURE SUSTAINABILITY (2021)

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Review Multidisciplinary Sciences

Dynamic structural property of organic-inorganic metal halide perovskite

Jin-Wook Lee et al.

Summary: Unique organic-inorganic hybrid semiconducting materials, known as perovskite solar cells, have achieved a significant breakthrough in the field of photovoltaics with a power conversion efficiency of 25.5%. The dynamic properties of the A site cationic molecules and PbI6 octahedrons in these materials have attracted a large number of researchers due to their dramatically different properties from traditional semiconductors.

ISCIENCE (2021)

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Article Nanoscience & Nanotechnology

Shaping Perovskites: In Situ Crystallization Mechanism of Rapid Thermally Annealed, Prepatterned Perovskite Films

Antonio Guenzler et al.

Summary: This study investigates the crystallization mechanisms of flash infrared-annealed perovskite films grown on substrates with lithographically patterned Au nucleation seeds. The study shows that by increasing the nucleation site density, the proportion of larger crystallites is increased, leading to longer charge carrier lifetimes in regions with large crystallites on the domain boundaries. This combination of rapid thermal annealing with nucleation control is a promising approach to improve perovskite crystallinity and the performance of optoelectronic devices.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Nanoscience & Nanotechnology

Impact of Vertical Inhomogeneity on the Charge Extraction in Perovskite Solar Cells: A Study by Depth-Dependent Photoluminescence

E. Regalado-Perez et al.

Summary: The study analyzes the vertical inhomogeneity of perovskite films in perovskite solar cells (PSCs) using depth-dependent photoluminescence (PL) achieved with different excitation wavelengths. An analytical representation parametrized with a factor, b, is introduced to understand the relation between inhomogeneity and charge recombination. Lower values of b correlate to lower vertical inhomogeneity and reduced recombination. Devices with lower vertical inhomogeneity, based on planar SnO2, show more efficient charge carrier extraction.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Nanoscience & Nanotechnology

Mechanism of Additive-Assisted Room-Temperature Processing of Metal Halide Perovskite Thin Films

Maged Abdelsamie et al.

Summary: Thiocyanate-containing additive MASCN can promote the crystallization of perovskite films and the formation of perovskite phase, contributing to growth through collision and drying processes. The characteristics of intermediate phases formed during this process and their kinetics of formation/dissociation play a crucial role in nucleation and growth of the perovskite phase.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Passivation Properties and Formation Mechanism of Amorphous Halide Perovskite Thin Films

Susan A. Rigter et al.

Summary: The addition of acetate precursors promotes rapid desolvation for making a variety of compositions of amorphous lead halide perovskite films. By controlling the amount of acetate, the transition from fully crystalline to fully amorphous films can be tuned, resulting in an intermediate state with crystalline islands embedded in an amorphous matrix.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Physical

Using In Situ Optical Spectroscopy to Elucidate Film Formation of Metal Halide Perovskites

Konstantin Schoetz et al.

Summary: Research interest in halide perovskites has increased due to high-efficient devices. High-quality perovskite layers are essential for these devices, and in situ optical spectroscopy is a powerful tool for studying their formation.

JOURNAL OF PHYSICAL CHEMISTRY A (2021)

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Article Multidisciplinary Sciences

Efficient perovskite solar cells via improved carrier management

Jason J. Yoo et al.

Summary: Metal halide perovskite solar cells have shown great potential to disrupt the silicon solar cell market with their improved performance, yet still face limitations in light-harvesting due to charge carrier recombination. Efforts to enhance charge carrier management offer a path to increase device performance and approach the theoretical efficiency limit of PSCs.

NATURE (2021)

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Article Multidisciplinary Sciences

Stabilized tilted-octahedra halide perovskites inhibit local formation of performance-limiting phases

Tiarnan A. S. Doherty et al.

Summary: This study successfully introduced octahedral tilting into pure alpha-FAPbI(3) thin films by using surface-bound ethylenediaminetetraacetic acid, ensuring extremely stability against thermal, environmental, and light stressors.

SCIENCE (2021)

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Review Chemistry, Multidisciplinary

Bulk Passivation and Interfacial Passivation for Perovskite Solar Cells: Which One is More Effective?

Jintao Wang et al.

Summary: Perovskite solar cells have promising photovoltaic applications, but suffer from poor stability. Recent advances in defect passivation in bulk films and interfaces through additive strategies were discussed, along with the impact of defect passivation and ion migration on stability performance. Challenges for commercialization prospects were also highlighted.

ADVANCED MATERIALS INTERFACES (2021)

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Article Multidisciplinary Sciences

Phase segregation in mixed-halide perovskites affects charge-carrier dynamics while preserving mobility

Silvia G. Motti et al.

Summary: The study investigates the impact of halide segregation on the charge-carrier dynamics and transport properties of mixed halide perovskite films using optical-pump terahertz-probe spectroscopy. Surprisingly, halide segregation has negligible impact on the charge-carrier mobilities, but affects recombination dynamics through charge funnelling. Enhanced lattice anharmonicity in the segregated regions supports ionic migration and contributes to fast charge funnelling into narrow-bandgap domains.

NATURE COMMUNICATIONS (2021)

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Article Multidisciplinary Sciences

Tuning structural isomers of phenylenediammonium to afford efficient and stable perovskite solar cells and modules

Cheng Liu et al.

Summary: The study focuses on understanding the energy barrier of 2D perovskite formation and proposes a method to prevent the formation of in-plane favored 2D perovskite layers, leading to improved device performance.

NATURE COMMUNICATIONS (2021)

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Article Multidisciplinary Sciences

Implementing an intermittent spin-coating strategy to enable bottom-up crystallization in layered halide perovskites

Yajie Yan et al.

Summary: The random orientation of layered crystals in 2D perovskites impedes the out-of-plane carriers transport and hence undermines the photovoltaic performance. Here, the authors discover that the crystallization can be regulated by intermittent spin-coating strategy, significantly enhancing crystal orientation and carrier transport, leading to a substantial improvement in solar cell efficiency.

NATURE COMMUNICATIONS (2021)

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Article Chemistry, Physical

Halide Segregation in Mixed-Halide Perovskites: Influence of A-Site Cations

Alexander J. Knight et al.

Summary: Mixed-halide perovskite films of MAPb(Br0.5I0.5)(3) and FA(0.83)Cs(0.17)Pb(Br0.4I0.6)(3) exhibit clear differences in compositional and optoelectronic changes associated with halide segregation. MAPb(Br0.5I0.5)(3) shows low-barrier ionic pathways that enhance stability against halide segregation, while FA(0.83)Cs(0.17)Pb(Br0.4I0.6)(3) lacks such pathways and undergoes considerable ionic rearrangement under prolonged illumination.

ACS ENERGY LETTERS (2021)

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Article Multidisciplinary Sciences

Iodine reduction for reproducible and high-performance perovskite solar cells and modules

Shangshang Chen et al.

Summary: Organic iodide perovskite precursors can be oxidized to I-2, impacting the performance and reproducibility of PSCs, but adding benzylhydrazine hydrochloride can effectively improve the situation. The stabilized efficiency of PSCs has been greatly enhanced after treatment.

SCIENCE ADVANCES (2021)

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Review Chemistry, Multidisciplinary

Perovskite Solar Cells for Space Applications: Progress and Challenges

Yongguang Tu et al.

Summary: Metal halide perovskites have versatile optoelectronic properties that make them promising candidates for next-generation space photovoltaic technology, despite being in the early stages of research compared to other practical space photovoltaics. The review highlights recent progress in perovskite solar cells for space applications, focusing on performance evolution and mechanism exploration under extreme space environments.

ADVANCED MATERIALS (2021)

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Article Engineering, Chemical

Low-Temperature Blade-Coated Perovskite Solar Cells

Adriano S. Marques et al.

Summary: Spin coating remains the primary choice for deposition in lab-scale perovskite solar cell assembly, with other methods still lagging in device efficiency and perovskite control. The development of a blade-coating route for all layers of perovskite solar cells offers a scalable method for large-area production, with potential improvements in device performance through ink composition tuning.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2021)

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Article Energy & Fuels

Degradation mechanisms of perovskite solar cells under vacuum and one atmosphere of nitrogen

Renjun Guo et al.

Summary: Research shows that perovskite solar cells operated under vacuum exhibit light-induced phase segregation, lattice shrinkage, and morphology deformation, while those operated under nitrogen only show lattice shrinkage, resulting in better device stability.

NATURE ENERGY (2021)

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Article Chemistry, Multidisciplinary

Surface Reconstruction of Halide Perovskites During Post-treatment

Shaun Tan et al.

Summary: In recent years, postfabrication surface treatment strategies have played a crucial role in improving the stability and performance of halide perovskite photovoltaics. This study utilized complementary surface-sensitive and depth-resolved techniques to observe the reconstruction of the perovskite surface induced by the common solvent isopropyl alcohol. The findings suggest that isopropyl alcohol assists in the adsorption process of organic ammonium salts to the surface, enhancing their defect passivation effects.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Multidisciplinary Sciences

Pseudo-halide anion engineering for α-FAPbI3 perovskite solar cells

Jaeki Jeong et al.

Summary: The research introduces a new concept of using formate anion to suppress defects in metal halide perovskite films and enhance film crystallinity, leading to improved efficiency and stability of solar cells.

NATURE (2021)

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Article Physics, Multidisciplinary

Three-dimensional coherent x-ray diffraction imaging of ferroelastic domains in single CsPbBr3 perovskite nanoparticles

D. Dzhigaev et al.

Summary: The study investigated twinned ferroelastic domains in single 500 nm CsPbBr3 particles using 3D Bragg coherent X-ray diffraction imaging, unveiling a preferential double-domain structure and suggesting the possibility of a deterministic formation process. The results provide valuable insights for both improving the performance of perovskite-based devices and understanding ferroelastic nanoscale materials, paving the way for real-time imaging of domain dynamics in ferroic systems.

NEW JOURNAL OF PHYSICS (2021)

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Article Energy & Fuels

Temperature-Dependent Crystallization Mechanisms of Methylammonium Lead Iodide Perovskite From Different Solvents

Oleksandra Shargaieva et al.

Summary: Hybrid perovskites are promising semiconducting materials for solution-processed optoelectronic devices, with the quality of perovskite thin films being critical for device performance. By investigating the crystallization process from a range of solvents, the binding strength of solvents within solvate-intermediate phases can be quantified, enabling prediction of optimal processing temperatures.

FRONTIERS IN ENERGY RESEARCH (2021)

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Article Multidisciplinary Sciences

Discovery of temperature-induced stability reversal in perovskites using high-throughput robotic learning

Yicheng Zhao et al.

Summary: The stability of perovskite-based photovoltaics is still a topic that needs more attention. Recent research reveals that the impact of cations on perovskite stability may reverse at temperatures below 100 degrees Celsius, compared to accelerated ageing tests at higher temperatures.

NATURE COMMUNICATIONS (2021)

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Article Multidisciplinary Sciences

Slot-die coating large-area formamidinium-cesium perovskite film for efficient and stable parallel solar module

Zhichun Yang et al.

Summary: This study utilized diphenyl sulfoxide (DPSO) additive to enhance the efficiency and stability of perovskite solar cells, resulting in the successful fabrication of high-efficiency solar modules.

SCIENCE ADVANCES (2021)

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Article Nanoscience & Nanotechnology

The Impact of Solvent Vapor on the Film Morphology and Crystallization Kinetics of Lead Halide Perovskites during Annealing

Yu Zhong et al.

Summary: By controlling the solvent vapor concentration, the grain size of perovskite can be adjusted, and the formation of low-dimensional perovskite during SVAA was observed. The study results indicate that perovskite growth follows an Ostwald ripening mechanism at higher solvent concentrations.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Review Chemistry, Physical

In-situ and operando spectroscopies for the characterization of catalysts and of mechanisms of catalytic reactions

Francisco Zaera

Summary: Catalysis in industrial chemical processes has long been studied through various spectroscopic techniques like vibrational and X-ray spectroscopies, allowing for a molecular-level understanding of catalytic mechanisms. These techniques help researchers explore the intricate details of catalytic processes and advancements in the field.

JOURNAL OF CATALYSIS (2021)

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Article Chemistry, Physical

High-Throughput Robotic Synthesis and Photoluminescence Characterization of Aqueous Multinary Copper-Silver Indium Chalcogenide Quantum Dots

Oleksandr Stroyuk et al.

Summary: The feasibility of high-throughput robot-assisted synthesis of complex CAISSe quantum dots by spontaneous alloying of aqueous glutathione-capped Ag-In-S, Cu-In-S, Ag-In-Se, and Cu-In-Se QDs is demonstrated. The composition-dependent character of the nonradiative recombination in QDs is found to be lower for mixed copper-silver-based QDs compared to Cu- or Ag-only QDs, indicating potential applications in photovoltaics and photochemistry. The synergy of high-throughput robotic synthesis and characterization is expected to lead to a self-learning synthetic platform for the production of metal chalcogenide QDs for various light-related applications.

PARTICLE & PARTICLE SYSTEMS CHARACTERIZATION (2021)

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Article Chemistry, Multidisciplinary

Unveiling Crystal Orientation in Quasi-2D Perovskite Films by In Situ GIWAXS for High-Performance Photovoltaics

Dong Liang et al.

Summary: GIWAXS was used to investigate the crystal orientation of quasi-2D perovskites during film fabrication process, revealing the impact of intermediate phases on crystalline growth and proposing a strategy of using simple additives to suppress their formation. This approach led to the successful fabrication of high-oriented quasi-2D perovskite solar cells with improved performance.

SMALL (2021)

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Article Multidisciplinary Sciences

Multication perovskite 2D/3D interfaces form via progressive dimensional reduction

Andrew H. Proppe et al.

Summary: Many top-performing perovskite photovoltaic devices utilize 2D/3D interfaces to enhance efficiency and stability. This study reveals the gradual dimensional reduction process from 3D to 2D perovskites.

NATURE COMMUNICATIONS (2021)

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Article Multidisciplinary Sciences

Importance of methylammonium iodide partial pressure and evaporation onset for the growth of co-evaporated methylammonium lead iodide absorbers

Karl L. Heinze et al.

Summary: Vacuum-based co-evaporation technique is explored for the growth of MAPbI3 thin films, revealing insights into crystallization and phase evolution. Optimization of chamber pressure and deposition sequence leads to improved efficiency and device performance.

SCIENTIFIC REPORTS (2021)

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Article Chemistry, Multidisciplinary

Structural and Trap-State Density Enhancement in Flash Infrared Annealed Perovskite Layers

Alica Brunova et al.

Summary: This study investigates the effect of adding methylammonium chloride (MACI) on the structure and trap-state density of perovskite. The results show that adding 10% MACI to the perovskite precursor solution significantly improves the crystallographic orientation of the perovskite layers while reducing the trap-state density by one order of magnitude. Through time-resolved GIWAXS, the most favorable time window for processing perovskite films with the lowest mosaicity and trap-state density is identified.

ADVANCED MATERIALS INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Revealing phase evolution mechanism for stabilizing formamidinium-based lead halide perovskites by a key intermediate phase

Zi-Ang Nan et al.

Summary: This study investigates the phase transition process of FA-based perovskites and identifies a key intermediate, providing insights into the phase evolution and stabilization mechanism. The findings deepen the understanding of the roles of cations and anions in maximizing halogen and cage concentrations, and offer suggestions for fabricating high-performance and stable PCSs by controlling various factors.

CHEM (2021)

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Article Chemistry, Physical

Effect of Light-Induced Halide Segregation on the Performance of Mixed-Halide Perovskite Solar Cells

Kunal Datta et al.

Summary: The study shows that light-induced halide segregation affects the performance of mixed-halide perovskite solar cells, resulting in a loss of short-circuit current density and red-shifted photoluminescence. Partial substitution of organic cations by cesium ions can reduce the negative impact of photogenerated charge carriers locating in iodide-rich domains and mitigate the loss in photovoltaic performance. Ultrasensitive photocurrent spectroscopy indicates that cesium ions lower the density of sub-band-gap defects and suppress defect growth under illumination.

ACS APPLIED ENERGY MATERIALS (2021)

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Article Chemistry, Physical

Regulating the crystalline phase of intermediate films enables FA1-xMAxPbI3 perovskite solar cells with efficiency over 22%

Fa-Zheng Qiu et al.

Summary: The study demonstrates that FA(1-x)MA(x)PbI(3) perovskite intermediate films prepared using the sequential deposition method at room temperature exhibit superior performance and can achieve high efficiency in solar cells. Furthermore, after aging for 1200 hours in ambient air, unencapsulated devices still maintain a high efficiency.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Multidisciplinary

Compositional heterogeneity in CsyFA1-yPb(BrxI1-x)3 perovskite films and its impact on phase behavior

Julien Barrier et al.

Summary: Hybrid organic-inorganic lead halide perovskite semiconductors show promise for high-efficiency photovoltaics, but their heterogeneity and its impact on material properties require further investigation. Using synchrotron X-ray diffraction to study the evolution of crystal structure is an effective method for evaluating heterogeneity and its effects.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Review Chemistry, Physical

Metal halide perovskite solar cells by modified chemical vapor deposition

Longbin Qiu et al.

Summary: Metal halide perovskite solar cells are a promising emerging photovoltaic technology facing challenges in scalable fabrication, operational stability, and environmental impact. Modified chemical vapor deposition (CVD) shows potential for large-area and uniform coating of perovskite layers at a low cost, with additional advantages such as solvent-free processing and compatibility with industrial manufacturing. This review presents the recent development of perovskite solar cells and modules using modified CVD, discussing differences with solution coating processing and highlighting the potential for cost-effective scalable fabrication.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Materials Science, Multidisciplinary

Moisture tolerant solar cells by encapsulating 3D perovskite with long-chain alkylammonium cation-based 2D perovskite

Bhushan P. Kore et al.

Summary: Long-chain alkylammonium cation-based 2D perovskites are effective coatings for 3D perovskites in improving stability and performance of perovskite solar cells, with only a 20% drop in power conversion efficiency after six months of operation in a humid environment.

COMMUNICATIONS MATERIALS (2021)

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Review Chemistry, Multidisciplinary

Upscaling perovskite solar cells via the ambient deposition of perovskite thin films

Kuan Liu et al.

Summary: This review summarizes the recent progress in upscaling of organic-inorganic halide perovskites processed in an ambient environment. It discusses the challenges and limitations involved, as well as provides a brief overview of robust strategies for the fabrication of efficient perovskite solar cells using printing-friendly techniques under ambient conditions, which are crucial for future deployment of this technology.

TRENDS IN CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Evolutionary exploration of polytypism in lead halide perovskites

Zhenzhu Li et al.

Summary: The thermodynamics of polytypism in CsPbI3 and CsPbBr3 are evaluated using total energies obtained from density functional theory. An axial Ising-type model Hamiltonian is paramaterized to explore the polytype phase space with a genetic algorithm, identifying distinct features of polytypism in the ground-state structures of CsPbX3 polytypes. Predictions of polytypes with low ordering energies suggest the formation of distinct phases or stacking faults within perovskite grains.

CHEMICAL SCIENCE (2021)

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Review Chemistry, Physical

Layered metal halide perovskite solar cells: A review from structure-properties perspective towards maximization of their performance and stability

Matheus S. de Holanda et al.

Summary: Perovskite solar cell technology has reached its full potential in terms of power conversion efficiency but still faces challenges in long-term stability. Layered perovskite solar cells offer a wide range of compositional variations to tune photophysical characteristics for device performance. Understanding the structural organization and properties of layered perovskites is crucial for improving the efficiency and stability of solar cells.

ECOMAT (2021)

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Article Materials Science, Multidisciplinary

Reduced graphene oxide in perovskite solar cells: the influence on film formation, photophysics, performance, and stability

Paulo Ernesto Marchezi et al.

Summary: The study demonstrates that the addition of reduced graphene oxide can influence the formation and properties of perovskite films, increasing grain size and improving device stability.

JOURNAL OF MATERIALS CHEMISTRY C (2021)

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Article Nanoscience & Nanotechnology

Using pulsed mode scanning electron microscopy for cathodoluminescence studies on hybrid perovskite films

Jordi Ferrer Orri et al.

Summary: The use of pulsed mode scanning electron microscopy cathodoluminescence (CL) is helpful in studying hybrid perovskite films, providing insights into their emission properties and carrier dynamics. Optimization of acquisition parameters allows for hyperspectral mapping and time-resolved measurements of these films, revealing heterogeneity in emission properties and shortened lifetimes of charge carriers compared to photoluminescence data. This work represents a promising advancement in investigating hybrid perovskite semiconductors at the nanoscale using CL.

NANO EXPRESS (2021)

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Article Chemistry, Physical

X-ray stability and degradation mechanism of lead halide perovskites and lead halides

Sebastian Svanstrom et al.

Summary: Lead halide perovskites have shown to be more stable under X-ray irradiation when fully inorganic, compared to those containing organic cations. The degradation of these materials occurs through two pathways induced by the radiolysis of the lead halide cage and the radiolysis of the organic cation, providing valuable insight for their use in high radiation environments.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2021)

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Article Chemistry, Physical

Quantifying the energy loss for a perovskite solar cell passivated with acetamidine halide

Ligang Yuan et al.

Summary: This study investigates the passivation of defects in polycrystalline perovskite films using acetamidine halide, leading to reduced trap state densities and improved efficiencies in perovskite solar cells and LED devices. Passivation with acetamidine halide significantly decreases energy loss and enhances stability of the devices.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Materials Science, Multidisciplinary

Blade-coating Perovskite Films with Diverse Compositions for Efficient Photovoltaics

Jun-Xing Zhong et al.

Summary: This research highlights recent advances in the hot-assisted blade-coating or air knife-assisted blade-coating of different perovskite compositions for single-junction or tandem PSCs, focusing on ink formulation engineering strategies, crystal growth mechanisms, crystallization kinetics, and optoelectronic properties of the different perovskite compositions.

ENERGY & ENVIRONMENTAL MATERIALS (2021)

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Review Green & Sustainable Science & Technology

Progress in blade-coating method for perovskite solar cells toward commercialization

Runsheng Wu et al.

Summary: Hybrid organic-inorganic halide perovskite solar cells have attracted attention in the photovoltaic community due to their unique properties, but the device area is a challenge for commercial applications. Various fabrication methods have been proposed to manufacture large-area PSCs, with this review focusing on progress in blade coating techniques and optimized strategies for perovskite film morphology. The challenges and opportunities for PSC commercialization have also been discussed.

JOURNAL OF RENEWABLE AND SUSTAINABLE ENERGY (2021)

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Article Chemistry, Physical

Fabrication of efficient CsPbBr3 perovskite solar cells by single-source thermal evaporation

Juan Li et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2020)

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Review Chemistry, Physical

A Review on Additives for Halide Perovskite Solar Cells

Shuang Liu et al.

ADVANCED ENERGY MATERIALS (2020)

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Review Chemistry, Physical

Structural Evolution During Perovskite Crystal Formation and Degradation: In Situ and Operando X-Ray Diffraction Studies

Laura E. Mundt et al.

ADVANCED ENERGY MATERIALS (2020)

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Review Chemistry, Multidisciplinary

The Role of the Interfaces in Perovskite Solar Cells

Shuyan Shao et al.

ADVANCED MATERIALS INTERFACES (2020)

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Article Nanoscience & Nanotechnology

Acetamidinium-Substituted Methylammonium Lead Iodide Perovskite Solar Cells with Higher Open-Circuit Voltage and Improved Intrinsic Stability

Pallavi Singh et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Chemistry, Multidisciplinary

Room-Temperature Partial Conversion of α-FAPbI3 Perovskite Phase via PbI2 Solvation Enables High-Performance Solar Cells

Dounya Barrit et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Revealing the Dynamics of Hybrid Metal Halide Perovskite Formation via Multimodal In Situ Probes

Tze-Bin Song et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Extending Carrier Lifetimes in Lead Halide Perovskites with Alkali Metals by Passivating and Eliminating Halide Interstitial Defects

Lu Qiao et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Multidisciplinary

Lead Iodide Thin Films via rf Sputtering

Jose Maria Clemente da Silva Filho et al.

CRYSTAL GROWTH & DESIGN (2020)

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Article Chemistry, Physical

Phase Diagram of Methylammonium/Formamidinium Lead Iodide Perovskite Solid Solutions from Temperature-Dependent Photoluminescence and Raman Spectroscopies

Adrian Francisco-Lopez et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2020)

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Article Materials Science, Multidisciplinary

Highly efficient and rapid manufactured perovskite solar cells via Flash InfraRed Annealing

Sandy Sanchez et al.

MATERIALS TODAY (2020)

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Article Chemistry, Multidisciplinary

In Situ Observation of Vapor-Assisted 2D-3D Heterostructure Formation for Stable and Efficient Perovskite Solar Cells

Zhou Liu et al.

NANO LETTERS (2020)

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Article Multidisciplinary Sciences

Strain engineering and epitaxial stabilization of halide perovskites

Yimu Chen et al.

NATURE (2020)

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Article Multidisciplinary Sciences

Triple-halide wide-band gap perovskites with suppressed phase segregation for efficient tandems

Jixian Xu et al.

SCIENCE (2020)

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Review Chemistry, Multidisciplinary

A Technical Introduction to Transmission Electron Microscopy for Soft-Matter: Imaging, Possibilities, Choices, and Technical Developments

Linda E. Franken et al.

SMALL (2020)

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Review Energy & Fuels

A review on perovskite solar cells: Evolution of architecture, fabrication techniques, commercialization issues and status

Priyanka Roy et al.

SOLAR ENERGY (2020)

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Review Chemistry, Physical

Electron-Beam-Related Studies of Halide Perovskites: Challenges and Opportunities

Junhui Ran et al.

ADVANCED ENERGY MATERIALS (2020)

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Review Chemistry, Physical

Optical Absorption-Based In Situ Characterization of Halide Perovskites

Finn Babbe et al.

ADVANCED ENERGY MATERIALS (2020)

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Article Materials Science, Multidisciplinary

Slot-die coating of perovskite solar cells: An overview

Rahul Patidar et al.

MATERIALS TODAY COMMUNICATIONS (2020)

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Article Chemistry, Multidisciplinary

Tapered Cross-Section Photoelectron Spectroscopy of State-of-the-Art Mixed Ion Perovskite Solar Cells: Band Bending Profile in the Dark, Photopotential Profile Under Open Circuit Illumination, and Band Diagram

Michael Wussler et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Chemistry, Multidisciplinary

First Proof-of-Principle of Inorganic Lead Halide Perovskites Deposition by Magnetron-Sputtering

Claudia Borri et al.

NANOMATERIALS (2020)

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Article Chemistry, Physical

Characterization of charge carrier behavior in photocatalysis using transient absorption spectroscopy

Tina Jingyan Miao et al.

JOURNAL OF CHEMICAL PHYSICS (2020)

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Article Chemistry, Multidisciplinary

Vacuum-Induced Degradation of 2D Perovskites

Yvonne J. Hofstetter et al.

FRONTIERS IN CHEMISTRY (2020)

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Article Multidisciplinary Sciences

Regulating strain in perovskite thin films through charge-transport layers

Ding-Jiang Xue et al.

NATURE COMMUNICATIONS (2020)

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Article Chemistry, Physical

The Application of Electron Backscatter Diffraction on Halide Perovskite Materials

Sun Hongyu et al.

ADVANCED ENERGY MATERIALS (2020)

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Review Chemistry, Physical

Photoemission Spectroscopy Characterization of Halide Perovskites

Solene Bechu et al.

ADVANCED ENERGY MATERIALS (2020)

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Article Chemistry, Physical

Ion Migration-Induced Amorphization and Phase Segregation as a Degradation Mechanism in Planar Perovskite Solar Cells

Diego Di Girolamo et al.

ADVANCED ENERGY MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Passivation Mechanism Exploiting Surface Dipoles Affords High-Performance Perovskite Solar Cells

Fatemeh Ansari et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Article Chemistry, Multidisciplinary

In Situ Analysis Reveals the Role of 2D Perovskite in Preventing Thermal-Induced Degradation in 2D/3D Perovskite Interfaces

Albertus A. Sutanto et al.

NANO LETTERS (2020)

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Article Multidisciplinary Sciences

Performance-limiting nanoscale trap clusters at grain junctions in halide perovskites

Tiarnan A. S. Doherty et al.

NATURE (2020)

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Article Nanoscience & Nanotechnology

Origin of Ionic Inhomogeneity in MAPb(IxBr1-x)3 Perovskite Thin Films Revealed by In-Situ Spectroscopy during Spin Coating and Annealing

Carolin Rehermann et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Chemistry, Multidisciplinary

Impact of Processing on Structural and Compositional Evolution in Mixed Metal Halide Perovskites during Film Formation

Maged Abdelsamie et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Chemistry, Multidisciplinary

In Situ Grazing-Incidence Wide-Angle Scattering Reveals Mechanisms for Phase Distribution and Disorientation in 2D Halide Perovskite Films

Justin M. Hoffman et al.

ADVANCED MATERIALS (2020)

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Review Chemistry, Multidisciplinary

High-Efficiency Perovskite Solar Cells

Jin Young Kim et al.

CHEMICAL REVIEWS (2020)

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Article Chemistry, Physical

Formamidinium Haloplumbate Intermediates: The Missing Link in a Chain of Hybrid Perovskites Crystallization

Andrey A. Petrov et al.

CHEMISTRY OF MATERIALS (2020)

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Article Nanoscience & Nanotechnology

Postpassivation of Multication Perovskite with Rubidium Butyrate

Jose Carlos Germino et al.

ACS PHOTONICS (2020)

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Article Chemistry, Physical

Multisource Vacuum Deposition of Methylammonium-Free Perovskite Solar Cells

Yu-Hsien Chiang et al.

ACS ENERGY LETTERS (2020)

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Article Chemistry, Physical

Microscopic Degradation in Formamidinium-Cesium Lead Iodide Perovskite Solar Cells under Operational Stressors

Nengxu Li et al.

JOULE (2020)

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Article Chemistry, Physical

Self-Elimination of Intrinsic Defects Improves the Low-Temperature Performance of Perovskite Photovoltaics

Yihua Chen et al.

JOULE (2020)

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Article Chemistry, Physical

Robot-Based High-Throughput Screening of Antisolvents for Lead Halide Perovskites

Ening Gu et al.

JOULE (2020)

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Article Energy & Fuels

Efficient Hybrid Mixed-Ion Perovskite Photovoltaics: In Situ Diagnostics of the Roles of Cesium and Potassium Alkali Cation Addition

Ming-Chun Tang et al.

SOLAR RRL (2020)

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Article Nanoscience & Nanotechnology

Surface, Interface, and Bulk Electronic and Chemical Properties of Complete Perovskite Solar Cells: Tapered Cross-Section Photoelectron Spectroscopy, a Novel Solution

Chittaranjan Das et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Nanoscience & Nanotechnology

Nanoscale Charge Accumulation and Its Effect on Carrier Dynamics in Tri-cation Perovskite Structures

David Toth et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Chemistry, Multidisciplinary

In Situ Imaging of Ferroelastic Domain Dynamics in CsPbBr3 Perovskite Nanowires by Nanofocused Scanning X-ray Diffraction

Lucas A. B. Marcal et al.

ACS NANO (2020)

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Article Chemistry, Physical

Pressure Engineered Optical Properties and Carrier Dynamics of FAPbBr3 Nanocrystals Encapsulated by Siliceous Nanosphere

Laizhi Sui et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2020)

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Article Chemistry, Physical

Removing Instability-Caused Low-Frequency Features in Small Perturbation Spectra of Perovskite Solar Cells

Sandheep Ravishankar et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2020)

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Article Chemistry, Physical

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